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Experimental observation of multiple topological nodal structure in LaSb_(2)

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Science China(physics,Mechanics & Astronomy) 2024年第4期67卷 138-145页

作者： Yuxi Qiao Fuyi Wang Huaiqiang Wang Zicheng Tao Zhicheng Jiang Zhengtai Liu Soohyun Cho Fayuan Zhang Qingkai Meng Wei Xia Yichen Yang Zhe Huang Jishan Liu Zhonghao Liu Zengwei Zhu Shan Qiao Yanfeng Guo Haijun Zhang Dawei Shen state key laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China National Synchrotron Radiation laboratory and School of Nuclear Science and TechnologyUniversity of Science and Technology of ChinaHefei 230026China National laboratory of Solid state Microstructures School of PhysicsNanjing UniversityNanjing 210093China School of physics and Technology Nanjing Normal UniversityNanjing 210023China School of Physical Science and Technology ShanghaiTech UniversityShanghai 201210China Shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210China Shenzhen Institute for Quantum Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Wuhan National high Magnetic field Center and School of physics Huazhong University of Science and TechnologyWuhan 430074China ShanghaiTech laboratory for Topological physics ShanghaiTech UniversityShanghai 201210China Institute of high-Pressure physics School of Physical Science and Technology Ningbo UniversityNingbo 315211China Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

Unconventional fermions in the immensely studied topological semimetals are the source for rich exotic topological ***,using symmetry analysis and first-principles calculations,we propose the coexistence of multiple topological nodal structure in LaSb_(2),including topological nodal surfaces,nodal lines and in particular eightfold degenerate nodal points,which have been scarcely observed in a single ***,utilizing angle-resolved photoemission spectroscopy,we confirm the existence of nodal surfaces and eightfold degenerate nodal points in LaSb_(2).The intriguing multiple topological nodal structure might play a crucial role in giving rise to the large linear *** work renews the insights into the exotic topological phenomena in LaSb_(2).

关键词： eightfold degenerate points multiple topological nodal structure angle-resolved photoemission spectroscopy linear unsaturated magnetoresistance

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Superradiance of ultracold cesium Rydberg |65D_(5/2)> → |66P_(3/2)>

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Chinese physics B 2024年第5期33卷 425-428页

作者：郝丽萍韩小萱白素英游秀芬焦月春赵建明 Department of Materials and Chemical Engineering Taiyuan UniversityTaiyuan 030032China Department of physics Taiyuan Normal UniversityJinzhong 030619China School of physics and Information Engineering Shanxi Normal UniversityTaiyuan 030031China state key laboratory of Quantum Optics and Quantum Optics Devices Institute of Laser SpectroscopyShanxi UniversityTaiyuan 030006China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China

We investigate Rydberg |65D_(5/2)> → |66P_(3/2)> superradiance in dense ultracold cesium atoms,where the ground atoms are excited to |65D_(5/2)> Rydberg states via two-photon excitation in a standard magneto-optical *** superradiant spectrum of |65D_(5/2)> → |66P_(3/2)> is obtained using the state-selective field ionization *** observe its dynamic evolution process by varying the delay time of ionization field *** results show that the evolution process of |65D_(5/2)> →|66P_(3/2)> is much shorter than its radiation lifetime at room temperature,which verifies the superradiance *** dependence of the superradiance process on Rydberg atoms number N_(e) and principal quantum number n is *** results show that the superradiance becomes faster with increasing N_(e),while it is suppressed for stronger van der Waals(vdW) *** has potential applications in quantum technologies,and the Rydberg atom is an ideal medium for *** system is effective for studying the strong two-body interaction between Rydberg atoms.

关键词： Rydberg atom superradiance van der Waals interaction

A Yb optical clock with a lattice power enhancement cavity

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Chinese physics B 2024年第3期33卷 70-74页

作者：王春云姚远师浩森于洪浮马龙生蒋燕义 state key laboratory of Precision Spectroscopy East China Normal UniversityShanghai 200062China

We construct a power enhancement cavity to form an optical lattice in an ytterbium optical *** is demonstrated that the intra-cavity lattice power can be increased by about 45 times,and the trap depth can be as large as 1400Er when laser light with a power of only 0.6 W incident to the lattice *** high trap depths are the key to accurate evaluation of the lattice-induced light shift with an uncertainty down to~1×*** probing the ytterbium atoms trapped in the power-enhanced optical lattice,we obtain a 4.3 Hz-linewidth Rabi spectrum,which is then used to feedback to the clock laser for the close loop operation of the optical lattice *** evaluate the density shift of the Yb optical lattice clock based on interleaving measurements,which is-0.46(62)*** result is smaller compared to the density shift of our first Yb optical clock without lattice power enhancement cavity mainly due to a larger lattice diameter of 344μm.

关键词： optical atomic clock optical lattice optical cavity Stark shift

Enhancing multifunctional photocatalysis with acetate-assisted cesium doping and unlocking the potential of Z-scheme solar water splitting

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Carbon Energy 2024年第3期6卷 178-195页

作者： Mengmeng Ma Jingzhen Li Xiaogang Zhu Kong Liu Kaige Huang Guodong Yuan Shizhong Yue Zhijie Wang Shengchun Qu key laboratory of Semiconductor Materials Science Beijing Key Laboratory of Low Dimensional Semiconductor Materials and DevicesInstitute of SemiconductorsChinese Academy of SciencesBeijingChina Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijingChina Department of physics College of Physical Science and TechnologyXiamen UniversityXiamenChina state key laboratory for Superlattices and Microstructures Institute of SemiconductorsChinese Academy of SciencesBeijingChina

Graphitic carbon nitride(g-C_(3)N_(4))has been extensively doped with alkali metals to enlarge photocatalytic output,in which cesium(Cs)doping is predicted to be the most ***,the sluggish diffusion and doping kinetics of precursors with high melting points,along with imprecise regulation,have raised the debate on whether Cs doping could make *** this matter,we attempt to confirm the positive effects of Cs doping on multifunctional photocatalysis by first using cesium acetate with the character of easy *** optimized Csdoped g-C_(3)N_(4)(CCN)shows a 41.6-fold increase in visible-light-driven hydrogen evolution reaction(HER)compared to pure g-C_(3)N_(4) and impressive degradation capability,especially with 77%refractory tetracycline and almost 100%rhodamine B degradedwithin an *** penetration ofCs+is demonstrated to be a mode of interlayer doping,and Cs–N bonds(especially with sp^(2) pyridine N in C═N–C),along with robust chemical interaction and electron exchange,are *** atomic configuration triggers the broadened spectral response,the improved charge migration,and the activated photocatalytic ***,we evaluate the CCN/cadmium sulfide hybrid as a Z-scheme configuration,promoting the visible HER yield to 9.02 mmol g^(−1) h^(−1),which is the highest ever reported among all CCN *** work adds to the rapidly expanding field of manipulation strategies and supports further development of mediating served for photocatalysis.

关键词： acetate-assisted cesium doping multifunctional photocatalysis Z-scheme

Efficient terahertz generation from van der Waalsα-In_(2)Se_(3)

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Chinese Optics Letters 2024年第1期22卷 141-146页

作者：段诗婕杨鸣周溯媛张隆辉韩锦森孙旭王广刘昌勤康冬冬王小伟陈家浩戴佳钰 Department of physics College of ScienceNational University of Defense TechnologyChangsha 410073China Hunan key laboratory of Extreme Matter and Applications(XMAL) Changsha 410073China Hunan key laboratory for Micro-Nano Energy Materials and Devices School of Physics and OptoelectronicsXiangtan UniversityXiangtan 411105China Guangxi key laboratory of Automatic Detecting Technology and Instrument Guilin University of Electronic TechnologyGuilin 541004China

Two-dimensional(2D)van der Waals materials have attracted tremendous attention due to their versatile physical properties and flexible manipulation *** the various types of van der Waals materials,α-In_(2)Se_(3)is remarkable for its intrinsic 2D ferroelectricity and high-performance opto-electronic ***,the study of theα-In_(2)Se_(3)system in terahertz(THz)radiation is scarce,although it is promising for electrically controlled THz field *** investigate theα-In_(2)Se_(3)in different thicknesses and report that the THz generation efficiency induced by femtosecond laser pulses can be largely improved by reducing the thickness from the ***,we reveal the surge current in thin film coupled with THz emission exhibits a different Auger recombination mode,which is helpful in understanding the mechanism and provides insights into the design of 2D highly efficient THz devices.

关键词： van der Waals terahertz carrier dynamics

Quantum control for time-dependent noise by inverse geometric optimization

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Science China(physics,Mechanics & Astronomy) 2024年第9期Mechanics & Astronomy) .卷 55-61页

作者： Xiaodong Yang Yingcheng Li Ran Liu Xinfang Nie Tao Xin Dawei Lu Jun Li Institute of Quantum Precision Measurement State Key Laboratory of Radio Frequency Heterogeneous IntegrationCollege of Physics and Optoelectronic EngineeringShenzhen University state key laboratory of Surface physics Department of PhysicsCenter for Field Theory and Particle Physicsand Institute for Nanoelectronic Devices and Quantum ComputingFudan University Shenzhen Institute for Quantum Science and Engineering and Department of physics Southern University of Science and Technology Guangdong Provincial key laboratory of Quantum Science and Engineering Southern University of Science and Technology Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area(Guangdong)

Quantum systems are exceedingly difficult to engineer because they are sensitive to various types of noises. In particular, timedependent noises are frequently encountered in experiments but how to overcome them remains a challenging problem. In this work, we propose a flexible robust control technique to resist time-dependent noises based on inverse geometric optimization working in the filter-function formalism. The basic idea is to parameterize the control filter function geometrically and minimize its overlap with the noise spectral density. This then effectively reduces the noise susceptibility of the controlled system evolution. We show that the proposed method can produce high-quality robust pulses for realizing desired quantum evolutions under realistic noise models. Also, we demonstrate this method in examples including dynamical decoupling and quantum sensing protocols to enhance their performances.

关键词： time-dependent noise robust control quantum gates and states dynamical decoupling quantum sensing

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Observation of maximal intrinsic chirality empowered by dual quasi-bound states in the continuum in a planar metasurface

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Photonics Research 2024年第2期12卷 244-252页

作者： XIN QI JIAJU WU FENG WU SONG ZHAO CHAO WU YUEYANG MIN MINA REN YUFEI WANG HAITAO JIANG YUNHUI LI ZHIWEI GUO YAPING YANG WANHUA ZHENG HONG CHEN YONG SUN MOE key laboratory of Advanced Micro-Structured Materials School of Physics Science and EngineeringTongji UniversityShanghai 200092China School of Optoelectronic Engineering Guangdong Polytechnic Normal UniversityGuangzhou 510665China l3 Shanghai key laboratory of Special Artificial Microstructure Materials and Technology School of Physics Science and EngineeringTongji UniversityShanghai 200092China Department of Electrical Engineering Tongji UniversityShanghai 201804China state key laboratory on Integrated Optoelectronics Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China

Metasurfaces with spin-selective transmission play an increasingly critical role in realizing optical chiral responses,especially for strong intrinsic chirality,which is limited to complex three-dimensional *** this paper,we propose a planar metasurface capable of generating maximal intrinsic chirality and achieving dual-band spinselective transmission utilizing dual quasi-bound states in the continuum(quasi-BICs)caused by the structural symmetry ***,the value of circular dichroism(CD)and the transmittance of two kinds of circular polarization states can be arbitrarily controlled by tuning the asymmetry *** CD approaching unity with the maximum transmittance up to 0.95 is experimentally achieved in the dual ***,assisted by chiral BICs,the application in polarization multiplexed near-field image display is also *** work provides a new avenue to flexibly control intrinsic chirality in planar structure and offers an alternative strategy to develop chiral sensing,multiband spin-selective transmission,and high-performance circularly polarized wave *** basic principle and design method of our experiments in the microwave regime can be extended to other bands,such as the terahertz and infrared wavelengths.

关键词： planar intrinsic quasi

laser manufacturing of spatial resolution approaching quantum limit

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Light(Science & Applications) 2024年第3期13卷 421-428页

作者： Xiao-Jie Wang Hong-Hua Fang Zhen-Ze Li Dan Wang Hong-Bo Sun state key laboratory of Precision Measurement Technology and Instruments Department of Precision InstrumentTsinghua UniversityBeijing 100084China state key laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin University2699 Qianjin StreetChangchun 130012China

Atomic and close-to-atom scale manufacturing is a promising avenue toward single-photon emitters,single-electron transistors,single-atom memory,and quantum-bit devices for future communication,computation,and sensing *** manufacturing is outstanding to this end for ease of beam manipulation,batch production,and no requirement for *** is,however,suffering from optical diffraction ***,we report a spatial resolution improved to the quantum limit by exploiting a threshold tracing and lock-in method,whereby the two-order gap between atomic point defect complexes and optical diffraction limit is surpassed,and a feature size ofphysics is that the uncertainty of local atom thermal motion dominates electron excitation,rather than the power density slope of the incident *** show that the colour centre yield in hexagonal boron nitride is transformed from stochastic to deterministic,and the emission from individual sites becomes polychromatic to *** a result,single colour centres in the regular array are deterministically created with a unity yield and high positional accuracy,serving as a step forward for integrated quantum technological applications.

关键词： quantum limit resolution

Generating electron spin qubit in metal-organic frameworks via spontaneous hydrolysis

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Chinese Chemical Letters 2024年第7期35卷 529-533页

作者： Xian-Fa Jiang Chongyun Shao Zhongwen Ouyang Zhao-Bo Hu Zhenxing Wang You Song state key laboratory of Coordination Chemistry School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Wuhan National high Magnetic field Center&School of physics Huazhong University of Science and TechnologyWuhan 430074China Chaotic Matter Science Research Center Faculty of Materials Metallurgy and ChemistryJiangxi University of Science and TechnologyGanzhou 341000China Shanghai Institute of Optics and Fine Mechanics Chinese Academy of SciencesShanghai 201800China Jiangxi Provincial key laboratory of Functional Molecular Materials Chemistry Jiangxi University of Science and TechnologyGanzhou 341000China

Qubit,as the basic unit of quantum operations,has at least two quantum states for *** itself has no superimposable quantum states,but after injecting N atoms,the resulted nitrogenvacancy centers form excellent-performance *** the same purpose,we can also obtain qubits by modifying the matrix without effective quantum ***-1({Cu_(3)(BTC)_(2)(H_(2)O)_(3)},BTC=1,3,5-benzene-tricarboxylate)with S=0 ground state is electron paramagnetic resonance(EPR)silent,so it is not a qubit ***,the spontaneously hydrolyzed HKUST-1 produces dilute uncoupled Cu^(Ⅱ)ions with S=1/*** this paper,we utilized the hydrolysis products of HKUST-1 to obtain qubits and assembled a core-shell structural HKUST-1@ZIF-8 by ZIF-8({Zn(mim)_(2)},mim=2-methylimidazole)coated over HKUST-1 for controlling the *** experimental results clearly show that the qubits come from hydrolyzed Cu^(Ⅱ)***,the dilute uncoupled Cu^(Ⅱ)ions in this assembly can effectively reduce the decoherence of *** EPR studies show that the T_(2) of this compound is 1067 ns at 10 K.

关键词： Hydrolysis Qubit Decoherent times Metal-organic framework Core-shell structure