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Microstructure evolution and shape memory behaviors of Ni_(47)Ti_(44)Nb_(9)alloy subjected to multistep thermomechanical loading with different prestrain levels

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Journal of Materials Science & Technology 2024年第4期171卷 80-93页

作者： Y.H.zhang H.li Z.w.Yang X.liu Q.F.Gu State Key laboratory of Solidification Processing School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Shaanxi Key laboratory of High-Performance Precision Forming Technology and Equipment Northwestern Polytechnical UniversityXi’an 710072China

Ni_(47)Ti_(44)Nb_(9)shape memory alloy(SMA)is a promising material in the aerospace field due to its wide transformation *** application of shape memory effect depends on multistep thermomechan-ical loading,viz.,low-temperature deformation and subsequent heating to ***-temperature deformation prestrain plays a pivotal role in shape memory properties tailoring of SMA ***,microstructure evolution and deformation mechanisms of Ni_(47)Ti_(44)Nb_(9)SMA subjected to vari-ous prestrain levels are still *** this end,microstructure evolution and shape memory behaviors of Ni_(47)Ti_(44)Nb_(9)alloy subjected to multistep thermomechanical loading with prestrain levels of 8%-16%at-28℃(M_(s)+30℃)were *** results demonstrate that the stress-strain curve of the specimen exhibits four distinct stages at a maximal prestrain of 16%.whereas stageⅡand stageⅢend at prestrains of∼8%and∼12%,*** stageⅡ,the stress-induced martensitic transformation is accompanied by the dislocation slip of the NiTi matrix andβ-Nb *** stageⅢ,in addition to the higher density of dislocations and further growth of stress-induced martensite variants(SIMVs),(001)compound twins are introduced as a result of the(001)deformation twinning in stress-induced ***{20-1}martensite twins are gradually introduced in stageⅣ.Correspondingly,after subsequent unloading and heating,a higher density of{114}austenite twins form in the specimen with a larger prestrain of 16%.with increasing prestrain from 8%to 16%,the recoverable strainε_(re)^(T)upon heating increases first and then ***ε_(re)^(T)obtains a maximum of 7.03%at 10%prestrain and de-creases to 6.17%at 16%*** increase ofε_(re)^(T)can be attributed to the formation of new SIMVs,the further growth of existing SIMVs,and the recoverable(001)compound *** the decrease ofε_(re)^(T)is mainly associated with the irrecoverable strain by{20−1}martensite *** effe

关键词： Ni_(47)Ti_(44)Nb_(9)shape memory alloy wide transformation hysteresis Thermomechanical loading Microstructure evolution Shape memory behaviors Stress-induced martensitic transformation Deformation twinning

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Photo-responsive functional materials based on light-driven molecular motors

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light(Science & Applications) 2024年第3期13卷 407-420页

作者： Yanping Deng Guiying long Yang zhang wei Zhao Guofu Zhou Ben l.Feringa Jiawen Chen SCNU-UG International Joint laboratory of Molecular Science and Displays National Center for International Research on Green OptoelectronicsSouth China Normal UniversityGuangzhou 510006China Stratingh Institute for Chemistry University of GroningenNijenborgh 49747AG GroningenThe Netherlands

In the past two decades,the research and development of light-triggered molecular machines have mainly focused on developing molecular devices at the nanoscale.A key scientific issue in the field is how to amplify the controlled motion of molecules at the nanoscale along multiple length scales,such as the mesoscopic or the macroscopic scale,or in a more practical perspective,how to convert molecular motion into changes of properties of a macroscopic ***-driven molecular motors are able to perform repetitive unidirectional rotation upon irradiation,which offers unique opportunities for responsive macroscopic *** several reviews that focus on the design,synthesis and operation of the motors at the nanoscale,photo-responsive macroscopic materials based on light-driven molecular motors have not been comprehensively *** the present review,we first discuss the strategy of confining absolute molecular rotation into relative rotation by grafting motors on ***,examples of self-assemble motors in supramolecular polymers with high internal order are ***,we will focus on building of motors in a covalently linked system such as polymeric gels and polymeric liquid crystals to generate complex responsive ***,a perspective toward future developments and opportunities is *** review helps us getting a more and more clear picture and understanding on how complex movement can be programmed in light-responsive systems and how man-made adaptive materials can be invented,which can serve as an important guideline for further design of complex and advanced responsive materials.

关键词： functions materials material

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Efficient fidelity estimation: alternative derivation and related applications

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Communications in Theoretical Physics 2024年第9期76卷 18-22页

作者： Diego S Starke Marcos l w Basso Jonas Maziero Physics Department Center for Natural and Exact Sciences Federal University of Santa Maria Center for Natural and Human Sciences Federal University of ABC Avenue of the States

In[***.A 107 012427 (2023)],Baldwin and Jones prove that Uhlmann–Jozsa’s fidelity between two quantum statesρandσ,i.e.,■,can be written in a simplified form as ■.In this article,we give an alternative proof of this result,using a function power series expansion and the properties of the trace *** approach not only reinforces the validity of the simplified expression but also facilitates the exploration of novel dissimilarity functions for quantum states and more complex trace functions of density operators.

关键词： Chebyshev polynomials efficient fidelity estimation Rényi entropy Ulhmann-Jozsa fidelity

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N-doped graphene quantum dot-decorated N-TiO2/P-doped porous hollow g-C_(3)N_(4) nanotube composite photocatalysts for antibiotic photodegradation and H2 production

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International Journal of Minerals,Metallurgy and Materials 2024年第1期31卷 165-178页

作者： Jingshu Yuan Yao zhang Xiaoyan zhang Junjie zhang Shen’gen zhang Institute for Advanced Materials and Technology University of Science and Technology BeijingBeijing 100083China Xi’an Fanyi University Xi’an 710105China Shunde Graduate School of University of Science and Technology Beijing Foshan 528399China State Key laboratory of lunar and Planetary Sciences Macao University of Science and TechnologyMacao SAR 820000China

Exclusive responsiveness to ultraviolet light (~3.2 eV) and high photogenerated charge recombination rate are the two primary drawbacks of pure TiO_(2). we combined N-doped graphene quantum dots (N-GQDs), morphology regulation, and heterojunction construction strategies to synthesize N-GQD/N-doped TiO_(2)/P-doped porous hollow g-C_(3)N_(4) nanotube (PCN) composite photocatalysts (denoted as G-TPCN). The optimal sample (G-TPCN doped with 0.1wt% N-GQD, denoted as 0.1% G-TPCN) exhibits significantly enhanced photoabsorption, which is attributed to the change in bandgap caused by elemental doping (P and N), the improved light-harvesting resulting from the tube structure, and the upconversion effect of N-GQDs. In addition, the internal charge separation and transfer capability of0.1% G-TPCN are dramatically boosted, and its carrier concentration is 3.7, 2.3, and 1.9 times that of N-TiO_(2), PCN, and N-TiO_(2)/PCN(TPCN-1), respectively. This phenomenon is attributed to the formation of Z-scheme heterojunction between N-TiO_(2) and PCNs, the excellent electron conduction ability of N-GQDs, and the short transfer distance caused by the porous nanotube structure. Compared with those of N-TiO_(2), PCNs, and TPCN-1, the H2 production activity of 0.1%G-TPCN under visible light is enhanced by 12.4, 2.3, and 1.4times, respectively, and its ciprofloxacin (CIP) degradation rate is increased by 7.9, 5.7, and 2.9 times, respectively. The optimized performance benefits from excellent photoresponsiveness and improved carrier separation and migration efficiencies. Finally, the photocatalytic mechanism of 0.1% G-TPCN and five possible degradation pathways of CIP are proposed. This study clarifies the mechanism of multiple modification strategies to synergistically improve the photocatalytic performance of 0.1% G-TPCN and provides a potential strategy for rationally designing novel photocatalysts for environmental remediation and solar energy conversion.

关键词： N-doped TiO_(2) N-doped graphene quantum dots P-doped g-C_(3)N_(4) porous hollow nanotube heterojunction photocatalysis

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Fluorescent Double Network Hydrogels with Ionic Responsiveness and High Mechanical Properties for Visual Detection

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Journal of wuhan University of Technology(Materials Science) 2024年第2期39卷 487-496页

作者：郑湾 lIU lerong lü Hanlin wANG Yuhang lI Feihu zhang Yixuan 陈艳军 wANG Yifeng School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China

we developed a fluorescent double network hydrogel with ionic responsiveness and high mechanical properties for visual *** nanocomposite hydrogel of laponite and polyacrylamide serves as the first network,while the ionic cross-linked hydrogel of terbium ions and sodium alginate serves as the second *** double-network structure,the introduction of nanoparticles and the reversible ionic crosslinked interactions confer high mechanical properties to the *** ions are not only used as the ionic cross-linked points,but also used as green emitters to endow hydrogels with fluorescent *** the basis of the “antenna effect” of terbium ions and the ion exchange interaction,the fluorescence of the hydrogels can make selective responses to various ions(such as organic acid radical ions,transition metal ions) in aqueous solutions,which enables a convenient strategy for visual detection toward ***,the fluorescent double network hydrogel fabricated in this study is promising for use in the field of visual sensor detection.

关键词： visual detection ionic responsiveness fluorescent hydrogels double network hydrogels mechanical property

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Impacts of major volcanic eruptions over the past two millennia on both global and Chinese climates:A review

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Science China Earth Sciences 2024年第1期67卷 61-78页

作者： weiyi SUN Deliang CHEN Guonian lÜ liang NING Chaochao GAO Renhe zhang Bin wANG Jian lIU Key laboratory for Virtual Geographic Environment Ministry of EducationState Key Laboratory Cultivation Base of Geographical Environment Evolution of Jiangsu ProvinceJiangsu Center for Collaborative Innovation in Geographical Information Resource Development and ApplicationSchool of Geography ScienceNanjing Normal UniversityNanjing 210023China Regional Climate Group Department of Earth SciencesUniversity of GothenburgGothenburg 40530Sweden College of Environmental and Resource Science Zhejiang UniversityHangzhou 310058China Department of Atmospheric and Oceanic Sciences&Institute of Atmospheric Sciences Fudan UniversityShanghai 200437China Department of Atmospheric Sciences and Atmosphere-Ocean Research Center University of Hawaii at ManoaHonoluluHI 96825USA Jiangsu Provincial Key laboratory for Numerical Simulation of large Scale Complex Systems School of Mathematical ScienceNanjing Normal UniversityNanjing 210023China Open Studio for the Simulation of Ocean-Climate-Isotope Qingdao National Laboratory for Marine Science and TechnologyQingdao 266237China

Major volcanic eruptions(MVEs)have attracted increasing attention from the scientific *** studies have explored the climatic impact of MVEs over the past two ***,proxy-based reconstructions and climate model simulations indicate divergent responses of global and China’s regional climates to ***,we used multiple data from observations,reconstructions,simulations,and assimilations to summarize the historical facts of MVEs,the characteristics and mechanisms of their climatic impact,and directions for future *** reviewed volcanic datasets and determined intensive MVE periods;these periods corresponded to the years 530–700,1200‒1460,and 1600‒1840 *** tropical MVEs,a substantial cooling effect is observed throughout the globe and China on the interannual-interdecadal time scales but an inconsistent cooling magnitude is detected between reconstructions and *** the first summer after tropical MVEs,a decrease in global and monsoonal precipitation is *** reconstructions and simulations,an increased precipitation is seen for the Yangtze River Basin,while large uncertainties in precipitation changes are present for other regions of *** drought can be induced by frequent eruptions and volcanism superimposed on low solar irradiation and internal *** affect climate directly through the radiative effect and indirectly by modulating internal variability,such as the El Niño‒Southern Oscillation(ENSO)and Atlantic Multidecadal Oscillation(AMO).However,changes in the phase,amplitude,and periodicity of ENSO and AMO after MVEs and the associated mechanisms remain controversial,which could account for model-reconstruction ***,other internal variability,uncertainties in reconstruction methods and aerosol‒climate models,and climate background may also induce model-reconstruction *** gaps and directions for future research are also discussed.

关键词： Major volcanic eruption Climate variability Mechanism Past two millennia Internal variability

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Reversing free-electron transfer of sulfide cocatalyst for exceptional photocatalytic H_(2)evolution

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Journal of Materials Science & Technology 2024年第4期171卷 147-149页

作者： Yanfeng zhang Zhenyi zhang National Experimental Chemistry Teaching Center Hebei Key Laboratory of Inorganic Nano-materialsCollege of Chemistry and Materials ScienceHebei Normal UniversityShijiazhuang 050024China Key laboratory of New Energy and Rare Earth Resource Utilization of State Ethnic Affairs Commission Key Laboratory of Photosensitive Materials and Devices of Liaoning ProvinceSchool of Physics and Materials EngineeringDalian Minzu UniversityDalian 116600China

Recently,Yu and co-workers deeply explore the potential impact of free electron transfer between co-catalysts and photocatalyst carriers on H_(2)evolution efficiency of active sites over MoS_(2+x).They pro-pose an electron-reversal tactics to evade the unexpected electron transfer and synchronously regulate the above transfer in a beneficial orientation for weakening hydrogen adsorption on S ***,this highlight not only discusses and summarizes the essences of electron reversal and the optimized H ad-sorption/desorption mechanism,but also emphasizes the significance of femtosecond transient absorp-tion spectroscopy(fs-TAS)and in-situ irradiated X-ray photoelectron spectroscopy(ISI-XPS)for revealing charge transfer dynamics and *** anticipate that this highlight can disseminate a new per-spective on the roles of photocatalyst carriers in improving cocatalytic H_(2)-production kinetics.

关键词： Photocatalysis Cocatalyst Electron reversal Antibonding-orbital occupancy S–H bonds

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A synthesis of the Cretaceous wildfire record related to atmospheric oxygen levels?

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Journal of Palaeogeography 2024年第1期13卷 149-164页

作者： Da-wei lü wen-Xu Du Zhi-Hui zhang Yuan Gao Tian-Tian wang Jin-Cheng Xu Ao-Cong zhang Cheng-Shan wang Shandong Provincial Key laboratory of Depositional Mineralization and Sedimentary Minerals College of Earth Sciences and EngineeringShandong University of Science and TechnologyQingdao 266590Shandong ProvinceChina School of Earth Sciences and Resources China University of GeosciencesBejing 100083China Institute of Earth Sciences China University of Geosciences(Bejing)Beijing 100083China

The Cretaceous was a significant greenhouse period in Earth's history with higher atmospheric CO_(2) levels and temperatures than today. Although evidence of combustion has been widely described from the Cretaceous deposits, our understanding of the spatiotemporal diversification pattern and process of the Cretaceous wildfires is still limited. In this study, we comprehensively synthesize a total of 271 published Cretaceous wildfire occurrences based on the by-products of burning, including fossil charcoal, pyrogenic inertinite(fossil charcoal in coal), and pyrogenic polycyclic aromatic hydrocarbons(PAHs). Spatially, the dataset shows a distinctive distribution of reported wildfire evidence characterized by high concentration in the middle latitudinal areas of the Northern Hemisphere(30°N-60°N) over the Cretaceous. Temporally, an overall increasing trend of the reported wildfire data from the Early Cretaceous to the late Cretaceous is coincident with higher atmospheric O_(2) levels. However, the spatial and temporal patterns may result from many types of factors, such as taphonomy, preservation, and researcher biases, instead of a real picture of the Cretaceous wildfire evolution. To better understand the spatiotemporal diversification of the Cretaceous wildfire, more investigations on the record of wildfire occurrences during this period would be necessary in the future.

关键词： wildfire Cretaceous Atmospheric oxygen Taphonomy Charcoal

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low crude protein formulation with supplemental amino acids for its impacts on intestinal health and growth performance of growing-finishing pigs

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Journal of Animal Science and Biotechnology 2024年第4期15卷 1590-1606页

作者： Marcos Elias Duarte wanpuech Parnsen Shihai zhang Marvio l.T.Abreu Sung woo Kim Department of Animal Science North Carolina State UniversityRaleighNC 27695USA

Background low crude protein(CP)formulations with supplemental amino acids(AA)are used to enhance intestinal health,reduce costs,minimize environmental impact,and maintain growth performance of ***,extensive reduction of dietary CP can compromise growth performance due to limited synthesis of non-essential AA and limited availability of bioactive compounds from protein supplements even when AA requirements are ***,implementing a low CP formulation can increase the net energy(NE)content in feeds causing excessive fat *** supplementation of functional AA,coupled with low CP formulation could further enhance intestinal health and glucose metabolism,improving nitrogen utilization,and growth *** experiments were conducted to evaluate the effects of low CP formulations with supplemental AA on the intestinal health and growth performance of growing-finishing *** In Exp.1,90 pigs(19.7±1.1 kg,45 barrows and 45 gilts)were assigned to 3 treatments:CON(18.0%CP,supplementing lys,Met,and Thr),lCP(16.0%CP,supplementing lys,Met,Thr,Trp,and Val),and lCPT(16.1%CP,lCP+0.05%SID Trp).In Exp.2,72 pigs(34.2±4.2 kg Bw)were assigned to 3 treatments:CON(17.7%CP,meeting the requirements of lys,Met,Thr,and Trp);lCP(15.0%CP,meeting lys,Thr,Trp,Met,Val,Ile,and Phe);and VlCP(12.8%CP,meeting lys,Thr,Trp,Met,Val,Ile,Phe,His,and leu).In Exp.3,72 pigs(54.1±5.9 kg Bw)were assigned to 3 treatments and fed experimental diets for 3 phases(grower 2,finishing 1,and finishing 2).Treatments were CON(18.0%,13.8%,12.7%CP for 3 phases;meeting lys,Met,Thr,and Trp);lCP(13.5%,11.4%,10.4%CP for 3 phases;meeting lys,Thr,Trp,Met,Val,Ile,and Phe);and lCPG(14.1%,12.8%,11.1%CP for 3 phases;lCP+Glu to match SID Glu with CON).All diets had 2.6 Mcal/kg *** In Exp.1,overall,the growth performance did not differ among *** lCPT increased(Plaudin-1 expression in the duodenum and *** lCP and lCPT increased(P<0.05)CAT-1,4F2hc,and B0AT exp

关键词： Amino acids Growing-finishing pigs Growth performance Intestinal health low crude protein formulation Net energy

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Continued evolution of H10N3 influenza virus with adaptive mutations poses an increased threat to mammals

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Virologica Sinica 2024年第4期39卷 546-555页

作者： Ding S. Zhou J. Xiong J. Du X. Yang w. Huang J. liu Y. Huang l. liao M. zhang J. Qi w. State Key laboratory for Animal Disease Control and Prevention South China Agricultural University Guangzhou 510642 China National Avian Influenza Para-Reference laboratory Guangzhou 510642 China Key laboratory of Zoonoses Ministry of Agriculture and Rural Affairs Guangzhou 510642 China National and Regional Joint Engineering laboratory for Medicament of Zoonoses Prevention and Control Guangzhou 510642 China College of Animal Science and Technology Zhongkai University of Agriculture and Engineering Guangzhou 510550 China Key laboratory of Zoonoses Prevention and Control of Guangdong Province Guangzhou 510642 China State Key laboratory of Agricultural Microbiology College of Veterinary Medicine Huazhong Agricultural University Wuhan 430070 China

The H10 subtype avian influenza virus (AIV) poses an ongoing threat to both birds and humans. Notably, fatal human cases of H10N3 and H10N8 infections have drawn public attention. In 2022, we isolated two H10N3 viruses (A/chicken/Shandong/0101/2022 and A/chicken/Shandong/0603/2022) from diseased chickens in China. Genome analysis revealed that these viruses were genetically associated with human-origin H10N3 virus, with internal genes originating from local H9N2 viruses. Compared to the H10N8 virus (A/chicken/Jiangxi/102/2013), the H10N3 viruses exhibited enhanced thermostability, increased viral release from erythrocytes, and accumulation of hemagglutinin (HA) protein. Additionally, we evaluated the pathogenicity of both H10N3 and H10N8 viruses in mice. we found that viral titers could be detected in the lungs and nasal turbinates of mice infected with the two H10N3 viruses, whereas H10N8 virus titers were detectable in the lungs and brains of mice. Notably, the proportion of double HA Q222R and G228S mutations in H10N3 viruses has increased since 2019. However, the functional roles of the Q222R and G228S double mutations in the HA gene of H10N3 viruses remain unknown and warrant further investigation. Our study highlights the potential public health risk posed by the H10N3 virus. A spillover event of AIV to humans could be a foretaste of a looming pandemic. Therefore, it is imperative to continuously monitor the evolution of the H10N3 influenza virus to ensure targeted prevention and control measures against influenza outbreaks. © 2024 The Authors

关键词： Avian influenza virus (AIV) Evolution H10N3 Pathogenicity

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