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Methane and nitrous oxide emissions from municipal wastewater treatment plants in China:A plant-level and technology-specific study

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Environmental Science and Ecotechnology 2024年第4期20卷 123-130页

作者： Haiyan Li Liangfang You He Du Bowen Yu Lu Lu Bo Zheng Qiang Zhang Kebin He Nanqi Ren School of Civil and Environmental Engineering Harbin Institute of TechnologyShenzhen518055China shenzhen key laboratory of ecological remediation and carbon sequestration Institute of Environment and EcologyTsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen518055China Ministry of Education key laboratory for Earth System Modeling Department of Earth System ScienceTsinghua UniversityBeijing100084China State key Joint laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China

Wastewater treatment is an important source of greenhouse gases(GHGs).Yet large uncertainties remain in the quantification of GHG emissions from municipal wastewater treatment plants(MWWTPs)in China.A high-resolution and technology-specific emission inventory is still lacking to support mitigation strategies of *** we develop a plant-level and technology-based MWWTP emission inventory for China covering 8703 plants and 19 treatment technology categories by compiling and harmonizing the most up-to-date facility-level ***'s methane(CH_(4))and nitrous oxide(N_(2)O)emissions from MWWTPs in 2020 are estimated to be 150.6 Gg and 22.0 Gg,respectively,with the uncertainty range of-30%to 37%and-30%to 26%at 95%confidence *** find an emission inequality across cities,with the richest cities emitting two times more CH_(4)and N_(2)O per capita from municipal wastewater treatment than the poorest *** emitted CH_(4)and N_(2)O are dominated by Anaerobic/Anoxic/Oxic-,Sequencing Batch Reactor-,Oxidation Ditch-,and Anoxic/Oxic-based MWWTPs of less than 20 years *** the relatively young age structure of China's MWWTPs,the committed emissions highlight the importance of reducing on-site GHG emissions by optimization of operating conditions and innovation *** emission differences among our estimates,previous studies,and the Intergovernmental Panel on Climate Change guidelines are largely attributed to the uncertainties in emission factors,implying the urgent need for more plant-integrated measurements to improve the accuracy of emission accounting.

关键词： Methane Nitrous oxide Emissions Municipal wastewater treatment plants

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Trends and drivers of anthropogenic NOx emissions in China since 2020

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Environmental Science and Ecotechnology 2024年第5期21卷 287-293页

作者： Hui Li Bo Zheng Yu Lei Didier Hauglustaine Cuihong Chen Xin Lin Yi Zhang Qiang Zhang Kebin He shenzhen key laboratory of ecological remediation and carbon sequestration Institute of Environment and EcologyTsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China State Environmental Protection key laboratory of Sources and Control of Air Pollution Complex Beijing 100084China State Environmental Protection key laboratory of Environmental Planning and Policy Simulation and Center of Air Quality Simulation and System Analysis Chinese Academy of Environmental PlanningBeijing 100041China Laboratoire des Sciences du Climat et de l’Environnement LSCE/IPSLCEA-CNRS-UVSQUniversite Paris-SaclayGif-sur-YvetteFrance Center for Satellite Application on Ecology and Environment Ministry of Ecology and Environment of ChinaBeijing 100094China Institute of Future Human Habitats Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China Ministry of Education key laboratory for Earth System Modeling Department of Earth System ScienceTsinghua UniversityBeijing 100084China State key Joint laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China

Nitrogen oxides(NOx),significant contributors to air pollution and climate change,form aerosols and ozone in the ***,timely,and transparent information on NOx emissions is essential for decision-making to mitigate both haze and ozone ***,a comprehensive understanding of the trends and drivers behind anthropogenic NOx emissions from Chinadthe world's largest emitterdhas been lacking since 2020 due to delays in emissions *** we show a consistent decline in China's NOx emissions from 2020 to 2022,despite increased fossil fuel consumption,utilizing satellite observations as constraints for NOx emission estimates through atmospheric *** reduction is corroborated by data from two independent spaceborne instruments:the TROPOspheric Monitoring Instrument(TROPOMI)and the Ozone Monitoring Instrument(OMI).Notably,a reduction in transport emissions,largely due to the COVID-19 lockdowns,slightly decreased China's NOx emissions in *** subsequent years,2021 and 2022,reductions in NOx emissions were driven by the industry and transport sectors,influenced by stringent air pollution *** satellite-based inversion system developed in this study represents a significant advancement in the real-time monitoring of regional air pollution emissions from space.

关键词： China's NOx emissions Pollution control Socio-economic drivers Atmospheric inversion

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Virus-Host Interactions Drive Contrasting Bacterial Diel Dynamics in the Ocean

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Research 2024年第2期6卷 389-399页

作者： Xiaowei Chen Chen Hu Wei Wei Yunlan Yang Markus G.Weinbauer Hongbo Li Shiying Ren Ruije Ma YVibin Huang Tingwei Luo Nianzhi Jiao Rui Zhang State key laboratory of Marine Environmental Science College of Ocean and Earth SciencesFujian Key Laboratory of Marine Carbon SequestrationXiamen UniversityXiamen 361102PR China College of the Environment and Ecology Xiamen UniversityXiamen 361102PR China Research Center for Environmental Ecology and Engineering School of Environmental Ecology and Biological EngineeringWuhan Institute of TechnologyWuhan 430205PR China Sorbonne Universités UPMCUniversitéParis 06CNRSLaboratoire d'Oceanographie de Villefranche(LOV)Villefranche-sur-Mer 06230France National Marine Environmental Monitoring Center Ministry of Ecological EnvironmentDalian 116023PR China Department of Ocean Sciences University of CaliforniaSanta CruzCAUSA NOAA/OAR Pacific Marine Environmental laboratory SeattleWAUSA Institute for Advanced Study Shenzhen UniversityShenzhen 518055PR China

Marine organisms perform a sea of diel *** diel dynamics have been shown to be driven by light,energy resources,circadian rhythms,and the coordinated coupling of photoautotrophs and heterotrophic ***,we explore the diel fluctuation of viral production and decay and their impact on the total and active bacterial community in the coastal and open seawaters of the South China *** results showed that the night-production diel pattern of lytic viral production was concurrent with the lower viral decay at night,contributing to the accumulation of the viral population size during the night for surface *** diel variations in bacterial activity,community composition,and diversity were found highly affected by viral *** was revealed by the finding that bacterial community diversity was positively correlated to lytic viral production in the euphotic zone of the open ocean but was negatively related to lysogenic viral production in the coastal *** distinct but contrasting correlations suggest that viral life strategies can not only contribute to diversifying bacterial community but also potentially piggyback their host to dominate bacterial community,suggesting the tightly synchronized depth-dependent and habitat-specific diel patterns of virus-host *** further implies that viruses serve as an ecologically important driver of bacterial diel dynamics across the ocean,highlighting the viral roles in bacterial ecological and biogeochemical processes in the ocean.

关键词： coastal ocean Marine

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A review on Bi_(2)WO_(6)-based photocatalysts synthesis, modification, and applications in environmental remediation, life medical, and clean energy

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Frontiers of Environmental Science & Engineering 2024年第7期18卷 87-108页

作者： Wei Mao Xuewu Shen Lixun Zhang Yang Liu Zehao Liu Yuntao Guan Guangdong Provincial Engineering Technology Research Center for Urban Water Cycle and Water Environment Safety Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China State Environmental Protection key laboratory of Microorganism Application and Risk Control School of EnvironmentTsinghua UniversityBeijing 100084China

Photocatalysis has emerged a promising strategy to remedy the current energy and environmental crisis due to its ability to directiy convert clean solar energy into chemical *** tungstate(Bi_(2)WO_(6))has been shown to be an excellent visible light response,a well-defined perovskite crystal structure,and an abundance of oxygen atoms(providing efficient channels for photogenerated carrier transfer)due to their suitable band gap,effective electron migration and separation,making them ideal *** has been extensively applied as photocatalyst in aspects including pollutant removal,carbon dioxide reduction,solar hydrogen production,ammonia synthesis by nitrogen photocatalytic reduction,and cancer *** this review,the fabrication and application of Bi_(2)WO_(6) in photocatalysis were comprehensively *** photocatalytic properties of BizwO-based materials were significantly enhanced by carbon modification,the construction of heterojunctions,and the atom doping to improve the photogenerated carrier migration rate,the number of surface active sites,and the photoexcitation ability of the *** addition,the potential development directions and the existing challenges to improve the photocatalytic performance of Bi_(2)WO_(6)-based materials were discussed.

关键词： Bismuth tungstate Synthesis and modification Photocatalytic application Environmental remediation Clean energy Medical science

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互花米草有利于我国海岸带蓝碳功能提升

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Science Bulletin 2024年第12期69卷 1991-2000页

作者：张靖凡毛德华刘纪化陈雅萍 Matthew Kirwan Christian Sanders 周金戈卢哲覃国铭黄幸运李慧焉恒琦焦念志苏纪兰王法明 Guangdong key laboratory of Applied Botany Xiaoliang Research Station of Tropical Coastal Ecosystemsthe CAS Engineering Laboratory for Ecological Restoration of Island and Coastal EcosystemsSouth China Botanical GardenChinese Academy of SciencesGuangzhou 510650China University of Chinese Academy of Sciences Beijing 100049China South China National Botanical Garden Chinese Academy of SciencesGuangzhou 510650China key laboratory of Wetland Ecology and Environment Northeast Institute of Geography and AgroecologyChinese Academy of SciencesChangchun 130102China Marine Research Institute Shandong UniversityQingdao 266237China School of Ecology Shenzhen Campus of Sun Yat-sen UniversityShenzhen 518107China Virginia Institute of Marine Science Gloucester PointVA 23062USA National Marine Science Centre School of EnvironmentScience and EngineeringSouthern Cross UniversityCoffs HarbourNSW 2450Australia Guangdong Eco-engineering Polytechnic Guangzhou 510520China carbon Neutral Innovation Research Center and Fujian key laboratory of Marine carbon sequestration Xiamen UniversityXiamen 361005China Second Institute of Oceanography State Oceanic AdministrationHangzhou 310012China Southern Marine Science and Engineering Guangdong laboratory(Zhuhai) Zhuhai 519082China School of Ecology and Environment Hainan UniversityHaikou 570228China

Spartina alterniflora has rapidly and extensively encroached on China's coastline over the past *** the coastal areas invaded by ***,at most 93%are ***,the effect of *** invasion on soil organic carbon(SOC)stocks of coastal mudflats has not been systematically studied on a national ***,we quantified the nationwide changes in SOC stocks in coastal mudflats associated with *** invasion between 1990 and *** found that *** invasion significantly enhanced SOC stocks in coastal ***,the benefit of *** invasion of coastal SOC stock may be weakened by continuing human *** found that *** invading mudflats added 2.3 Tg SOC stocks to China's coastal blue carbon,while 1.78 Tg SOC stocks were lost mainly due to human activities,resulted in a net SOC stock gain of 0.52 Tg *** findings overturned the traditionally thought that *** invasion would reduce ecosystem services by highlighting that the historical invasion of *** has broadly and consistently enhanced blue carbon stock in coastal China.

关键词： Spartina alterniflora invasion Mudflats China coastal wetland Blue carbon sequestration

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A survey of remote sensing-based aboveground biomass estimation methods in forest ecosystems

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International Journal of Digital Earth 2016年第1期9卷 63-105页

作者： Dengsheng Lu Qi Chen Guangxing Wang Lijuan Liu Guiying Li Emilio Moran Zhejiang Provincial key laboratory of carbon Cycling in Forest Ecosystems and carbon sequestration School of Environmental&Resource SciencesZhejiang A&F UniversityLin’AnChina Center for Global Change and Earth Observations Michigan State UniversityEast LansingMIUSA Department of Geography University of Hawaii at MānoaHonoluluHIUSA Department of Geography and Environmental Resources Southern Illinois University at CarbondaleCarbondaleILUSA

Remote sensing-based methods of aboveground biomass(AGB)estimation in forest ecosystems have gained increased attention,and substantial research has been conducted in the past three *** paper provides a survey of current biomass estimation methods using remote sensing data and discusses four critical issues–collection of field-based biomass reference data,extraction and selection of suitable variables from remote sensing data,identification of proper algorithms to develop biomass estimation models,and uncertainty analysis to refine the estimation ***,we discuss the impacts of scales on biomass estimation performance and describe a general biomass estimation *** optical sensor and radar data have been primary sources for AGB estimation,data saturation is an important factor resulting in estimation *** Detection and Ranging(lidar)can remove data saturation,but limited availability of lidar data prevents its extensive *** literature survey has indicated the limitations of using single-sensor data for biomass estimation and the importance of integrating multi-sensor/scale remote sensing data to produce accurate estimates over large *** research is needed to extract a vertical vegetation structure(*** height)from interferometry synthetic aperture radar(InSAR)or optical stereo images to incorporate it into horizontal structures(*** cover)in biomass estimation modeling.

关键词： aboveground biomass forest ecosystems parametric vs.nonparametric algorithms remote sensing uncertainty

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Recent Advances on Porous Materials for Synergetic Adsorption and Photocatalysis

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Energy & Environmental Materials 2022年第3期5卷 711-730页

作者： Tianqi Wang Bingbing Tian Bin Han Dingren Ma Mingzhe Sun Aamir Hanif Dehua Xia Jin Shang International Collaborative laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518060China School of Energy and Environment City University of Hong KongTat Chee AvenueKowloonHong Kong China Institute of Microscale Optoelectronics Shenzhen UniversityShenzhen 518060China key laboratory for City Cluster Environmental Safety and Green Development of the Ministry of Education Institute of Environmental and Ecological EngineeringGuangdong University of TechnologyGuangzhou 510006China School of Environmental Science and Engineering Sun Yat-Sen UniversityGuangzhou 510275China City University of Hong Kong shenzhen Research Institute Nanshan District8 Yuexing 1st RoadShenzhen Hi−Tech Industrial ParkShenzhen 518060China Department of Chemistry Islamic University of Science and TechnologyAwantipora 192122India

Porous photocatalysts are promising materials capable of simultaneously adsorbing and oxidizing/reducing target species,showing great potentials in environmental remediation and energy *** review offered a comprehensive overview of the recent progress in design,fabrication,and applications of porous photocatalysts,including carbon-based semiconductors,metal oxides/sulfides,metal–organic frameworks,and adsorbent–photocatalyst *** fundamental understanding of the structure–performance relationships of porous materials together with the in-depth insights into the synergetic effects between adsorption and photocatalysis was *** strategies to further improve the photocatalytic activity of porous photocatalysts were *** review would provide references and outlooks of constructing efficient porous materials for adsorptive and photocatalytic removal of pollutants and energy production.

关键词： adsorption photocatalysis porous materials synergetic effect

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Recent advances on electroactive CNT-based membranes for environmental applications:The perfect match of electrochemistry and membrane separation

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Chinese Chemical Letters 2020年第10期31卷 2539-2548页

作者： Yanbiao Liu Fuqiang Liu Ning Ding Xuemei Hu Chensi Shen Fang Li Manhong Huang Zhiwei Wang Wolfgang Sand Chong-Chen Wang Textile Pollution Controlling Engineering Center of Ministry of Environmental Protection College of Environmental Science and EngineeringDonghua UniversityShanghai 201620China Shanghai Institute of Pollution Control and ecological Security Shanghai 200092China key laboratory of Cleaner Production and Integrated Resource Utilization of China National Light Industry Beijing Technology and Business UniversityBeijing 100048China State key laboratory of Pollution Control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China Institute of Biosciences Freiberg University of Mining and TechnologyFreiberg 09599Germany Beijing key laboratory of Functional Materials for Building Structure and Environment remediation Beijing University of Civil Engineering and ArchitectureBeijing 100044China

Global climate change,growing population,and environmental pollution underscore the need for a greater focus on providing advanced water treatment *** electrochemical basedprocesses are becoming promising solutions,they still face challenges owing to mass transport and upscaling which hinder the exploitation of this *** design and reactor configuration are key factors for achieving operational *** electroactive membrane has proven to be a breakthrough technology integrating electrochemistry and membrane separation with an enhanced mass transport by *** this review article,we discuss recent progress in environmental applications of electroactive membranes with particular focus on those composed of carbon nanotubes(CNT)due to their intriguing physicochemical prope *** applications in degradation of refractory contaminants,detoxification and sequestration of toxic heavy metal ions,and membrane fouling alleviations are systematically *** then discuss the existing limitations and opportunities for future *** development of advanced electroactive systems depends on interdisciplinary collaborations in the areas of materials,electrochemistry,membrane development,and environmental sciences.

关键词： Electroactive membranes carbon nanotubes Organic pollutants Heavy mental ions Antifouling

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Coastal blue carbon in China as a nature-based solution toward carbon neutrality

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The Innovation 2023年第5期4卷 109-123页

作者： Faming Wang Jihua Liu Guoming Qin Jingfan Zhang Jinge Zhou Jingtao Wu Lulu Zhang Poonam Thapa Christian J.Sanders Isaac R.Santos Xiuzhen Li Guanghui Lin Qihao Weng Jianwu Tang Nianzhi Jiao Hai Ren Xiaoliang Research Station of Tropical Coastal Ecosystems Key Laboratory of Vegetation Restoration and Management of Degraded Ecosystemsand the CAS Engineering Laboratory for Ecological Restoration of lsland and Coastal EcosystemsSouth China Botanical GardenChinese Academy of SciencesGuangzhou 510650China Southern Marine Science and Engineering Guangdong laboratory(Guangzhou) Guangzhou 510650China Marine Research Institute Shandong UniversityQingdao 266237China University of Chinese Academy of Sciences Beijing 100049China National Marine Science Centre Faculty of Science and EngineeringSouther Cross UniversityCoffs HarbourNSW 2450Australia Department of Marine Sciences University of Gothenburg41319 GothenburgSweden State key laboratory of Estuarine and Coastal Research and Instiute of Eco-Chongming East China Normal UniversityShanghai 201100China key laboratory for Earth System Modeling Ministry of EducationDepartment of Earth System ScienceTsinghua UniversityBejing 100084China laboratory of Stable Isotope and Gulf Ecology Institute of Ocean EngineeringTsinghua's Shenzhen International Graduate SchoolShenzhen 518055China Department of Land Surveying and Geo-nformatics The Hong Kong Polytechnic UniversiyHongkong 99077China Innovative Research Center for carbon Neutralization Global ONCE ProgramXiamen 361005China

To achieve the Paris Agreement,China pledged to become“carbon Neutral”by the *** addition to massive decarbonization,this would require significant changes in ecosystems toward negative CO_(2)*** ability of coastal blue carbon ecosystems(BCEs),including mangrove,salt marsh,and seagrass meadows,to sequester large amounts of CO_(2)makes their conservation and restoration an important“nature-based solution(NbS)”for climate adaptation and *** this review,we examine how BCEs in China can contribute to climate *** the national scale,the BCEs in China store up to 118 Tg C across a total area of 1,440,377 ha,including over 75%as unvegetated tidal *** annual sedimental C burial of these BCEs reaches up to 2.06 Tg C year^(−1),of which most occurs in salt marshes and tidal *** lateral C flux of mangroves and salt marshes contributes to 1.17 Tg C year^(−1)along the Chinese *** and restoration of BCEs benefit climate change mitigation and provide other ecological services with a value of$32,000 ha^(−1)year^(−1).The potential practices and technologies that can be implemented in China to improve BCE C sequestration,including their constraints and feasibility,are also *** directions are suggested to improve blue carbon estimates on aerial extent,carbon stocks,sequestration,and mitigation *** and preserving BCEs would be a cost-effective step to achieve carbon Neutral by 2060 in China despite various barriers that should be removed.

关键词： tidal coastal carbon

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Eco-engineering approaches for ocean negative carbon emission

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Science Bulletin 2022年第24期67卷 2564-2573,M0004页

作者： Chuanlun Zhang Tuo Shi Jihua Liu Zhili He Helmuth Thomas Hailiang Dong Buki Rinkevich Yuze Wang Jung-Ho Hyun Markus Weinbauer Celeste López-Abbate Qichao Tu Shucheng Xie Youhei Yamashita Pavel Tishchenko Quanrui Chen Rui Zhang Nianzhi Jiao Southern Marine Science and Engineering Guangdong laboratory(Guangzhou) Guangzhou 511458China shenzhen key laboratory of Marine Geo-Omics Research Southern University of Science and TechnologyShenzhen 518055China Institute of Marine Science and Technology Shandong UniversityQingdao 266237China Environmental Microbiomics Research Center School of Environmental Science and EngineeringSouthern Marine Science and Engineering Guangdong LaboratorySun Yat-sen UniversityZhuhai 510006China Helmholtz-Center Hereon Institute of Carbon CyclesGeesthacht D-21502Germany Center for Geomicrobiology and Biogeochemistry Research State Key Laboratory of Biogeology and Environmental GeologyChina University of GeosciencesBeijing 100083China Israel Oceanographic&Limnological Research National Institute of OceanographyHaifa Tel Shikmona 3109701Israel Department of Ocean Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Marine Science and Convergence Engineering Hanyang University ERICA CampusAnsanGyeonggi-do 15588South Korea Laboratoire d’Océanographie de Villefranche(LOV) Sorbonne Université-CNRS UMR7093Institut de la Mer de Villefranche(IMEV)Villefranche BP28France Instituto Argentino de Oceanografía Consejo Nacional de Investigaciones Científicas y TécnicasBahía Blanca 8000Argentina State key laboratory of Biogeology and Environmental Geology China University of GeosciencesWuhan 430074China Faculty of Environmental Earth Science Hokkaido UniversityHokkaido 060-0810Japan V.I.Il’ichev Pacific Oceanological Institute Far Eastern BranchRussian Academy of SciencesVladivostok 690041Russia State key laboratory of Marine Environmental Science Institute of Marine Microbes and EcospheresCollege of Ocean and Earth SciencesXiamen UniversityXiamen 361102China

The goal of achieving carbon neutrality in the next 30-40 years is approaching worldwide consensus and requires coordinated efforts to combat the increasing threat of climate *** main sets of actions have been proposed to address this grand *** is to reduce anthropogenic CO2emissions to the atmosphere,and the other is to increase carbon sinks or negative emissions,i.e.,removing CO2from the *** we advocate eco-engineering approaches for ocean negative carbon emission(ONCE),aiming to enhance carbon sinks in the marine *** international program is being established to promote coordinated efforts in developing ONCE-relevant strategies and methodologies,taking into consideration ecological/biogeochemical processes and mechanisms related to different forms of carbon(inorganic/organic,biotic/abiotic,particulate/dissolved) for *** focus on marine ecosystem-based approaches and pay special attention to mechanisms that require transformative research,including those elucidating interactions between the biological pump(BP),the microbial carbon pump(MCP),and microbially induced carbonate precipitation(MICP).Eutrophic estuaries,hypoxic and anoxic waters,coral reef ecosystems,as well as aquaculture areas are particularly considered in the context of efforts to increase their capacity as carbon *** approaches are thus expected to be beneficial for both carbon sequestration and alleviation of environmental stresses.

关键词： carbon neutrality Ocean negative carbon emission Biological pump Microbial carbon pump Microbially induced carbonate precipitation Ocean alkalinity

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