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Selection of Negative Charged Acidic Polar Additives to Regulate Electric Double Layer for Stable Zinc Ion Battery

Nano-Micro Letters 2024年第12期16卷 342-356页

作者： Xing Fan Lina Chen Yongjing Wang Xieyu Xu Xingxing Jiao Peng zhou Yangyang Liu Zhongxiao Song jiang zhou State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an 710049People’s Republic of China School of Materials Science and Engineering Harbin Institute of Technology(Shenzhen)Shenzhen 518055People’s Republic of China Research Institute of Frontier Science Southwest Jiaotong UniversityChengdu 610031People’s Republic of China Hunan Provincial Key Defense Laboratory of High Temperature Wear-Resisting Materials and Preparation Technology Hunan University of Science and TechnologyXiangtan 411201People’s Republic of China School of Instrument Science and Technology Xi’an Jiaotong UniversityXi’an 710049People’s Republic of China School of Materials Science and Engineering Hunan Provincial Key Laboratory of Electronic Packaging and Advanced Functional MaterialsCentral South UniversityChangsha 410083People’s Republic of China

Zinc-ion batteries are promising for large-scale electrochemical energy storage systems,which still suffer from interfacial issues,e.g.,hydrogen evolution side reaction(HER),self-corrosion,and uncontrollable dendritic Zn *** the regulation of electric double layer(EDL)has been verified for interfacial issues,the principle to select the additive as the regulator is still ***,several typical amino acids with different characteristics were examined to reveal the interfacial behaviors in regulated EDL on the Zn *** charged acidic polarity(NCAP)has been unveiled as the guideline for selecting additive to reconstruct EDL with an inner zincophilic H_(2)O-poor layer and to replace H_(2)O molecules of hydrated Zn^(2+)with NCAP *** the synergistic effects of EDL regulation,the uncontrollable interface is significantly stabilized from the suppressed HER and anti-self-corrosion with uniform ***,by adding NCAP glutamate,a high average Coulombic efficiency of 99.83%of Zn metal is achieved in Zn|Cu asymmetrical cell for over 2000 cycles,and NH4V4O10|Zn full cell exhibits a high-capacity retention of 82.1%after 3000 cycles at 2 A g^(-1).Recapitulating,the NCAP principle posted here can quicken the design of trailblazing electrolyte additives for aqueous Zn-based electrochemical energy storage systems.

关键词： Aqueous Zn-ion batteries Zn metal anode Negative charged acidic polar additives Electric double-layer regulation

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Growth of two-inch free-standing heteroepitaxial diamond on Ir/YSZ/Si(001)substrates via laser-patterned templates

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Journal of Semiconductors 2024年第9期45卷 4-6页

作者： Pengfei Qu Peng Jin Guangdi zhou zhen Wang Zhanguo Wang Laboratory of Solid-State Optoelectronic Information Technology Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

As an ultra-wide bandgap semiconductor,diamond garners significant interest due to its exceptional physical properties^([1–3]).These superior characteristics make diamonds highly promising for applications in power electronics^([4]),deep-ultraviolet detectors^([5]),high-energy particle detectors^([6]),and quantum devices based on color centers^([7]).

关键词： template exceptional diamond

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Bifurcation analysis of an SIS epidemic model with a generalized non-monotonic and saturated incidence rate

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International Journal of Biomathematics 2024年第4期17卷 39-73页

作者： Chunxian Huang zhenkun jiang Xiaojun Huang Xiaoliang zhou School of Mathematics and Statistics Lingnan Normal University Zhanjiang Guangdong 524048P.R.China

In this paper,a new generalized non-monotonic and saturated incidence rate was introduced into a susceptible-infected-susceptible(SIS)epidemic model to account for inhibitory effect and crowding *** dynamic properties of the model were studied by qualitative theory and bifurcation *** is shown that when the infuence of psychological factors is large,the model has only disease-free equilibrium point,and this disease-free equilibrium point is globally asymptotically stable;when the influence of psychological factors is small,for some parameter conditions,the model has a unique endemic equilibrium point,which is a cusp point of co-dimension two,and for other parameter conditions the model has two endemic equilibrium points,one of which could be weak focus or *** addition,the results of the model undergoing saddle-node bifurcation,Hopf bifurcation and Bogdanov-Takens bifurcation as the parameters vary were also *** results shed light on the impact of psychological behavior of susceptible people on the disease transmission.

关键词： SIS epidemic model generalized non-monotone and saturated incidence rate saddle-node bifurcation Hopf bifurcation Bogdanov-Takens bifurcation

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An electrochemiluminescent magneto-immunosensor for ultrasensitive detection of hs-cTnI on a microfluidic chip

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Nanotechnology and Precision Engineering 2024年第3期7卷 13-23页

作者： Yun Hui zhen Zhao Weiliang Shu Fengshan Shen Weijun Kong Shengyong Geng zhen Xu Tianzhun Wu Wenhua zhou Xuefeng Yu Shenzhen Key Laboratory of Micro/Nano Biosensing Shenzhen Institutes of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China Shenzhen Institutes of Advanced Technology Chinese Academy of SciencesShenzhen 518055China Biomedical Imaging Science and System Key Laboratory Chinese Academy of SciencesShenzhen 518055China

Sensitive detection and precise quantitation of trace-level crucial biomarkers in a complex sample matrix has become an important area of *** example,the detection of high-sensitivity cardiac troponin I (hs-cTnI) is strongly recommended in clinical guidelines for early diagnosis of acute myocardial *** on the use of an electrode modified by single-walled carbon nanotubes (SWCNTs) and a Ru(bpy)32+-doped silica nanoparticle (Ru@SiO2)/tripropylamine (TPA) system,a novel type of electrochemiluminescent (ECL) magnetoimmunosensor is developed for ultrasensitive detection of *** this approach,a large amount of[Ru(bpy)3]2+is loaded in SiO2(silica nanoparticles) as luminophores with high luminescent efficiency and SWCNTs as electrode surface modification material with excellent electrooxidation ability for ***,a hierarchical micropillar array of microstructures is fabricated with a magnet placed at each end to efficiently confine a single layer of immunomagnetic microbeads on the surface of the electrode and enable 7.5-fold signal enhancement In particular,the use of transparent SWCNTs to modify a transparent ITO electrode provides a two-order-of-magnitude ECL signal amplification.A good linear calibration curve is developed for hs-cTnI concentrations over a wide range from 10 fg/ml to 10 ng/ml,with the limit of detection calculated as 8.720 fg/ml (S/N=3).This ultrasensitive immunosensor exhibits superior detection performance with remarkable stability,reproducibility,and *** recoveries are obtained in the detection of hs-cTnI in human serum,providing a potentia analysis protocol for clinical applications.

关键词： Electrochemiluminescent magneto-immunosensor Microﬂuidic chip High-sensitivity cardiac troponin I Single-walled carbon nanotube [Ru(bpy)3]2+-doped silica nanoparticle

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Unlocking supercapacitive energy storage potential:Catalyzing electrochemically inactive manganese oxides to active MnO_(2)via heterostructure reconstruction

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Nano Research 2024年第7期17卷 5897-5906页

作者： Baohong Zhang Tao jiang Xinyan zhou Xiaoyu Fan Binbin Jia Lidong Li School of Chemistry Beihang UniversityBeijing 100191China College of Materials and Chemical Engineering Key Laboratory of Inorganic Nonmetallic Crystalline and Energy Conversion MaterialsChinaThree Gorges UniversityYichang 443002China Chinese Academy of Sciences(CAS)Key Laboratory of Nanosystem and Hierarchy Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190China Shanghai GTX Semiconductor Co. Ltd.Shanghai 201806China

Advancing supercapacitor system performance hinges on the innovation of novel electrode materials seamlessly integrated within distinct ***,we introduce a direct approach for crafting nanorod arrays featuring crystalline/amorphous CuO/MnO_(2)−*** reconfigured heterostructure results in an elevated content of electrochemically active MnO_(2).The nanorod arrays serve as efficient capacitive anodes and are easily prepared via low-potential electrochemical *** resulting structure spontaneously forms a p–n heterojunction,developing a built-in electric field that dramatically facilitates the charge transport *** intrinsic electric field,in conjunction with the crystalline/amorphous architecture,enables a large capacitance of 1.0 F·cm^(−2)at 1.0 mA·cm^(−2),an ultrahigh rate capability of approximately 85.4%at 15 mA·cm^(−2),and stable cycling performance with 92.4%retention after 10,000 *** calculations reveal that the presence of heterojunctions allows for the optimization of the electronic structure of this composite,leading to improved conductivity and optimized OH−adsorption *** work provides new insights into the rational design of heterogeneous nanostructures,which hold great potential in energy storage applications.

关键词： reconfiguration active MnO_(2) crystalline/amorphous structure p-n heterojunction supercapacitor

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Rh(Ⅱ)-catalyzed intermolecular carboamination of pyridines via double Csp^(2)-H bond activations

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Science China Chemistry 2024年第1期67卷 374-382页

作者： Zhongfeng Luo Jingxing jiang Lifang Zou Xiaoyu zhou Junshan Liu Zhuofeng Ke Fengjuan Chen Huanfeng jiang Wei Zeng Key Laboratory of Functional Molecular Engineering of Guangdong Province School of Chemistry and Chemical EngineeringSouth China University of TechnologyGuangzhou 510641China School of Materials Science and Engineering PCFM LabSun Yat-sen UniversityGuangzhou 510275China Guangdong Provincial Key Laboratory of Chinese Medicine Pharmaceutics School of Traditional Chinese MedicineSouthern Medical UniversityGuangzhou 510515China

We disclose the development of the Rh-catalyzed amine-directed remote 5,6-carboamination protocol of pyridines via dual Csp^(2)-H functionalizations.A variety of readily available 2-aminopyridines and 1,2,3-triazoles are allowed for coupling cyclization to access polyfunctionalized *** studies including DFT calculations unveil that relay carbenoidelectrophilic addition to pyridines and the sequential pyridyl Csp^(2)-H amination are involved in this *** postsynthetic utility of this methodology is showcased by versatile and site-selective modification of azaindoles.

关键词： Rh-catalysis azaindoles pyridyl Csp^(2)-H bond carboamination coupling-cyclization

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Traditional Meiyu-Baiu has been suspended by global warming

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National Science Review 2024年第7期11卷 126-134页

作者： Zhicong Yin Xiaolei Song Botao zhou Wenhao jiang Huopo Chen Huijun Wang Key Laboratory of Meteorological Disaster Ministry of Education/Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University of Information Science&Technology Nansen-Zhu International Research Centre Institute of Atmospheric PhysicsChinese Academy of Sciences

More than 1000 years, the Meiyu–Baiu have shaped the uniqueness of natural resources, civilization and culture in the Yangtze River Basin of China and the main islands of Japan. In recent decades, frequent rainstorms and droughts have seemingly diminished the misty features of traditional Meiyu–Baiu ***, there is still no consensus on whether their traditional nature is suspended. In this study, we quantitatively demonstrate that the Meiyu–Baiu almost completely lost their traditional features during 1961–2023, ～80% of which can be attributed to anthropogenic warming. Furthermore, in a warmer future,the traditional Meiyu–Baiu will be more unlikely to appear. This study underscores the urgency in adapting to climate shift because destructive extremes are measurably taking the place of mild and maternal rains.

关键词： global warming Meiyu–Baiu extremes human activity culture and civilization

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Prediction of Coefficient of Restitution for Impact Elastoplastic Spheres Considering Finite Plate Thickness

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Chinese Journal of Mechanical Engineering 2024年第4期37卷 183-193页

作者： Yunfeng Fan Hao Wang Tao zhou Limin Zou Zhinong jiang Minghui Hu State Key Laboratory of High-end Compressor and System Technology Beijing University of Chemical TechnologyBeijing 100029China China Ship Research and Development Academy Beijing 100101China Key Lab of Engine Health Monitoring-Control and Networking of Ministry of Education Beijing University of Chemical TechnologyBeijing 100029China Beijing Key Laboratory of High-End Mechanical Equipment Health Monitoring and Self-Recovery Beijing University of Chemical TechnologyBeijing 100029China

Collisions between objects are a relatively common phenomenon in *** of collision processes can greatly contribute to solving problems such as impact-rub faults and particle *** coefficient of restitution is a critical parameter in the analysis of collision *** experiments have shown that the coefficient of restitution is closely related to the plate thickness,and the smaller the plate thickness,the more inaccurate the coefficient of restitution predicted by the existing model,which seriously affects the process of collision *** remedy this shortcoming,this paper proposes a plate thickness influence factor with the ratio of sphere diameter to plate thickness as the *** plate thickness influence factor can optimize the coefficient of restitution model to effectively predict the coefficient of restitution of impacting elastoplastic spheres with finite plate ***,the validity of the new model is verified using a large amount of experimental data.

关键词： Collision Coefficient of restitution Energy loss Sphere

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Evolving molecular subtyping of breast cancer advances precision treatment

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Cancer Biology & Medicine 2024年第9期21卷 731-739页

作者： Rui Shan Lei-Jie Dai Zhi-Ming Shao Yi-zhou jiang Department of Breast Surgery Fudan University Shanghai Cancer CenterShanghai 200032China Department of Oncology Shanghai Medical CollegeFudan UniversityShanghai 200032China

Breast cancer is the second most prevalent cancer *** 2022,approximately 2.3 million newly diagnosed cases of female breast cancer occurred worldwide,and more than 665 thousand people lost their lives to this disease^... 详细信息

关键词： breast cancer Breast

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Sulphur-template method for facile manufacturing porous silicon electrodes with enhanced electrochemical performance

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Chinese Chemical Letters 2024年第8期35卷 433-436页

作者： Peng zhou Ziang jiang Yang Li Peng Xiao Feixiang Wu Powder Metallurgy Research Institute School of Metallurgy and EnvironmentCentral South UniversityChangsha 410083China

Sulphur(S)-template method based on conventional slurry-casting method has been developed to pro-duce porous silicon(Si)*** facile fabrication technology is suitable for current production line and expected to be widely applied to various electrode materials under large volume change during ***,S particles as template agent are mixed with active material Si,carbon conductor and binder forming uniform *** casting and drying,the electrodes are immersed in carbon disul-fide solution to remove S particles rapidly,generating pores in-situ at the original position of S *** analysis shows that the pores inside electrodes are able to shorten lithium ion diffusion paths,reduce normal expansion rate and decrease formation of cracks in the Si electrode(2 mg_(Si)/cm^(2)),demonstrating a reversible capacity of 951 mAh/g at 0.5 A/g after 100 cycles(with a capacity retention of 99.5%)and a capacity of-826 mAh/g at 2 A/g.

关键词： Sulphur-template Porous electrodes Silicon anodes Low volume expansion Lithium-ion batteries

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