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Corrosion and in vitro cytocompatibility investigation on the designed Mg-Zn-Ag metallic glasses for biomedical application

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Journal of Magnesium and Alloys 2024年第4期12卷 1566-1580页

作者： Jian wang Lingzhong Meng Weixin Xie Chen Ji Ronghua wang Pinghu Zhang Liling Jin Liyuan Sheng yufeng Zheng School of Mechanical Engineering Yangzhou UniversityYangzhou225127China Department of Materials Science and Engineering Seoul National UniversitySeoulSouth Korea Huizhou Port Customs Huizhou516081China Jiangsu Key Laboratory of Integrated Traditional chinese and Western Medicine for Prevention and Treatment of Senile Diseases Institute of Translational MedicineMedical CollegeYangzhou UniversityYangzhou225009China Center for Research in Computational Thermochemistry(CRCT) Department of Chemical EngineeringEcole polytechnique de MontréalMontréalQuébecH3C 3A7Canada Shenzhen Institute Peking UniversityShenzhen 518057China PKU-HKUST ShenZhen-HongKong Institution Shenzhen518057China

In the present work,seven Mg-Zn-Ag alloys with the nominal composition of Mg_(96-x)Zn_(x)Ag_(4)(x=17,20,23,26,29,32,35 in at.%)were prepared by induction melting and single-roller *** X-ray diffraction(XRD)analyses indicate the metallic glasses with three composition of Mg_(73)Zn_(23)Ag_(4),Mg_(70)Zn_(26)Ag_(4),and Mg_(67)Zn_(29)Ag_(4)were obtained *** differential scanning calorimetry(DSC)measurement was used to obtain the characteristic temperature of Mg-Zn-Ag metallic glasses for the glass-forming ability *** maximum glass transition temperature(Trg)was found to be 0.525 with a composition close to Mg_(67)Zn_(29)Ag_(4),which results in the best glass-forming ***,the immersion test in simulated body fluid(SBF)demonstrate the relative homogeneous corrosion behavior of the Mg-Zn-Ag metallic *** corrosion rate of Mg-Zn-Ag metallic glasses in SBF solution decreases with the increase of Zn *** sample Mg_(67)Zn_(29)Ag_(4)has the lowest corrosion rate of 0.19mm/yr,which could meet the clinical application requirement *** in vitro cell experiments show that the Madin-Darby canine kidney(MDCK)cells cultured in sample Mg_(67)Zn_(29)Ag_(4)and its extraction medium have higher ***,the Mg-Zn-Ag metallic glasses exhibit obvious inhibitory effect on human rhabdomyosarcoma(RD)tumor *** present investigations on the glass-forming ability,corrosion behavior,cytocompatibility and tumor inhibition function of the Mg-Zn-Ag based metallic glass could reveal their biomedical application possibility.

关键词： Metallic glasses Mg-Zn-Ag Corrosion behavior In vitro cytocompatibility

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Room-temperature Self-healing and Recyclable PDMS Elastomers with Superior Mechanical Properties for Triboelectric Nanogenerators

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chinese Journal of Polymer Science 2024年第10期42卷 1566-1577,I0014页

作者： Shu-Juan wang Lu wang Hong-Zhe Su Zhi-Cheng Wu Qiao-Gen Zhang Wei Fan Xin-Li Jing School of Chemistry Joint Innovation Center of Thermal Protection MaterialsXi’an Jiaotong UniversityXi’an710049China School of Electrical Engineering Xi’an Jiaotong UniversityXi’an710049China School of Textile Science and Engineering Xi’an Polytechnic UniversityXi’an710048China

Polydimethylsiloxane(PDMS)is an electron-withdrawing material that is widely used in triboelectric nanogenerators(TENGs).However,PDMS has poor mechanical properties after curing and is easily damaged when subjected to long-term ***,the long-term stable operation of TENGs under mechanical deformation cannot be *** this work,multiple hydrogen bonds and aromatic disulfide bonds were introduced into PDMS *** elastomers exhibited high toughness(a tensile strength of 1.91 MPa and an elongation at break of 340%),good recyclability,and room-temperature self-healing properties(healing efficiency of 96.4%in 24 h).Recyclable sandwich-like triboelectric nanogenerators with excellent electrical output performance(13.5 V)and room-temperature self-healing performance(24 h,98%recovery of self-generating performance)were prepared by utilizing the hydrogen bonding between the PDMS elastomer and *** work reported herein offers theoretical guidance and a compelling strategy for developing high-performance TENG negative friction layers.

关键词： Polydimethylsiloxane Aromatic disulfide bonds Hydrogen bonds Room temperature self-healing Triboelectric nanogenerator

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共同富裕进程中的数字普惠金融作用研究——基于我国254个地级市面板数据的分析

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经济问题 2024年第6期 1-9页

作者：方先明王宇南京大学商学院江苏南京210093

数字普惠金融利用数字技术手段实现金融服务的“精准滴灌”与“低成本覆盖”,为实现共同富裕提供了重要抓手。首先,基于“发展与共享”理念测度地级市共同富裕水平;然后,以我国254个地级市的面板数据检验数字普惠金融对共同富裕的作用... 详细信息

数字普惠金融利用数字技术手段实现金融服务的“精准滴灌”与“低成本覆盖”,为实现共同富裕提供了重要抓手。首先,基于“发展与共享”理念测度地级市共同富裕水平;然后,以我国254个地级市的面板数据检验数字普惠金融对共同富裕的作用。结果表明:总体上,数字普惠金融发展能够显著促进共同富裕水平的提升;细分子维度来看,数字普惠金融覆盖广度、使用深度和数字化程度均能显著促进共同富裕水平提升;区域数字基础设施建设能正向调节数字普惠金融的促进作用。拓展性分析表明,数字普惠金融对共同富裕的促进作用存在非线性,以数字普惠金融指数、产业结构、教育水平和城镇化水平作为门槛变量时,这种非线性关系均显著。研究结果不仅为数字普惠金融发展能够促进共同富裕提供了经验证据,而且还揭示了“完善数字基础设施建设,充分消弭数字鸿沟”“关注数字普惠金融门槛效应,充分释放数字红利”是进一步发挥数字普惠金融促进作用的关键要点。

关键词：数字普惠金融发展与共享共同富裕门槛效应

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差异与多元:列斐伏尔都市空间问题的方法论探索

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苏州大学学报（哲学社会科学版） 2024年第5期45卷 19-27页

作者：车玉玲王洁苏州大学哲学系江苏苏州215123

在当代大都市社会,资本主义根据自己需要的样态塑造了都市空间,空间自身的生产成为资本增殖的新途径。以资本逻辑建构的当代都市空间,具有单调性与同质性的鲜明特征。列斐伏尔作为都市马克思主义学派的代表人物,不仅开辟了社会批判理论... 详细信息

在当代大都市社会,资本主义根据自己需要的样态塑造了都市空间,空间自身的生产成为资本增殖的新途径。以资本逻辑建构的当代都市空间,具有单调性与同质性的鲜明特征。列斐伏尔作为都市马克思主义学派的代表人物,不仅开辟了社会批判理论的空间转向,在分析都市空间问题时也采用了不同于以往社会批判理论的新方法。列斐伏尔指出,当前人类历史已进入具有后现代特征的都市时代,继续沿用现代性的分析工具已经无法解决后现代的都市问题,因此必须建构与当代都市空间相符合的方法论原则,即“都市总问题式”“三元空间辩证法”和“节奏分析的方法论”,才能恢复差异与多元在都市空间的地位,从而实现总体的人的解放。当前中国城镇化正处于高速发展时期,如何避免西方城镇化发展中的负面效应,走出具有中国特色的社会主义城镇化新道路,是当代城市发展研究的必要议题。列斐伏尔城市方法论研究的“空间转向”对于研究中国当代城市问题具有启示意义。

关键词：列斐伏尔都市空间方法论都市总问题式三元辩证法节奏分析

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飞机防除冰机理及超疏水材料的机载应用

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科学技术与工程 2024年第1期24卷 72-87页

作者：王瑜王歆铖南京工业大学城市建设学院南京211816

飞机表面结冰改变飞机的飞行动力学特性,严重威胁了飞行安全,因此飞机防除冰技术对于安全飞行有重要意义。首先,通过分析飞机结冰的基本原理、类型、影响等,介绍现有的防除冰技术的方法及优缺点对比,详细综述了超疏水材料的润湿性模型... 详细信息

飞机表面结冰改变飞机的飞行动力学特性,严重威胁了飞行安全,因此飞机防除冰技术对于安全飞行有重要意义。首先,通过分析飞机结冰的基本原理、类型、影响等,介绍现有的防除冰技术的方法及优缺点对比,详细综述了超疏水材料的润湿性模型、机理等,同时对超疏水材料研究现状进行了全面综述并对其特定条件(超疏水特性失效)进行分析,特别指出了存在的问题和挑战。其次,在单一防除冰系统缺陷的基础上提出了复合型防除冰系统,并对几种复合防除冰系统进行介绍且将其与单一防除冰系统进行对比。此外,针对超疏水材料应用可能出现的问题,提出了一种回路热管+超疏水材料相结合的飞机防除冰系统。最后,就超疏水表面与复合型防除冰系统存在的问题进行分析与展望,认为主被动复合型防除冰系统具有良好的应用潜力。

关键词：结冰机理超疏水表面回路热管复合型防除冰系统

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Strain sensor on a chip for quantifying the magnitudes of tensile stress on cells

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Microsystems & Nanoengineering 2024年第3期10卷 305-315页

作者： yuyin Zhang yue wang Hongze Yin Jiahao wang Na Liu Songyi Zhong Long Li Quan Zhang Tao yue School of Mechatronics Engineering and Automation Shanghai UniversityShanghaiChina School of Future Technology Shanghai UniversityShanghaiChina Key Laboratory of Advanced Manufacturing Technology of Zhejiang Province School of Mechanical EngineeringZhejiang UniversityHangzhouChina Shanghai Key Laboratory of Intelligent Manufacturing and Robotics Shanghai UniversityShanghaiChina Shanghai Institute of Intelligent Science and Technology Tongji UniversityShanghaiChina

During cardiac development,mechanotransduction from the in vivo microenvironment modulates cardiomyocyte growth in terms of the number,area,and arrangement ***,the response of cells to different degrees of mechanical stimuli is ***-on-a-chip,as a platform for investigating mechanical stress stimuli in cellular mimicry of the in vivo microenvironment,is limited by the lack of ability to accurately quantify externally induced ***,previous technology lacks the integration of external stimuli and feedback sensors in microfluidic platforms to obtain and apply precise amounts of external ***,we designed a cell stretching platform with an in-situ *** in-situ liquid metal sensors can accurately measure the mechanical stimulation caused by the deformation of the vacuum cavity exerted on *** platform was applied to human cardiomyocytes(AC16)under cyclic strain(5%,10%,15%,20 and 25%),and we found that cyclic strain promoted cell growth induced the arrangement of cells on the membrane to gradually unify,and stabilized the cells at 15%amplitude,which was even more effective after 3 days of *** platform’s precise control and measurement of mechanical forces can be used to establish more accurate in vitro microenvironmental models for disease modeling and therapeutic research.

关键词： stress deformation arrangement

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Enhanced Photocatalytic Activity of Z-scheme Meso-BiVO_(4)-Au-CdS for Degradation of Rhodamine B

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Journal of Wuhan University of Technology(Materials Science) 2024年第4期39卷 869-876页

作者：张雁伟 wang Yanze LI Junguo XIE Jingjing 王文宣 FU Zhengyi State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Hubei Longzhong Laboratory Xiangyang 441000China

We synthesized BiVO_(4)mesocrystals with ordered assembly structure,and studied the structural order and the relationship between the photodegradation of Rhodamine *** nanoparticles(NPs)were successfully loaded onto Meso-BiVO_(4)by light-assisted induction,and Cd nanoparticles were further selected to be deposited on Au nanoparticles to form Z-scheme photocatalyst Meso-BiVO_(4)-Au-CdS *** try and propose to analyze its ordered assembly structure by XRD for the first *** results show that Meso-BiVO_(4)is a mesocrystal with highly exposed(001)plane and directional assembly *** charge separation efficiency of all samples was studied by PL *** results show that the Z-scheme Meso-BiVO_(4)-Au-CdS can promote the charge separation and obtain the best carrier separation ***,it has the best photocatalytic activity in the experiment of photocatalytic degradation of rhodamine *** main active species in the degradation process were confirmed by free radical trapping experiment,and the degradation mechanism was put forward.

关键词： biomineralization photosynthesis mesocrystal photocatalysis TiO_(2) BiVO_(4)

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Evolution of the porous structure for phosphoric acid etching carbon as cathodes in Li–O_(2) batteries:Pyrolysis temperature-induced characteristics changes

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Carbon Energy 2024年第1期6卷 172-181页

作者： Feiyang Yang Ying Yao yunkai Xu Cong wang Meiling wang Jingjie Ren Cunzhong Zhang Feng Wu Jun Lu Beijing Key Laboratory of Environmental Science and Engineering School of Materials Science and EngineeringBeijing Institute of TechnologyBeijingChina Beijing Institute of Technology Chongqing Innovation Center ChongqingChina College of Chemical and Biological Engineering Zhejiang UniversityHangzhouChina

Although biomass-derived carbon(biochar)has been widely used in the energy field,the relation between the carbonization condition and the physical/chemical property of the product remains ***,we revealed the carbonization condition's effect on the morphology,surface property,and electrochemical performance of the obtained *** open slit pore structure with shower-puff-like nanoparticles can be obtained by finely tuning the carbonization temperature,and its unique pore structure and surface properties enable the Li–O_(2) battery with cycling longevity(221 cycles with 99.8%Coulombic efficiency at 0.2 mA cm^(−2) and controlled discharge–charge depths of 500 mAh g^(−1))and high capacity(16,334 mAh g^(−1) at 0.02 mA cm^(−2)).This work provides a greater understanding of the mechanism of the biochar carbonization procedure under various pyrolysis conditions,paving the way for future study of energy storage devices.

关键词： biomass Li-O_(2) battery oxygen catalysts porous carbon temperature parameters

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Tailoring Classical Conditioning Behavior in TiO_(2) Nanowires:ZnO QDs-Based Optoelectronic Memristors for Neuromorphic Hardware

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Nano-Micro Letters 2024年第7期16卷 265-280页

作者： Wenxiao wang Yaqi wang Feifei Yin Hongsen Niu Young-Kee Shin Yang Li Eun-Seong Kim Nam-Young Kim School of Information Science and Engineering University of JinanJinan 250022People’s Republic of China RFIC Centre NDAC CentreKwangwoon UniversityNowon-guSeoul 139-701South Korea Department of Electronics Engineering Kwangwoon UniversityNowon-GuSeoul 139-701South Korea School of Microelectronics Shandong UniversityJinan 250101People’s Republic of China Department of Molecular Medicine and Biopharmaceutical Sciences Seoul National UniversitySeoul 08826South Korea

Neuromorphic hardware equipped with associative learn-ing capabilities presents fascinating applications in the next generation of artificial ***,research into synaptic devices exhibiting complex associative learning behaviors is still ***,an optoelec-tronic memristor based on Ag/TiO_(2) Nanowires:ZnO Quantum dots/FTO was proposed and constructed to emulate the biological associative learning *** implementation of synaptic behaviors,including long and short-term plasticity,and learning-forgetting-relearning behaviors,were achieved in the device through the application of light and electrical *** the optoelectronic co-modulated characteristics,a simulation of neuromorphic computing was conducted,resulting in a handwriting digit recognition accuracy of 88.9%.Furthermore,a 3×7 memristor array was constructed,confirming its application in artificial visual *** importantly,complex biological associative learning behaviors were emulated by mapping the light and electrical stimuli into conditioned and unconditioned stimuli,*** training through associative pairs,reflexes could be triggered solely using light ***-sively,under specific optoelectronic signal applications,the four features of classical conditioning,namely acquisition,extinction,recovery,and generalization,were elegantly *** work provides an optoelectronic memristor with associative behavior capabilities,offering a pathway for advancing brain-machine interfaces,autonomous robots,and machine self-learning in the future.

关键词： Artificial intelligence Classical conditioning Neuromorphic computing Artificial visual memory Optoelectronic memristors ZnO Quantum dots

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Model reduction of fractional impedance spectra for time–frequency analysis of batteries, fuel cells, and supercapacitors

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Carbon Energy 2024年第1期6卷 108-141页

作者： Weiheng Li Qiu-An Huang yuxuan Bai Jia wang Linlin wang yuyu Liu yufeng Zhao Xifei Li Jiujun Zhang Institute for Sustainable Energy/College of Sciences Shanghai UniversityShanghaiChina Shanxi Key Laboratory of Nanomaterials and Nanotechnology School of Mechanical and Electrical EngineeringXi'an University of Architecture and TechnologyXi'anShaanxiChina Xi'an Key Laboratory of New Energy Materials and Devices School of Materials Science and EngineeringInstitute of Advanced Electrochemical EnergyXi'an University of TechnologyXi'anShaanxiChina

Joint time–frequency analysis is an emerging method for interpreting the underlying physics in fuel cells,batteries,and *** increase the reliability of time–frequency analysis,a theoretical correlation between frequency-domain stationary analysis and time-domain transient analysis is urgently *** present work formularizes a thorough model reduction of fractional impedance spectra for electrochemical energy devices involving not only the model reduction from fractional-order models to integer-order models and from high-to low-order RC circuits but also insight into the evolution of the characteristic time constants during the whole reduction *** following work has been carried out:(i)the model-reduction theory is addressed for typical Warburg elements and RC circuits based on the continued fraction expansion theory and the response error minimization technique,respectively;(ii)the order effect on the model reduction of typical Warburg elements is quantitatively evaluated by time–frequency analysis;(iii)the results of time–frequency analysis are confirmed to be useful to determine the reduction order in terms of the kinetic information needed to be captured;and(iv)the results of time–frequency analysis are validated for the model reduction of fractional impedance spectra for lithium-ion batteries,supercapacitors,and solid oxide fuel *** turn,the numerical validation has demonstrated the powerful function of the joint time–frequency *** thorough model reduction of fractional impedance spectra addressed in the present work not only clarifies the relationship between time-domain transient analysis and frequency-domain stationary analysis but also enhances the reliability of the joint time–frequency analysis for electrochemical energy devices.

关键词： battery,fuel cell,supercapacitor fractional impedance spectroscopy model reduction time-frequency analysis

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