Methane and nitrous oxide emissions from municipal wastewater treatment plants in China:A plant-level and technology-specific study
作者机构:School of Civil and Environmental EngineeringHarbin Institute of TechnologyShenzhen518055China Shenzhen Key Laboratory of Ecological Remediation and Carbon SequestrationInstitute of Environment and EcologyTsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen518055China Ministry of Education Key Laboratory for Earth System ModelingDepartment of Earth System ScienceTsinghua UniversityBeijing100084China State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing100084China
出 版 物:《Environmental Science and Ecotechnology》 (环境科学与生态技术(英文))
年 卷 期:2024年第20卷第4期
页 面:123-130页
核心收录:
学科分类:083002[工学-环境工程] 0830[工学-环境科学与工程(可授工学、理学、农学学位)] 08[工学]
基 金:supported by the Shenzhen Science and Technology Innovation Commission(No.RCBS20210609103731062,No.WDZC20220810110301001) Guangdong Basic and Applied Basic Research Foundation(No.2021A1515110887) H.L.acknowledge additional support from the Shenzhen Overseas High-Level Talent Project
主 题:Methane Nitrous oxide Emissions Municipal wastewater treatment plants
摘 要:Wastewater treatment is an important source of greenhouse gases(GHGs).Yet large uncertainties remain in the quantification of GHG emissions from municipal wastewater treatment plants(MWWTPs)in China.A high-resolution and technology-specific emission inventory is still lacking to support mitigation strategies of *** we develop a plant-level and technology-based MWWTP emission inventory for China covering 8703 plants and 19 treatment technology categories by compiling and harmonizing the most up-to-date facility-level *** s methane(CH_(4))and nitrous oxide(N_(2)O)emissions from MWWTPs in 2020 are estimated to be 150.6 Gg and 22.0 Gg,respectively,with the uncertainty range of-30%to 37%and-30%to 26%at 95%confidence *** find an emission inequality across cities,with the richest cities emitting two times more CH_(4)and N_(2)O per capita from municipal wastewater treatment than the poorest *** emitted CH_(4)and N_(2)O are dominated by Anaerobic/Anoxic/Oxic-,Sequencing Batch Reactor-,Oxidation Ditch-,and Anoxic/Oxic-based MWWTPs of less than 20 years *** the relatively young age structure of China s MWWTPs,the committed emissions highlight the importance of reducing on-site GHG emissions by optimization of operating conditions and innovation *** emission differences among our estimates,previous studies,and the Intergovernmental Panel on Climate Change guidelines are largely attributed to the uncertainties in emission factors,implying the urgent need for more plant-integrated measurements to improve the accuracy of emission accounting.