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npj Flexible Electronics 2023年第1期7卷 524-534页

作者： T.S.Lopes J.P.Teixeira m.A.Curado B.R.Ferreira A.J.N.Oliveira J.m.V.Cunha m.monteiro A.Violas J.R.S.Barbosa P.C.Sousa I.Çaha J.Borme K.Oliveira J.Ring W.C.Chen Y.Zhou K.Takei E.Niemi F.L.Deepak m.Edoff G.Brammertz P.A.Fernandes B.Vermang P.m.P.Salomé INL-International Iberian Nanotechnology Laboratory Avenida Mestre JoséVeiga4715-330 BragaPortugal Hasselt University imo-imomecMartelarenlaan 423500 HasseltBelgium Imec imo-imomecThor Park 83203600 GenkBelgium EnergyVille imo-imecThorPark 83203600 GenkBelgium CFisUC Department of PhysicsUniversity of CoimbraP-3004-516 CoimbraPortugal Departamento de Física Universidade de AveiroCampus Universitário de Santiago3810-193 AveiroPortugal i3N Universidade de AveiroCampus Universitário de Santiago3810-193 AveiroPortugal Obducat AB Medicon Village22363 LundSweden Ångström Laboratory Department of Engineering SciencesUppsala University75121 UppsalaSweden midsummer AB Elektronikhõjden 6SE-17543 JãrfãllaSweden CIETI Departamento de FísicaInstituto Superior de Engenharia do PortoInstituto Politécnico do Porto4200-072 PortoPortugal

The incorporation of interface passivation structures in ultrathin Cu(In,Ga)Se_(2)based solar cells is *** fabrication used an industry scalable lithography technique—nanoimprint lithography(NIL)—for a 15×15 cm^(2)dielectric layer *** with a NIL nanopatterned dielectric layer are benchmarked against electron-beam lithography(EBL)patterning,using rigid *** NIL patterned device shows similar performance to the EBL patterned *** impact of the lithographic processes in the rigid solar cells’performance were evaluated via X-ray Photoelectron Spectroscopy and through a Solar Cell Capacitance *** device on stainless-steel showed a slightly lower performance than the rigid approach,due to additional challenges of processing steel substrates,even though scanning transmission electron microscopy did not show clear evidence of impurity ***,time-resolved photoluminescence results strongly suggested elemental diffusion from the flexible ***,bending tests on the stainless-steel device demonstrated the mechanical stability of the CIGS-based device.

关键词： lithography ultrathin rigid

A comparative study on emergent pollutants photo-assisted degradation using ruthenium modified titanate nanotubes and nanowires as catalysts

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Journal of Environmental Sciences 2020年第6期32卷 38-51页

作者： Beatriz Barrocas m.Conceicao Oliveira Helena I.S.Nogueira Sara Fateixa Olinda C.monteiro Centro de Química Estrutural Faculdade de CienciasUniversidade de LisboaLisboa 1749-016Portugal Centro Química Estrutural Instituto Superior TécnicoUniversidade de LisboaLisboa 1049-001Portugal Department of Chemistry CICECO-Aveiro Institute of MaterialsUniversity of AveiroAveiro 3810-193Portugal

Several methods have been used to tailor nanomaterials structure and ***,slight changes in the structure outcomes expressive improvements in the optical and photocatalytic properties of semiconductor *** this context,the influence of the metal doping and the morphology on a catalyst performance was studied in this ***,ruthenium doped titanate nanotubes(RuTNT)were synthesised for the first time using an amorphous Ru-containing ***,the photocatalytic performance of this sample was compared to the one obtained for ruthenium titanate nanowires(RuTNW),recently *** samples,RuTNW and RuTNT,were produced using the same Ru-containing precursor but distinct hydrothermal *** powders were structural,morphological and optical characterized by X-ray diffraction and fluorescence,transmission electron microscopy,Raman,X-ray photoelectron and photoluminescence *** variations on the structural and optical properties of the RuTNT and RuTNW nanoparticles,due to ruthenium incorporation were *** potential use as photocatalysts was evaluated on the hydroxyl radical photo-assisted *** samples were catalytic for this reaction,presenting better performances than the pristine counterparts,being RuTNT the best ***,the degradation of two emergent pollutants,caffeine and sulfamethazine,was *** demonstrated to be better photocatalyst than RuTNW for caffeine but identical performances were obtained for *** both catalysts,the degradation mechanism of the pollutants was explored through the identification and quantification of the intermediate compounds produced and several differences were *** indicates the importance of the structural and morphological aspects of a material on its catalytic performance.

关键词： Titanate nanotubes and nanowires Ruthenium doping Ru-Ti replacement Emergent pollutants Photocatalytic degradation

Degradation of duloxetine: Identification of transformation products by UHPLC-ESI(+)-HRmS/mS,in silico toxicity and wastewater analysis

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Journal of Environmental Sciences 2019年第8期31卷 113-123页

作者： Rodrigo A.Osawa Ana P.Carvalho Olinda C.monteiro m.Conceicao Oliveira m.Helena Florêncio Centro de Química e Bioquímica Faculdade de Ciências Universidade de Lisboa Laboratório de FTICR e Espectrometria de massa Estrutural Faculdade de Ciências Universidade de Lisboa Centro de Química Estrutural Instituto Superior Técnico Universidade de Lisboa

Duloxetine(DUL), an antidepressant drug, has been detected in surface water and wastewater effluents, however, there is little information on the formation of its transformation products(TPs). In this work, hydrolysis, photodegradation(UV irradiation) and chlorination experiments were performed on spiked distillated water, under controlled experimental conditions to simulate abiotic processes that can occur in the environment and wastewater treatment plants(WWTPs). Eleven TPs, nine from reaction with UV light and two from chlorine contact, were formed and detected by ultra-high performance liquid chromatography coupled to quadrupole time-of-flight mass spectrometry, and nine of them had their chemical structures elucidated upon analyses of their fragmentation patterns in mS/mS spectra. The formation and degradation of the TPs were observed. The parent compound was completely degraded after30 min in photodegradation and after 24 hr in chlorination. Almost all TPs were completely degraded in the experiments. The ecotoxicity and mutagenicity of the TPs were predicted based on several in silico models and it was found that a few of these products presented more ecotoxicity than DUL itself and six TPs showed positive mutagenicity. Finally, wastewater samples were analyzed and DUL and one TP, possibly formed by chlorination process, were detected in the effluent, which showed that WWTP not only did not remove DUL, but also formed a TP.

关键词： High resolution mass spectrometry Duloxetine Degradation processes Transformation products Wastewater analysis In silico toxicity

Replication of natural surface topographies to generate advanced cell culture substrates

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Bioactive materials 2023年第10期28卷 337-347页

作者： N.O.monteiro J.F.Fangueiro R.L.Reis N.m.Neves 3B’s Research Group I3Bs-Research Institute on BiomaterialsBiodegradables and BiomimeticsUniversity of MinhoHeadquarters of the European Institute of Excellence on Tissue Engineering and Regenerative MedicineAveParkParque de Ciencia e Tecnologi1Zona Industrial da Gandr14805-017BarcoGuimaraesPortugal ICVS/3B’s-PT Government Associate Laboratory Brag1Guimar˜aesPortugal

Surface topographies of cell culture substrates can be used to generate in vitro cell culture environments similar to the in vivo cell niches. In vivo, the physical properties of the extracellular matrix (ECm), such as its topography, provide physical cues that play an important role in modulating cell function. mimicking these properties remains a challenge to provide in vitro realistic environments for cells. Artificially generated substrates’ topographies were used extensively to explore this important surface cue. more recently, the replication of natural surface topographies has been enabling to exploration of characteristics such as hierarchy and size scales relevant for cells as advanced biomimetic substrates. These substrates offer more realistic and mimetic environments regarding the topographies found in vivo. This review will highlight the use of natural surface topographies as a template to generate substrates for in-vitro cell culture. This review starts with an analysis of the main cell functions that can be regulated by the substrate’s surface topography through cell-substrate interactions. Then, we will discuss research works wherein substrates for cell biology decorated with natural surface topographies were used and investigated regarding their influence on cellular performance. At the end of this review, we will highlight the advantages and challenges of the use of natural surface topographies as a template for the generation of advanced substrates for cell culture.

关键词： Biomimetic topography Cell culture substrates Natural surface topographies

Seismic performance of composite moment-resisting frames achieved with sustainable CFST members

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Frontiers of Structural and Civil Engineering 2016年第3期10卷 312-332页

作者： A. SILVA Y. JIANG L. mACEDO J. m. CASTRO R. monteiro N. SILVESTRE Department of Civil Engineering Faculty of Engineering University of Porto Porto 4099-002 Portugal Istituto Universitario di Studi Superiori di Pavia Pavia 27100 Italy IDmEC LAETA Department of Mechanical Engineering Instituto Superior Tecnico Universidade de Lisboa Lisboa 1649-004 Portugal

The main objective of the research presented in this paper is to study the bending behaviour of Concrete Filled Steel Tube （CFST） columns made with Rubberized Concrete （RuC）, and to assess the seismic performance of moment-resisting frames with these structural members. The paper describes an experimental campaign where a total of 36 specimens were tested, resorting to a novel testing setup, aimed at reducing both the preparation time and cost of the test specimens. Different geometrical and material parameters were considered, namely cross-section type, cross-section slenderness, aggregate replacement ratio, axial load level and lateral loading type. The members were tested under both monotonic and cyclic lateral loading, with different levels of applied axial loading. The test results show that the bending behaviour of CFST elements is highly dependent on the steel tube properties and that the type of infill does not have a significant influence on the flexural behaviour of the member. It is also found that Eurocode 4 is conservative in predicting the flexural capacity of the tested specimens. Additionally, it was found that the seismic design of composite moment- resisting frames with CFST columns, according to Eurocode 8, not only leads to lighter design solutions but also to enhanced seismic performance in comparison to steel frames.

关键词： concrete filled steel tubes rubberized concrete composite frames seismic performance assessment

On the Factors Affecting the Accuracy and Robustness of Smoothed-Radial Point Interpolation method

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Advances in Applied mathematics and mechanics 2017年第1期9卷 43-72页

作者： Abderrachid Hamrani Idir Belaidi Eric monteiro Philippe Lorong Research team mISP LEMIUniversity of M’Hamed Bougara de Boumerdes35000Algerie PImm Arts et M´etiers ParisTechCNRS151 bd de l’Hˆopital75013 ParisFrance

In order to overcome the possible singularity associated with the Point Interpolation method(PIm),the Radial Point Interpolation method(RPIm)was proposed by *** basis functions(RBF)was used in RPIm as basis functions for *** these radial basis functions include shape *** choice of these shape parameters has been and stays a problematic theme in RBF approximation and interpolation *** object of this study is to contribute to the analysis of how these shape parameters affect the accuracy of the radial *** RPIm is studied based on the global Galerkin weak form performed using two integration technics:classical Gaussian integration and the strain smoothing integration *** numerical performance of this method is tested on their behavior on curve fitting,and on three elastic mechanical problems with regular or irregular nodes distributions.A range of recommended shape parameters is obtained from the analysis of different error indexes and also the condition number of the matrix *** resulting RPIm methods perform very well in term of numerical *** Smoothed Radial Point Interpolation method(SRPIm)shows a higher accuracy,especially in a situation of distorted node scheme.

关键词： Radial Basis Function Radial Point Interpolation methods strain smoothing nodal integration Galerkin weak form

metal-organic frameworks of lanthanide iminodiacetates and tartrates:Synthesis,structural characterization and luminescence properties——Commemorating the 100th anniversary of the birth of Academician Guangxian Xu

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Journal of Rare Earths 2021年第5期39卷 487-494页

作者： melissa Fairley m.m.Varuni S.Livera Wanmin Chen Jorge H.S.K.monteiro Adam Schmitt Ana de Bettencourt-Dias Sue Roberts Zhiping Zheng Department of Chemistry and Biochemistry University of ArizonaTucsonAZ 85721USA Department of Chemistry Southern University of Science and TechnologyShenzhen 518055China Department of Chemistry University of NevadaRenoNV 89557USA

Two series of lanthanide-containing metal-organic frameworks(Ln-mOFs)of the general formula{[Ln(HIDA)_(2)H_(2)O]ClO_(4)·H_(2)O}_n(Ln=La(1),Nd(2),Eu(3),Gd(4),Tb(5),Eu:Tb(6);H_(2)IDA=iminodiacetic acid)and[Ln(TT)(HTT)(H_(2)O)_3]_n(Ln=Eu(7),Gd(8),Tb(9),Dy(10),and Eu:Tb(11);H_(2)TT=tartaric acid)were synthesized by reacting Ln(ClO_(4))_3 with iminodiacetic acid and L-tartaric acid,*** compounds were structurally characterized by single-crystal X-ray *** analyses are co nsistent with the corre sponding crystallographically generated *** reover,the luminescence properties of both the single and mixed-lanthanide complexes were *** infrared,red,and green emissions that are characteristic of Nd(Ⅲ),Eu(Ⅲ),and Tb(Ⅲ)are observed for 2,3/7,and 5/9,*** the two mixed-lanthanide complex systems 6 and 11,depending on the relative amount of Eu(Ⅲ)and Tb(Ⅲ),the color of emission can be *** is found that a small amount of Eu(Ⅲ)is adequate for the observation of the most intense transition of Eu(Ⅲ).This is believed to be a result of energy transfer from Tb(Ⅲ)to Eu(Ⅲ)within the same complex-a conclusion supported by the significantly shortened lifetime of Tb(Ⅲ)and the accompanying enhanced lifetime of Eu(Ⅲ)in the mixedlanthanide complex with respect to the corresponding values for the pure Tb(Ⅲ)and Eu(Ⅲ)complexes with the same ligand.

关键词： Lanthanides metal-organic frameworks Luminescence Rare earths

Effect of Alloying Additions on the Oxidation of High Speed Steels under Dry and Wet Conditions

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中国腐蚀与防护学报 2009年第4期29卷 241-247页

作者： F. C. RIZZO m. J. monteiro S. R. J. SAUNDERS DCmm PUC Rio de Janeiro Brazil Bentley Surrey UK

An investigation has been carried out into the effects of chromium and vanadium content on the oxidation rate and on the adhesion of oxide scales grown on three different chemical compositions of high speed steels under dry and wet *** oxidation tests were carried out in a thermobalance at 650℃for up to 14.4 *** mass gain of the specimens increased with increasing contents of water vapour. Alloy composition had no effect on the oxidation rate in dry ***'adhesion'of the oxide scale was determined using indentation with a Rockwell C diamond and the pull adhesion test to determine the interfacial toughness and the tensile strength of the oxide metal bond,***,the results of the investigation indicated that oxide adhesion was lowest for the specimens exposed to dry conditions, and that with increasing water vapour content,the scale was more *** test results showed that an increase in the V concentration was deleterious to oxide adhesion in both the dry and wet environments,whereas an increase in the Cr-content had little effect on adhesion.

关键词：合金腐蚀氧化金属材料

Behavior of wood basic density according to environmental variables

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Journal of Forestry Research 2022年第2期33卷 497-505页

作者： Gabriel marcos Vieira Oliveira Josémárcio de mello Carlos Rogério de mello JoséRoberto Soares Scolforo Eder Pereira miguel Thiago Campos monteiro Brazil Institute of Agricultural and Forestry Defense of Espírito Santo(IDAF) Av.Lourival Lugon Moulinnº300CentroJerônimo MonteiroES CEP:29.550-000Brazil Department of Forestry Sciences Universidade Federal de Lavras-UFLACaixa Postal 3037LavrasMG CEP:37.200-000Brazil Engineering Department Universidade Federal de Lavras-UFLACaixa Postal 3037LavrasMG CEP:37.200-000Brazil Forestry Engineering Department Faculdade de TecnologiaUniversity of Brasilia-UnBCampus Universitário Darcy RibeiroCaixa Postal 4357Asa Norte-BrasíliaDF CEP:70910-900Brazil Department of Forestry Engineering and Technology Universidade Federal do Paraná-UFPRAv.Pref.Lothário Meissner632Jardim BotânicoCuritibaPR CEP:80.210-170Brazil

The relationships between climate conditions and wood density in tropical forests are still poorly *** quantify spatial dependence of wood density in the state of minas Gerais(mG,Brazil),map spatial distribution of density,and correlate density with climate variables,we extracted data from the Forest Inventory of minas Gerais for 1988 trees scaled throughout the territory and measured wood density of discs removed from the *** variables were extracted from the database of the Ecological-Economic Zoning of minas *** spatial analysis,tree densities were measured at 44 georeferenced sampling *** data were subjected to exploratory analysis,variography,cross-validation,model selection,and ordinary *** relationships between wood density and environmental variables were calculated using dispersion matrices,linear correlation,and *** density proved to be highly spatially dependent,reaching a correlation of 96%,and was highly continuous over a distance of 228 *** distribution of wood density followed a continuous gradient of 514-659 kg m^(−3),enabling corre-lation with environment *** was correlated with mean annual precipitation(−0.57),temperature(0.63),and evapotranspiration(0.83).Geostatistical methods proved useful in predicting wood density in native tropical forests with different climate *** results confirmed the sensitivity of wood density to climate change,which could affect future carbon stock in forests.

关键词： Biomass Climate variables Geostatistics Hardwood Forest inventory minas Gerais