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Journal of Oceanology and Limnology 2024年第5期42卷 1634-1650页

作者： Ming CONG Zhaoshun LI Wenwen TIAN Yuanmei LI Jiasen LÜ School of Ocean Yantai UniversityYantai 264005China School of Life Sciences Yantai UniversityYantai 264005China

Previous studies have revealed that ammonia nitrogen has several adverse effects on clam Ruditapes ***,knowledge is lacking regarding the related proteins involved in the toxicological responses,which is vital to elucidate the underlying mechanism of ammonia *** this study,clams *** were exposed to ammonia nitrogen for 21 d at two environmentally relevant *** tandem mass tags approach(TMT)was applied to assay the differentially expressed proteins(DEPs)in clam gill tissues on the 3 rd and 21 st ***,a total of 7263 proteins were *** analyses revealed that clam protein profiles changed in dose-and time dependent manner after ammonia nitrogen *** inferred that the clams may face heavy challenges after ammonia exposure,such as unbalanced gender ratio,lysosomal disease,energy lack,neurological disorders,altered glutamine metabolism,increased lipid synthesis,and impaired *** profiles of enzyme activities of glutaminase and glutamine synthase provided direct evidence to verify the related inference from proteome *** of the inferred toxic effects merit further *** study identified important proteins related to ammonia nitrogen toxicity in the clam and indicated the severe stress of marine ammonia pollution on the healthy development of mollusc aquaculture.

关键词： ammonia nitrogen Ruditapes philippinarum proteomic analysis toxicity

Migration mechanism of atrazine in the simulated lake icing process at different freezing temperatures based on density function theory

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Journal of Environmental Sciences 2024年第10期144卷 45-54页

作者： Yan Zhang Hao Lin Aixin Yu Xiaozhuang Wang Yucan Liu Tongshuai Liu Chen Zhao Rui Mei School of Civil Engineering Yantai UniversityYantai 264005China

Atrazine causes concern due to its resistant to biodegradation and could be accumulated in aquatic organisms,causing pollution in *** study measured the concentration of atrazine in ice and the water under ice through a simulated icing experiment and calculated the distribution coefficient K to characterize its migration ability in the freezing ***,density functional theory(DFT)calculations were employed to expatiate the migration law of atrazine during icing *** to the results,it could release more energy into the environment when atrazine staying in water phase(-15.077 kcal/mol)than staying in ice phase(-14.388 kcal/mol),therefore it was beneficial for the migration of atrazine from ice to *** explains that during the freezing process,the concentration of atrazine in the ice was lower than that in the *** calculations indicated thatwhen the temperature decreases from268 to 248 K,the internal energy contribution of the compound of atrazine and ice molecule(water cluster)decreases at the same vibrational frequency,resulting in an increase in the free energy difference of the compound from-167.946 to-165.390 kcal/*** demonstrated the diminished migratory capacity of *** study revealed the environmental behavior of atrazine during lake freezing,which was beneficial for the management of atrazine and other pollutants during freezing and environmental protection.

关键词： Density functional theory(DFT) Icing process Atrazine Migration behavior Free energy

The Al_(2)O_(3)and Mn/Al_(2)O_(3)sorbents highly utilized in destructive sorption of NF_(3)

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Chinese Journal of Chemical Engineering 2024年第1期65卷 54-62页

作者： Yanfei Pan Hejian Li Li Zheng Xiufeng Xu School of Chemistry and Chemical Engineering Yantai UniversityYantai 264005China

NF_(3)is commonly used as an etching and cleaning gas in semiconductor industry,however it is a strongly greenhouse ***,the destruction of disposal NF_(3)is an urgent task to migrate the greenhouse *** the technologies for NF_(3)abatement,the destructive sorption of NF_(3)over metal oxides sorbents is an effective ***,the search for a highly reactive and utilized sorbent for NF_(3)destruction is in great *** this work,AlOOH supported on carbon-sphere(AlOOH/CS)as precursors were synthesized hydrothermally and heat-treated to prepare the Al_(2)O_(3)*** influence of AlOOH/CS hydrothermal temperatures on the reactivity of derived Al_(2)O_(3)sorbents for NF_(3)destruction was investigated,and it is shown that the Al2O3 from AlOOH/CS hydro-thermalized at 120℃is superior to ***,the optimized Al_(2)O_(3)was covered by Mn(OH)x to prepare Mn/Al_(2)O_(3)sorbents via changing hydrothermal temperatures and Mn *** results show that the Mn/Al_(2)O_(3)sorbents are more utilized than bare Al_(2)O_(3)in NF_(3)destructive sorption due to the promotional effect of Mn_(2)O_(3)as surface layer on the fluorination of Al_(2)O_(3)as substrate,especially the optimal 5%Mn/Al2O3(160℃)exhibits a utilization percentage as high as 90.4%,and remarkably exceeds all the sorbents reported so *** findings are beneficial to develop more efficient sorbents for the destruction of NF_(3).

关键词： Greenhouse gas NF_(3)destructive sorption Sorbents Al_(2)O_(3) Mn/Al_(2)O_(3) Reactivity

Seasonal changes in gut microbiota of sea cucumber over natural aestivation cycle

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Journal of Oceanology and Limnology 2024年第3期42卷 849-864页

作者： Ye ZHAO Han WANG Haona WANG Lijie ZHANG Hao SUN Yanying ZHANG Ocean School Yantai UniversityYantai 264005China

Sea cucumber Apostichopus japonicus is an ideal model organism for marine invertebrate aestivation;it annually enters a“sleeping state”for nearly 3 months when ambient water temperature range is 25–30℃.The natural fasting is accompanied by remodeling the intestinal biota and function,which is a part of host biology and could affect the gut *** investigatesd the impact of annual aestivation on gut microbiota using high-throughput sequencing of 16S rRNA *** reveal a notable alteration in the composition of gut bacteria during aestivation during which various indigenous families and genera that exhibit a preference for dietary glycans(e.g.,family Rhodobacteraceae and Flavobacteriaceae)decreased,while the taxa capable of utilizing substrates derived from the host(e.g.,genus Akkermansia and Prevotella)increased,and so did certain opportunistic pathogenic ***,the investigation delved into the gut morphology and immunity response of *** and reveal that the intestine of *** undergoes substantial atrophy and degeneration during ***,there was an observed augmentation in the levels of acid and neutral mucin within mucous cells,as well as an enhanced immune defense response(as evidenced by increased gene expression of AjTLR3,LITAF,Ajp105,and LYZ).These results imply that the composition of sea cucumber gut microbiota differed between aestivation and active periods,which potentially affects the intestinal functions of the host and the symbiotic relationship between host and its microbiota over the activeaestivation cycle.

关键词： Apostichopus japonicus aestivation gut microbiota diet Illumina sequencing

Probing inelastic signatures of dark matter detection via polarized nucleus

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Chinese Physics C 2024年第10期48卷 72-85页

作者： Zai Yun Junwei Sun Bin Zhu Xuewen Liu Department of Physics Yantai UniversityYantai 264005China

We investigate the inelastic signatures of dark matter-nucleus interactions,explicitly focusing on the ramifications of polarization,dark matter splitting,and the Migdal *** detection experiments,crucial for testing the existence of dark matter,encounter formidable obstacles,such as indomitable neutrino backgrounds and elusive determination of dark matter *** overcome these challenges,we explore the potential of polarized-target dark matter scattering,examining the impact of nonvanishing mass splitting,and the role of the Migdal effect in detecting dark *** analysis demonstrates the valuable utility of the polarized triple-differential event rate as an effective tool for examining inelastic dark *** enables us to investigate angular and energy dependencies,providing valuable insights into the scattering process.

关键词： inelastic dark matter polarized target dark matter direct detection

A SINGULAR DIRICHLET PROBLEM FOR THE MONGE-AMPÈRE TYPE EQUATION

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Acta Mathematica Scientia 2024年第5期44卷 1965-1983页

作者： Zhijun ZHANG Bo ZHANG School of Mathematics and Information Science Yantai UniversityYantai264005China

We consider the singular Dirichlet problem for the Monge-Ampère type equation{\rm det}\D^2 u=b(x)g(-u)(1+|\nabla u|^2)^{q/2},\u<0,\x\in\Omega,\u|_{\partial\Omega}=0,whereΩis a strictly convex and bounded smooth domain inℝn,q∈[0,n+1),g∈C∞(0,∞)is positive and strictly decreasing in(0,∞)with\lim\limits_{s\rightarrow 0^+}g(s)=\infty,and b∈C∞(Ω)is positive inΩ.We obtain the existence,nonexistence and global asymptotic behavior of the convex solution to such a problem for more general b and *** approach is based on the Karamata regular variation theory and the construction of suitable sub-and super-solutions.

关键词： Monge-Ampère equation a singular boundary value problem the unique convex solution global asymptotic behavior

Investigating the Impact of Ocean Acidification on Anti-Stress Mechanisms in Sepia esculenta Larvae Based on Transcriptome Profiling

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Journal of Ocean University of China 2024年第4期23卷 1054-1066页

作者： WANG Yongjie LIU Xiumei LV Tingjin WANG Weijun SUN Guohua YANG Jianmin LI Zan School of Agriculture Ludong UniversityYantai 264025China College of Life Sciences Yantai UniversityYantai 264005China yantai Institute of Marine Economy Yantai 264003China

With the rapid development of oil,energy,power and other industries,CO_(2) emissions rise sharply,which will cause a large amount of CO_(2) in the air be absorbed by the ocean and lead to ocean *** growth and development of organisms can be seriously affected by acidified *** esculenta is a mollusk with high nutritional and economic value and is widely cultured in offshore waters of *** are the early life forms of the organism and are more vulnerable to changes in the external *** low pH will lead to some adverse reactions in larvae,which will affect metabolism,immune response and other life *** this study,we sequenced the transcriptome of *** subjected to acidified seawater stress and identified 1072differentially expressed genes(DEGs).The detected atypical expression of DEGs substantiates cellular malformation and translocation in *** under low pH ***,this also substantiates the notable impact of ocean acidification on *** DEGs were used for functional enrichment analysis of GO and KEGG,and the top twenty items of the biological process classification in GO terms and 11 KEGG signaling pathways were significantly ***,the constructed proteinprotein interaction network(PPI)was used to analyze protein-protein interactions,and 12 key DEGs and 3 hub genes were *** reliability of 12 genes was verified by quantitative RT-PCR.A comprehensive analysis of the KEGG signaling pathway and PPI revealed that ocean acidification leads to abnormalities in lipid metabolism in *** larvae,which can lead to cancer development and metastasis,accompanied by some degree of *** results of the study will help to further investigate the physiological processes of *** when stimulated by ocean acidification,and provide a reference to cope with the captive breeding of *** affected by acidification.

关键词： Sepia esculenta ocean acidification protein-protein interaction network transcriptome immunity

An improved bound on accelerated light dark matter

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Science China(Physics,Mechanics & Astronomy) 2024年第2期67卷 105-118页

作者： Liangliang Su Lei Wu Bin Zhu Department of Physics and Institute of Theoretical Physics Nanjing Normal UniversityNanjing 210023China School of Physics Yantai UniversityYantai 264005China

Light(sub-GeV)dark matter has gained increasing interest in terms of direct *** dark matter is a promising candidate that can generate detectable nuclear recoil energy within the sub-GeV *** of the large kinetic energy,its interactions with the nucleus are predominantly governed by inelastic scattering,including quasi-elastic and deep inelastic *** this work,we calculated the inelastic effects in dark matter-Earth scattering mediated by a vector *** analysis revealed that the impact of inelastic scattering relies on the mediator mass and the kinetic energy spectrum of dark *** results exhibited considerable disparity:the upper bounds of the exclusion limit for the spin-independent cross-section between accelerated dark matter and nuclei via a heavy mediator differ by several tens of times when inelastic scattering is considered.

关键词： accelerated dark matter inelastic scattering direct detection experiment

Neutral color and self-healable electrochromic system based on CuI/Cu and I_(3)^(-)/I^(-)conversions

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Nano Research 2024年第5期17卷 4437-4443页

作者： Junsen Zhong Bingkun Huang Kunjie Yang Zuju Ma Lingyu Du Ning Luo Fengjiao Tang Chuanxin Hou Fuyi Jiang Litao Kang College of Environment and Materials Engineering Yantai UniversityYantai 264005China School of Energy and Power Engineering Shandong UniversityJinan 250061China Shandong Laboratory of Advanced Materials and Green Manufacturing(yantai) Yantai 264001China

The electrochromic(EC)mechanisms of inorganic materials are usually based on reversible cation insertion/extraction or metal deposition/dissolution,which are plagued by ion trapping and dendrite growth,*** this paper,a novel conversion-type electrochromic mechanism is proposed,by making good use of the CuI/Cu redox *** CuI-based electrochromic system shows a neutral color switching from transparent and dim *** simply increasing the bleaching voltage,I_(3)^(-)/I^(-)redox couple can be further *** generated I_(3)^(-)will readily react with Cu,effectively improving the conversion reversibility and thereby rejuvenating the degraded electrochromic *** to the well-designed electrode and the self-healing ability,this conversion electrochromic system achieves rapid response times(tcoloring:23 s,tbleaching:6 s),decant optical modulation amplitude(26.4%),high coloration efficiency(86.15 cm^(2)·C^(-1)),admirable cyclic durability(without performance degradation after 480 cycles)and excellent optical memory ability(transmittance variation<1%after 10 h open-circuit storage).The establishment of this conversion-type electrochromism may inspire the exploration of novel electrochromic materials and devices.

关键词： electrochromic CuI conversion reaction self-healing neutral color

Pressure-Driven Energy Band Gap Narrowing of λ-N_(2)

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Chinese Physics Letters 2024年第4期41卷 173-177页

作者：李月刘静仪吴彬彬陶雨耿延雷王晓丽雷力 Institute of Atomic and Molecular Physics Sichuan UniversityChengdu 610065China School of Physics and Electronic Information Yantai UniversityYantai 264005China

Probing the energy band gap of solid nitrogen at high pressures is of importance for understanding pressuredriven changes in electronic structures and insulator-to-metal transitions under high *** λ-N_(2) formed by cold compression is known to be the most stable one in all solid nitrogen phases observed so *** optimizing the optical system,we successfully measured the high-pressure absorption spectra of λ-N_(2) covering the polymericnitrogen synthetic pressures(124 GPa-165 GPa).The measured optical band gap decreases with increasing pressure,from 2.23 eV at 124 GPa to 1.55 eV at 165 GPa,with a negative pressure coefficient of-18.4 meV/GPa,which is consistent with the result from our ab initio total-energy calculations(-22.6 meV/GPa).The extrapolative metallization pressure for theλ-N_(2) is around 288(18)GPa,which is close to the metallization pressure(280 GPa)for the η-N_(2) expected by previous absorption edge and direct electrical *** results provide a direct spectroscopic evidence for the pressure-driven band gap narrowing of solid nitrogen.

关键词： absorption transitions spectroscopic