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The component-activity interrelationship of cobalt-based bifunctional electrocatalysts for overall water splitting:Strategies and performance

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Journal of Energy Chemistry 2024年第4期91卷 453-474页

作者： mingjie sun Riyue Ge Sean Li Liming Dai Yiran Li Bin Liu Wenxian Li School of Materials Science and Engineering Shanghai UniversityShanghai 200444China Institute of Textiles and Clothing The Hong Kong Polytechnic UniversityHong Kong SAR 999077China School of Materials Science and Engineering University of New South WalesSydneyNew South Wales 2052Australia UNSW Materials&Manufacturing Futures Institute UNSW SydneyNew South Wales 2052Australia School of Chemical Engineering University of New South WalesSydneyNew South Wales 2052Australia

Cobalt-based electrocatalysts take advantage of potentially harmonizable microstructure and flexible coupling effects compared to commercial noble metal-based catalytic ***,conventional water electrolysis systems based on cobalt-based monofunctional hydrogen evolution reaction(HER)or oxygen evolution reaction(OER)catalysts have certain shortcomings in terms of resource utilization and *** contrast,cobalt-based bifunctional catalysts(CBCs)have attracted much attention in recent years for overall water splitting systems because of their practicality and reduced preparation cost of *** review aims to address the latest development in CBCs for total *** main modification strategies of CBCs are systematically classified in water electrolysis to provide an overview of how to regulate their morphology and electronic ***,the catalytic performance of CBCs in total-hydrolysis is summarized according to the types of cobalt-based phosphides,sulfides and oxides,and the mechanism of strengthened electrocatalytic ability is emphasized through combining experiments and theoretical *** efforts are finally suggested to focus on exploring the dynamic conversion of reaction intermediates and building near-industrial CBCs,designing advanced CBC materials through micro-modulation,and addressing commercial applications.

关键词： Cobalt Bifunctional electrocatalysis Water splitting Modification strategies Electrocatalytic performances

Vasorelaxant effect of osthole on isolated thoracic aortic rings in rats

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Journal of Traditional Chinese Medicine 2019年第4期39卷 492-501页

作者： Huang Ying Kong Liting Wang Yanping sun mingjie Cui Haifeng Zhai Huaqiang LüCheng Fan Danping Experimental Research Center China Academy of Chinese Medical SciencesBeijing 100700China School of Chinese Materia Medica Beijing University of Chinese MedicineBeijing 100029China Institute of Basic Research in Clinical Medicine China Academy of Chinese Medical SciencesBeijing 100700China

OBJECTIVE: To investigate the effect of osthole on isolated thoracic aortic rings, and to determine the potential mechanism of ***: Thoracic aortas were isolated from Wistar rats, and were suspended in tissue organ chambers for vascular tension measurement. The effect of cumulative osthole(10-9, 10-8, 10-7, 10-6, and 10-5 mol/L) on endothelium-intact and endothelium-denuded thoracic aortic rings pre-contracted with phenylephrine(PE, 10-6 mol/L) or KCl(6 × 10-2 mol/L) was recorded. Histomorphological changes of thoracic aorta were analyzed by hematoxylin-eosin. The effects of different osthole concentrations on endothelium-intact aortic rings, which were pre-inhibited with the non-selective nitric oxide synthase inhibitor L-Arg(NO2)-OMe·HCl(3 × 10-4 mol/L), endothelium-derived nitric oxide synthase inhibitor Nω-nitro-L-arginine(3 × 10-4 mol/L), guanylate cyclase inhibitor 1 H-[1,2,4] oxadiazolo [4,3-α]quinoxaline-1-one(10-5 mol/L), cyclooxygenase inhibitor indometacin(10-5 mol/L), and the Ca2+-activated potassium channel inhibitor tetraethylammonium nitrate(10-5 mol/L), and then contracted with PE, were examined. Aortic rings incubated with osthole(10-5 mol/L), phentolamine(10-5 mol/L), or verapamil(10-5 mol/L) in Ca2+-free Krebs-Henseleit solution(KHS) were stimulated with PE or ***: There was a dose-dependent increase in vasorelaxation of isolated thoracic aortic rings(both with and without endothelium) with increasing osthole concentration. Hematoxylin-eosin staining showed that osthole significantly improved thoracic aorta ring morphology. Compared with the control group, there were also significant differences after incubation with L-Arg(NO2)-OMe ω-nitro-L-arginine, and 1 H-[1,2,4] oxadiazo·lo HCl,N [4,3-α] quinoxaline-1-one(P < 0.05 for all). The relaxation rate of the rings in the osthole group incubated with indometacin and tetraethylammonium nitrate were similar to controls. In Ca2+-free KHS, the PE-induced contraction was similar between

关键词： Aorta,thoracic Osthole Phentolamine Verapamil Vasorelaxation Calcium Nitric oxide

Protection of Immuno-Compromised Mice from Lethal Infection of Klebsiella pneumonia by rAAV2-BPI23-Fcγ1 Gene Transfer

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Cellular & Molecular Immunology 2008年第6期5卷 439-445页

作者： Jing Li Qingli Kong Zhe Lv Yuanzhi Guan Yong Qiu Chen Li mingjie sun Zhenlong Liu Yunqing An Department of Immunology Capital Medical University Beijing 100069China Laboratory Department Capital Institute of Pediatrics Beijing 100020China Department of Microbiology Institute of Basic Medical Sciences ChineseAcademy of Medical Sciences ＆ Peking Union Medical College Beijing100005 China Laboratory Department Beijing Shijitan Hospital Beijing 100038 China China Rehabilitation Center Institute of Medical Sciences Beijing 100077China

In previous research, chimerical BPI23-Fcy1 gene which consisted of human bactericidal/permeability increasing protein （BPI） gene of encoding the functional N terminus （amino acid residues 1 to 199） of human BPI and Fcy1 gene of encoding the Fc segment of human immunoglobulin G1 was successfully reconstructed within a recombinant adeno-associated virus serotype 2 （rAAV2） vector as rAAV2-BPI23-Fcy1. Here, to evaluate the potentiality of applying gene therapy to gram negative bacterial （GNB） infection in high-risk patients, we investigated protection of immuno-compromised mice and immunocompetent mice from challenge with minimal lethal dose （MLD） Klebsiella pneumonia infection after rAAV2-BPI23-Fcy1 gene transferred. The results showed that the survival rate of rAAV2-BPI23-Fcy1 transferred immunocompetent mice as well as immuno-compromised mice （40.0% and 44.4%, respectively） were significant higher than that of corresponding control mice （6.7% and 4.4%, respectively）; the bacteria counting, level of endotoxin and proinflammatory cytokines in the rAAV2-BP123-Fcy1 transferred immuno-compromised mice were markedly lower than that of rAAV2-EGFP and rAAV2-Null transferred immuno- compromised mice. Our data suggest that rAAV2-BPI23-Fcy1 gene transferring offered immuno-compromised mice with resistance against GNB infection, so it is quite potential in preventing GNB infection of clinical high-risk patients. Cellular ＆ Molecular Immunology. 2008;5（6）：439-445.

关键词： rAAV2 BPI immuno-compromised mouse Klebsiella pneumonia gene transfer

Fast and deterministic optical phased array calibration via pointwise optimisation

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Light(Advanced Manufacturing) 2023年第2期4卷 39-47页

作者： Jingwen Shan Hanyi Zhang Lijing Li Weijie Deng mingjie sun Department of Opto-electronic Engineering Beihang UniversityBeijing 100191China Key Laboratory of Optical System Advanced Manufacturing Technology Chinese Academy of SciencesChangchun.*mingjie.sun@***

Owing to the structural errors in the optical phased array,an initial random phase reduces the quality of the deflection *** most commonly applied approach to phase calibration is based on adaptive ***,adaptive optimisation approaches have slow convergence and low diffraction *** proposed a pointwise optimisation approach to achieve fast and accurate beam *** approach conducts phase calibration,combining global traversal and local searches individually for each array *** built a phase-calibration optical system containing a one-dimensional optical waveguide phase array for further verification and designed the relevant *** simulation and experimental results demonstrate that the pointwise optimisation approach accelerates the calibration process and improves the diffraction efficiency.

关键词： Beam deflection Optical phase array Phase calibration

Effects of lead pollution on soil microbial community diversity and biomass and on invertase activity

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Soil Ecology Letters 2023年第1期5卷 118-127页

作者： Xin sun mingjie sun Ying Chao Xiaoyang Shang Hui Wang Hong Pan Quangang Yang Yanhong Lou Yuping Zhuge National Engineering Research Center for Efficient Utilization of Soil and Fertilizer Resources College of Resources and EnvironmentShandong Agricultural UniversityTai’an 271018China Tai’an Hi-Tech Industrial Development Zone Tai’an 271000China Rizhao Municipal Bureau of Agricultural and Rural Affairs Rizhao 276800China Key Laboratory of Technologies and Models for Cyclic Utilization from Agricultural Resources Ministry of Agriculture and Rural AffairsBeiJing 100125China

Lead(Pb)pollution is one of the most widespread and harmful environmental problems *** of changes in soil properties and microbial functional diversity due to land use is needed to establish a basis for remediation of soil *** study aimed to investigate soils contaminated by Pb from different sources and to analyze the functional diversity and metabolism of soil microbial communities using Biolog *** pollution(>300 mg kg-1)significantly influenced the diversity and metabolic functions of soil microbial ***,Pb contamination significantly reduced soil microbial biomass carbon(C)and nitrogen(N)levels and catalase activity while increasing invertase ***,Biolog EcoPlate assays revealed that Pb pollution reduced the general activities of soil microorganisms,suppressing their ability to utilize C *** Pb-contaminated areas lacking vegetation cover,Shannon,Simpson,and McIntosh diversity indices of soil microorganisms were significantly *** microbial diversity and biomass C and N levels were affected by land use and soil properties,respectively,whereas soil enzyme activity was primarily affected by the interaction between land use and soil *** results provide a reference and a theoretical basis for developing soil quality evaluation and remediation strategies.

关键词： Lead pollution Biolog Microbial functional diversity Soil enzyme activities Environment toxicity

Lotus seedpod-inspired internal vascularized 3D printed scaffold for bone tissue repair

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Bioactive Materials 2021年第6期6卷 1639-1652页

作者： Xiaoyu Han mingjie sun Bo Chen Qimanguli Saiding Junyue Zhang Hongliang Song Lianfu Deng Peng Wang Weiming Gong Wenguo Cui Department of Orthopedics Jinan Central HospitalShandong First Medical University&Shandong Academy of Medical Sciences105 Jiefang RoadLixia DistrictJinanShandong250013PR China Shanghai Key Laboratory for Prevention and Treatment of Bone and Joint Diseases Shanghai Institute of Traumatology and OrthopedicsRuijin HospitalShanghai Jiao Tong University School of Medicine197 Ruijin 2nd RoadShanghai200025PR China

In the field of bone defect repair,3D printed scaffolds have the characteristics of personalized customization and accurate internal ***,how to construct a well-structured vascular network quickly and effectively inside the scaffold is essential for bone repair after ***,inspired by the unique biological structure of“lotus seedpod”,hydrogel microspheres encapsulating deferoxamine(DFO)liposomes were prepared through microfluidic technology as“lotus seeds”,and skillfully combined with a three-dimensional(3D)printed bioceramic scaffold with biomimetic“lotus”biological structure which can internally grow blood *** this composite scaffold system,DFO was effectively released by 36%in the first 6 h,which was conducive to promote the growth of blood vessels inside the scaffold *** the following 7 days,the release rate of DFO reached 69%,which was fundamental in the formation of blood vessels inside the scaffold as well as osteogenic differentiation of bone mesenchymal stem cells(BMSCs).It was confirmed that the composite scaffold could significantly promote the human umbilical vein endothelial cells(HUVECs)to form the vascular morphology within 6 h in *** vivo,the composite scaffold increased the expression of vascularization and osteogenic related proteins Hif1-α,CD31,OPN,and OCN in the rat femoral defect model,significantly cutting down the time of bone *** sum up,this“lotus seedpod”inspired porous bioceramic 3D printed scaffold with internal vascularization functionality has broad application prospects in the future.

关键词： 3D scaffolds Drug release Neovascularization Osteogenesis Regeneration

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温度对光纤准直器的角度偏移影响分析

光子学报 2006年第10期35卷 1509-1513页

作者：孙鸣捷浙江大学现代光学仪器国家重点实验室国家光学仪器工程技术研究中心杭州310027

通过对光纤准直器准直失配,即离轴耦合、偏角耦合、间距耦合三种情况的耦合损耗进行分析,发现角度偏移对耦合效率影响最大.实验中随着温度周期性的变化,光斑位置也出现了有一定规律性的变化.实验通过确定光斑位置的变化量从而求出鞍型... 详细信息

通过对光纤准直器准直失配,即离轴耦合、偏角耦合、间距耦合三种情况的耦合损耗进行分析,发现角度偏移对耦合效率影响最大.实验中随着温度周期性的变化,光斑位置也出现了有一定规律性的变化.实验通过确定光斑位置的变化量从而求出鞍型和拱型支承架在温度循环时的角度偏移为519μrad和395μrad,并导致了0.944dB和0.718dB的耦合损耗;在温度冲击时的角度偏移为986μrad和138μrad,并导致了1.793dB和0.251dB的耦合损耗.实验结果表明拱型支承架在两种不同的温度变化情况下均优于鞍型支承架.

关键词：光纤准直器光纤支承架激光焊接角度偏移

基于单光子雪崩二极管阵列的成像技术研究进展(特邀)

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光子学报 2022年第8期51卷 182-198页

作者：孙鸣捷王知冠北京航空航天大学仪器科学与光电工程学院北京100191 北京航空航天大学未来空天技术学院/高等理工学院北京100191

单光子雪崩二极管以其极高的光子灵敏度以及超快的响应时间在各领域被广泛应用。随着半导体技术的发展,集成多个像素以及时间测量电路的单光子雪崩二极管阵列逐渐普及。成像是一种以光子作为媒介获取目标物体信息的手段,基于单光子雪崩... 详细信息

单光子雪崩二极管以其极高的光子灵敏度以及超快的响应时间在各领域被广泛应用。随着半导体技术的发展,集成多个像素以及时间测量电路的单光子雪崩二极管阵列逐渐普及。成像是一种以光子作为媒介获取目标物体信息的手段,基于单光子雪崩二极管的成像系统可以利用更丰富的光子计数以及光子时间信息实现极端环境下的目标探测。单光子雪崩二极管阵列具备并行采集光子信息的能力,进一步提高了光子信息的探测效率,能够替代传统单光子成像中单点探测器加扫描结构的探测体系,推动生物显微成像、散射成像以及非视域成像等技术的进步。本文梳理了单光子雪崩二极管阵列的发展历程以及技术趋势,按照是否需要光子时间信息分类介绍了单光子雪崩二极管阵列在成像方面的典型应用,结合应用分析了单光子雪崩二极管阵列相比于其他探测器的优势,对单光子雪崩二极管阵列的应用前景进行了展望。

关键词：单光子雪崩二极管阵列成像系统时间相关光子计数技术生物光子学散射成像非视域成像

像素有效形状对微扫描红外超分辨成像的影响(英文)

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红外与激光工程 2015年第1期44卷 48-52页

作者：孙鸣捷于康龙北京航空航天大学仪器科学与光电工程学院北京100091

超分辨成像是基于过采样来降低频率混叠、提高图像分辨率的技术,而像素有效形状是超分辨相关研究的重要对象。基于实际的红外焦平面阵型提出了"Z"形有效形状模型,并分析了常用的方形模型和"Z"形模型分别得到调制传递函数(MTF)的差别。... 详细信息

超分辨成像是基于过采样来降低频率混叠、提高图像分辨率的技术,而像素有效形状是超分辨相关研究的重要对象。基于实际的红外焦平面阵型提出了"Z"形有效形状模型,并分析了常用的方形模型和"Z"形模型分别得到调制传递函数(MTF)的差别。还提出了形状边界到中心点的差值越小,其得到的MTF越大的假设,通过对不同形状模型的MTF推导分析和数值模拟,其结果证实了这一假设。数值模拟结果还表明圆形模型具有最大的MTF值。上述结论对未来的红外焦平面阵型设计与生产具有参考意义。

关键词：微扫描红外超分辨成像像素有效形状