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Comparison of antimony and arsenic behaviour at the river-lake junction in the middle of the Yangtze River Basin

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Journal of Environmental Sciences 2024年第2期136卷 189-200页

作者： Huiji Liu wei zeng Ziyang Lai Mengchang He Chunye Lin wei Ouyang Xitao Liu State Key Laboratory of Water Environment Simulation School of EnvironmentBeijing Normal UniversityBeijing 100875China Advanced Interdisciplinary Institute of Environment and Ecology Beijing Normal UniversityZhuhai 519087China

As typical metalloid toxic elements widely distributed in environmental media,the geochemical behaviour of antimony(Sb)and arsenic(As)affects environmental *** selected the surface waters and sediments at the river-lake junction of Dongting Lake as the research objects,analysed the concentration and chemical partitioning of Sb and As,assessed its contamination and ecological risk levels,and discussed its sources and potential influencing *** concentrations of dissolved Sb and As in surface waters were low(<5.46μg/L),and the concentrations of Sb and As in surface sediments were 2.49-22.65mg/kg and 11.10-136.34 mg/kg,*** and As in sediments were mainly enriched in the fraction of residues,but the proportion of As in bioavailability was significantly higher than that of *** the contamination level of Sb was higher than that of As,the risk assessment code(RAC)showed that the ecological risk level of As was higher than that of *** erosion and mining activities(in the midstream of Zijiang River)were the main contaminated sources of Sb,while As was affect mainly by rainwater *** contamination and ecological risk of Sb in the inlet of the Zijiang River should receive considerable attention,while those of As in the inlet of the Xiangjiang River should also be seriously *** study highlights the need for multi-index-based assessments of contamination and ecological risk and the importance of further studies on the environmental behaviour of metalloids in specific hydrological conditions,such as river-lake junctions.

关键词： Contamination Ecological risks Antimony(Sb) Arsenic(As) River-lake junction Dongting Lake

Understory seedlings of Quercus mongolica survive by phenological escape

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Forest Ecosystems 2024年第2期11卷 236-246页

作者： Shixiong Wu Ying Liu Lulu He wei zeng Qijing Liu College of Forestry Beijing Forestry UniversityBeijing100083China

Understanding understory seedling regeneration mechanisms is important for the sustainable development of temperate primary forests in the context of increasingly intense climate warming *** poor regeneration of dominant tree species,however,is one of the biggest challenges it faces at the ***,the regeneration of the shade-intolerant Quercus mongolica seedling is difficult in primary forests,which contrasts with the extreme abundance of understory seedlings in secondary *** mechanism behind the interesting phenomenon is still *** study used in-situ monitoring and nursery-controlled experiment to investigate the survival rate,growth performance,as well as nonstructural carbohydrate (NSC) concentrations and pools of various organ tissues of seedlings for two consecutive years,further analyze the understory light availability and simulate the foliage carbon (C) gain in the secondary and primary *** suggested that seedlings in the secondary forest had greater biomass allocation aboveground,height and specific leaf area (SLA) in summer,which allowed the seedling to survive longer in the canopy closure *** light availability and positive C gain in early spring and late autumn are key factors affecting the growth and survival of understory seedlings in the secondary forest,whereas seedlings in the primary forest had annual negative carbon *** the growing season,the total NSC concentrations of seedlings gradually decreased,whereas those of seedlings in the secondary forest increased significantly in autumn,and were mainly stored in roots for winter consumption and the following year's summer shade period,which was verified by the nursery-controlled experiment that simulated autumn enhanced light availability improved seedling survival rate and NSC *** conclusion,our results revealed the survival trade-off strategies of Quercus mongolica seedlings and highlighted the necessity of high light availability d

关键词： Carbon gain Nonstructural carbohydrate Recruitment Trade-off Biomass allocation

Rh(Ⅱ)-catalyzed intermolecular carboamination of pyridines via double Csp^(2)-H bond activations

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Science China Chemistry 2024年第1期67卷 374-382页

作者： Zhongfeng Luo Jingxing Jiang Lifang Zou Xiaoyu Zhou Junshan Liu Zhuofeng Ke Fengjuan Chen Huanfeng Jiang wei zeng Key Laboratory of Functional Molecular Engineering of Guangdong Province School of Chemistry and Chemical EngineeringSouth China University of TechnologyGuangzhou 510641China School of Materials Science and Engineering PCFM LabSun Yat-sen UniversityGuangzhou 510275China Guangdong Provincial Key Laboratory of Chinese Medicine Pharmaceutics School of Traditional Chinese MedicineSouthern Medical UniversityGuangzhou 510515China

We disclose the development of the Rh-catalyzed amine-directed remote 5,6-carboamination protocol of pyridines via dual Csp^(2)-H functionalizations.A variety of readily available 2-aminopyridines and 1,2,3-triazoles are allowed for coupling cyclization to access polyfunctionalized *** studies including DFT calculations unveil that relay carbenoidelectrophilic addition to pyridines and the sequential pyridyl Csp^(2)-H amination are involved in this *** postsynthetic utility of this methodology is showcased by versatile and site-selective modification of azaindoles.

关键词： Rh-catalysis azaindoles pyridyl Csp^(2)-H bond carboamination coupling-cyclization

Enhanced SERS aptasensor for sensitive detection of saxitoxin based on HAuCl/HOreaction system and Pt/Au nanozyme

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Food Science and Human Wellness 2024年

作者： Yueqing Li Xuemei Tang wei zeng Ting Wu Long Wu School of Food Science and Engineering， Key Laboratory of Tropical Fruits and Vegetables Quality and Safety for State Market Regulation， Hainan University

Saxitoxin （STX） is a marine biotoxin produced by cyanobacteria and methanobacteria， which is harmful to humans and aquatic organisms. Therefore， it is urgent to establish an efficient， sensitive and selective method for the screening of STX. In this paper， based on the HAuCl4/H2O2reaction system， gold nanoparticles （Au NPs） decorated Fe3O4magnetic beads (Fe3O4@Au NPs) and Pt/Au nanozymes （Pt/Au NZs）， an enhanced SERS aptasensor was proposed for sensitive and selective detection of STX. Firstly， SERS tag （4-MBA） and aptamer modified Fe3O4@Au NPs were hybridized with complementary DNA modified Pt/Au NZs （Pt/Au-cDNA） to form the specific complexes. Wherein， aptamer acted as capture agent to specifically recognize STX， Pt/Au NZs catalyzed HAuCl4/H2O2reaction to enhance SERS signal， and Fe3O4facilitated the magnetic separation and simple detection operations. The SERS aptasensor achieved sensitive detection of STX with a wide linear range from 0.02 μmol/L to 0.8 μmol/L and a low detection limit of 13 nmol/L （LOD， S/N=3）. To evaluate the performance of this method， STX were detected in the spiked seafood samples with recoveries from 78.75% to 150% with relative errors below 6.52%. Besides， the SERS aptasensor behaved good stability and repeatability， revealing its promising potential in STX detection and food safety detection.

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Sentient Mountains and Seas: Vast and Tranquil Liaoning

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China & The World Cultural Exchange 2024年第2期 24-25页

作者： zeng wei(Photo) 不详

Liaoning has a long winter snowperiod with abundant snow,which is soft and thick in nature,presenting enchanting snow-white scenery away from biting *** is the most suitablefor outdoor ice&snow sports,with ice&snow and hot springs complementing ***14toDecember 20,2023,"Nihao!China"—2024China lce&Snow Tourism Overseas Promotion Season"launched"Liaoning Overseas Promotion Week".

关键词： Liaoning winter abundant

Fragility crossover mediated by covalent-like electronic interactions in metallic liquids

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Materials Futures

Materials Futures 2024年第2期3卷 117-130页

作者： Hui-Ru Zhang Liang Gao Yu-Hao Ye Jia-Xin Zhang Tao Zhang Qing-Zhou Bu Qun Yang zeng-wei Zhu Shuai wei Hai-Bin Yu Wuhan National High Magnetic Field Center and School of Physics Huazhong University of Science and TechnologyWuhan 430074People’s Republic of China Department of Chemistry Aarhus University8000 AarhusDenmark iMAT Centre for Integrated Materials Research Aarhus University8000 AarhusDenmark

Fragility is one of the central concepts in glass and liquid sciences,as it characterizes the extent of deviation of viscosity from Arrhenius behavior and is linked to a range of glass ***,the intervention of crystallization often prevents the assessment of fragility in poor glass-formers,such as supercooled metallic *** experimental data on their compositional dependence are scarce,let alone fundamentally *** this work,we use fast scanning calorimetry to overcome this obstacle and systematically study the fragility in a ternary La–Ni–Al system,over previously inaccessible composition *** observe fragility dropped in a small range with the Al alloying,indicating an alloying-induced fragility *** use x-ray photoelectron spectroscopy,resistance measurements,electronic structure calculations,and DFT-based deep-learning atomic simulations to investigate the cause of this fragility *** results show that the fragility crossover can be fundamentally ascribed to the electronic covalency associated with the unique Al–Al *** findings provide insight into the origin of fragility in metallic liquids from an electronic structure perspective and pave a new way for the design of metallic glasses.

关键词： metallic glass fragility fast scanning calorimetry density functional theory deep learning potential

The DUF579 proteins GhIRX15s regulate cotton fiber development by interacting with proteins involved in xylan synthesis

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The Crop Journal 2024年第4期12卷 1112-1125页

作者： Mengyun Li Feng Chen Jingwen Luo Yanan Gao Jinglong Cai wei zeng Monika S.Doblin Gengqing Huang Wenliang Xu Hubei Key Laboratory of Genetic Regulation and Integrative Biology School of Life SciencesCentral China Normal UniversityWuhan 430079HubeiChina Zhejiang Provincial Key Laboratory of Plant Evolutionary Ecology and Conservation School of Life SciencesTaizhou UniversityTaizhou 318000ZhejiangChina La Trobe Institute for Sustainable Agriculture&Food School of AgricultureBiomedicine and EnvironmentLa Trobe UniversityBundooraVIC 3086Australia

Cotton provides the most abundant natural fiber for the textile *** mature cotton fiber largely consists of secondary cell walls with the highest proportion of cellulose and a small amount of hemicellulose and *** dissect the roles of hemicellulosic polysaccharides during fiber development,four IRREGULAR XYLEM 15(IRX15)genes,GhIRX15-1/-2/-3/-4,were functionally characterized in *** genes encode DUF579 domain-containing proteins,which are homologs of AtIRX15 involved in xylan *** four GhIRX15 genes were predominantly expressed during fiber secondary wall thickening,and the encoded proteins were localized to the Golgi *** GhIRX15 gene could restore the xylan deficient phenotype in the Arabidopsis irx15irx15l double *** of GhIRX15s in cotton resulted in shorter mature fibers with a thinner cell wall and reduced cellulose content as compared to the wild ***,GhIRX15-2 and GhIRX15-4 formed homodimers and *** addition,the GhIRX15s showed physical interaction with glycosyltransferases GhGT43C,GhGT47A and GhGT47B,which are responsible for synthesis of the xylan backbone and reducing end ***,the GhIRX15s can form heterocomplexes with enzymes involved in xylan modification and side chain synthesis,such as GhGUX1/2,GhGXM1/2 and *** findings suggest that GhIRX15s participate in fiber xylan biosynthesis and modulate fiber development via forming large multiprotein complexes.

关键词： Cotton fiber Xylan biosynthesis GhIRX15s Protein-protein interaction Protein complexes

由格物致知到知行合一:论出版学的实践品格——从《关于推进出版学科专业共建工作的实施意见》说起

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河南大学学报（社会科学版） 2024年第2期64卷 146-151,156页

作者：曾巍华中师范大学文学院、文化传播研究中心湖北武汉430079

出版活动是人类知识生产与传播的实践活动,出版的实践属性决定了出版学的实践品格。从出版现象出发,通过观察与思考,能够揭示出版现象的存在方式和运行规律,实现由感性认识到理性认识的知识飞跃。而在时间维度中梳理出版史,可呈现出版... 详细信息

出版活动是人类知识生产与传播的实践活动,出版的实践属性决定了出版学的实践品格。从出版现象出发,通过观察与思考,能够揭示出版现象的存在方式和运行规律,实现由感性认识到理性认识的知识飞跃。而在时间维度中梳理出版史,可呈现出版现象的动态演变,进而聚焦其中的推动因素,即具有能动性的实践主体。进入“现场”的实地调研,既可以将知识应用于实践进行检验,又可以发现并解决问题,实现社会服务功能。出版学研究,应坚持用辩证唯物主义、历史唯物主义、实践唯物主义的眼光来看问题,坚持理论与实践紧密结合,由“格物致知”达至“知行合一”,以学科共建为契机,加快中国出版学自主知识体系构建。

关键词：出版学知识生产出版史出版实践自主知识体系

Mental health and insomnia problems in healthcare workers after the COVID-19 pandemic:A multicenter cross-sectional study

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World Journal of Psychiatry 2024年第5期14卷 704-714页

作者： wei Ding Min-Zhong Wang Xian-wei zeng Zhen-Hua Liu Yao Meng Hui-Ting Hu Yuan Zhang Yu-Guang Guan Fan-Gang Meng Jian-Guo Zhang Shu Wang Department of Public Health Liaocheng People’s HospitalLiaocheng 252000Shandong ProvinceChina Department of Neurology Shandong Provincial Hospital Affiliated to Shandong First Medical UniversityJinan 250021Shandong ProvinceChina Department of Neurosurgery Qilu Hospital of Shandong UniversityJinan 250012Shandong ProvinceChina Sleep Medicine Center Shandong Provincial Hospital Affiliated to Shandong First Medical UniversityJinan 250021Shandong ProvinceChina Department of Neurology The First Affiliated Hospital of Shandong First Medical UniversityJinan 250014Shandong ProvinceChina Department of Neurology Heze Mudan People’s HospitalHeze 274000Shandong ProvinceChina Neonatal Center Beijing Children's HospitalCapital Medical UniversityNational Center for Children's HealthBeijing 100045China Department of Neurosurgery SanBo Brain HospitalCapital Medical UniversityBeijing 100093China Department of Neurosurgery Beijing Tiantan HospitalCapital Medical UniversityBeijing 100070China

BACKGROUND Healthcare workers(HCWs)are at increased risk of contracting coronavirus disease 2019(COVID-19)as well as worsening mental health problems and *** problems can persist for a long period,even after the ***,less is known about this *** To analyze mental health,insomnia problems,and their influencing factors in HCWs after the COVID-19 *** This multicenter cross-sectional,hospital-based study was conducted from June 1,2023 to June 30,2023,which was a half-year after the end of the COVID-19 ***-stratified population-based cluster sampling was applied at the provincial level for Chinese *** such as anxiety,depression,and insomnia were evaluated by the Generalized Anxiety Disorder-7,Patient Health Questionnaire-9,and Insomnia Severity *** influencing the symptoms were identified by multivariable logistic *** A total of 2000 participants were invited,for a response rate of 70.6%.A total of 1412 HCWs[618(43.8%)doctors,583(41.3%)nurses and 211(14.9%)nonfrontline],254(18.0%),231(16.4%),and 289(20.5%)had symptoms of anxiety,depression,and insomnia,respectively;severe symptoms were found in 58(4.1%),49(3.5%),and 111(7.9%)of the ***,female sex,and hospitalization for COVID-19 were risk factors for anxiety,depression,and insomnia symptoms;moreover,death from family or friends was a risk factor for insomnia *** the COVID-19 outbreak,most[1086(76.9%)]of the participating HCWs received psychological interventions,while nearly all[994(70.4%)]of them had received public psychological *** 102(7.2%)of the HCWs received individual counseling from *** Although the mental health and sleep problems of HCWs were relieved after the COVID-19 pandemic,they still faced challenges and greater risks than did the general *** risk factors would help in providing targeted *** addition,although a major proportion of

关键词： COVID-19 Mental health Psychological symptoms Insomnia Sleep disorders Cross-sectional study Epidemiological study