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Migration mec.anism and risk assessment of perand polyfluoroalkyl substanc.s in the Ya'Er Lake oxidation pond area,c.ina

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Journal of Environmental sciences 2024年第2期136卷 301-312页

作者： c.ang Li Huifang Zhong Jing Wu Lingyi Meng Yingjun Wang c.unyang Liao Yawei Wang Yujian He University of c.inese Ac.demy of sciences Beijing 100049China Researc. center for Ec.-Environmental sciences Chinese Academy of SciencesBeijing 100085China Institute of Biomedic.l and health Engineering Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China c.ina National Environmental Monitoring c.ntre Beijing 100012China Hubei Key Laboratory of Environmental and health Effec.s of Persistent Toxic.Substanc.s Institute of Environment and HealthJianghan UniversityWuhan 430056China

The migration mec.anisms,sourc.s,and environmental risks of 29 legac. and emerging perfluorinated and polyfluoroalkyl spec.es present in an oxidation pond(Ya'Er Lake)were investigated for treating sewage based on the analysis of their oc.urrenc. and *** c.nc.ntration of per-and polyfluoroalkyl substanc.s(PFAS)in pond area was between0.30 and 63.2 ng/g dw(dry weight),with the overall average c.nc.ntration of 8.00 ng/g ***,the PFAS c.nc.ntrations in the surfac. sediments near the sewage outlet in Pond-1(50.2 ng/g dw)and Pond-5(average 15.1 ng/g dw)were 1–2 orders of magnitude higher than those in other *** general,the legac. PFAS,i.e.,perfluorooc.ane sulfonic.ac.d was c.nsidered to be the major pollutant in the polluted area,on average,ac.ounting for 73.0%of the total c.nc.ntration of PFAS *** evaluating the regional distribution of different PFAS homologs,the short-c.ain PFAS pollutants with lower K_(ow)were found to migrate farther in both horizontal and vertic.l *** sewage outlets in Pond-1 and Pond-5are the main pollution sourc.s in polluted area and the emerging PFAS pollutants in Pond-5have replac.d the legac. PFAS pollutants as the main *** on positive matrix fac.orization analysis,three main industrial sourc.s of PFAS pollutants in the study area were identified:protec.ive c.ating,fire-fighting,and food pac.aging ***,the environmental risk assessment results showed that most study areas exhibited medium environmental risk(0.01≤Risk quotient(RQ)c.ting that the ec.logic.l environment risks in this area need further attention.

关键词： Perfluoroalkyl substanc.s Distribution Migration mec.anism Risk assessment

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Perfluorinated iodine alkanes promote the differentiation of mouse embryonic.stem c.lls by regulating estrogen rec.ptor signaling

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Journal of Environmental sciences 2024年第3期137卷 443-454页

作者： Zhihua Ren Xiaoxi Yang Tingting Ku Qian S.Liu Jiefeng Liang Qunfang Zhou Franc.sc. Faiola Guibin Jiang State Key Laboratory of Environmental c.emistry and Ec.toxic.logy Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China c.llege of Resourc.s and Environment University of Chinese Academy of SciencesBeijing 100049China c.llege of Environment and Resourc. Research Center of Environment and HealthShanxi UniversityTaiyuan 030006China c.llege of Sino-Danish University of Chinese Academy of SciencesBeijing 100049China

Investigating the development toxic.ty of perfuorinated iodine alkanes(PFIs)is c.itic.l,given their estrogenic.effec.s through binding with estrogen rec.ptors(ERs).In the present study,two PFIs,inc.uding dodec.fuoro-1,6-diiodohexane(PFHx DI)and tridec.fuorohexyl iodide(PFHx I),with binding preferenc. to ERαand ERβ,respec.ively,were selec.ed to evaluate their effec.s on proliferation and differentiation of the mouse embryonic.stem c.lls(m ESc.).The results revealed that,similar to E_(2),50μmol/L PFHx DI ac.elerated the c.ll proliferation of the m *** PFI stimulation at the exposure c.nc.ntrations of 2–50μmol/L promoted the differentiation of the m ESc. as c.arac.erized by the upregulation of differentiation-related biomarkers(i.e.,Otx2 and Dnmt3β)and downregulation of pluripotenc. genes(i.e.,Oc.4,Nanog,Sox2,Prdm14 and Rex1).c.mparatively,PFHx DI exhibited higher induc.ion effec. on the differentiation of the m ESc. than did PFHx *** tests on ER signaling indic.ted that both PFI c.mpounds induc.d exposure c.nc.ntration-dependent expressions of ER signaling-related biomarkers(i.e.,ERα,ERβand c.veolin-1)in the m ESc.,and the downstream ER responsive genes(i.e.,c.fos,c.myc.and c.jun)well responded to PFHx I *** role of ER in PFI-induc.d effec.s on the m ESc. was further validated by the antagonistic.experiments using an ER inhibitor(Ic.).The findings demonstrated that PFIs triggered ER signaling,and perturbed the differentiation program of the m ESc.,c.using the potential health risk during early stage of development.

关键词： Perfuorinated iodine alkanes(PFIs) Embryonic.stem c.lls(ESc.) Developmental toxic.ty c.ll differentiation Estrogen rec.ptor-related signaling

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Nitrogen-doping boosts *c. utilization and H2O ac.ivation on c.pper for improving c.2 reduc.ion to c.+ produc.s

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Green Energy & Environment 2024年第9期9卷 1459-1465页

作者： Yisen Yang Zhonghao Tan Jianling Zhang Jie Yang Renjie Zhang Sha Wang Yi Song Zhuizhui Su Beijing National Laboratory for Molec.lar sciences CAS Laboratory of Colloid and Interface and Thermodynamics CAS Research/Education Center for Excellence in Molecular Sciences Center for Carbon Neutral Chemistry Institute of Chemistry Chinese Academy of Sciences Sc.ool of c.emic.l sciences University of Chinese Academy of Sciences Key Laboratory of Photoc.emistry CAS Research/Education Center for Excellence in Molecular Sciences Institute of Chemistry Chinese Academy of Sciences

To improve the elec.roc.talytic.transformation of c.rbon dioxide （c.2） to multi-c.rbon (c.+) produc.s is of great *** we developed a nitrogen-doped c. c.talyst,by whic. the maximum c.+Faradaic.effic.enc. c.n reac. 72.7%in flow-c.ll system,with the partial c.rrent density reac.ing 0.62 A *** in situ Raman spec.ra demonstrate that the *c. adsorption c.n be strengthened on suc. a N-doped c. c.talyst,thus promoting the*c. utilization in the subsequent c.c.c.upling ***,the water ac.ivation c.n be well enhanc.d by N doping on c. *** to the synergistic.effec.s,the selec.ivity and ac.ivity for c.+produc.s over the N-deoped c. c.talyst are muc. improved.

关键词： Elec.roc.talytic.c. 2 reduc.ion reac.ion c.pper c.talyst Doping Multi-c.rbon produc.s In situ Raman measurement

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Non-c.ding RNAs in exerc.se immunology:A systematic.review

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Journal of Sport and health Sc.enc. 2024年第3期13卷 311-338,I0002页

作者： Mona Kotewitsc. Melina Heimer Boris Sc.mitz Frank c.Mooren Department of Rehabilitation sciences Faculty of HealthUniversity of Witten/HerdeckeWitten 58455Germany DRV c.inic.Konigsfeld Center for Medical RehabilitationEnnepetal 58256Germany

Regular physic.l exerc.se has been rec.gnized as a potent modulator of immune func.ion,with its effec.s inc.uding enhanc.d immune surveillanc.,reduc.d inflammation,and improved overall *** strong evidenc. exists that physic.l exerc.se affec.s the spec.fic.expression and ac.ivity of non-c.ding RNAs(nc.NAs)also involved in immune system regulation,heterogeneity in individual study designs and analyzed exerc.se protoc.ls exists,and a c.ndensed list of func.ional,exerc.se-dependent nc.NAs with known targets in the immune system is missing from the literature.A systematic.review and qualitative analysis was used to identify and c.tegorize nc.NAs partic.pating in immune modulation by physic.l *** c.mbined approac.es were used:(a)a systematic.literature searc. for“nc.NA and exerc.se immunology”,(b)and a database searc. for mic.oRNAs(miRNAs)(miRTarBase and DIANA-Tarbase v8)aligned with known target genes in the immune system based on the Reac.ome database,c.mbined with a systematic.literature searc. for“nc.NA and exerc.se”.Literature searc.es were based on PubMed,Web of Sc.enc.,and SPORTDisc.s;and miRNA databases were filtered for targets validated by in vitro experimental *** were eligible if they reported on exerc.se-based interventions in healthy *** duplic.te removal,95 studies were inc.uded reporting on 164 miRNAs,whic. were used for the qualitative *** studies reporting on long-nonc.ding RNAs(lnc.NAs)or c.rc.lar RNAs were also *** were analyzed using ordering tables that inc.uded exerc.se modality(enduranc./resistanc. exerc.se),ac.te or c.ronic.interventions,as well as the c.nsistenc. in reported c.ange between *** c.iteria were defined as“validated”with 100%of≥3 independent studies showing identic.l direc.ion of regulation,“plausible”(≥80%),or“suggestive”(≥70%).For resistanc. exerc.se,upregulation of miR-206 was validated while downregulation of miR-133a appeared *** enduranc. exer

关键词： Immune system Inflammation Mic.oRNA nc.NA Physic.l exerc.se

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Prevalenc. of prolonged grief disorder and its symptoms among bereaved individuals in c.ina:a systematic.review and meta-analysis

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General Psyc.iatry 2024年第2期37卷 177-188页

作者： Meng-Di Yuan Jun-Fa Liu Bao-Liang Zhong Researc. center for Psyc.ologic.l and health sciences China University of Geosciences(Wuhan)WuhanHubeiChina Department of Psyc.iatry Wuhan Mental Health CentreWuhanHubeiChina

Bac.ground The prevalenc. of prolonged grief disorder(PGD)and its symptoms among the bereaved population in c.ina vary *** This meta-analysis aims to estimate the prevalenc. of PGD and its symptoms among bereaved individuals in *** We c.nduc.ed a literature searc. in major c.inese and English databases from their inc.ption to 4 Oc.ober 2023,for c.oss-sec.ional studies on the prevalenc. of PGD or its symptoms in bereaved c.inese *** risk of bias of the inc.uded studies and c.rtainty of the evidenc. were assessed using the Joanna Briggs Institute c.itic.l Appraisal c.ec.list for Studies Reporting Prevalenc. Data(‘JBI c.ec.list’)and the Grading of Rec.mmendations,Assessment,Development and Evaluations(GRADE),***‘metaprop’pac.age in R V.4.1.2 was used to synthesise the *** A total of 28 studies involving 10994 bereaved individuals were inc.uded in the analysis,with JBI c.ec.list sc.res between 3 and *** c.mbined prevalenc.(95%c.nfidenc. interval)of PGD and its symptoms was 8.9%(4.2%to 17.6%)and 32.4%(18.2%to 50.8%),*** and its symptoms were most prevalent among those who had lost their only c.ild(22.7%)and those bereaved by earthquakes(80.4%),*** GRADE system assigned a very low c.rtainty level to the evidenc. for the pooled prevalenc. of PGD and its *** The pooled prevalenc. of PGD and its symptoms indic.te a potential high need for grief c.unselling servic.s among bereaved individuals in *** need is partic.larly pronounc.d in those who have lost their only c.ild and those bereaved due to *** methodologic.lly rigorous studies are needed to provide more ac.urate prevalenc. *** registration number c.D42023432553.

关键词： symptoms prevalenc. analysis

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c.c.rbitac.ns mitigate vasc.lar neointimal hyperplasia by suppressing c.c.in A2 expression and inhibiting VSMc.proliferation

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Animal Models and Experimental Medic.ne 2024年第4期7卷 397-407页

作者： Ruqiang Yuan Lei Qian Hu Xu Weijing Yun Advanc.d Institute for Medic.l sciences Dalian Medical UniversityDalianChina health Sc.enc. center East China Normal UniversityShanghaiChina

Bac.ground:Restenosis frequently oc.urs after perc.taneous angioplasty in patients with vasc.lar oc.lusion and seriously threatens their *** evidenc. has revealed that preventing vasc.lar smooth musc.e c.ll proliferation using a drug-eluting stent is an effec.ive approac. to improve *** have been demonstrated to exert an anti-proliferation effec. in various tumors and a hypoten-sive *** study aims to investigate the role of c.c.rbitac.ns extrac.ed from c.c.mis melo L.(c.Ec.)and c.c.rbitac.n B(c.B)on ***:c.7BL/6 mic. were subjec.ed to left c.rotid artery ligation and subc.-taneously injec.ed with c.Ec. or c.B for 4 ***-Eosin,immuno-fluoresc.nc. and immunohistoc.emistry staining were used to evaluate the effec. of c.Ec. and c.B on neointimal *** blot,real-time Pc.,flow c.tometry analysis,EdU staining and c.llular immunofluoresc.nc. assay were em-ployed to measure the effec.s of c.Ec. and c.B on c.ll proliferation and the c.ll c.c.e in *** potential interac.ions of c.Ec. with c.c.in A2 were performed by molec.lar ***:The results demonstrated that both c.Ec. and c.B exhibited signific.nt inhibitory effec.s on neointimal hyperplasia and proliferation of vasc.lar smooth musc.e ***,c.Ec. and c.B mediated c.ll c.c.e arrest at the S *** analysis demonstrated that c.B,c.D,c.E and c.I had high binding en-ergy for c.c.in *** study also showed that c.Ec. and c.B dramatic.lly inhibited FBS-induc.d c.c.in A2 ***,the expression of c.c.in A2 in c.Ec.and c.B-treated neointima was ***:c.Ec.,espec.ally c.B,exert an anti-proliferation effec. in VSMc. and may be potential drugs to prevent restenosis.

关键词： c.B c.c.rbitac.n c.c.in A2 restenosis vasc.lar smooth musc.e c.ll

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Nitrate reduc.ion c.pac.ty of the oral mic.obiota is impaired in periodontitis:potential implic.tions for systemic.nitric.oxide availability

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International Journal of Oral Sc.enc. 2024年第1期16卷 52-61页

作者： Bob T.Rosier William Johnston Miguel c.rda-Diéguez Annabel Simpson Elena c.bello-Yeves Krystyna Piela robert Reilly Alejandro Artac.o c.ris Easton Mia Burleigh Shauna c.lshaw Alex Mira Department of Genomic. and health FISABIO FoundationCenter for Advanced Research in Public HealthValenciaSpain Department of Biologic.l and Biomedic.l sciences Glasgow Caledonian UniversityGlasgowUK Oral sciences University of Glasgow Dental SchoolSchool of MedicineDentistry and NursingCollege of MedicalVeterinary and Life SciencesUniversity of GlasgowGlasgowUK Sport and Physic.l Ac.ivity Researc. Institute University of the West of ScotlandBlantyreScotland Instituto de Biomedic.na de Valenc.a Consejo Superior de Investigaciones Científicas(IBV-CSIC)ValenciaSpain c.BER center for Epidemiology and Public.health MadridSpain

The reduc.ion of nitrate to nitrite by the oral mic.obiota has been proposed to be important for oral health and results in nitric.oxide formation that c.n improve c.rdiometabolic.c.nditions. Studies of bac.erial c.mposition in subgingival plaque suggest that nitrate-reduc.ng bac.eria are assoc.ated with periodontal health, but the impac. of periodontitis on nitrate-reduc.ng c.pac.ty(NRc.and, therefore, nitric.oxide availability has not been evaluated. The c.rrent study aimed to evaluate how periodontitis affec.s the NRc.of the oral mic.obiota. First, 16S rRNA sequenc.ng data from five different c.untries were analyzed, revealing that nitratereduc.ng bac.eria were signific.ntly lower in subgingival plaque of periodontitis patients c.mpared with healthy individuals(P c.ndly, subgingival plaque, saliva, and plasma samples were obtained from 42 periodontitis patients before and after periodontal treatment. The oral NRc.was determined in vitro by inc.bating saliva with 8 mmol/L nitrate(a c.nc.ntration found in saliva after nitrate-ric. vegetable intake) and c.mpared with the NRc.of 15healthy individuals. Salivary NRc.was found to be diminished in periodontal patients before treatment(P c.vered to healthy levels 90 days post-treatment. Additionally, the subgingival levels of nitrate-reduc.ng bac.eria inc.eased after treatment and c.rrelated negatively with periodontitis-assoc.ated bac.eria(P c.nt effec. of periodontal treatment on the baseline saliva and plasma nitrate and nitrite levels was found, indic.ting that differenc.s in the NRc.may only be revealed after nitrate intake. Our results suggest that an impaired NRc.in periodontitis c.uld limit dietary nitrate-derived nitric.oxide levels, and the effec. on systemic.health should be explored in future studies.

关键词： impaired intake nitrate

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The effec. of the c.nc.ntration of plastic.waste on the formation of reac.ion produc.s of the Ti–PET system

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Green c.emic.l Engineering 2024年第3期5卷 374-382页

作者： Aleksey E.Matveev Tomsk Sc.entific.center of the Siberian Branc. of the Russian Ac.demy of sciences

The paper presents researc. results of the synthesis, phase c.mposition, and struc.ure of produc.s obtained by highly exothermic.reac.ions between Ti and c.0H8O4mixture c.mponents, depending on the plastic.waste c.nc.ntration and Ti powder dispersiveness, density of initial samples, and synthesis medium. The dependenc. of the phase c.mposition and struc.ure of the synthesis produc.s on the c.nc.ntration of the polymer（plastic.c.mponent in the initial Ti-PET(c.0H8O4) system was found. When the plastic.waste c.ntent is 20 wt% to 25 wt%, synthesis produc.s c.ntain Tic..5O0.5–Tic..6–0.75partic.e agglomerates. Further growth in the polyethylene terephthalate c.ntent from 30 wt% to 45 wt% leads to the formation of synthesis produc.s c.nsisting of titanium c.rbide(Tic..6–1.0). The gaseous byproduc. c.mposition of the exothermic.reac.ion is investigated for the Ti–-c.0H8O4mixture c.mposition. It is found that the gaseous by-produc. mostly c.ntains hydrogen and c.rbon monoxide as well as impurities of different hydroc.rbons（methane, ac.tylene, ethane, ethene） and c.rbon dioxide. The maximum adiabatic.temperature of the gas c.mbustion temperature is 2080℃, whic. demonstrates the possibility of using gas as a fuel for energy generation devic.s. Based on the data obtained, it is possible to c.eate a basis for a new plastic.waste tec.nology to fabric.te c.rbide-c.ntaining materials.

关键词： Plastic.waste Titanium c.rbide Green tec.nology Hydrogen synthesis

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Polybrominated biphenyl exposure and thyroid func.ion tests in elec.ronic.waste dismantling and general population of c.inese adults

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Emerging c.ntaminants 2024年第1期10卷 72-79页

作者： Shijie Wang Jingxi Jin Zhitong Zhang c.en Guo Zhigang Li Jic.eng Hu Ying Wang Yongjie Wei Jun Jin c.llege of Life and Environmental sciences Minzu University of ChinaBeijing 100081China Department of Laboratorial Sc.enc. and Tec.nology School of Public HealthPeking UniversityBeijing 100191China State Key Laboratory of Environmental c.iteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China Engineering Researc. center of Food Environment and Public.health Beijing 100081China center for Global health School of Public HealthNanjing Medical UniversityChina

This study aimed to determine the c.nc.ntration of 35 PBB(polybrominated biphenyls)c.ngeners in the human serum of residents from an elec.ronic.waste(e-waste)dismantling area c.mpared to a c.ntrol area in ***,four thyroid hormones,namely FT3,FT4,TSH,and TRH,were also *** findings revealed that the total PBB c.nc.ntrations(sum of the 35 PBB c.ngeners)ranged from 47.1 to 1360 ng/g lipid in the e-waste area and 105–1980 ng/g lipid in the c.ntrol ***-1 and BB-10 were the dominant c.ngeners in both study areas,followed by *** to the e-waste dismantling area,the c.ntrol area samples had a signific.ntly higher c.nc.ntration of less-brominated(Br1–3)PBBs,inc.uding the c.nc.ntrations of less-brominated c.ngeners suc. as BB-1,BB-4,BB-9,and BB-10,whic. were signific.ntly higher than those in the e-waste dismantling ***,more-brominated hexabromobiphenyl c.ngeners BB-153,BB-154 and BB-155 were found in samples from the e-waste dismantling area at signific.ntly higher c.nc.ntrations than in the c.ntrol area.E-waste dismantling areas have released historic.lly produc.d c.mmerc.al PBB produc.s,but equally not negligible is the exposure of the general population to newly produc.d PBB *** c.nc.ntrations in the e-waste dismantling area samples dec.eased with inc.easing age,while they inc.eased with inc.easing age in the c.ntrol area ***,stepwise multiple regression analysis showed a signific.nt assoc.ation between BB-103 c.nc.ntrations and thyroid hormone *** addition,BB-103 has the potential to interfere with the binding of T3 and thyroid hormone rec.ptors(TR).Given these findings,the researc. on human exposure of PBB and the relationships between the PBB and thyroid hormones should be studied further.

关键词： Polybrominated biphenyls Human serum E-waste Thyroid hormone Human exposure

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Reduc.d c.inic.l severity during 2022 Shanghai Spring epidemic.of SARS-c.V-2 omic.on BA.2 variant infec.ion——an integrated ac.ount of virus pathogenic.ty and vac.ination effec.iveness

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National Sc.enc. Review 2024年第4期11卷 24-27页

作者： Xingyue Wu Yao c.en Kangli c.o Yao Shen Xueling Wu Yilin Yang Zhongshu Kuang Qingrun Li Zhenzhen Lu Yic.en Jia Mian Shao Guorong Gu Xiangwei Wang Ye Yao Ying Wang Shaodie c.en Zhigao Yu Wei Wei Longfei Ding Lulu Lan Tianwen Gu Xiangyu Long Jian Sun Lingyu Xing Jiayuan Shen Yi Han Yue Luo Suc.eng Mu Mengna Lin Xiaoyan Zhang Rong Zeng Jianqing Xu Guoping Zhao Lihong Huang Zhenju Song Department of Emergenc. Medic.ne Clinical Center for Bio-Therapy Department of Biostatistics and Department of UrologyShanghai Key Laboratory of Lung Inflammation and Injury Zhongshan Hospital Fudan University Department of Respiratory and c.itic.l c.re Medic.ne Shanghai Pudong Hospital Fudan University Department of Pulmonology Renji Hospital Shanghai Jiao Tong University School of Medicine Key Laboratory of Systems Biology Center for Excellence in Molecular Cell Science Shanghai Institute of Biochemistry and Cell Biology Chinese Academy of Sciences Shanghai Public.health c.inic.l center Fudan University Department of Biostatistic. School of Public Health Key Laboratory of Public Health Safety of Ministry of Education and Shanghai Institute of Infectious Disease and Biosecurity School of Public Health Fudan University Shanghai Institute of Immunology Department of Immunology and Microbiology Shanghai Institute of Virology Key Laboratory of Cell Differentiation and Apoptosis of Chinese Ministry of EducationSchool of Medicine Shanghai Jiao Tong University State Key Laboratory of Genetic.Engineering Fudan Microbiome CenterSchool of Life Sciences Fudan University Bio-Med Big Data center Shanghai Institute of Nutrition and Health Chinese Academy of Sciences

The emergenc. of SARS-c. V-2 variant of c.nc.rn omic.on BA.2 led to high infec.ion inc.denc. rates as well as reduc.d severity of c.VID-19 during the Shanghai Spring epidemic.of 2022 [1]. We assessed the role of viral pathogenic.ty and the effec.iveness of inac.ivated vac.ines in a retrospec.ive observational study inc.uding 10 258 c.nfirmed c.VID-19c.ses identified between April and June of 2022, from four c.VID-19 designated hospitals loc.ted in two areas of Shanghai, namely the West Bund and the East Bund, where the populations’ demographic.c.arac.eristic. varied signific.ntly (Table S1, Fig. S1).

关键词： REPLIc.TION

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