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Molecular packing tuning via chlorinated end group enables efficient binary organic solar cells over 18.5%

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Carbon Energy 2024年第3期6卷 196-203页

作者： Yafeng Li Zhenyu Chen Xingzheng Yan Ziyi ge Zhejiang Business Technology Institute NingboZhejiangChina Zhejiang Engineering Research Center for Energy Optoelectronic Materials and Devices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingboZhejiangChina Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijingChina

Designing novel nonfullerene acceptors(NFAs)is of vital importance for the development of organic solar cells(OSC).Modification on the side chain and end group are two powerful tools to construct efficient ***,based on the high-performance L8BO,we selected 3-ethylheptyl to substitute the inner chain of 2-ethylhexyl,obtaining the backbone of *** we introduced different halogen atoms of fluorine and chlorine on 2-(3-oxo-2,3-dihydro-1Hinden-1-ylidene)malononitrile end group(EG)to construct efficient NFAs named BON3-F and BON3-Cl,*** donor D18 was chosen to combine with two novel NFAs to construct OSC ***,D18:BON3-Cl-based device shows a remarkable power conversion efficiency(PCE)of 18.57%,with a high open-circuit voltage(V_(OC))of 0.907 V and an excellent fill factor(FF)of 80.44%,which is one of the highest binary PCE of devices based on D18 as the ***,BON3-F-based device shows a relatively lower PCE of 17.79%with a decreased FF of 79.05%.The better photovoltaic performance is mainly attributed to the red-shifted absorption,higher electron and hole mobilities,reduced charge recombination,and enhanced molecular packing in the D18:BON3-Cl ***,we performed stability tests on two binary systems;the D18:BON3-Cl and D18:BON3-F devices maintain 88.1%and 85.5%of their initial efficiencies after 169 h of storage at 85°C in an N2-filled glove box,*** work demonstrates the importance of selecting halogen atoms on EG and provides an efficient binary system of D18:BON3-Cl for further improvement of PCE.

关键词： binary organic solar cell chlorinated end group molecular packing

Digital light processing based multimaterial 3D printing: challenges, solutions and perspectives

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INTERNATIONAL JOURNAL OF EXTREME MANUFACTURING 2024年第4期6卷 151-174页

作者： Cheng, Jianxiang Yu, Shouyi Wang, Rong ge, Qi Southern Univ Sci & Technol Shenzhen Key Lab Soft Mech & Smart Mfg Shenzhen 518055 Peoples R China Southern Univ Sci & Technol Dept Mech & Energy Engn Shenzhen 518055 Peoples R China

Multimaterial (MM) 3D printing shows great potential for application in metamaterials, flexible electronics, biomedical devices and robots, since it can seamlessly integrate distinctive materials into one printed structure. Among numerous MM 3D printing technologies, digital light processing (DLP) MM 3D printing is compatible with a wide range of materials from hydrogels to ceramics, and can print MM 3D structures with high resolution, high complexity and fast speed. This paper introduces the fundamental mechanisms of DLP 3D printing, and reviews the recent advances of DLP MM 3D printing technologies with emphasis on material switching methods and material contamination issues. It also summarizes a number of typical examples of DLP MM 3D printing systems developed in the past decade, and introduces their system structures, working principles, material switching methods, residual resin removal methods, printing steps, as well as the representative structures and applications. Finally, we provide perspectives on the directions of the further development of DLP MM 3D printing technology. Review the recent advances of digital light processing multimaterial 3D printing. Summarize critical challenges in digital light processing multimaterial 3D printing. Provide perspectives on directions of further development of multimaterial 3D printing.

关键词： multimaterial 3D printing digital light processing multimaterial 3D structures SOFT MATTER STEREOLITHOGRAPHY TEMPERATURE FABRICATION

Attack-Resilient Distributed Cooperative Control of Virtually Coupled High-Speed Trains via Topology Reconfiguration

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IEEE/CAA Journal of Automatica Sinica 2024年第4期11卷 1066-1068页

作者： Shunyuan Xiao Xiaohua ge Qing Wu the Institute of Advanced Technology Nanjing University of Posts and TelecommunicationsNanjing 210023China the School of Science Computing and Engineering TechnologiesSwinburne University of TechnologyMelbourne VIC 3122Australia the School of Engineering and Technology Central Queensland UniversityRockhampton QLD 4701Australia

Dear Editor,This letter addresses the resilient distributed cooperative control problem of a virtually coupled train convoy under stochastic disturbances and cyber *** main purpose is to achieve distributed coordinati... 详细信息

关键词： prescribed Speed trains

An ultra-thin bolt tension sensor and online monitoring system:For application in hydropower plant unit

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Frontiers of Structural and Civil Engineering 2024年第9期18卷 1388-1400页

作者： Shaoquan ZHANG Yanke TAN Hanbin ge Qilin ZHANG Department of Civil Engineering Meijo UniversityNagoya 4688502Japan College of Civil Engineering Tongji UniversityShanghai 200092China

The condition of bolted connections significantly affects the structural ***,conventional bolt tension sensors fail to provide precise measurements due to their bulky size or inadequate *** study employs the piezoresistive effect of crystalline silicon material to fabricate an ultrathin *** sensor exhibits a linear relationship between pressure and voltage,an exceptional stability at varying temperatures,and a superior resistance to corrosion,making it adaptable and user-friendly for applications of high-strength bolt tension monitoring.A monitoring system,incorporating the proposed sensor,has also been *** system provides real-time display of bolt tension and enables the assessment of sensor and structural conditions,including bolt loosening or component *** efficacy of the proposed sensor and monitoring system was validated through a project carried out at the Xiluodu Hydropower *** to the results,the sensor and online monitoring system effectively gauged and proficiently conveyed and stored bolt tension *** addition,correlations were created between bolt tensions and essential unit parameters,such as water head,active power,and pressures at vital points,facilitating anomaly detection and early warning.

关键词： ultra-thin sensor high-strength bolt tension online monitoring system anomaly alarm hydro-generator units

Constructal design of a rectangular porous fin considering minimization of maximum temperature difference and pumping power consumption

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Science China(Technological Sciences) 2024年第3期67卷 919-929页

作者： LIU XiaoYe FENG HuiJun CHEN Lingen ge YanLin Institute of Thermal Science and Power Engineering Wuhan Institute of TechnologyWuhan 430205China College of Power Engineering Naval University of EngineeringWuhan 430033China Hubei Provincial Engineering Technology Research Center of Green Chemical Equipment Wuhan 430205China School of Mechanical&Electrical Engineering Wuhan Institute of TechnologyWuhan 430205China

A heat dissipation model of a rectangular porous fin is established based on constructal theory. First, the constructal design of rectangular porous fin is conducted by selecting a complex function minimization, which composed of linear weighting sum of maximum temperature difference and pumping power consumption, as optimization objective. Effects of gap height, air inlet velocity, total porous fin volume and porosity on the optimal constructs are investigated, respectively. The findings show that the complex function can attain its double minimum at a value of 0.802 when the fin length and number are optimized, and the corresponding optimal fin length and number are 8.01 mm and 10, respectively. In comparison to original design, the complex function and maximum temperature difference after twice optimization are decreased by 19.80% and 66.31%, ***, the comprehensive performance of porous fin is improved by simultaneously optimizing the fin length and number. The artificial neural network is applied to predict the fin performances, which is used to conduct multi-objective optimization based on NSGA-II algorithm. Optimal structure of porous fin for multiple requirements is gained by LINMAP and TOPSIS decisionmaking strategies. The findings in this study can serve as theoretical guides for fin thermal designs of electronic devices.

关键词： constructal theory rectangular porous fin pumping power consumption maximum temperature difference complex function multi-objective optimization

Design of an automated robotic microinjection system for batch injection of zebrafish embryos and larvae

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Microsystems & Nanoengineering 2024年第1期10卷 89-103页

作者： Zhongyi Guo Nana Ai Wei ge Qingsong Xu Department of Electromechanical Engineering Faculty of Science and TechnologyUniversity of MacaoMacaoChina Department of Biomedical Sciences and Centre of Reproduction Development and Aging(CRDA)Faculty of Health SciencesUniversity of MacaoMacaoChina

This paper presents the design of a vision-based automated robotic microinjection system for batch injection of both zebrafish embryos and larvae.A novel visual recognition algorithm based on an automatic threshold and excessive dilatation is introduced to accurately identify the center of zebrafish embryos and larval yolks.A corresponding software system is developed using the producer-consumer model as the framework structure,and a friendly user interface is designed to allow operators to choose from a range of desired functions according to their different *** addition,a novel microstructural agarose device is designed and fabricated to simultaneously immobilize mixed batches of embryos and ***,a prototype microinjection system is fabricated by integrating hardware devices with visual *** experimental study is conducted to verify the performance of the robotic microinjection *** results show that the reported system can accurately identify zebrafish embryos and larvae and efficiently complete batch microinjection tasks of the mixtures with an injection success rate of 92.05%in 13.88 s per *** with manual and existing microinjection systems,the proposed system demonstrates the merits of versatility,excellent efficiency,high success rate,high survival rate,and sufficient stability.

关键词： zebra automated hardware

Energy and exergy analyses and optimizations for two-stage TEC driven by two-stage TEG with Thomson effect

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Science China(Technological Sciences) 2024年第4期67卷 1077-1093页

作者： CHEN Lingen ge YanLin FENG HuiJun REN TingTing Institute of Thermal Science and Power Engineering Wuhan Institute of TechnologyWuhan 430205China Hubei Provincial Engineering Technology Research Center of Green Chemical Equipment Wuhan 430205China School of Mechanical&Electrical Engineering Wuhan Institute of TechnologyWuhan 430205China

Based on the non-equilibrium thermodynamics and energy and exergy analyses,a thermodynamic model of two-stage thermoelectric(TE)cooler(TTEC)driven by two-stage TE generator(TTEG)(TTEG-TTEC)combined TE device is established with involving Thomson effect by fitting method of variable physical parameters of TE *** total number of TE elements as constraint,influences of number distributions of TE elements on three device performance indictors,that is,cooling load,maximum COP and maximum exergetic efficiency,are *** number distributions of TE elements are optimized with three maximum performance indictors as the objectives,*** of hot-junction temperature of TTEG and coldjunction temperature of TTEC on optimization results are analyzed,and difference between optimization results corresponding to three performance indicators are *** performance intervals and optimal variable intervals are *** of Thomson effect on three general performance indicators,three optimal performance indicators and optimal variables are comparatively *** effect reduces three general performance indicators and three optimal performance indicators of *** hot-and cold-junction temperatures of TTEG and TTEC are 450,305,325 and 295 K,respectively,Thomson effect reduced maximum cooling load,maximum COP and maximum exergetic efficiency from 9.528 W,9.043×10^(-2)and2.552%to 6.651 W,6.286×10^(-2)and 1.752%,respectively.

关键词： non-equilibrium thermodynamics cooling load COP exergetic efficiency combined thermoelectric device performance optimization

End-group modulation of phenazine based non-fullerene acceptors for efficient organic solar cells with high open-circuit voltage

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Journal of Energy Chemistry 2024年第1期88卷 461-468,I0011页

作者： Yahui Zhang Yafeng Li Ruixiang Peng Yi Qiu Jingyu Shi Zhenyu Chen Jinfeng ge Cuifen Zhang Zheng Tang Ziyi ge School of Materials Science and Engineering Shanghai UniversityShanghai 200444China Zhejiang Business Technology Institute Ningbo 315012ZhejiangChina Zhejiang Provincial Engineering Research Center of Energy Optoelectronic Materials and Devices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201ZhejiangChina Center for Advanced Low-dimension Materials College of Materials Science and EngineeringDonghua UniversityShanghai 201620China

Phenazine-based non-fullerene acceptors(NFAs)have demonstrated great potential in improving the power conversion efficiency(PCE)of organic solar cells(OSCs).Halogenation is known to be an effective strategy for increasing optical absorption,refining energy levels,and improving molecular packing in organic ***,a series of NFAs(Pz IC-4H,Pz IC-4F,Pz IC-4Cl,Pz IC-2Br)with phenazine as the central core and with/without halogen-substituted(dicyanomethylidene)-indan-1-one(IC)as the electron-accepting end group were synthesized,and the effect of end group matched phenazine central unit on the photovoltaic performance was systematically *** photophysical and morphological analyses revealed that the PM6:Pz IC-4F blend involves efficient exciton dissociation,higher charge collection and transfer rates,better crystallinity,and optimal phase ***,OSCs based on PM6:Pz IC-4F as the active layer exhibited a PCE of 16.48%with an open circuit voltage(Voc)and energy loss of 0.880 V and 0.53 e V,***,this work demonstrated a promising approach by designing phenazine-based NFAs for achieving high-performance OSCs.

关键词： Organic solar cells Non-fullerene acceptor Phenazine Central core End group

Nitrogen isotope stratigraphy of the Early Cambrian successions in the Tarim Basin:Spatial variability of nitrogen cycling and its implication for paleo-oceanic redox conditions

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Acta geochimica 2024年第4期43卷 785-801页

作者： Bi Zhu Xuefeng Li Lu ge Yongquan Chen Institute of Earth’s Critical Zone School of Earth Sciences and EngineeringHohai UniversityNanjing 210098China Research Institute of Exploration and Development Tarim Oil Field CompanyPetroChinaKorlaChina

The Early Cambrian represents a critical time period characterized by extraordinary biological innovations and dynamic redox conditions in *** isotopic signatures of ancient sediments have the potential to elucidate the evolutionary path of marine redox states and the biogeochemical nitrogen cycle within the water column of the Early Cambrian *** existing research on this topic has predominantly focused on South China,the exploration of other continental margins has been limited,leaving contradictory hypotheses *** this study,pairedδ^(15)N andδ^(13)C org analyses were performed on the Lower Cambrian successions from the Shiairike section(inner ramp)and Well Tadong 2(deep shelf/basin)in the northwestern and eastern Tarim Basin,*** data from the Shiairike section reveal a discernible shift in the operation of different nitrogen cycles for the black chert-shale unit,also referred to as the black rock series in Chinese literature,of the Yurtus Formation(Fortunian stage to lower Stage 3).Oscillatingδ^(15)N values for its lower part are suggestive of alternating anaerobic assimilation of NH 4+and denitrification/*** is likely attributed to a shallow,unstable chemocline consistent with the upwelling and incursion of deep,anoxic waters during a major *** contrast,aerobic nitrogen cycling,indicated by positiveδ^(15)N values of>2‰,dominated the upper part alongside a reduction in upwelling *** the other hand,theδ^(15)N signatures of Xishanbulake and Xidashan Formations of Well Tadong 2,which encompass a time interval from the Cambrian Fortunian Age to Age 4,are indicative of N_(2)fixation by diazotrophs as the major nitrogen *** two studied intervals,although not time-equivalent,exhibit separated states of nitrogen cycling at least during the deposition of the Yurtus black rock *** spatially different nitrogen cycling of the studied sections is compatible with a redox-stratified ocean dur

关键词： Nitrogen isotopes Early Cambrian Tarim Black rock series