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Enhanced Photocatalytic H_(2)-production Activity of CdS Nanoflower using Single Atom Pt and Graphene Quantum Dot as Dual Cocatalysts

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Chinese Journal of Structural Chemistry 2022年第6期41卷 6-14页

作者： Yi Yang Jinsong Wu Bei Cheng Liuyang Zhang Ahmed Abdullah Al-Ghamdi swelm wageh Youji Li State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Nanostructure Research Centre(NRC)Wuhan University of TechnologyWuhan 430070China Laboratory of Solar Fuel Faculty of Materials Science and ChemistryChina University of GeosciencesWuhan 430074China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia College of Chemistry and Chemical engineering Jishou UniversityJishouHunan 416000China

Single-atom catalysts have high catalytic activity due to their unique quantum size effects and optimal atom utilization.Herein,visi-ble-light-responsive photocatalysts were designed by coupling CdS with graphene quantum dots(GQDs)and platinum single atoms(PtSAs).GQDs and PtSAs were successively loaded on ultrathin CdS nanosheets through freeze-drying and in-situ photocatalytic reduction.The synergistic effect between PtSAs and GQDs results in superior photocatalytic activity with a hydrogen production rate of 13488μmol h^(-1)g^(-1)as well as the maximum apparent quantum efficiency(AQE)of 35.5%in lactic acid aqueous solution,which is 62 times higher than that of pristine CdS(213μmol g^(-1)h^(-1)).The energy conversion efficiency is ca.13.05%.As a photosensitizer and an electron reservoir,GQDs can not only extend the light response of CdS to the visible-light region(400-800 nm),but also promotes the separation of photoinduced electron-hole pairs.Meanwhile,PtSAs,with unique electronic and geometric features,can provide more efficient proton reduction sites.This finding provides an effective strategy to remarkably improve the photocatalytic H_(2) production performance.

关键词： hierarchical nanostructure single-atom catalysts graphene quantum dots CdS nanosheets hydrogen production

一种乳酸菌-金属有机框架复合物用于强化肿瘤乏氧光动力和免疫治疗

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Science China Materials 2023年第1期66卷 363-374页

作者：李田忠王金勇陈桐楷 swelm wageh Ahmed AAl-Ghamdi 于江天谢中建张晗 Interdisciplinary Center of High Magnetic Field Physics of Shenzhen University College of Physics and Optoelectronic EngineeringDepartment of OtolaryngologyShenzhen Institute of Translational MedicineShenzhen Second People’s Hospitalthe First Affiliated HospitalShenzhen UniversityShenzhen 518060China Shenzhen International Institute for Biomedical Research Shenzhen 518000China Science and Technology Innovation Center Guangzhou University of Chinese MedicineGuangzhou 510405China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia Institute of Pediatrics Shenzhen Children’s HospitalShenzhen 518038China

开发长期有效的癌症治疗技术仍然是科研工作者和临床医生面临的重要任务.厌氧型乳酸菌(LAB)具有天然的乏氧倾向性,可自发富集在缺氧的肿瘤微环境中.金属有机框架(MOF)是一类独特的纳米材料,其中的ZIF-67可以自发分解过氧化氢产氧,且析... 详细信息

开发长期有效的癌症治疗技术仍然是科研工作者和临床医生面临的重要任务.厌氧型乳酸菌(LAB)具有天然的乏氧倾向性,可自发富集在缺氧的肿瘤微环境中.金属有机框架(MOF)是一类独特的纳米材料,其中的ZIF-67可以自发分解过氧化氢产氧,且析氧能力可被光照增强.然而,LAB或MOF单独应用于肿瘤治疗的效果并不令人满意.在本文中,我们制备了一种MOF修饰的乳酸菌制剂,用以在缺氧性肿瘤中局部产生活性氧(ROS)助力光动力治疗,同时精准诱导宿主肿瘤免疫.这些细菌表面被ZIF-67纳米材料修饰(LAB@ZIF-67),经体内循环后富集在肿瘤微环境中.细菌表面的ZIF-67可以被CT-26细胞吸收,并且在光照后检测到细胞内快速生成ROS.体内实验表明,该细菌复合物可通过光动力疗法消灭肿瘤,同时诱导肿瘤特异的炎性反应,招募巨噬细胞和T细胞实现肿瘤的免疫治疗.此类材料-细菌复合物为今后研发肿瘤主动靶向药物和癌症免疫疗法提供了新思路.

关键词：肿瘤微环境金属有机框架光动力免疫治疗肿瘤免疫缺氧性巨噬细胞厌氧型

核壳Au@NiS;助催化剂实现高效TiO;光催化制氢（英文）

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物理化学学报 2022年

作者： swelm wageh Ahmed A.Al-Ghamdi 徐全龙 Department of Physics， Faculty of Science， King Abdulaziz University 温州大学化学与材料工程学院，浙江省碳材料技术研究重点实验室

The convertion of solar energy into hydrogen energy with high energy density by photocatalysis is a green and eco-friendly avenue to solve the energy crisis and environmental pollution issues;. Unfortunately， most photocatalysts usually suffer from the rapid quenching of photogenerated carriers and depressed interfacial H;-generation dynamics;.

关键词：

Fully depleted vdW heterojunction based high performance photovoltaic photodetector

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Journal of Materiomics 2023年第6期9卷 1039-1047页

作者： Yonghong Zeng Fanxu Meng Sidi Fan Pengfei Wang Cuiyun Kou Mingyi Sun Haiguo Hu Rui Cao swelm wageh Omar A.Al-Hartomy Abul Kalam Bowen Du Wenchao Ding Songrui Wei Zhinan Guo Qiuliang Wang Han Zhang College of Physics and Optoelectronic Engineering Institute of Microscale OptoelectronicsInternational Collaborative Laboratory of 2D Materials for Optoelectronics Science and TechnologyInterdisciplinary Center of High Magnetic Field Physics of Shenzhen UniversityShenzhen UniversityShenzhen518060China Guangzhou Key Laboratory of Sensing Materials and Devices Center for Advanced Analytical ScienceSchool of Chemistry and Chemical EngineeringGuangzhou UniversityGuangzhou510006China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah21589Saudi Arabia Research Center for Advanced Materials Science(RCAMS) Department of ChemistryCollege of ScienceKing Khalid UniversityP.O.Box 9004Abha61413Saudi Arabia Foshan Electrical and Lighting Co. LTD64 North Fenjiang RoadFoshanChina Institute of Electrical Engineering Chinese Academy of SciencesBeijing100190China Center of Characterization and Analysis Jilin Institute of Chemical TechnologyJilin132022China

Van der Waals(vdW)heterojunctions,with their unique electronic and optoelectronic properties,have become promising candidates for photodetector applications.Amplifying the contribution of the depletion region in vdW heterojunction,which would enhance both of the collection efficiency and speed of the photogenerated carriers,presents an effective strategy for achieving high performance vdW heterojunction photodetectors.Herein,a fully depleted vdW heterojunction photodetector is built on two-dimensional(2D)semiconductor materials(GaTe and InSe)layered on a pattered bottom electrode in vertical structure,in which the generation and motion of carriers are exclusively achieved in the depletion region.Attributed to the intrinsic built-in electric field,the elimination of series resistance and the depletion region confinement of carriers,the as-fabricated photodetector exhibits prominent photovoltaic properties with a high open-circuit voltage of 0.465 V,as well as photoresponse characteristics with outstanding responsivity,detectivity and photoresponse speed of 63.7 A/W,3.88×10^(13)Jones,and 32.7 ms respectively.The overall performance of this fully depleted GaTe/InSe vdW heterojunctions photodetectors are ranking high among the top level of 2D materials based photodetectors.It indicates the device architecture can provide new opportunities for the fabrication of high-performance photodetectors.

关键词： Two-dimensional material van der waals heterojunction Fully depleted photodetector Photovoltaic

TiO2 nanosheets with exposed {001} facets for photocatalytic applications

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Nano Research 2016年第1期9卷 3-27页

作者： Chimmikuttanda Ponnappa Sajan swelm wageh Ahmed. A. Al-Ghamdi Jiaguo Yu Shaowen Cao State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 China Department of Physics Faculty of Science King Abdulaziz University Jeddah 21589 Saudi Arabia Physics and Engineering Mathematics Department Faculty of Electronic Engineering Menoufia University Menouf32952 Egypt

TiO2 nanosheets with highly reactive {001} facets （{001}-TiO2） have attracted great attention in the fields of science and technology because of their unique properties. In recent years, many efforts have been made to synthesize {001}-TiO2 and to explore their applications in photocatalysis. In this review, we summarize the recent progress in preparing {001}-TiO2 using different techniques such as hydrothermal, solvothermal, alcohothermal, chemical vapor deposition （CVD）, and sol gel-based techniques. Furthermore, the enhanced efficiency of {001}-TiO2 by modification of carbon materials, surface deposition of transition metals, and non-metal doping is reviewed. Then, the applications of {001}-TiOR-based photocatalysts in the degradation of organic dyes, hydrogen evolution, carbon dioxide （CO2） reduction, bacterial disinfection, and dye-sensitized solar cells are summarized. We believe this entire review on TiO2 nanosheets with {001] facets can further inspire researchers in associated fields.

关键词： TiO2,nanosheets,{001} facets,photocatalysis

A CRISPR/Cas12a-empowered surface plasmon resonance platform for rapid and specific diagnosis of the Omicron variant of SARS-CoV-2

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National Science Review 2022年第8期9卷 100-109页

作者： Zhi Chen Jingfeng Li Tianzhong Li Taojian Fan Changle Meng Chaozhou Li Jianlong Kang Luxiao Chai Yabin Hao Yuxuan Tang Omar A.Al-Hartomy swelm wageh Abdullah G.Al-Sehemi Zhiguang Luo Jiangtian Yu Yonghong Shao Defa Li Shuai Feng William J.Liu Yaqing He Xiaopeng Ma Zhongjian Xie Han Zhang Department of Physics Faculty of Science King Abdulaziz University Research Center for Advanced Materials Science (RCAMS) King Khalid University Department of Chemistry College of Science King Khalid University Zhongmin (Shenzhen) Intelligent Ecology Co.Ltd Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic Engineering Shenzhen University Department of Laboratory Medicine Shenzhen Children’s Hospital Optoelectronics Research Center School of Science Minzu University of China NHC Key Laboratory of Biosafety National Institute for Viral Disease Control and Prevention Chinese Center for Disease Control and Prevention Research Unit of Adaptive Evolution and Control of Emerging Viruses Chinese Academy of Medical Sciences Institute of Pathogenic Organism Shenzhen Center for Disease Control and Prevention Shenzhen Engineering Laboratory of Phosphorene and Optoelectronics Respiratory Department Shenzhen Children’s Hospital Institute of Pediatrics Shenzhen Children’s Hospital International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education 3. Shenzhen Institute of Translational Medicine 4. Department of Otolaryngology Shenzhen Second People’s Hospital 5. the First Affiliated Hospital 6. Institute of Microscale Optoelectronics Shenzhen University 7. Shenzhen International Institute for Biomedical Research 8. Shenzhen Han’s Tech Limited Company 9. Shenzhen Metasensing Tech Limited Company

The outbreak of the COVID-19 pandemic was partially due to the challenge of identifying asymptomatic and presymptomatic carriers of the virus, and thus highlights a strong motivation for diagnostics with high sensitivity that can be rapidly deployed. On the other hand, several concerning SARS-Co V-2 variants,including Omicron, are required to be identified as soon as the samples are identified as ‘positive’.Unfortunately, a traditional PCR test does not allow their specific identification. Herein, for the first time,we have developed MOPCS(Methodologies of Photonic CRISPR Sensing), which combines an optical sensing technology-surface plasmon resonance(SPR) with the ‘gene scissors’ clustered regularly interspaced short palindromic repeat(CRISPR) technique to achieve both high sensitivity and specificity when it comes to measurement of viral variants. MOPCS is a low-cost, CRISPR/Cas12a-systemempowered SPR gene-detecting platform that can analyze viral RNA, without the need for amplification,within 38 min from sample input to results output, and achieve a limit of detection of 15 fM. MOPCS achieves a highly sensitive analysis of SARS-Co V-2, and mutations appear in variants B.1.617.2(Delta),B.1.1.529(Omicron) and BA.1(a subtype of Omicron). This platform was also used to analyze some recently collected patient samples from a local outbreak in China, identified by the Centers for Disease Control and Prevention. This innovative CRISPR-empowered SPR platform will further contribute to the fast, sensitive and accurate detection of target nucleic acid sequences with single-base mutations.

关键词： surface plasmon resonance CRISPR SARS-CoV-2 Omicron variant

2D-ultrathin MXene/DOXjade platform for iron chelation chemo-photothermal therapy

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Bioactive Materials 2022年第8期7卷 76-85页

作者： Yunjie Xu Yingwei Wang Jusung An Adam C.Sedgwick Mingle Li Jianlei Xie Weibin Hu Jianlong Kang Sajal Sen Axel Steinbrueck Bin Zhang Lijun Qiao swelm wageh Jonathan F.Arambula Liping Liu Han Zhang Jonathan L.Sessler Jong Seung Kim Shenzhen Engineering Laboratory of Phosphorene and Optoelectronics International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of EducationShenzhen Institute of Translational MedicineDepartment of OtolaryngologyShenzhen Second People’s HospitalThe First Affiliated HospitalCollege of Optoelectronic EngineeringShenzhen UniversityShenzhen518060China Department of Chemistry Korea UniversitySeoul02841South Korea Department of Hepatobiliary and Pancreatic Surgery Shenzhen People’s HospitalSecond Clinical Medical College of Jinan UniversityShenzhen518020China Department of Chemistry The University of Texas at AustinAustinTX78712-1224USA Hunan Key Laboratory of Nanophotonics and Devices School of Physics and ElectronicsCentral South University932 South Lushan RoadChangsha410083China Institute of Translation Medicine Shenzhen Second People’s Hospital First Affiliated Hospital of Shenzhen University Shenzhen518035China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah21589Saudi Arabia

An increased demand for iron is a hallmark of cancer cells and is thought necessary to promote high cell proliferation,tumor progression and metastasis.This makes iron metabolism an attractive therapeutic target.Unfortunately,current iron-based therapeutic strategies often lack effectiveness and can elicit off-target toxicities.We report here a dual-therapeutic prodrug,DOXjade,that allows for iron chelation chemo-photothermal cancer therapy.This prodrug takes advantage of the clinically approved iron chelator deferasirox(ExJade®)and the topoisomerase 2 inhibitor,doxorubicin(DOX).Loading DOXjade onto ultrathin 2D Ti_(3)C_(2) MXene nanosheets produces a construct,Ti_(3)C_(2)-PVP@DOXjade,that allows the iron chelation and chemotherapeutic functions of DOXjade to be photo-activated at the tumor sites,while potentiating a robust photothermal effect with photothermal conversion efficiencies of up to 40%.Antitumor mechanistic investigations reveal that upon activation,Ti_(3)C_(2)-PVP@DOXjade serves to promote apoptotic cell death and downregulate the iron depletion-induced iron transferrin receptor(TfR).A tumor pH-responsive iron chelation/photothermal/chemotherapy antitumor effect was achieved both in vitro and in vivo.The results of this study highlight what may constitute a promising iron chelation-based phototherapeutic approach to cancer therapy.

关键词： 2D MXene Nanomedicine Prodrug Iron chelation Photothermal therapy

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S型异质结CO_(2)还原光催化剂

物理化学学报 2021年第6期37卷 3-4页

作者： swelm wageh Ahmed AAl-Ghamdi 刘丽君 Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia 武汉纺织大学化学与化工学院武汉430200

Photocatalytic CO_(2) reduction to solar fuels attracts great interest due to the growing fossil fuel shortage and global warming. Developing high-efficiency photocatalyst is the key for the solar fuel production ~(1,2). TiO_(2), as an inert, nontoxic and earth-abundant semiconductor, has been widely used for photocatalytic CO_(2) reduction.

关键词： reduction. abundant (2)

Design principle of S-scheme heterojunction photocatalyst

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Journal of Materials Science & Technology 2022年第29期124卷 171-173页

作者： Quanlong Xu S.wageh Ahmed A.Al-Ghamdi Xin Li Key laboratory of Carbon Materials of Zhejiang Province College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou325027China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah21589Saudi Arabia Institute of Biomass Engineering Key Laboratory of Energy Plants Resource and UtilizationMinistry of Agriculture and Rural AffairsSouth China Agricultural UniversityGuangzhou510642China

Recently,a new opinion was put forward on general design standards for S-scheme heterojunction photocatalyst.Four types of S-scheme heterojunctions were analyzed.Specifically,the critical understanding on the curved Fermi level at the interface of S-scheme heterojunction is helpful to strengthen and promote the basic theory of photocatalysis.

关键词： S-scheme heterojunction p-type semiconductor n-type semiconductor Curved Fermi level