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CdS/聚合物梯形产氢光催化剂及其原位光照电子转移机制

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Chinese Journal of Ca.alysis 2022年第3期43卷 586-588页

作者： S.Wageh Ahmed a.al-Ghamdi omar a.al-hartomy Maged F.alotaibi 王临曦阿卜杜勒阿齐兹国王大学理学院物理系吉达沙特阿拉伯中国地质大学(武汉)材料与化学学院太阳燃料实验室湖北武汉430074中国

氢气是公认的洁净、高效、可再生的能源载体,有望替代目前广泛使用的化石燃料.太阳能光催化产氢是实现高效、低成本、可持续生产氢能的一种途径.然而,单一组分光催化剂的性能受限于光生电子-空穴的快速复合,并且不能同时满足宽的太阳光... 详细信息

氢气是公认的洁净、高效、可再生的能源载体,有望替代目前广泛使用的化石燃料.太阳能光催化产氢是实现高效、低成本、可持续生产氢能的一种途径.然而,单一组分光催化剂的性能受限于光生电子-空穴的快速复合,并且不能同时满足宽的太阳光吸收范围和强的氧化还原能力的要求,因此需要构建异质结来增强光生载流子的分离并保持高效光吸收和强氧化还原能力.异质结包括II型异质结、Z型(分为传统Z型和全固态Z型)异质结和梯型(Step-scheme,S型)异质结.在II型异质结中,光生电子从较高迁移至较低的导带,而光生空穴从较低迁移至较高的价带.该原理中光生载流子的转移会使其氧化还原能力降低,同时光生电子-空穴间的吸引和同种电荷间的互斥不利于载流子的转移.Z型异质结利用溶解的氧化还原离子对(传统的Z型异质结)或导电材料(全固态Z型异质结)作为电荷转移和分离的穿梭器.然而,具有更强氧化还原能力的光生载流子会优先与该离子对反应或通过导电材料复合,使氧化还原能力下降.S型异质结通过费米能级差产生的电荷转移形成内建电场,在光照下,内建电场促使氧化还原能力较弱的电子-空穴对结合,而保留氧化还原能力强的电子-空穴对,增强光生载流子的传递分离与光催化剂的活性.目前,Cheng等(Adv.Mater.,2021,33,2100317)通过原位生长硫化镉(CdS)与芘-三苯胺交替共聚物(PT),形成一种无机有机梯型(S型)复合异质结光催化剂(CP).负载了1%Pt助催化剂的2%PT/CdS光催化剂显示出高达9.28 mmol h^(-1) g^(-1)的产氢速率,较好的性能归因于S型异质结的高电子-空穴分离效率和强氧化还原活性.利用开尔文探针和原位光照X射线光电子能谱(ISI-XPS)研究了S型异质结的电子转移机理.在光照下,CdS的电势升高而PT的电势降低,说明CdS中的光生电子转移至PT与其中的光生空穴结合,这与S型异质结的电子转移机理是一致的.CdS的ISI-XPS谱图结果表明,在黑暗条件下,CP中Cd 3d和S 2p的结合能低于它们在CdS中的结合能,说明有电子净流入CdS使其结合能降低;在光照下,Cd 3d和S 2p的结合能则升高,说明电子由CdS转移至PT中.该S型异质结光催化剂成功光催化分解水制氢的案例表明,该研究方向具有潜力.

关键词： S型异质结电子转移机理开尔文探针表面电势图像原位光照X射线光电子能谱

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A new fractional order 6D chaotic model:Study of model dynamics,system structure graph,electronic circuit realization and fractional control

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Journal of Ocean Engineering and Science 2024年第2期9卷 112-125页

作者： M.Higazy Norah almalki Shabbir Muhammad a.al-Ghamdi Department of Mathematics and Statistics College of ScienceTaif UniversityP.O.Box 11099Taif 21944Saudi Arabia Department of Physics and Engineering Mathematics Faculty of Electronic EngineeringMenoufia UniversityMenouf 32952Egypt Research Center for Advanced Materials Science(RCAMS) King Khalid UniversityP.O.Box 9004Abha 61413Saudi Arabia Department of Chemistry College of ScienceKing Khalid UniversityP.O.Box 9004Abha 61413Saudi Arabia Department of Physics Faculty of ScienceKing Abdulaziz UniversityP.O.Box 80203Jeddah 21589Saudi Arabia

A new fractional 6D chaotic model is constructed in this paper.The new fractional 6D chaotic model has six positive parameters plus the fractional order with eight nonlinear terms.The complicated chaotic dy-namics of the new fractional 6D model is presented and a.alyzed.The basic properties of this model are studied and its chaotic attractors,dissipative feature,symmetry,equilibrium points,Lyapunov Exponents are investigated.The new dynamics of the 6D fractional model is numerically simulated using Matlab software.In addition,utilizing the graph theory tools certain structural characteristics are calculated.An electrical circuit is built to implement the new 5.4 fractional order 6D model.Finally,an active fractional order controller is proposed to control the new model at different fractional orders.The chaos of the new model is very useful and can be used to produce random keys for data encryption.

关键词： Chaotic systems Fractional calculus Lyapunov exponents Chaotic attractors Adjacency matrix Hermitian matrix Electronic circuit realization

Au/MXene based ultrafast all-optical switching

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Frontiers of physics 2023年第3期18卷 147-153页

作者： Yule Zhang Feng Zhang Bowen Du Hualong Chen S.Wageh omar a.al-hartomy Abdullah G.al-Sehemi Bin Zhang Han Zhang International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education Institute of Microscale Optoelectronics and Translational MedicineThe First Affiliated Hospital(Shenzhen Second People’s Hospital)College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia Research Center for Advanced Materials Science(RCAMS) King Khalid UniversityP.O.Box 9004Ab-ha61413Saudi Arabia

all-optical switches have arisen great attention due to their ultrafast speed as compared with electric switches.However,the excellent optical properties and strong interaction of two-dimensional(2D)material MXene show great potentials in next-generation all-optical switching.As a solution,we propose all-optical switching used Au/MXene with switching full width at half maximum(FWHM)operating at 290 fs.Compared with pure MXene,the Au/MXene behaves outstanding performances due to local surface plasmon resonance(LSPR),including broadband differential transmission,strong near-infrared on/off ratio enhancement.Remarkably,this study enhances understanding of Au/MXene based ultrafast all-optical switching red-shifted about 34 nm in comparison to MXene,validating all optical properties of Au/MXene opening the way to the implementation of optical interconnection and optical switching.

关键词： Au/MXene ultrafast all-optical switching Au/MXene carrier lifetime

Findings on three endocommensal scuticociliates(Protista,Ciliophora)from freshwater mollusks,including their morphology and molecular phylogeny with descriptions of two new species

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Marine Life Science & Technology 2024年第2期6卷 212-235页

作者： Tao Li Tengyue Zhang Mingjian Liu Zhe Zhang Jiachen Zhang Junhua Niu Xiangrui Chen Saleh a.al‑Farraj Weibo Song Institute of Evolution and Marine Biodiversity Ocean University of China and Key Laboratory of Evolution and Marine Biodiversity(Ministry of Education)Qingdao 266003China The Key Laboratory of Zoological Systematics and Application College of Life SciencesHebei UniversityBaoding 071002China College of Marine Life Sciences Ocean University of ChinaQingdao 266003China School of Marine Sciences Ningbo UniversityNingbo 315800China Zoology Department College of ScienceKing Saud University11451 RiyadhSaudi Arabia Laboratory for Marine Biology and Biotechnology Laoshan LaboratoryQingdao 266237China

Species of the ciliate genera Myxophyllum and Conchophthirus are found as endocommensals of terrestrial and freshwater mollusks,respectively.So far,there have been few studies of these genera and morphological data for most members are often incomplete.In the present work,two new species,Myxophyllum weishanense sp.***.and Conchophthirus paracurtus sp.nov.,and a known species,Conchophthirus lamellidens,were isolated from hosts in Lake Weishan Wetland,China.Taxonomic studies indicate that M.weishanense sp.***.can be recognized mainly by the combination of about 60 somatic kineties on both ventral and dorsal sides and the presence of caudal cilia.Conchophthirus paracurtus sp.***.differs from congeners in its body shape and size,having a glabrous area on the posterior right side,and having fewer somatic kineties.In addition,differences in their ITS2(Internally Transcribed Spacer 2)secondary structures support the discrimination of the two new species from their highly similar congeners.An improved diagnosis for the poorly known species,C.lamel-lidens is also provided.Phylogenetic a.alyses reveal that members of the genus Myxophyllum belong to a fully supported clade that is sister to a large,poorly supported clade consisting of Hemispeiridae,Ancistridae,and several lineages of the nonmonophyletic Cyclidiidae.The Myxophyllum clade also includes Protophyra ovicola JQ956552,a possible misidenti-fication.Sequences of the two new Conchophthirus species cluster with other congeners in a fully supported clade that is unrelated to either the‘typical’thigmotrichs or to pleuronematids,thus conflicting with the traditional classification,and may represent an orphan scuticociliate lineage.

关键词： Ciliates Endocommensal ITS2 secondary structure Mollusks New taxa Wetland

A CRISPR/Cas12a-empowered surface plasmon resonance platform for rapid and specific diagnosis of the Omicron variant of SARS-CoV-2

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National Science Review 2022年第8期9卷 100-109页

作者： Zhi Chen Jingfeng Li Tianzhong Li Taojian Fan Changle Meng Chaozhou Li Jianlong Kang Luxiao Chai Yabin Hao Yuxuan Tang omar a.al-hartomy Swelm Wageh Abdullah G.al-Sehemi Zhiguang Luo Jiangtian Yu Yonghong Shao Defa Li Shuai Feng William J.Liu Yaqing He Xiaopeng Ma Zhongjian Xie Han Zhang Department of Physics Faculty of Science King Abdulaziz University Research Center for Advanced Materials Science (RCAMS) King Khalid University Department of Chemistry College of Science King Khalid University Zhongmin (Shenzhen) Intelligent Ecology Co.Ltd Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic Engineering Shenzhen University Department of Laboratory Medicine Shenzhen Children’s Hospital Optoelectronics Research Center School of Science Minzu University of China NHC Key Laboratory of Biosafety National Institute for Viral Disease Control and Prevention Chinese Center for Disease Control and Prevention Research Unit of Adaptive Evolution and Control of Emerging Viruses Chinese Academy of Medical Sciences Institute of Pathogenic Organism Shenzhen Center for Disease Control and Prevention Shenzhen Engineering Laboratory of Phosphorene and Optoelectronics Respiratory Department Shenzhen Children’s Hospital Institute of Pediatrics Shenzhen Children’s Hospital International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education 3. Shenzhen Institute of Translational Medicine 4. Department of Otolaryngology Shenzhen Second People’s Hospital 5. the First Affiliated Hospital 6. Institute of Microscale Optoelectronics Shenzhen University 7. Shenzhen International Institute for Biomedical Research 8. Shenzhen Han’s Tech Limited Company 9. Shenzhen Metasensing Tech Limited Company

The outbreak of the COVID-19 pandemic was partially due to the challenge of identifying asymptomatic and presymptomatic carriers of the virus, and thus highlights a strong motivation for diagnostics with high sensitivity that can be rapidly deployed. On the other hand, several concerning SARS-Co V-2 variants,including Omicron, are required to be identified as soon as the samples are identified as ‘positive’.Unfortunately, a traditional PCR test does not allow their specific identification. Herein, for the first time,we have developed MOPCS(Methodologies of Photonic CRISPR Sensing), which combines an optical sensing technology-surface plasmon resonance(SPR) with the ‘gene scissors’ clustered regularly interspaced short palindromic repeat(CRISPR) technique to achieve both high sensitivity and specificity when it comes to measurement of viral variants. MOPCS is a low-cost, CRISPR/Cas12a-systemempowered SPR gene-detecting platform that can a.alyze viral RNA, without the need for amplification,within 38 min from sample input to results output, and achieve a limit of detection of 15 fM. MOPCS achieves a highly sensitive a.alysis of SARS-Co V-2, and mutations appear in variants B.1.617.2(Delta),B.1.1.529(Omicron) and BA.1(a subtype of Omicron). This platform was also used to a.alyze some recently collected patient samples from a local outbreak in China, identified by the Centers for Disease Control and Prevention. This innovative CRISPR-empowered SPR platform will further contribute to the fast, sensitive and accurate detection of target nucleic acid sequences with single-base mutations.

关键词： surface plasmon resonance CRISPR SARS-CoV-2 Omicron variant

Fully depleted vdW heterojunction based high performance photovoltaic photodetector

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Journal of Materiomics 2023年第6期9卷 1039-1047页

作者： Yonghong Zeng Fanxu Meng Sidi Fan Pengfei Wang Cuiyun Kou Mingyi Sun Haiguo Hu Rui Cao Swelm Wageh omar a.al-hartomy Abul Kalam Bowen Du Wenchao Ding Songrui Wei Zhinan Guo Qiuliang Wang Han Zhang College of Physics and Optoelectronic Engineering Institute of Microscale OptoelectronicsInternational Collaborative Laboratory of 2D Materials for Optoelectronics Science and TechnologyInterdisciplinary Center of High Magnetic Field Physics of Shenzhen UniversityShenzhen UniversityShenzhen518060China Guangzhou Key Laboratory of Sensing Materials and Devices Center for Advanced Analytical ScienceSchool of Chemistry and Chemical EngineeringGuangzhou UniversityGuangzhou510006China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah21589Saudi Arabia Research Center for Advanced Materials Science(RCAMS) Department of ChemistryCollege of ScienceKing Khalid UniversityP.O.Box 9004Abha61413Saudi Arabia Foshan Electrical and Lighting Co. LTD64 North Fenjiang RoadFoshanChina Institute of Electrical Engineering Chinese Academy of SciencesBeijing100190China Center of Characterization and a.alysis Jilin Institute of Chemical TechnologyJilin132022China

Van der Waals(vdW)heterojunctions,with their unique electronic and optoelectronic properties,have become promising candidates for photodetector applications.Amplifying the contribution of the depletion region in vdW heterojunction,which would enhance both of the collection efficiency and speed of the photogenerated carriers,presents an effective strategy for achieving high performance vdW heterojunction photodetectors.Herein,a fully depleted vdW heterojunction photodetector is built on two-dimensional(2D)semiconductor materials(GaTe and InSe)layered on a pattered bottom electrode in vertical structure,in which the generation and motion of carriers are exclusively achieved in the depletion region.Attributed to the intrinsic built-in electric field,the elimination of series resistance and the depletion region confinement of carriers,the as-fabricated photodetector exhibits prominent photovoltaic properties with a high open-circuit voltage of 0.465 V,as well as photoresponse characteristics with outstanding responsivity,detectivity and photoresponse speed of 63.7 A/W,3.88×10^(13)Jones,and 32.7 ms respectively.The overall performance of this fully depleted GaTe/InSe vdW heterojunctions photodetectors are ranking high among the top level of 2D materials based photodetectors.It indicates the device architecture can provide new opportunities for the fabrication of high-performance photodetectors.

关键词： Two-dimensional material van der waals heterojunction Fully depleted photodetector Photovoltaic

CRISPR-Cas12a-Empowered Electrochemical Biosensor for Rapid and Ultrasensitive Detection of SARS-CoV-2 Delta Variant

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Nano-Micro Letters 2022年第10期14卷 83-94页

作者： Chenshuo Wu Zhi Chen Chaozhou Li Yabin Hao Yuxuan Tang Yuxuan Yuan Luxiao Chai Taojian Fan Jiangtian Yu Xiaopeng Ma omar Aal-hartomy SWageh Abdullah Gal-Sehemi Zhiguang Luo Yaqing He Jingfeng Li Zhongjian Xie Han Zhang International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of EducationInstitute of Microscale OptoelectronicsCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060People’s Republic of China Shenzhen International Institute for Biomedical Research Shenzhen 518116People’s Republic of China Department of Respiratory Shenzhen Children’s HospitalShenzhen 518038People’s Republic of China Institute of Pediatrics Shenzhen Children’s HospitalShenzhen 518038People’s Republic of China Shenzhen Han’s Tech Limited Company Shenzhen 518000People’s Republic of China Hospital of Guangzhou Medical University Qingyuan city People’s HospitalQingyuan 511518People’s Republic of China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia Research Center for Advanced Materials Science(RCAMS) King Khalid UniversityP.O.Box 9004Abha 61413Saudi Arabia Department of Chemistry College of ScienceKing Khalid UniversityP.O.Box 9004Abha 61413Saudi Arabia Zhongmin(Shenzhen)Intelligent Ecology Co. LtdShenzhen 518055People’s Republic of China Shenzhen Center for Disease Control and Prevention Shenzhen 518055People’s Republic of China

Coronavirus disease 2019(COVID-19)is a highly contagious disease caused by severe acute respiratory syndrome coronavirus 2(SARS-CoV-2).The gold standard method for the diagnosis of SARS-CoV-2 depends on quantitative reverse transcription-polymerase chain reaction till now,which is time-consuming and requires expensive instrumentation,and the confirmation of variants relies on further sequencing techniques.Herein,we first proposed a robust technique-methodology of electrochemical CRISPR sensing with the advantages of rapid,highly sensitivity and specificity for the detection of SARS-CoV-2 variant.To enhance the sensing capability,gold electrodes are uniformly decorated with electro-deposited gold nanoparticles.Using DNA template identical to SARS-CoV-2 Delta spike gene sequence as model,our biosensor exhibits excellent a.alytical detection limit(50 fM)and high linearity(R2=0.987)over six orders of magnitude dynamic range from 100 fM to 10 nM without any nucleic-acid-amplification assays.The detection can be completed within 1 h with high stability and specificity which benefits from the CRISPR-Cas system.Furthermore,based on the wireless micro-electrochemical platform,the proposed biosensor reveals promising application ability in point-of-care testing.

关键词： SARS-COV-2 variant Methodology of electrochemical CRISPR sensing(MOECS) Gold nanoparticles(AuNPs) Point-of-care testing(POCT)

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Improving Thyroid Disorder Diagnosis via Ensemble Stacking and Bidirectional Feature Selection

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Computers, Materials & Continua 2024年第3期78卷 4225-4241页

作者： Muhammad Armghan Latif Zohaib Mushtaq Saad Arif Sara Rehman Muhammad Farrukh Qureshi Nagwan Abdel Samee Maali alabdulhafith Yeong Hyeon Gu Mohammed a.al-masni Department of Computer and Information System Cleveland State UniversityOhio44115USA Department of Electrical Electronics and Computer SystemsCollege of Engineering and TechnologyUniversity of SargodhaSargodha40100Pakistan Department of Mechanical Engineering College of EngineeringKing Faisal UniversityAl-Ahsa31982Saudi Arabia Department of Biomedical Engineering Riphah International UniversityIslamabad44000Pakistan Department of Electrical Engineering Riphah International UniversityIslamabad44000Pakistan Department of Information Technology College of Computer and Information SciencesPrincess Nourah bint Abdulrahman UniversityP.O.Box 84428Riyadh11671Saudi Arabia Department of Artificial Intelligence College of Software and Convergence TechnologySejong UniversitySeoul05006Korea

Thyroid disorders represent a significant global health challenge with hypothyroidism and hyperthyroidism as two common conditions arising from dysfunction in the thyroid gland.Accurate and timely diagnosis of these disorders is crucial for effective treatment and patient care.This research introduces a comprehensive approach to improve the accuracy of thyroid disorder diagnosis through the integration of ensemble stacking and advanced feature selection techniques.Sequential forward feature selection,sequential backward feature elimination,and bidirectional feature elimination are investigated in this study.In ensemble learning,random forest,adaptive boosting,and bagging classifiers are employed.The effectiveness of these techniques is evaluated using two different datasets obtained from the University of California Irvine-Machine Learning Repository,both of which undergo preprocessing steps,including outlier removal,addressing missing data,data cleansing,and feature reduction.Extensive experimentation demonstrates the remarkable success of proposed ensemble stacking and bidirectional feature elimination achieving 100%and 99.86%accuracy in identifying hyperthyroidism and hypothyroidism,respectively.Beyond enhancing detection accuracy,the ensemble stacking model also demonstrated a streamlined computational complexity which is pivotal for practical medical applications.It significantly outperformed existing studies with similar objectives underscoring the viability and effectiveness of the proposed scheme.This research offers an innovative perspective and sets the platform for improved thyroid disorder diagnosis with broader implications for healthcare and patient well-being.

关键词： Ensemble learning random forests boosting dimensionality reduction machine learning smart healthcare computer aided diagnosis

Diagnostic accuracy of ePOS score in predicting DNR labeling after ICU admission:A prospective observational study(ePOS-DNR)

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Journal of Intensive Medicine 2024年第2期4卷 216-221页

作者： omar E.Ramadan Ahmed F.Mady Mohammed a.al-Odat Ahmed N.Balshi Ahmed W.aletreby Taisy J.Stephen Sheena R.Diolaso Jennifer Q.Gano Waleed Th.aletreby Department of Critical Care King Saud Medical CityRiyadhSaudi Arabia Anesthesia Department Faculty of MedicineAin Shams UniversityCairoEgypt Anesthesia Department Faculty of MedicineTanta UniversityTantaEgypt Faculty of Medicine Alexandria UniversityAlexandriaEgypt Nursing Department King Saud Medical CityRiyadhSaudi Arabia

Background Resuscitation can sometimes be futile and making a do-not-resuscitate(DNR)decision is in the best interest of the patient.The electronic poor outcome screening(ePOS)score was developed to predict 6-month poor outcomes of critically ill patients.We explored the diagnostic accuracy of the ePOS score in predicting DNR decisions in the intensive care unit(ICU).Methods This study was conducted at the ICU of a tertiary referral hospital in Saudi Arabia between March and May 2023.Prospectively,we calculated ePOS scores for all eligible consecutive admissions after 48 h in the ICU and recorded the DNR orders.The ability of the score to predict DNR was explored using logistic regression.Youden's ideal cut-off value was calculated using the DeLong method,and different diagnostic accuracy measures were generated with corresponding 95%confidence intervals(CIs).Results We enrolled 857 patients,125 received a DNR order and 732 did not.The average ePOS score of DNR and non-DNR patients was 28.2±10.7 and 15.2±9.7,respectively.ePOS score,as a predictor of DNR order,had an area under receiver operator characteristic(AUROC)curve of 81.8%(95%CI:79.0 to 84.3,Pal cut-off value>17 was associated with a sensitivity of 87.2(95%CI:80.0 to 92.5,Palue of 29.2(95%CI:24.6 to 33.8,Palue of 96.7(95%CI:95.1 to 98.3,P17 may help guide clinical decisions to withhold or commence resuscitative measures.

关键词： Do-not-resuscitate(DNR) Resuscitation Intensive care unit(ICU) Diagnostic accuracy Sensitivity Specificity