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Emissions of intermediate volatility organic compound from waste cooking oil biodiesel and marine gas oil on a ship auxiliary engine

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Journal of Environmental Sciences 2020年第5期32卷 262-270页

作者： Penghao Su Yuejiao Hao Zhe Qian Weiwei zhang jing Chen Fan zhang Fang Yin Daolun feng Yingjun Chen Yifan Li Department of Environmental Engineering Shanghai Maritime UniversityShanghai 201306China College of Environmental Science and Engineering Tongji UniversityShanghai 200092China Key Lab of Geographic Information Science of Ministry of Education of China School of Geographic SciencesEast China Normal UniversityShanghai 200142China International Joint Research Center for Persistent Toxic Substances(IJRC-PTS) Shanghai Maritime UniversityShanghai 200135China School of Environmental Engineering Fudan UniversityShanghai 200433China International Joint Research Center for Persistent Toxic Substances(IJRC-PTS) State Key Laboratory of Urban Water Resource and EnvironmentSchool of Municipal and Environmental EngineeringHarbin Institute of TechnologyHarbin 150090China

Ship auxiliary engines contribute large amounts of air pollutants when at ***,including that from waste cooking oil(WCO),can favor a reduction in the emission of primary pollutant when used with internal combustion *** study investigated the emissions of gaseous intermediate-volatile organic compounds(IVOCs)between WCO biodiesel and marine gas oil(MGO)to further understand the differences in secondary organic aerosol(SOA)production of *** revealed that WCO exhaust exhibited similar IVOC composition and volatility distribution to MGO exhaust,despite the differences between fuel *** WCO biodiesel could reduce IVOC emissions by 50%as compared to MGO,and thus reduced the SOA production from *** compositions and volatility distributions of exhaust IVOCs varied to those of their fuels,implying that fuel-component-based SOA predicting model should be used with more cautions when assessing SOA production of WCO and MGO *** biodiesel is a cleaner fuel comparing to conventional MGO on ship auxiliary engines with regard to the reductions in gaseous IVOC emissions and corresponding SOA *** the tests were conducted on test bench,the results could be considered as representative due to the widely applications of the test engine and MGO fuel on real-world ships.

关键词： Waste cooking oil biodiesel Marine gas oil Marine auxiliary engine Intermediate-volatility organic compounds Secondary organic aerosol

Effect of solidification mode on microstructure evolution and properties of magnesium alloy with long-period stacking ordered phase

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Journal of Iron and Steel Research International 2024年第5期31卷 1127-1138页

作者： Hao Li Hong-mei Chen Xu zhang Qian-hao Zang jing zhang Di feng Yan-xin Qiao Yu-hang Guo School of Materials Science and Engineering Jiangsu University of Science and TechnologyZhenjiang212100JiangsuChina School of Metallurgy and Materials Engineering Jiangsu University of Science and TechnologySuzhou215600JiangsuChina

The solidification methods of electromagnetic stirring(EMS)and non-electromagnetic stirring were employed to prepare Mg–6Gd–3Y–xZn–0.6Zr(x=1,1.5,2,3)*** evolution of alloy microstructures and the changes in properties were analyzed for different Zn *** has been observed that in alloys without electromagnetic stirring,as the Zn content increases,the alloy structure gradually *** primary second phase transitions from Mg5RE phase to long-period stacking ordered(LPSO)phase,resulting in improved hardness and *** alloys subjected to electromagnetic stirring,there is a relatively higher content of the second phase,primarily consisting of LPSO *** applying electromagnetic stirring,the quantity and the type of LPSO phase in the alloy *** alloy structure becomes more uniform with electromagnetic stirring,resulting in increased hardness and reduced hardness gradients within the *** mechanical properties of alloys with electromagnetic stirring are superior to those without electromagnetic stirring.

关键词： Rare earth magnesium alloy LPSO phase Electromagnetic stirring Casting Property

Utilizing dual-pathway energy transfer in upconversion nanoconjugates for reinforced photodynamic therapy

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Nano Research 2024年第4期17卷 2941-2948页

作者： Ruohao zhang Yu Lu Yifei Zhou Kehong Lv Xinyu Fu jitong Gong Shuang Yao Xiaozhen Wang jing feng Hongjie zhang State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026China College of Chemistry Jilin UniversityChangchun 130012China Department of Breast Surgery General Surgery Centerthe First Hospital of Jilin UniversityChangchun 130021China Department of Chemistry Tsinghua UniversityBeijing 100084China

Enhancing the therapeutic effect of existing treatments or developing new non-invasive treatments are important measures to achieve high-efficiency treatment of malignant *** therapy(PDT)is an emerging treatment modality,and the key for achieving high-efficiency PDT is to select light with strong tissue penetration depth and enhance the generation of reactive oxygen species(ROS).Although the upconversion nanoparticles(UCNPs)modified with the photosensitizers could achieve PDT with strong penetration depth under near-infrared light irradiation,the ROS generated by traditional single-pathway PDT is still ***,we developed a novel nanoconjugate(UCNP-Ce6/AIEgen)for dual-pathway reinforced PDT,in which the UCNPs were co-modified with chlorin e6(Ce6)and luminogen with aggregation-induced emission(AIEgen).Due to the presence of AIEgen,UCNP-Ce6/AIEgen could avoid aggregation-caused luminescence quenching in biological water environments and convert upconversion luminescence(UCL)of UCNPs to Ce6-activatable ***,under the irradiation of 808 nm laser,UCNP-Ce6/AIEgen can not only undergo direct lanthanide-triplet energy transfer to activate Ce6,but also convert the UCL of UCNPs to the light that can activate Ce6 through Fӧrster resonance energy transfer to generate more ROS,thus promoting tumor cell *** work broadens the applications of nanoconjugates of lanthanide-based inorganic materials and organic dyes,and provides a conception for reinforced PDT of tumors.

关键词： upconversion nanoparticle aggregation-induced emission direct lanthanide-triplet energy transfer Förster resonance energy transfer photodynamic therapy

Effect of AMPS(2-acrylamido-2-methylpropane sulfonic acid) content on the properties of polymer gels

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Petroleum Science 2022年第2期19卷 697-706页

作者： Tian-Ci zhang ji-jiang Ge Hao Wu Hong-Bin Guo Bao-Lei jiao Zhen Qian School of Petroleum Engineering China University of Petroleum(East China)Qingdao266580ShandongChina Petroleum Engineering Institute Northwest Branch of SinopecUrumqi830011XinjiangChina

The BST oilfield in the northwestern Taklamakan Desert is a fractured carbonate reservoir,but issues of water breakthrough are becoming increasingly severe with the development of water ***,the high-temperature and high-salt conditions(130°C,71695 mg/L)of the BST oilfield pose challenges for the development of plugging *** this study,the effects of 2-acrylamido-2-methylpropane sulfonic acid(AMPS)content on AM/AMPS copolymers and gels were studied through viscosity measurements,nuclear magnetic resonance(NMR),and cryo-scanning electron microscope(Cryo-SEM).Moreover,the AMPS stabilization mechanism of the polymers and gels was *** and salt-tolerant gel systems were developed,and their gelation properties,thermal stability,injection capacity,and plugging ability were *** results showed inconsistencies between the effects of AMPS content on the polymers and *** the polymers,the thermal stability increased with increased AMPS content in the ***,excessive AMPS content resulted in poor gelation and low *** developed gel systems with S30 polymer(AMPS content is approximately 26%)exhibited excellent thermal stability,controllable gelation time,good injection capacity,and plugging *** field application results indicated that most production wells had a positive response,with reduced water-cut and increased daily oil production.

关键词： Gels 2-Acrylamido-2-methylpropane sulfonic acid Enhanced oil recovery Hydrolysis Syneresis

Experimental investigation of the flow characteristics of jet pumps for zero flow-ratio conditions

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Journal of Hydrodynamics 2023年第6期35卷 1146-1156页

作者： Yun-zhi Liang jiong Wang Zu-ti zhang Bin ji Huai-yu Cheng Xin-ping Long Key Lab of Jet Theory and New Technology of Hubei Province Wuhan UniversityWuhan430072China School of Power and Mechanical Engineering Wuhan UniversityWuhan430072China State Key Laboratory of Water Resources Engineering and Management Wuhan UniversityWuhan430072China

Experimental research was conducted on the performance curves and the cavity evolution for different flow and geometric parameters in jet pumps for zero flow ratio(ZFR)*** pressure ratio,Pr,flow ratio,qr,were used in place of the conventional performance parameters h,q,to characterize the jet pump flow performance.A super cavitation cavity in the jet pump was observed to fill most of the flow channel,which hindered further increases of the flow rate and increased qr to one,thus,created a critical point on the new P_(r)-q_(r)^(2)*** the critical point,P_(r)was proportional to q_(r)^(2)with a coefficient that was much more sensitive to the area ratio than the relative throat length and the diffusion *** the critical point,the flow rate reached its maximum,the limiting flow rate,which only depended on the total inlet pressure and the area *** total inlet pressure was proportional to the square of the limiting flow rate with a flow coefficient that was only a quadratic function of the area ratio.

关键词： Jet pump performance curve zero flow-ratio super-cavitation

Effects of Co and Nb on the Crack of Additive Manufacturing Nickel-Based Superalloys

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Acta Metallurgica Sinica(English Letters) 2024年第9期37卷 1601-1610页

作者： Kejie Tan jinli Xie Hailong Qin Bin Xu Guichen Hou jinguo Li Zhongnan Bi ji zhang Beijing Key Laboratory of Advanced High Temperature Materials Central Iron&Steel Research InstituteBeijing100081China Beijing GAONA Materials&Technology Co. LTDBeijing100081China Superalloys Division Institute of Metal ResearchChinese Academy of SciencesShenyang110016China

Increasing the print quality is the critical requirement for the additive manufactured complex part of aero-engines of nickel-based superalloys.A study of the effects of Co and Nb on the crack is performed focusing on the selective laser melting(SLM)nickel-based *** this paper,the solvus temperature of γ',crack characteristics,microstructure,thermal expansion,and mechanical properties of SLM nickel-based superalloy are investigated by varying the content of Co and *** alloy with 15Co/0Nb shows the highest comprehensive *** increases the crack risk and thermal deformation,and then Co accelerates the stress ***,Co is an extremely important alloying element for improving the quality of SLM nickel-based ***,the crack growth kinetics and the strain difference are discussed to reveal the SLM crack regular that is affected by time or *** analysis work on the effect of alloying elements can obtain an effective foundational theory to guide the composition optimization of SLM nickel-based superalloys.

关键词： Nickel-based superalloys Selective laser melting Element effect Crack

In situ modification of heavy oil catalyzed by nanosized metal-organic framework at mild temperature and its mechanism

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Chinese Journal of Chemical Engineering 2024年第3期67卷 166-173页

作者： Li Wang ji-Xiang Guo Rui-Ying Xiong Chen-Hao Gao Xiao-Jun zhang Dan Luo The Unconventional Oil and Gas Institute China University of Petroleum-BeijingBeijing 102200China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China

Two catalysts, nano-sized cobalt-metal-organic framework(Co-MOF) and nickel(Ni)-MOF, were successfully prepared by the modification method. Tetralin(C10H12) was used as the hydrogen donor for the catalytic cracking and hydrogenation modification study of the dehydrated crude oil from the Shengli Oilfield. The optimal reaction conditions were determined through orthogonal experiments, and the components of the crude oil and modified oil samples were analyzed. The results revealed that the nanoMOF catalysts were successfully prepared and exhibited high catalytic activity. They could catalyze the cracking of large molecules in heavy oil at mild temperatures(<300°C), leading to the decomposition of the hydrogen donor. When the mass fraction of the catalyst was 0.2%, the mass fraction of the hydrogen donor was 1%, and the reaction temperature was 280°C, the Ni-MOF showed the best catalytic viscosity reduction effect. It could reduce the viscosity of heavy oil at 50°C from 15761.9 m Pa.s to 1266.2 m Pa.s,with a viscosity reduction rate of 91.97%. The modification effect of Co-MOF was the next best, which could reduce the viscosity of heavy oil to 2500.1 m Pa.s with a viscosity reduction rate of 84.14%. Molecular dynamics simulations revealed a strong interaction force between the MOF surface and asphaltene molecules. In the process of heavy-oil catalytic hydrogenation, the nano-MOF catalyst exhibited high catalytic activity. On the one hand, the empty d orbitals outside the metal atoms in the catalyst could polarize the carbon atoms in the organic matter, accelerating the breaking of long chains. On the other hand, the metal atoms in the catalyst could bond with the carbon σ bonds, breaking the carbon-carbon bonds. This disrupted the structure of the recombined components in the crude oil, irreversibly reducing the viscosity of the heavy oil and improving its fluidity.

关键词： Nano-sized MOF Petroleum Viscosity reduction Catalyst Nanomaterials

A two-dimensional tetragonal structure of vanadium telluride

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Nano Research 2023年第5期16卷 7749-7755页

作者： Zizhao Liu Ye Tao Zhiqiang Cui Yi ji Xuhan Zhou Peigen Li Yunwei zhang Dingyong Zhong School of Physics Sun Yat-sen UniversityGuangzhou 510275China State Key Laboratory of Optoelectronic Materials and Technologies Sun Yat-sen UniversityGuangzhou 510275China

The family of vanadium chalcogenides with variable stoichiometry and abundant crystallographic structures are promising platforms for realizing exotic emergent ***,we report on a novel two-dimensional(2D)tetragonal structure of vanadium telluride(VTe)grown by molecular beam *** atomic structures and electronic properties are revealed by scanning tunneling microscopy and first-principles *** from the hexagonal or trigonal lattices of 2D VTe_(2),the 2D VTe with a V:Te ratio of 1:1 exhibits an uncommon square ***-zero differential conductivity at the Fermi energy detected by scanning tunneling spectroscopy reveals the metallic feature of ***,Friedel oscillations are observed near chiral point defects and domain walls,illustrating the itinerant nature of the electrons close to the Fermi *** firstprinciples structure searches identify a 2D body-centered cubic(bcc)-like structure with a favorable formation energy to be the candidate of the metallic phase of the tetragonal VTe obtained *** on our calculations the 2D bcc-like structure possesses a strong 2D antiferromagnetic *** work enriches the family of vanadium chalcogenides and provides a possible 2D antiferromagnetic material for fabricating advanced spintronic devices.

关键词： vanadium telluride molecular beam epitaxy scanning tunneling microscopy two-dimensional magnetism first-principles calculation

Review of precipitation strengthening in ultrahigh-strength martensitic steel

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 256-269页

作者： Zhihao Tian Chunlei Shang Chaolei zhang Xiaoye Zhou Honghui Wu Shuize Wang Guilin Wu Junheng Gao jiaming Zhu Xinping Mao Institute for Carbon Neutrality University of Science and Technology BeijingBeijing 100083China Institute of Steel Sustainable Technology Liaoning Academy of MaterialsShenyang 110004China Department of Materials Science and Engineering Shenzhen MSU-BIT UniversityShenzhen 518172China Institute of Materials Intelligent Technology Liaoning Academy of MaterialsShenyang 110004China School of Civil Engineering Shandong UniversityJinan 250061China

Martensite is an important microstructure in ultrahigh-strength steels,and enhancing the strength of martensitic steels often involves the introduction of precipitated phases within the martensitic *** considerable research efforts devoted to this area,a systematic summary of these advancements is *** review focuses on the precipitates prevalent in ultrahigh-strength martensitic steel,primarily carbides(e.g.,MC,M_(2)C,and M_(3)C)and intermetallic compounds(e.g.,Ni Al,Ni_(3)X,and Fe_(2)Mo).The precipitation-strengthening effect of these precipitates on ultrahigh-strength martensitic steel is discussed from the aspects of heat treatment processes,microstructure of precipitate-strengthened martensite matrix,and mechanical ***,a perspective on the development of precipitation-strengthened martensitic steel is presented to contribute to the advancement of ultrahigh-strength martensitic *** review highlights significant findings,ongoing challenges,and opportunities in the development of ultrahigh-strength martensitic steel.

关键词： ultrahigh-strength martensitic steel precipitation strengthening mechanical property carbide intermetallic compound