Toward scalable fabrication of electrochemical paper sensor without surface functionalization
作者机构:State Key Laboratory of Pulp and Paper EngineeringSouth China University of Technology(SCUT)Guangzhou 510640China Institute for Bioscience and Biotechnology Research(IBBR)University of MarylandCollege ParkMD 20742USA State Key Laboratory of Biobased Material and Green PapermakingShandong Academy of SciencesQilu University of TechnologyJinan 250353China School of Resource and Environmental ScienceHubei Biomass-Resource Chemistry and Environmental Biotechnology Key LaboratoryWuhan UniversityWuhan 430079China
出 版 物:《npj Flexible Electronics》 (npj-柔性电子(英文))
年 卷 期:2022年第6卷第1期
页 面:99-106页
核心收录:
学科分类:08[工学] 0805[工学-材料科学与工程(可授工学、理学学位)] 080502[工学-材料学]
基 金:supported by the National Key Research and Development Program of China (2019YFE0114400) the Taishan Industrial Leading Talent Project (20180215) the United States National Science Foundation (CBET-1932963)
主 题:composite surface portable
摘 要:Paper-based electrochemical sensors provide the opportunity for low-cost,portable and environmentally friendly single-use chemical analysis and there are various reports of surface-functionalized paper *** we report a composite paper electrode that is fabricated through designed papermaking using cellulose,carbon fibers(CF),and graphene oxide(GO).The composite paper has well-controlled structure,stable,and repeatable properties,and offers the electrocatalytic activities for sensitive and selective chemical *** demonstrate that this CF/GO/cellulose composite paper can be reduced electroche mically using relatively mild conditions and this GO reduction confers electrocatalytic properties to the composite ***,we demonstrate that this composite paper offers sensing performance(sensitivity and selectivity)comparable to,or better than,paperbased sensors prepared by small-batch surface-modification(e.g.,printing)*** envision this coupling of industrialized papermaking technologies with interfacial engineering and electrochemical reduction can provide a platform for single-use and portable chemical detection for a wide range of applications.