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Investigation of hydroxyl-terminated polybutadiene propellant breaking characteristics and mechanism impacted by submerged cavitation water jet

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Defence Technology（防务技术） 2024年第3期33卷 559-572页

作者： Wenjun Zhou Meng Zhao Bo Liu Youzhi Ma Youzhi Zhang Xuanjun Wang zhijian laboratory Rocket Force University of EngineeringXi’an710025China

A submerged cavitation water jet(SCWJ)is an effective method to recycle solid propellant from obsolete solid engines by the breaking *** propellant's breaking modes and mechanical process under SCWJ impact are *** study aims to understand those impact breaking *** hydroxyl-terminated polybutadiene(HTPB)propellant was chosen as the research material,and a self-designed test system was used to conduct impact tests at four different working *** high-speed camera characterized crack propagation,and the DIC method calculated strain change during the impact ***,micro and macro fracture morphologies were characterized by scanning electron microscope(SEM)and computed tomography(CT)*** results reveal that the compressive strain concentration region locates right below the nozzle,and the shear strain region distributes symmetrically with the jet axis,which increases to 4% at first 16th ms,the compressive strain rises to 2% and 6% in the axial and transverse direction,*** two tensile cracks formed first at the compression strain concentrate region,and there generate many shear cracks around the tensile cracks,and those shear cracks that develop and aggregate cause the cracks to become wider and cut through the tensile cracks,forming the tensile-shear cracks and the impact parts eventually *** HTPB propellant forms a breaking hole shaped conical after impact 10 *** mass loss increases by 17 times at maximum,with the working pressure increasing by three ***,the damage value of the breaking hole remaining on the surface increases by 7.8 times while 2.9 times in the depth of the breaking *** breaking efficiency is closely affected by working *** failure modes of HTPB impacted by SCWJ are classified as tensile crack-dominated and tensile-shear crack-dominated damage mechanisms.

关键词： Submerged cavitation water jet Hydroxyl-terminated polybutadiene propellant Breaking characteristics Failure modes

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Relative orbit determination algorithm of space targets with passive observation

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Journal of Systems Engineering and Electronics 2024年第3期35卷 793-804页

作者： DAI Chenchao QIANG Hongfu ZHANG Degang HU Shaolei GONG Baichun zhijian laboratory Rocket Force University of EngineeringXi’an 710025China College of Astronautics Nanjing University of Aeronautics and AstronauticsNanjing 210016China China Flight Test Research Institute Xi’an 710089China Beijing Institute of Control and Electronic Technology Beijing 100038China

Angles-only relative orbit determination for space non-cooperative targets based on passive sensor is subject to weakly observable problem of the relative state between two spacecraft. Previously, the evidence for angles-only observability was found by using cylindrical dynamics, however, the solution of orbit determination is still not provided. This study develops a relative orbit determination algorithm with the cylindrical dynamics based on differential evolution. Firstly, the relative motion dynamics and line-of-sight measurement model for nearcircular orbit are established in cylindrical coordinate ***, the observability is qualitatively analyzed by using the dynamics and measurement model where the unobservable geometry is found. Then, the angles-only relative orbit determination problem is modeled into an optimal searching frame and an improved differential evolution algorithm is introduced to solve the problem. Finally, the proposed algorithm is verified and tested by a set of numerical simulations in the context of highEarth and low-Earth cases. The results show that initial relative orbit determination(IROD) solution with an appropriate accuracy in a relative short span is achieved, which can be used to initialize the navigation filter.

关键词： angles-only measurement relative orbit determination cylindrical coordinate differential evolution

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Breaking the boundaries of biological penetration depth:X-ray luminescence in light theranostics

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Science China Chemistry 2024年第4期67卷 1056-1059页

作者： zhijian Yang Qiaohong Xu Qiushui Chen Huanghao Yang New Cornerstone Science laboratory Key Laboratory for Analytical Science of Food Safety and Biology of Ministry of EducationCollege of ChemistryFuzhou UniversityFuzhou 350002China Fujian Science&Technology Innovation laboratory for Optoelectronic Information of China Fuzhou 350108China

Advances in luminescence materials have markedly propelled research in light theranostics,spanning luminescence biosensing[1],in vivo optical imaging[2],photodynamic therapy[3],optogenetics[4],and related fields[5-7].Nevertheless,conventional light sources have limited penetration depths within deep tissues,and the current state of light theranostics in superficial tissues does not fulfill the requirements for deep tissue treatments in clinical applications.

关键词： luminescence light spanning

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Influence of vibration on the lubrication effect of a splash-lubricated gearbox

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第4期25卷 324-339页

作者： Yi LIU Kailin ZHANG Shuai SHAO Hongxu XIANG zhijian YE State Key laboratory of Rail Transit Vehicle System Southwest Jiaotong UniversityChengdu 610031China

In this study,we investigate the effect of rail vibrations on the lubrication and efficiency of a splash-lubricated gearbox;specifically,the gearbox of a rail-transit vehicle.A high-fidelity 3D numerical model of the gearbox in a moving reference system is described,as well as computational fluid dynamics(CFD)simulations of the gearbox with different vibration *** effects of rotational speed,oil-immersion depth,and different oil-injection volume rates on lubrication and efficiency are *** propose a method of evaluating the internal lubrication condition of a splash-lubricated gearbox and quantitatively compare the effects of different operating parameters on lubrication and ***,our experiment to verify the feasibility of the simulation method is *** results show that with vibration,the churning loss and oil supply for the bearings are significantly higher than those under static *** addition,among different vibrational directions,lateral vibration has the greatest influence on the lubrication condition and efficiency of the *** the studied railway-vehicle gearbox,the best lubrication condition is achieved at a rotational speed of 1600 r/min and an oil-immersion depth of two times the tooth height(***).Rotational speed is the operating parameter that has the most significant effect on the lubrication and efficiencyofthegearbox.

关键词： Comprehensive lubrication evaluation Churning loss Moving reference system Splash lubrication Vibrational excitation Gearbox

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Recent progress of cobalt-based electrocatalysts for water splitting: Electron modulation, surface reconstitution, and applications

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Nano Research 2024年第4期17卷 2234-2269页

作者： zhijian Liang Di Shen Lei Wang Honggang Fu Key laboratory of Functional Inorganic Material Chemistry Ministry of Education of the People’s Republic of ChinaHeilongjiang UniversityHarbin 150080China

Electrocatalytic water splitting is an essential and effective means to produce green hydrogen energy structures,so it is necessary to develop non-precious metal catalysts to replace precious ***-based catalysts present effective alternatives due to the diverse valence states,adjustable electronic structures,and plentiful *** this review,the catalytic mechanisms of hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)for electrocatalytic water splitting are ***,the synthesis strategies of various cobalt-based catalysts are systematically summarized,followed by the relationships between the structure and performance ***,the effects of d-band center and spin regulation for cobalt-based catalysts are also ***,the dynamic electronic and structural devolution of cobalt-based catalysts are elucidated by combining a series of in-situ ***,we highlight the challenges and future developed directions of cobalt-based catalysts for electrocatalytic water splitting.

关键词： cobalt-based electrocatalysts water splitting electron modulation surface reconfiguration

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Unveiling the tailorable electrochemical properties of zeolitic imidazolate framework-derived Ni-doped LiCoO_(2) for lithium-ion batteries in half/full cells

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Journal of Energy Chemistry 2024年第6期93卷 229-242,I0006页

作者： Jian-En Zhou Yiqing Liu zhijian Peng Quanyi Ye Hua Zhong Xiaoming Lin Ronghua Zeng Yongbo Wu Jiaye Ye Guangdong Provincial International Joint Research Center for Energy Storage Materials Key Laboratory of Theoretical Chemistry of EnvironmentMinistry of EducationSchool of ChemistrySouth China Normal UniversityGuangzhou 510006GuangdongChina School of Chemistry and Physics Faculty of ScienceQueensland University of TechnologyBrisbaneQLD 4001Australia Key laboratory of Atomic and Subatomic Structure and Quantum Control(Ministry of Education) Guangdong Basic Research Center of Excellence for Structure and Fundamental Interactions of MatterSchool of PhysicsSouth China Normal UniversityGuangzhou 510006GuangdongChina Guangdong Provincial Key laboratory of Quantum Engineering and Quantum Materials Guangdong-Hong Kong Joint Laboratory of Quantum MatterSouth China Normal UniversityGuangzhou 510006GuangdongChina

As a prevailing cathode material of lithium-ion batteries(LIBs),LiCoO_(2)(LCO)still encounters the tricky problems of structural collapse,whose morphological engineering and cation doping are crucial for surmounting the mechanical strains and alleviating phase degradation upon ***,we propose a strategy using a zeolitic imidazolate framework(ZIF)as the self-sacrificing template to directionally prepare a series of LiNi_(0.1)Co_(0.9)O_(2)(LNCO)with tailorable electrochemical *** rational selection of sintering temperature imparts the superiority of the resultant products in lithium storage,during which the sample prepared at 700℃(LNCO-700)outperforms its counterparts in cyclability(156.8 mA h g^(-1)at 1 C for 200 cycles in half cells,1 C=275 mA g^(-1))and rate capability due to the expedited ion/electron transport and the strengthen mechanical *** feasibility of proper Ni doping is also divulged by half/full cell tests and theoretical study,during which LNCO-700(167 mA h g^(-1)at 1 C for 100 cycles in full cells)surpasses LCO-700 in battery performance due to the mitigated phase deterioration,stabilized layered structu re,ameliorated electro nic co nductivity,a nd exalted lithium sto rage *** work systematically unveils tailorable electrochemical behaviors of LNCO to better direct their practical application.

关键词： Lithium-ion batteries Zeolitic imidazolate framework LiNi_(0.1)Co_(0.9)O_(2) Electrochemical properties

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The transcriptional control of LcIDL1–LcHSL2 complex by LcARF5 integrates auxin and ethylene signaling for litchi fruitlet abscission

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Journal of Integrative Plant Biology 2024年第6期66卷 1206-1226页

作者： Xingshuai Ma Zidi He Ye Yuan zhijian Liang Hang Zhang Vilde Olsson Lalun Zhuoyi Liu Yanqing Zhang Zhiqiang Huang Yulian Huang Jianguo Li Minglei Zhao State Key laboratory for Conservation and Utilization of Subtropical Agro-Bioresources Guangdong Laboratory for Lingnan Modern AgricultureKey Laboratory of Biology and Genetic Improvement of Horticultural Crops(South China)Ministry of Agriculture and Rural AffairsGuangdong Litchi Engineering Research CenterCollege of HorticultureSouth China Agricultural UniversityGuangzhou 510642China Dongguan Botanical Garden Dongguan 523128China Section for Genetics and Evolutionary Biology Department of BiosciencesUniversity of OsloBlindernveien 31Oslo 0316Norway College of Agriculture Guangxi UniversityNanning 530004China

At the physiological level,the interplay between auxin and ethylene has long been recognized as crucial for the regulation of organ abscission in ***,the underlying molecular mechanisms remain ***,we identified transcription factors involved in indoleacetic acid(IAA)and ethylene(ET)signaling that directly regulate the expression of INFLORESCENCE DEFICIENT IN ABSCISSION(IDA)and its receptor HAESA(HAE),which are key components initiating ***,litchi IDAlike 1(LcIDL1)interacts with the receptor HAESA-like2(LcHSL2).Through in vitro and in vivo experiments,we determined that the auxin response factor LcARF5 directly binds and activates both LcIDL1 and ***,we found that the ETHYLENE INSENSITIVE 3-like transcription factor LcEIL3 directly binds and activates *** expression of IDA and HSL2 homologs was enhanced in Lc ARF5and Lc EIL3 transgenic Arabidopsis plants,but reduced in ein3 eil1 ***,the expressions of LcIDL1 and LcHSL2 were significantly decreased in Lc ARF5-and LcEIL3-silenced fruitlet abscission zones(FAZ),which correlated with a lower rate of fruitlet *** of auxin led to an increase in 1-aminocyclopropane-1-carboxylic acid(the precursor of ethylene)levels in the litchi FAZ,followed by abscission *** this process,LcRF5 and LcEIL3 were induced in the ***,our findings suggest that the molecular interactions between litchi AUXIN RESPONSE FACTOR 5(LcARF5)-LcIDL1/LcHSL2 and LcEIL3–LcIDL1 signaling modules play a role in regulating fruitlet abscission in litchi and provide a long-sought mechanistic explanation for how the interplay between auxin and ethylene is translated into the molecular events that initiate abscission.

关键词： auxin ethylene fruit abscission IDA–HAE/HSL2 litchi

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Enhancing zinc-air battery performance by constructing threedimensional N-doped carbon coating multiple valence Co and MnO heterostructures

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Nano Research 2024年第6期17卷 5104-5113页

作者： Qi Liu Panzhe Qiao Miaomiao Tong Ying Xie Xinxin Zhang Kuo Lin zhijian Liang Lei Wang Honggang Fu Key laboratory of Superlight Materials and Surface Technology of the Ministry of Education of the People’s Republic of China Harbin Engineering UniversityHarbin 150080China Key laboratory of Functional Inorganic Material Chemistry Ministry of Education of the People’s Republic of China Heilongjiang UniversityHarbin 150080China Shanghai Institute of Applied Physics Chinese Academy of SciencesShanghai 201204China

Developing highly-efficient bifunctional oxygen evolution reaction(OER)and oxygen reduction reaction(ORR)electrocatalysts is crucial for the widespread application of rechargeable Zn-air batteries(ZABs).Herein,an efficiency electrodeposition and pyrolytic strategy to synthesize the three-dimensional(3D)N-doped carbon coating multiple valence Co and MnO heterostructures supported on carbon cloth substrate(Co-MnO@NC/CC).It contains Co-Co,Co-N,and Co-O bonds,which synergistically enhance the oxygen reaction activity with *** exhibits a working potential of 1.473 V at 10 mA·cm^(−2)for OER and onset potential of 0.97 V for *** calculations demonstrate that the synergy between cobalt and manganese species could optimize the d-band center and reduce the energy barrier of Co-MnO@NC/CC for both OER and ORR ***,the MnO acts as the main OER active site could significantly optimize the energy barrier of O*→OOH*,thus further promoting the OER *** can be directly used as the air-cathode for both liquid-state and solid-state ZABs,which could afford a small voltage gap of 0.75 V at 10 mA·cm^(−2),a high power density of 172.5 mW·cm^(−2)and a long-term durability for 400 h,surpassing those of the Pt/C+RuO_(2)-based ***,the assembled batteries show potential applications in portable devices.

关键词： heterostructure synergy valence cobalt manganese oxide Zn-air battery

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Gelatin-Based Metamaterial Hydrogel Films with High Conformality for Ultra-Soft Tissue Monitoring

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Nano-Micro Letters 2024年第2期16卷 347-364页

作者： Yuewei Chen Yanyan Zhou Zihe Hu Weiying Lu Zhuang Li Ning Gao Nian Liu Yuanrong Li Jing He Qing Gao zhijian Xie Jiachun Li Yong He State Key laboratory of Fluid Power and Mechatronic Systems School of Mechanical EngineeringZhejiang UniversityHangzhou 310027People’s Republic of China School of Mechanical Engineering Guizhou UniversityGuiyang 550025People’s Republic of China Stomatology Hospital School of StomatologyZhejiang University School of MedicineClinical Research Center for Oral Diseases of Zhejiang ProvinceKey Laboratory of Oral Biomedical Research of Zhejiang ProvinceCancer Center of Zhejiang UniversityHangzhou 310006People’s Republic of China

Implantable hydrogel-based bioelectronics(IHB)can precisely monitor human health and diagnose ***,achieving biodegradability,biocompatibility,and high conformality with soft tissues poses significant challenges for *** is the most suitable candidate for IHB since it is a collagen hydrolysate and a substantial part of the extracellular matrix found naturally in most *** study used 3D printing ultrafine fiber networks with metamaterial design to embed into ultra-low elastic modulus hydrogel to create a novel gelatin-based conductive film(GCF)with mechanical *** regulation of GCF nearly covers soft tissue mechanics,an elastic modulus from 20 to 420 kPa,and a Poisson’s ratio from-0.25 to *** negative Poisson’s ratio promotes conformality with soft tissues to improve the efficiency of biological *** GCF can monitor heartbeat signals and respiratory rate by determining cardiac deformation due to its high ***,the gelatin characteristics of the biodegradable GCF enable the sensor to monitor and support tissue *** GCF metamaterial design offers a unique idea for bioelectronics to develop implantable sensors that integrate monitoring and tissue repair and a customized method for endowing implanted sensors to be highly conformal with soft tissues.

关键词： Implantable hydrogel-based bioelectronics Conformality 3D printing Metamaterial design

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基于低浓度掺杂TTF-HLCT一体化分子提供的多重激子循环通道增强深蓝光OLED的稳定性

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Science China Materials 2024年第7期67卷 2161-2168页

作者：唐振宇龚乐帆郭浩清杨爽罗骏唐荣肖静张震曲波陈志坚肖立新 State Key laboratory of Artificial Microstructure and Mesoscopic Physics School of PhysicsPeking UniversityBeijing 100871China College of Physics and Electronic Engineering Taishan UniversityTaian 271000China Key laboratory of Advanced Display and System Applications Ministry of EducationShanghai UniversityShanghai 200072China

目前,商用的深蓝有机发光二极管(OLED)使用的三重态-三重态融合(TTF)型发光材料只能捕获50%的三重态(T_(1))激子,导致其器件效率较低.基于窄带蓝色发射体的热激活延迟荧光(TADF)和超荧光策略可以实现接近100%的激子利用率,然而,在发射层... 详细信息

目前,商用的深蓝有机发光二极管(OLED)使用的三重态-三重态融合(TTF)型发光材料只能捕获50%的三重态(T_(1))激子,导致其器件效率较低.基于窄带蓝色发射体的热激活延迟荧光(TADF)和超荧光策略可以实现接近100%的激子利用率,然而,在发射层(EML)中停留的高能量T_(1)激子通常会导致不可避免的分子降解,从而限制了器件的使用寿命.为了解决这一问题,本文研究了一种TTF-杂化局域-电荷转移态(HLCT)一体化分子,旨在通过多个激子回收通道降低EML内T_(1)激子的密度,从而提高高效深蓝OLED的稳定性.通过TTF过程回收T_(1)激子,通过HLCT过程利用高能三重态(Tn)激子,可以提高EML中三重态激子的利用率.此外,低浓度掺杂的TTF-HLCT分子在TADF体系中可以减轻T_(1)激子猝灭造成的效率损失.最后,实现了外量子效率(EQE)为25.9%、CIE为(0.131,0.050)、蓝光指数(CE由CIEy校准)为312 cd A^(−1) CIE_(y)^(−1)的顶发射OLED,并且其寿命T90@1000 cd m^(−2)从0.5小时延长到6.1小时.本工作揭示了低浓度TTF-HLCT分子掺杂的潜力,作为一种可行的解决方案,可以最大限度地减少效率猝灭,并解决蓝光OLED的稳定性问题.

关键词： organic light-emitting diode stability multiple ex-citon recycling channels deep blue emission TTF-HLCT

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