Regulation of the activity,selectivity,and durability of Cu-based electrocatalysts for CO_(2) reduction

作     者：Chang Liu Jun Gong Zeyu Gao Li Xiao Gongwei Wang Juntao Lu Lin Zhuang Chang Liu;Jun Gong;Zeyu Gao;Li Xiao;Gongwei Wang;Juntao Lu;Lin Zhuang

作者机构：College of Chemistry and Molecular SciencesHubei Key Lab of Electrochemical Power SourcesWuhan UniversityWuhan 430072China The Institute for Advanced StudiesWuhan UniversityWuhan 430072China 

出 版 物：《Science China Chemistry》 (中国科学（化学英文版）)

年 卷 期：2021年第64卷第10期

页      面：1660-1678页

核心收录：

学科分类：083002[工学-环境工程] 0830[工学-环境科学与工程（可授工学、理学、农学学位）] 081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 080502[工学-材料学] 0805[工学-材料科学与工程（可授工学、理学学位）] 

基　　金：the National Natural Science Foundation of China(21991154 21991150 92045302) 

主　　题：CO_(2)electroreduction Cu-based catalysts activity selectivity durability 

摘      要：CO_(2)electroreduction offers a promising approach to alleviate global warming and reduce petroleum consumption simultaneously,due to its capability to convert the greenhouse gas CO_(2)to valuable fuels and chemicals by using renewable *** has an essential impact on the CO_(2)electroreduction *** the diverse exploited materials,Cu is the only monometallic electrocatalyst that can produce CO and ***,its activity,selectivity,and durability are not satisfactory for practical ***,we make a comprehensive survey of the recent progress in enhancing Cu-based electrocatalysts with the strategies such as oxidation pre-treatment,heteroatom doping,morphological control,and surface *** review provides an overview of the current status and future opportunities for Cu-catalyzed CO_(2)*** may contribute to the rational design of Cu-based electrocatalysts with improved performance and thus advance practical CO_(2)electrolyzer development.