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Tunning the bandgap of MnO_(2)homojunction by building active high-index facet to achieve rapid electron transfer for enhanced photocatalytic sterilization

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Journal of Materials science & Technology 2024年第1期168卷 265-275页

作者： Tao Zhang Bo Li Chaofeng Wang Shuilin Wu Shengli Zhu Hui Jiang Yufeng Zheng Zhaoyang Li Zhenduo Cui Yu Zhang Paul K Chu Xiangmei Liu biomedical Materials engineering Research Center Hubei Key Laboratory of Polymer MaterialsMinistry-of-Education Key Laboratory for the Green Preparation and Application of Functional MaterialsSchool of Materials Science and Engineering Hubei UniversityWuhan 430062China school of health science&biomedical engineering Hebei University of TechnologyTianjin 300401China school of Materials science&engineering Peking UniversityBeijing 100871China school of Materials science&engineering the Key Laboratory of Advanced Ceramics and Machining Technology by the Ministry of Education of ChinaTianjin UniversityTianjin 300072China Department of Orthopedics Guangdong Provincial People’s HospitalGuangdong Academy of Medical SciencesGuangzhou 510080China Department of Physics Department of Materials Science and Engineering and Department of Biomedical EngineeringCity University of Hong KongHong Kong 999077China

Photocatalysis has been a research hotspot in recent years,and the design and modification of photocat-alysts have been the key *** methods for designing photocatalysts,including constructing heterojunctions and homojunctions,have been developed on the basis of *** this study,two homojunctions of manganese dioxide(MnO_(2)),including a high-index crystal plane homojunction and a general homojunction,are prepared using a stepwise hydrothermal *** a capping agent,the high-index crystal surface of the MnO_(2)is *** is found that the electron transport efficiency be-tween the two components of the homojunction with high-index planes is higher and the adsorption capacity of the oxygen is stronger,which leads to higher photocatalytic *** addition,the newly designed high-index homojunction is used for the treatment of bacterial infections,and it kills Staphy-lococcus aureus(***)and Escherichia coli(***)at rates of 99.95%±0.04%and 99.31%±0.25%,*** also has excellent therapeutic effects on mouse wounds,which implies superb practical application *** work provides a new strategy for the improved design of homojunctions and the application of photocatalytic materials.

关键词： Photocatalysis Homojunction Bandgap High-index facet Antibacterial

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Laser speckle contrast imaging based on uniting spatiotemporal Fourier transform

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Chinese Optics Letters 2024年第1期22卷 98-104页

作者：翟林君杜永兆吴循循刁勇傅玉青 school of biomedical science Huaqiao UniversityQuanzhou 362021China College of engineering Huaqiao UniversityQuanzhou 362021China

We propose a laser speckle contrast imaging method based on uniting spatiotemporal Fourier ***,the raw speckle images are entirely transformed to the spatiotemporal frequency domain with a three-dimensional(3D)fast Fourier ***,the dynamic and static speckle components are extracted by applying 3D low-pass and high-pass filtering in the spatiotemporal frequency domain and inverse 3D Fourier ***,we calculate the time-averaged modulation depth with the average of both components to map the two-dimensional blood flow *** experiments demonstrate that the proposed method could effectively improve computational efficiency and imaging quality.

关键词： uniting spatiotemporal Fourier transform laser speckle contrast image fluctuation modulation 3D Fourier transform

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Tuning the diffusion constant to optimize the readout of positional information of spatial concentration patterns

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Chinese Physics B 2024年第8期33卷 579-586页

作者：江嘉杰罗春雄刘峰 The State Key Laboratory for Artificial Microstructures and Mesoscopic Physics School of PhysicsPeking UniversityBeijing 100871China Center for Quantitative Biology Peking UniversityBeijing 100871China Wenzhou Institute University of Chinese Academy of sciences Wenzhou 325001China Key Laboratory of Hebei Province for Molecular Biophysics Institute of BiophysicsSchool of Health Science&Biomedical EngineeringHebei University of TechnologyTianjin 300130China

Positional information encoded in spatial concentration patterns is crucial for the development of multicellular ***,it is still unclear how such information is affected by the physically dissipative diffusion *** we study one-dimensional patterning systems with analytical derivation and numerical *** find that the diffusion constant of the patterning molecules exhibits a nonmonotonic effect on the readout of the positional information from the concentration ***,there exists an optimal diffusion constant that maximizes the positional ***,we find that the energy dissipation due to the physical diffusion imposes a fundamental upper limit on the positional information.

关键词： pattern formation positional information mutual information diffusion

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Experimental realization of fractal fretwork metasurface for sound anomalous modulation

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Chinese Physics B 2024年第5期33卷 473-478页

作者：何佳杰于书萌江雪他得安 Department of biomedical engineering School of Information Science and TechnologyFudan UniversityShanghai 200433China Academy for engineering and Technology Fudan UniversityShanghai 200433China

Natural creatures and ancient cultures are full of potential sources to provide inspiration for applied *** by the fractal geometry in nature and the fretwork frame in ancient culture,here we design the acoustic metasurface to realize sound anomalous modulation,which manifests itself as an incident-dependent propagation behavior:sound wave propagating in the forward direction is allowed to transmit with high efficiency while in the backward direction is obviously *** quantitatively investigate the dependences of asymmetric transmission on the propagation direction,incident angle and operating frequency by calculating sound transmittance and energy *** compact fractal fretwork metasurface for acoustic anomalous modulation would promote the development of integrated acoustic devices and expand versatile applications in acoustic communication and information encryption.

关键词： acoustic metasurface fractal geometry sound anomalous modulation

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Effect of mechanical stresses on degradation behavior of high-purity magnesium in bone environments

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Journal of Materials science & Technology 2024年第4期171卷 252-261页

作者： Yan Yao Jie Xia Lizhen Wang Yuanming Gao Xili Ding Chao Wang Yubo Fan Key Laboratory of Biomechanics and Mechanobiology(Beihang University) Ministry of EducationBeijing Advanced Innovation Center for Biomedical EngineeringSchool of Biological Science and Medical EngineeringSchool of Engineering MedicineBeihang UniversityBeijing 100083China

High-purity(HP)magnesium(Mg)has emerged as a promising biomaterial for supporting functional bone *** previous study found that mechanical stresses and the surrounding fibrotic tissue(subcuta-neous)both play crucial roles in the degradation of HP ***,due to challenges in the degradation and regeneration process in vivo,it remains unclear how stress affects HP Mg degradation in bone en-vironments,limiting its further *** this study,novel loading devices were designed and the effects of tensile and compressive stresses on HP Mg degradation in vivo and in vitro bone environments were quantitatively *** addition,bone osteointegration around HP Mg was explored *** stress increases the degradation rate of HP Mg in vivo and in *** Mg degradation in vivo is more sensitive to stress factors than in vitro,but the sensitivity decreases with corrosion *** volume loss rate of HP Mg is multilinear with the applied stress and degradation *** volume of bone tissue surrounding HP Mg is larger in the no-stress group compared to the stressed groups,which is more pronounced with increasing implantation *** results provide valuable insights for optimiz-ing the design of HP Mg-based implants considering load *** will help to achieve a balance between the degradation rate of the implant and the regeneration rate of the surrounding bone.

关键词： High-purity magnesium Quantitative stresses Degradation Bone environments In vivo and in vitro

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In situ and on-line monitoring of cadmium in soil pore water using an automatic sampling integrated electrochemical sensor

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science China(Technological sciences) 2024年第9期67卷 2894-2904页

作者： KUANG JiaJie WEN JunLin CAI XiXi ZHOU LiHua YUAN Yong Guangdong Key Laboratory of Environmental Catalysis and health Risk Control School of Environmental Science and EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China school of biomedical and Pharmaceutical sciences Guangdong University of TechnologyGuangzhou 510006China

Cadmium(Cd) contamination in soil pore water is the primary pathway for Cd uptake by food crops,such as rice(Oryza sativa L.),posing significant risks to both food safety and human *** study presents a novel soil pore water metal sensor(SPW-Msensor) for in situ and online monitoring of Cd in soil pore water(Cd_(pw)).The SPW-Msensor integrates an automated sampling device,comprising a Rhizon sampler and a reciprocating series pump with an independent dual plunger drive,along with a portable electrochemical sensor consisting of a screen-printed electrode,flow cell,and portable *** SPW-Msensor enables the detection of Cd within a linear range of 50 to 300 ppb while exhibiting high anti-interference ***,it demonstrates excellent repeatability(relative standard deviation values(RSDs)<3.6%) across 30 measurements conducted within a 2-h *** method exhibits good agreement with results obtained using the standard ICP-MS method(RSDs<5%).Additionally,this study establishes a positive correlation between Cd_(pw)detected by the SPW-Msensor and total Cd concentration(Cd_(total)) in the soil with an R^(2) value equal to *** acquired from the SPW-Msensor can be utilized for predicting Cd_(total)through partial least squares regression modeling,achieving model quality score(Q^(2)) of 0.69,adjusted R^(2) of 0.9345,and root mean square error(RMSE) of *** SPW-Msensor demonstrates real-time monitoring capabilities for assessing Cd levels in acidified *** SPW-Msensor offers an efficient approach for in-situ and continuous monitoring of Cd_(pw)that provides valuable insights applicable to environmental and agricultural domains.

关键词： cadmium pore water electrochemical sensor in-situ monitoring soil

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Aberration correction for deformable-mirror-based remote focusing enables high-accuracy whole-cell super-resolution imaging

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Photonics Research 2024年第4期12卷 821-832页

作者： WEI SHI YINGCHUAN HE JIANLIN WANG LULU ZHOU JIANWEI CHEN LIWEI ZHOU ZEYU XI ZHEN WANG KE FANG YIMING LI Department of biomedical engineering Southern University of Science and TechnologyShenzhen 518055China

Single-molecule localization microscopy(SMLM)enables three-dimensional(3D)investigation of nanoscale structures in biological samples,offering unique insights into their ***,traditional 3D super-resolution microscopy using high numerical aperture(NA)objectives is limited by imaging depth of field(DOF),restricting their practical application to relatively thin biological ***,we developed a unified solution for thick sample super-resolution imaging using a deformable mirror(DM)which served for fast remote focusing,optimized point spread function(PSF)engineering,and accurate aberration *** effectively correcting the system aberrations introduced during remote focusing and sample aberrations at different imaging depths,we achieved high-accuracy,large DOF imaging(~8μm)of the whole-cell organelles[i.e.,nuclear pore complex(NPC),microtubules,and mitochondria]with a nearly uniform resolution of approximately 35 nm across the entire cellular volume.

关键词： enable mirror resolution

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Dynamic recrystallization mechanism, texture evolution development and mechanical characteristics of a Mg–8.7Gd–4.18Y–0.42Zr magnesium alloy by ECAP

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Progress in Natural science:Materials International 2024年第2期34卷 376-388页

作者： Ling Zhang Yinglong Li school of Materials science and engineering Northeastern University school of Mechanical and engineering Ningxia Institute of Science and Technology

Equal channel angle pressing is recognized for its ability to refine alloy grains and alter grain orientation, thereby achieve better mechanical performance of the magnesium alloy. This study investigates the microstructures,dynamic recrystallization mechanism, texture development, and mechanical performance of GW94K(Mg–8.7Gd–4.18Y–0.42Zr wt. %) Mg alloy following ECAP-4 passes at 400°C and 3 mm/min. Results show that when high-temperature deformation is undertaken, twin formation is suppressed while dislocation slip is facilitated, increasing dislocation density during deformation. Following ECAP deformation, the sample displayed higher fracture elongation, TYS, and UTS than the as-solutioned GW94K alloy. In particular, the GW94K alloy performed well mechanically after ECAP-4 passes, with an ultimate TYS of 231 MPa, an UTS of 290 MPa, and an elongation of 14.8 %. DDRX and shear bands induce CDRX, both of which are important in plastic deformation. as well as in modifying microstructure and grain orientation during ECAP deformation.

关键词： Dynamic recrystallization mechanism Equal channel angular pressing Magnesium alloy Mechanical performance Mg-Gd-Y-Zr alloy Texture development

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Multi-focus non-periodic scanning method for femtosecond lasers based on DMD and galvanometer scanners[Invited]

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Chinese Optics Letters 2024年第5期22卷 89-94页

作者：李华明王雨胡庆磊张卓宇吕晓华曾绍群 Britton Chance Center for biomedical Photonics Wuhan National Laboratory for OptoelectronicsHuazhong University of Science and TechnologyWuhan 430074China MOE Key Laboratory for biomedical Photonics Collaborative Innovation Center for Biomedical EngineeringSchool of Engineering SciencesHuazhong University of Science and TechnologyWuhan 430074China

Multi-focus parallel scanning can effectively increase laser fabrication ***,the conventional approach of using a spatial light modulator(SLM)to generate multi-foci and scan this fixed number of foci with galvanometer scanners can only achieve a periodic scanning trajectory due to the low switching speed of the *** we demonstrate a multifocus non-periodic scanning method for femtosecond lasers by using,instead,a fast-switching digital micromirror device(DMD)to generate a dynamic number of *** number of effective foci is quickly switched by introducing aberration to the undesired *** this way,the intensity allocated to each focus will not be affected by the number of foci,and a uniformity of 98%with different numbers of foci is achieved without adjusting the total laser ***,we validate the effectiveness of this scanning method by demonstrating corneal flap fabrication of porcine cornea in vitro.

关键词： multi-focus non-periodic trajectory digital micromirror device aberration control corneal cutting

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Thin-film flow technology in controlling the organization of materials and their properties Special Collection:Distinguished Australian Researchers

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Aggregate 2024年第1期5卷 115-129页

作者： Clarence Chuah Xuan Luo Javad Tavakoli Youhong Tang Colin L.Raston Flinders Institute for Nanoscale science and Technology College of Science and EngineeringFlinders UniversityAdelaideSouth AustraliaAustralia Centre for health Technologies School of Biomedical EngineeringFaculty of Engineering and Information TechnologyUniversity of Technology SydneySydneyNew South WalesAustralia

Centrifugal and shear forces are produced when solids or liquids *** systems and devices that use these forces,such as dynamic thin-film flow technology,are evolving continuously,improve material structure-property relationships at the nanoscale,representing a rapidly thriving and expanding field of research high with green chemistry metrics,consolidated at the inception of *** vortex fluidic device(VFD)provides many advantages over conventional batch processing,with fluidic waves causing high shear and producing large surface areas for micro-mixing as well as rapid mass and heat transfer,enabling reactions beyond diffusion *** these abilities allows for a green and innovative approach to altering materials for various research and industry applications by controlling small-scale flows and regulating molecular and macromolecular chemical reactivity,self-organization phenomena,and the synthesis of novel *** review highlights the aptitude of the VFD as clean technology,with an increase in efficiency for a diversity of top-down,bottom-up,and novel material transformations which benefit from effective vortex-based processing to control material structure-property relationships.

关键词： material nanoscale structure-property relationship thin film flow technology vortex fluidic device

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