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Impact of hydrolysis on surface area and energy storage applications of activated carbons produced from corn fiber and soy hulls

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Carbon Resources Conversion 2020年第1期3卷 19-28页

作者： zachary d.herde Ruchira dharmasena Gamini Sumanasekera Jaya Shankar Tumuluru Jagannadh Satyavolu Conn Center for Renewable Energy Research University of LouisvilleLouisvilleKYUSA Energy Systems Laboratory Idaho National LaboratoryIdaho FallsIDUSA School of Chemical and Biomolecular Eng Georgia Institute of TechnologyUnited States

Complete utilization of lignocellulosic biomass through the creation of value-added coproducts is one of the key strategies of the Bioenergy Technologies Office(BETO)for the cost-effective production of biofuels and biochemicals.A green approach to producing lightweight and high specific surface area(SSA)activated carbons(ACs)from sustainable biomass sources is of great interest to producers and users of energy devices such as batteries and *** direct conversion from biomass has been studied extensively,AC with relatively high surface areas can be produced more cost-effectively when leveraged as a co-product from a *** this paper,we discuss the production of high specific surface area activated carbons from residual fiber(fiber remaining after extraction of C5-sugars)generated as part of a C5 *** surface,morphological characteristics using SEM and TEM,and energy storage behavior of ACs produced using the C5 extracted residual fiber were evaluated in the present *** ACs produced from the residual fiber delivered an order of magnitude higher surface area than the one directly from corn pericarp fiber and soy *** surface area of the ACs produced from pre-hydrolysis ddG was only 10 m^(2)/g compared to 689 m^(2)/g for soy hulls whereas after hydrolysis these values increased significantly(ddG:1700 m^(2)/g and soy hulls:1300 m^(2)/g).TEM images indicated high exfoliation,explaining the change in surface area *** the same current density(500 mA/g)the cycling performance of the ACs increased as the surface area increased significantly.

关键词： Agricultural residues Hydrolysis Activated carbon Surface area characterization Surface morphology

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Facile synthesis of intra-nanogap enhanced Raman tags with different shapes

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Nano Research 2024年第9期17卷 8415-8423页

作者： Sanjun Fan Brian T.Scarpitti Zhewen Luo Abigail E.Smith Jian Ye zachary d.Schultz department of Chemistry and Biochemistry The Ohio State UniversityColumbusOhio 43210USA School of Biomedical Engineering Shanghai Jiao Tong UniversityShanghai 200030China

Hot spot engineering in plasmonic nanostructures plays a significant role in surface-enhanced Raman scattering(SERS)for bioanalysis and cell ***,creating stable,reproducible,and strong SERS signals remains challenging due to the potential interference from surrounding chemicals and locating SERS-active analytes into hot-spot ***,we developed a straightforward approach to synthesize intra-gap nanoparticles encapsulating 4-nitrobenzenethiol(4-NBT)as a reporter molecule within these gaps to avoid outside *** made three kinds of intra-gap nanoparticles using nanorods,bipyramids,and nanospheres as cores,in which the nanorods based intra-gap nanoparticles exhibit the highest SERS *** advantage of our method is the ease of preparation of high-yield and stable intra-gap nanoparticles characterized by a short incubation time(10 min)with 4-NBT and quick synthesis without requiring an additional step to centrifuge for the purification of core *** intense localized field in the synthesized hot spots of these plasmonic gap nanostructures holds great promise as a SERS substrate for a broad range of quantitative optical applications.

关键词： hot spot engineering surface enhanced Raman scattering intra-gap nanoparticles 4-nitrobenzenethiol

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Anneal-free ultra-low loss silicon nitride integrated photonics

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Light(Science & Applications) 2024年第8期13卷 1565-1577页

作者： debapam Bose Mark W.Harrington Andrei Isichenko Kaikai Liu Jiawei Wang Nitesh Chauhan zachary L.Newman daniel J.Blumenthal department of Electrical and Computer Engineering University of California Santa BarbaraSanta BarbaraCA 93106USA Octave Photonics LouisvilleCO 80027USA

Heterogeneous and monolithic integration of the versatile low-loss silicon nitride platform with low-temperature materials such as silicon electronics and photonics,III–V compound semiconductors,lithium niobate,organics,and glasses has been inhibited by the need for high-temperature annealing as well as the need for different process flows for thin and thick *** techniques are needed to maintain the state-of-the-art losses,nonlinear properties,and CMOS-compatible processes while enabling this next generation of 3d silicon nitride *** report a significant advance in silicon nitride integrated photonics,demonstrating the lowest losses to date for an anneal-free process at a maximum temperature 250℃,with the same deuterated silane based fabrication flow,for nitride and oxide,for an order of magnitude range in nitride thickness without requiring stress mitigation or *** report record low anneal-free losses for both nitride core and oxide cladding,enabling 1.77 dBm-1 loss and 14.9 million Q for 80 nm nitride core waveguides,more than half an order magnitude lower loss than previously reported sub 300℃ *** 800 nm-thick nitride,we achieve as good as 8.66 dBm-1 loss and 4.03 million Q,the highest reported Q for a low temperature processed resonator with equivalent device area,with a median of loss and Q of 13.9 dBm-1 and 2.59 million each *** demonstrate laser stabilization with over 4 orders of magnitude frequency noise reduction using a thin nitride reference cavity,and using a thick nitride micro-resonator we demonstrate OPO,over two octave supercontinuum generation,and four-wave mixing and parametric gain with the lowest reported optical parametric oscillation threshold per unit resonator *** results represent a significant step towards a uniform ultra-low loss silicon nitride homogeneous and heterogeneous platform for both thin and thick waveguides capable of linear and nonlinear photonic circuits and integrat

关键词： resonator thick free

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A Rare Case of Aortic Valve Endocarditis and Acute Meningitis due to Haemophilus influenzae

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Case Reports in Clinical Medicine 2024年第6期13卷 207-211页

作者： zachary M. Visinoni Justin d. Tse Christopher F. Pease department of Graduate Medical Education Internal Medicine Residency Sutter Roseville Medical Center Roseville USA Sutter Medical Group Roseville USA

HACEK organisms represent a rare but important group of causative pathogens in endocarditis. These bacteria have historically been associated with culture-negative endocarditis;however, modern laboratory techniques have made this less common. In this case, we present a 74-year-old man who presented with acute onset altered mentation, fever, and sepsis. He was ultimately found to have Haemophilus influenzae meningitis, cerebral empyema, aortic valve endocarditis, psoas myositis, and L2 - L3 diskitis with osteomyelitis. Although HACEK organisms are commonly found in the oropharynx and upper respiratory tract in humans, our patient did not report recent preceding dental or ENT procedures. H. influenzae is responsible for approximately 0.16% of all cases of bacterial endocarditis, representing a very limited subset. Although generally considered low virulent pathogens, this case demonstrates the unusual extent of infection from a HACEK organism, H. influenzae, causing aortic valve endocarditis as well as atypical non-cardiac sequelae, including acute meningitis.

关键词： HACEK Haemophilus influenzae Aortic Valve Endocarditis Bacterial Meningitis Cerebral Empyema

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Evaluation of Ruminal dry Matter disappearance and pH of dry Corn, High-Moisture Corn, and Rye under in Vitro Conditions

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Agricultural Sciences 2024年第3期15卷 327-332页

作者： Warren Carl Rusche zachary Kidd Foster Smith South dakota State University Brookings South Dakota USA

An in vitro experiment was conducted to evaluate the effects of grain type on in vitro dry matter disappearance (IVdMd) and pH using ruminal fluid and a buffer reagent. Five beef cows were used for ruminal fluid collection and ruminal fluid was pooled prior to use. The cows used for ruminal fluid collection were maintained on a forage-based diet (60:40 forage to concentrate) for 28 d prior to ruminal fluid collection. Three grain types were evaluated: 1) dry corn (89% dry matter;dRC), 2) high-moisture corn (72% dry matter;HMC) and 3) rye (89% dry matter;RYE). data were analyzed as a completely randomized design. A total of twenty-one replications of each grain type were used for statistical analysis (n = 63 tubes total). IVdMd was greater (P ≤ 0.05) by 97.1% and 46.4% for RYE compared to dRC and HMC, respectively. Additionally, IVdMd was greater (P = 0.05) by 34.6% for HMC compared to dRC. Final pH was decreased (P ≤ 0.05) for RYE by 12.3% and 2.8% for RYE compared to dRC and HMC, respectively. Also, final pH was decreased (P = 0.05) by 9.8% for HMC compared to dRC. These data indicate that corn harvest method (dry vs. high-moisture) influences IVdMd and final pH and that rye has a greater disappearance of dry matter and lower final pH than corn under in vitro conditions.

关键词： Corn Grain Processing Ruminal Fermentation Rye

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Conservative management of spinal pathology with autologous conditioned serum: A systematic review of the literature

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World Journal of Orthopedics 2024年第9期15卷 870-881页

作者： Christian J Rajkovic Matthew L Merckling Alyssa W Lee Galadu Subah Aryan Malhotra zachary d Thomas Sabrina L Zeller John V Wainwright Merritt d Kinon department of Neurosurgery Westchester Medical CenterValhallaNY 10595United States

BACKGROUNd Chronic inflammatory pain is associated with increased expression of interleukin(IL)-1,an inflammatory cytokine,and activity on its receptor(IL-1R).In response,the body produces IL-1R antagonist(IL-1Ra)to reduce this *** conditioned serum(ACS)is the only biologic therapy for spinal pathologies that enhances the action of endogenous IL-1Ra reserves to improve *** systematic review investigates the effectiveness of ACS in treating pain and dis-ability caused by spinal *** To evaluate the use of ACS as a conservative management option for spinal *** A systematic review of PubMed/Medline was performed to identify studies inve-stigating administration of ACS for treatment of any spinal *** Six articles were included,comprising 684 patients treated with epidural(n=133)or transforaminal(n=551)ACS *** had an average age of 54.0 years with slight female predominance(53.2%).The lumbar spine was most com-monly treated,with 567 patients(82.9%)receiving injections for lumbar radicu-lopathy(n=67),degenerative disc disease(ddd)(n=372),or spinal stenosis(n=128);cervical injections were performed in 109 patients(15.9%).Mean(Sd)follow-up was 21.7(4.8)weeks from first ACS *** studies investigating mecha-nical lumbar and lumbar or cervical radicular pain reported significant pain re-duction at final follow-up compared to *** achieved comparable or su-perior results to lumbar epidural steroid *** events were reported in 21 patients(3.1%),with no serious adverse *** ACS injection is a safe and effective intervention for pain reduction in many spinal pathologies,including cervical and lumbar radiculopathies.

关键词： Spine Autologous conditioned serum Orthokine Regenokine Epidural steroid injection Interleukin-1 Inter-leukin-1 receptor antagonist

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Utilizing multiphoton imaging and integrative clearing to reveal sex differences in neuroimmune interactions after nerve injury

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Neural Regeneration Research 2022年第11期17卷 2429-2430页

作者： zachary W.Castillo Michael d.Burton Neuroimmunology and Behavior Laboratory Department of NeuroscienceSchool of Behavioral and Brain SciencesCenter for Advanced Pain StudiesUniversity of Texas at Dallas

With the constant development of multiphoton microscopy,our ability to observe complex and dynamic biological processes deeper within living tissue,is steadily *** use multiphoton microscopy,because experiments can be conducted with little to no invasiveness or tissue damage over a long period of time with no photodamage(Mancuso et al.,2009).This allows for the introduction of tissue into the context of a three-dimensional 3d environment in which visualization of cellular activation and interaction is *** circumventing a distorted reconstruction with limited z-stacks,multiphoton imaging provides enhanced spatiotemporal resolution.

关键词： resolution. multiphoton distorted

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A Rare Case of Aortic Valve Endocarditis and Acute Meningitis due to Haemophilus influenzae

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Case Reports in Clinical Medicine（临床医学病理报告） 2024年第6期 207页

作者： zachary M.Visinoni Justin d.Tse Christopher F.Pease

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Bipolar depression:a review of treatment options

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General Psychiatry 2022年第4期35卷 230-239页

作者： Kate Levenberg zachary A Cordner Psychiatry and Behavioral Sciences Johns Hopkins School of MedicineBaltimoreMarylandUSA

Bipolar depression(Bd-d)is both common and incredibly challenging to *** treated individuals with Bd-d experience depression approximately 19%of the time,and subsyndromal depression an additional 18%.This stands in clear contrast to the approximately 10%of time spent in hypomania and 1%of time spent in *** this high illness burden,there remain relatively few treatment options approved by the US Food and drug Administration for *** the approved medications,four are second-generation antipsychotics(SGAs)and one is an SGA combined with an ***,particularly when used long-term,antipsychotics can pose a significant risk of adverse effects,raising the clinical conundrum of weighing the risks associated with longterm antipsychotic use versus the risk of relapse when patients are off ***,we review commonly used treatments for Bd-d,including antipsychotics,classic mood stabilisers,electroconvulsive therapy and *** then address the somewhat controversial topic of antidepressant use in ***,we summarise emerging treatment options and highlight ongoing clinical *** hope this review will help compare the risks and benefits of several common and novel options for the treatment of patients with *** doing so,we also hope this review will aid the individualised selection of treatments based on each patient’s history and treatment goals.

关键词： treatment spite approved

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The pervasive effects of lighting environments on sensory drive in bluefin killifish： an investigation into male/male competition, female choice, and predation

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Current Zoology 2018年第4期64卷 499-512页

作者： Lisa d. MITCHEM Shannon STANIS Nicholas M. SUTTON zachary TURNER Rebecca C. FULLER School of Integrative Biology University of Illinois Urbana IL 61801 USA department of Biology University of Virginia Charlottesville VA 22904 USA department of Mathematics University of Illinois Urbana IL 61801 USA

Sensory drive predicts that the conditions under which signaling takes place have large effects on signals, sensory systems, and behavior. The coupling of an ecological genetics approach with sen sory drive has been fruitful. An ecological genetics approach compares populations that experi ence different environments and asks whether population differences are adaptive and are the result of genetic and/or environmental variation. The multifaceted effects of signaling environ ments are wellexemplified by the bluefin killifish. In this system, males with blue anal fins are abundant in tanninstained swamps that lack UV/blue light but are absent in clear springs where UV/blue light is abundant. Past work indicates that lighting environments shape genetic and envir onmental variation in color patterns, visual systems, and behavior. Less is known about the select ive forces creating the across population correlations between UV/blue light and the abundance of blue males. Here, we present three new experiments that investigate the roles of lighting environ ments on male competition, female mate choice, and predation. We found strong effects of lighting environments on male competition where blue males were more likely to emerge as dominant in teastained water than in clear water. Our preliminary study on predation indicated that blue males may be less susceptible to predation in teastained water than in clear water. However, there was little evidence for female preferences favoring blue males. The resulting pattern is one where the effects of lighting environments on genetic variation and phenotypic plasticity match the direction of selection and favor the expression of blue males in swamps.

关键词： Lucania goodei adaptive plasticity intrasexual selection male competition private communication predation

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