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Ground-state mass of ^(22)Al and test of state-of-the-art ab initio calculations

Chinese Physics C 2024年第3期48卷 72-78页

作者：孙铭泽于越王新鹏王猛李健国张玉虎 K.Blaum 陈祖毅陈瑞九邓涵宇付超义葛文文黄文嘉焦红扬李红蕙李宏福罗胤芳廖挺 YuALitvinov 司敏帅鹏史金阳王茜邢元明徐星徐瑚珊许甫荣袁琪 T.Yamaguchi 颜鑫亮杨建成原有进周小红周旭张敏曾奇 CAS Key Laboratory of high Precision Nuclear Spectroscopy Institute of Modern PhysicsChinese Academy of SciencesLanzhou 730000China School of Nuclear Science and Technology University of Chinese Academy of SciencesBeijing 100049China Max-Planck-Institut für Kernphysik Saupfercheckweg 169117 HeidelbergGermany GSI helmholtzzentrum für Schwerionenforschung Planckstraße 164291 DarmstadtGermany Advanced Energy Science and Technology Guangdong Laboratory Huizhou516007China State Key Laboratory of Nuclear Physics and Technology School of PhysicsPeking UniversityBeijing 100871China Department of Physics Saitama UniversitySaitama 338-8570Japan School of Nuclear Science and Engineering East China University of TechnologyNanchang 330013China

The ground-state mass excess of the T_(z)=−2 drip-line nucleus ^(22)Al is measured for the first time as 18103(10)keV using the newly-developed Bρ-defined isochronous mass spectrometry method at the cooler storage ring in *** new mass excess value allowed us to determine the excitation energies of the two low-lying 1+states in ^(22)Al with significantly reduced uncertainties of 51 *** compared to the analogue states in its mirror nucleus ^(22)f,the mirror energy differences of the two 1^(+)states in the ^(22)Al-^(22)f mirror pair are determined to be−625(51)keV and−330(51)*** excitation energies and mirror energy differences are used to test the state-of-the-art ab initio valence-space in-medium similarity renormalization group calculations with four sets of interactions derived from the chiral effective field *** mechanism leading to the large mirror energy differences is investigated and attributed to the occupation of theπs_(1/2) orbital.

关键词： nuclear mass Bρ-defined IMS mirror energy difference ab initio VS-IMSRG calculations chiral interactions

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Genomic Mosaicism of the Brain:Origin,Impact,and Utility

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Neuroscience Bulletin 2024年第6期40卷 759-776页

作者： Jared h.Graham Johannes C.M.Schlachetzki Xiaoxu Yang Martin W.Breuss Department of Pediatrics Section of Clinical Genetics and MetabolismUniversity of Colorado School of MedicineAurora80045-2581COUSA Department of Cellular and Molecular Medicine University of California San DiegoLa Jolla92093-0021San DiegoCAUSA Department of Neurosciences University of California San DiegoLa Jolla92093-0021San DiegoCAUSA rady Children’s Institute for Genomic Medicine San Diego92123CAUSA

Genomic mosaicism describes the phenomenon where some but not all cells within a tissue harbor unique genetic ***,research focused on the impact of genomic mosaicism on clinical phenotype—motivated by its involvement in cancers and overgrowth *** recently,we increasingly shifted towards the plethora of neutral mosaic variants that can act as recorders of cellular lineage and environmental ***,we summarize the current state of the field of genomic mosaicism research with a special emphasis on our current understanding of this phenomenon in brain development and *** the field of genomic mosaicism has a rich history,technological advances in the last decade have changed our approaches and greatly improved our *** will provide current definitions and an overview of contemporary detection approaches for genomic ***,we will discuss the impact and utility of genomic mosaicism.

关键词： Genomics Brain development Brain homeostasis Genomic mosaicism

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Long-term open circuit microbial electrosynthesis system promotes methanogenesis

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Journal of Energy Chemistry 2020年第2期29卷 3-6页

作者： raúl Mateos Adrián Escapa María Isabel san-Martín heleen De Wever Ana Sotres Deepak Pant Chemical and Environmental Bioprocess Engineering Group Natural Resources Institute(IRENA)University of LeonLeon 24071Spain Department of Electrical Engineering and Automatic Systems Universidad de LeonLeon 24071Spain Reparation and Conversion Technology Flemish Institute for Technological Research(VITO)Mol 2400Belgium

Microbial electrosynthesis(MES) can potentially provide a mean for storing renewable energy surpluses as chemical energy. however, the fluctuating nature of these energy sources may represent a threat to MES, as the microbial communities that develop on the biocathode rely on the continuous existence of a polarized electrode. This work assesses how MES performance, product generation and microbial community evolution are affected by a long-period(6 weeks) power off(open circuit). Acetogenic and h2-producing bacteria activity recovered after reconnection. however, few days later syntrophic acetate oxidation bacteria and h2-consuming methanogens became dominant, producing Ch4 as the main product, via electromethanogenesis and the syntrophic interaction between eubacterial and archaeal communities which consume both the acetic acid and the hydrogen present in the cathode environment. Thus,the system proved to be resilient to a long-term power interruption in terms of electroactivity. At the same time, these results demonstrated that the system could be extensively affected in both end product generation and microbial communities.

关键词： Biocathode Electromethanogenesis Microbial electrosynthesis Microbial community dynamics Methanogens Acetogens

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分子筛改性铜硅催化剂对顺酐选择性加氢反应性能的影响

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石油炼制与化工 2024年第5期55卷 58-66页

作者：刘天意黄卫国邢闯伞晓广沈阳化工大学化学工程学院沈阳110142 浙江联盛化学股份有限公司浙江科技大学生物与化学工程学院

采用蒸氨法将不同分子筛掺杂在CuSi催化剂中,考察了ZSM-5,MOR,4A,5A分子筛对Cu基催化剂顺酐(MA)选择性加氢反应性能的影响。相比于未经分子筛掺杂的CuSi催化剂,分子筛掺杂催化剂的活性明显提高。CuSi-4A催化剂中Cu粒子的分散较差,导致... 详细信息

采用蒸氨法将不同分子筛掺杂在CuSi催化剂中,考察了ZSM-5,MOR,4A,5A分子筛对Cu基催化剂顺酐(MA)选择性加氢反应性能的影响。相比于未经分子筛掺杂的CuSi催化剂,分子筛掺杂催化剂的活性明显提高。CuSi-4A催化剂中Cu粒子的分散较差,导致其比表面积小,h 2在催化剂上的吸附能力最弱,CuSi-4A活性明显低于CuSi-MOR,CuSi-ZSM-5,CuSi-5A催化剂。而CuSi-MOR催化剂有丰富的Cu+,Cu粒子更小,表现出最佳的催化性能,在反应温度为280℃、氢酐摩尔比为79、质量空速为0.12 h-1的反应条件下,MA转化率高达99.6%,γ-丁内酯选择性为47.9%。在蒸氨法制备CuSi催化剂过程中掺杂分子筛,可提高金属分散度,为催化剂设计提供一定的借鉴。

关键词：顺酐 CuSi催化剂选择性加氢分子筛丁二酸酐 γ -丁内酯

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All-atom Molecular Dynamic Simulations and NMR Spectra Study on Intermolecular Interactions of N,N-dimethylacetamide-Water System

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Chinese Journal of Chemical Physics 2008年第3期21卷 221-226页

作者： Rong Zhang Zai-you Tan san-lai Luo Lab of Physical Chemistry College of Pharmacy Guangdong Pharmaceutical University Guangzhou510006 China

N,N-dimethylacetamide （DMA） has been investigated extensively in studying models of peptide bonds. An all-atom MD simulation and the NMR spectra were performed to investigate the interactions in the DMA- water system. The radial distribution functions （RDfs） and the hydrogen-bonding network were used in MD simulations. There are strong hydrogen bonds and weak C-h…O contacts in the mixtures, as shown by the analysis of the RDfs. The insight structures in the DMA-water mixtures can be classified into different regions by the analysis of the hydrogen-bonding network. Chemical shifts of the hydrogen atom of water molecule with concentration and temperatures are adopted to study the interactions in the mixtures. The results of NMR spectra show good agreement with the statistical results of hydrogen bonds in MD simulations.

关键词： All-atom simulation NMR spectrum DMA-water system hydrogen bond

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Multiple solutions for weighted nonlinear elliptic system involving critical exponents

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Science China Mathematics 2015年第1期58卷 161-178页

作者： NYAMOraDI Nemat hSU Tsing san Department of Mathematics Faculty of Sciences Razi University Department of Natural Sciences in the Center for General Education Chang Gung University

In this paper, by using the idea of category, we investigate how the shape of the graph of h（x） affects the number of positive solutions to the following weighted nonlinear elliptic system： = （ N-2-2a 2. where 0 is a smooth bounded domain in ]1N （N 〉 3）, A, cr 〉 0 are parameters, 0 ≤ μ 〈 μa a 2 ＇ h（x）, KI（X） and K2（x） are positive continuous functions in , 1 〈 q 〈 2, a, β 〉 1 and a ＋ β = 2＊（a,b）（2＊（a, b） 2N = N-2（1＋a-b） is critical Sobolev-hardy exponent）. We prove that the system has at least k nontrivial nonnegative solutions when the pair of the parameters （）, r） belongs to a certain subset of N2.

关键词： Caffarelli-Kohn-Nirenberg inequality variational method critical hardy-Sobolev exponent mul-tiple positive solutions

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EffECT Of ThE DEfECT STATES DENSITY ON OPTICAL BAND GAP Of CdIn_(2)O_(4)ThIN fILM

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Acta Metallurgica Sinica(English Letters) 2005年第3期18卷 403-410页

作者： h.S.san Z.G.Wu B.Li B.X.feng KeyLaboratoryforMagnetismandMagneticMaterialofMinistryofEducation LanzhouUniversityLanzhou730000China ShanghaiInstituteofTechnicalPhysics TheChineseAcademyofSciencesShanghai200083China

Transparent conducting oxides CdIn2O4 thin films were prepared by radio-frequenc y reactive sputtering from a Cd-In alloy target in Ar+O2 atmosphere. By transmis sion spectrum and hall measurement for different samples prepared at different s ubstrate temperatures, it could be found that the carrier concentration would in crease with the decrease of substrate temperature, but absorption edge showed an abrupt variation from a blue shift to a red shift. Theoretically, the paper for mulated the effect of high-density point defects on band structures; it embodied the formation of band tailing, Burstein-Moss shift and band-gap narrowing. The density of holes will influence the magnitude of optical band gap and transmitta nce of light. Since extrapolation method does not fit degenerate semiconductor m aterials, a more accurate method of obtaining optical band gap is curve fitting. In addition, ionized impurities scattering is the main damping mechanism of the free electrons in CdIn2O4 films, the density of ionized impurities induced by a ltering substrate temperature will affect the carriers mobility.

关键词： sputtering CdIn2O4 thin film electrical property optical property

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Synthesis of cleavable multi-functional mikto-arm star polymer by rafT polymerization: example of an anti-cancer drug 7-ethyl-10-hydroxycamptothecin(SN-38) as functional moiety

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Science China Chemistry 2014年第7期57卷 995-1001页

作者： WEI Xiaohu GUNATILLAKE Pathiraja A MOAD Graeme RIZZARDO Ezio ROSSELGONG Julien YANG WanTai ThANG san h. College of Materials Science and Engineering Beijing University of Chemical Technology Materials Science and Engineering The Commonwealth Scientific and Industrial Research Organisation(CSIRO)

Multi-functional mikto-arm star polymers containing three different arms [hydrophilic, SN-38-P（OEGMAs_9）11, cationizable, SN-38-P（DMAEMA）3s and hydrophobic, SN-38-P（BMA）26] were prepared by rafT polymerization via an arm-first approach using a cleavable cross-linker. The star polymers were cleaved to the linear arms with tributylphosphine as a reducing agent. The decrease in molecular weight observed is consistent with the initial stars having approximately five arms, Blue fluorescence was observed when a solution of mikto-arm star was irradiated under a 365 nm light proving the retention of the SN-38 moiety during star formation by rafT polymerization. Thus these polymer-drug conjugates can be considered as potential delivery vehicles for cancer therapy. The P（DMAEMA） arms can be quaternized using iodomethane, allowing star polymers to bind negatively charged small interfering RNA （siRNA） and potentially be used as a carrier for that material.

关键词： rafT mikto-arm star polymer-drug conjugate cleavable polymer siRNA delivery cancer therapy

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Microstructure and hardness of Mg-based composites reinforced with Mg_2Si particles

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rare Metals 2009年第4期28卷 396-400页

作者： Mustafa Aydin Cem zgür Osman san Mechanical Engineering Department Dumlupinar University Ceramic Engineering Department Dumlupinar University

Magnesium powders were mechanically alloyed with SiO2 powder particles having different particle sizes using nigh-energy ball milling techniques under Ar atmosphere for 1 h. The powders were consolidated with cold pressing under 560 MPa. They were then sintered at 550℃ for 45 min under Ar atmosphere. The composites obtained on the Mg-SiO2 system were investigated using the Archimedes principle, a differential scanning calorimeter, X-ray diffraction, optic microscopy, and scanning electron microscopy. for the mechanically alloyed powders, the solid-state reaction of the synthesis of Mg2Si and MgO progressed further during sintering of the materials. The results showed that the strengthening mechanisms were dependent on dispersion hardening of fine Mg2Si and MgO particulates dispersed homogeneously in the matrix. Mg-

关键词： based composites SiO2 mechanical alloying strengthening mechanism

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Ductal carcinoma in situ within a fibroadenoma:A case report and review of literature

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World Journal of radiology 2024年第3期16卷 58-68页

作者： Yazmin Olivares-Antúnez Yesika Janett Dávila-Zablah Joséraúl Vázquez-Ávila Gabriela Sofía Gómez-Macías María Teresa Mireles-Aguilar Margarita Lilia Garza-Montemayor Department of Diagnostic Breast Imaging Center Hospital Zambrano HellionTecnológico de MonterreyNuevo León 66260Mexico Department of Patology Service Hospital San JoséTecnológico de MonterreyNuevo León 64710Mexico Department of faculty of Medicine Hospital Universitario de la UANLNuevo León 64710Mexico. Department of Breast Surgery Center Hospital Zambrano HellionTecnológico de MonterreyNuevo León 66260Mexico

BACKGROUND fibroadenoma(fA)is the most common tumor found in young women,although it can occur in any age *** carcinoma in situ(DCIS)that is confined in a fA is rare;it is most frequently reported as an incidental *** SUMMARY We report a case of DCIS within a fA in a 46-year-old female without cancerrelated personal and family *** patient was diagnosed with a breast conglomerate of nodules and was followed for 1 *** the current control image study,we found suspicious microcalcification,as a new finding,within one of the ***,a core biopsy of the tumor,which appeared hypoechoic,oval,and circumscribed,was *** pathological diagnosis was ductal carcinoma in situ within a fibroepithelial *** patient underwent breastconserving surgery and received radiotherapy as well as endocrine therapy(tamoxifen).CONCLUSION We recommend a multidisciplinary approach for adequate treatment and followup.

关键词： Carcinoma in situ fibroadenoma Mammography Ultrasound Magnetic resonance imaging radiology Case report

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