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Influence of Local Cation Order on Electronic Structure and Optical Properties of Cation-Disordered semiconductor AgBiS_(2)

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Chinese Physics Letters 2024年第10期41卷 61-69页

作者： Xiaoyu Wang Muhammad Faizan Yuhao Fu Kun Zhou Yilin Zhang Xin He David J.Singh Lijun Zhang state key laboratory of Superhard Materials College of PhysicsJilin UniversityChangchun 130012China state key laboratory of Integrated Optoelectronics Key Laboratory of Automobile Materials of MOECollege of Materials Science and EngineeringJilin UniversityChangchun 130012China Department of Physics and Astronomy University of MissouriColumbiaMissouri 65211-7010USA

Site disorder exists in some practical semiconductors and can significantly impact their intrinsic properties both beneficially and ***,the uncertain local order and structure pose a challenge for experimental and theoretical ***,it hinders the investigation of the effects of the diverse local atomic environments resulting from the site *** employ the special quasi-random structure method to perform first-principles research on connection between local site disorder and electronic/optical properties,using cationdisordered AgBiS_(2)(rock salt phase)as an *** predict that cation-disordered AgBiS_(2)has a bandgap ranging from 0.6 to 0.8 eV without spin-orbit coupling and that spin-orbit coupling reduces this by approximately 0.3 *** observe the effects of local structural features in the disordered lattice,such as the one-dimensional chain-like aggregation of cations that results in formation of doping energy bands near the band edges,formation and broadening of band-tail states,and the disturbance in the local electrostatic potential,which significantly reduces the bandgap and *** influence of these ordered features on the optical properties is confined to alterations in the bandgap and does not markedly affect the joint density of states or optical *** study provides a research roadmap for exploring the electronic structure of site-disordered semiconductor materials,suggests that the ordered chain-like aggregation of cations is an effective way to regulate the bandgap of AgBiS_(2),and provides insight into how variations in local order associated with processing can affect properties.

关键词： stability. structure ordered

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Low-power soft transistors triggering revolutionary electronics

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The Innovation 2024年第3期5卷 21-22页

作者： Ziyang Liu Yaoshen Zhao Zhigang Yin state key laboratory of Power Transmission Equipment technology School of Electrical EngineeringChongqing UniversityChongqing 400044China

Transistors have been reshaping our lives since their initial appearance in the *** the central element of logic gates and integrated circuits(chips),they undoubtedly play an incomparable role in promoting the development of computers,smartphones,flat panel displays,Internet of Things,and even all electronic or electrical *** past decades have witnessed dominant transistors usually made from inorganic semiconductors such as silicon materials and metal oxides,which are advantageous to achieve high mobility,fast switching speed,and excellent ***,silicon transistors and metal oxide semiconductor field-effect transistors have been broadly used for electronic ***,these transistors are rigid and nearly approaching the fundamental limits on speed and power consumption,despite being manufactured at a much smaller scale to meet the projection of Moore’s *** future transistors with mechanical flexibility/robustness and low-power consumption are demanded,innovation in functional materials,device configurations,and integrated processing techniques to facilitate the evolution from rigid devices to soft,durable,and biocompatible devices is imperative.

关键词： approaching evolutionary doubt

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Single Ti atoms coupled with Ti-O clusters enable low temperature hydrogen cycling by sodium alanate

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Rare Metals 2024年第6期43卷 2671-2681页

作者： Zhuang-He Ren Xin Zhang Wen-Xuan Zhang Zhen-Guo Huang Li-Mei Yang Ya-Xiong Yang Zheng-Long Li Juan Li Wen-Ping Sun Ming-Xia Gao Hong-Ge Pan Yong-Feng Liu state key laboratory of Silicon and Advanced semiconductor Materials Zhejiang UniversityHangzhou 310027China School of Materials Science and Engineering Zhejiang UniversityHangzhou 310058China School of Civil&Environmental Engineering.University of technology Sydney Sydney2007 NSWAustralia Institute of Science and technology for New Energy Xi'an Technological UniversityXi'an 710021China College of Materials Science and Engineering Zhejiang University of TechnologyHangzhou 310014China

Ti-based catalysts are known to improve the hydrogen storage performance of NaAlH4by facilitating the dissociation/recombination of H-H and Al-H *** catalytic activity of metallic Ti species strongly depends on its particle size and *** clusters and even single atoms are therefore highly desirable,but their controllable fabrication has been highly *** rein,we demonstrate a novel facile sonochemical synthesis of a Ti-O clusters featuring single Ti atom catalyst at room *** reducing TiCl_(4)by MgBu_(2)with ultrasound instead of heating as driving force,numerous single Ti atoms coupled with Ti-O clusters with Ti loading on graphene(Ti_(1)/Ti-O@G)up to 22.6 wt%have been successfully *** prepared Ti_(1)/Ti-O@G contributes high reactivity and superior catalytic activity,therefore enabling full dehydrogenation of NaAlH_(4)at 80℃in thermogravimetric mode and re-hydrogenation at 30℃and 10 MPa with 4.9 wt% H_(2).This fact indicates for the first time that single Ti atom catalyst with high loading is highly effective in catalyzing hydrogen cycling of NaAlH4at remarkably reduced temperatures.

关键词： Hydrogen storage Nanocatalysis Transition metals Single Ti atoms NaAlH_(4)

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A modified supervised learning rule for training a photonic spiking neural network to recognize digital patterns

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Science China(Information Sciences) 2021年第2期64卷 202-210页

作者： Yahui ZHANG Shuiying XIANG Xingxing GUO Aijun WEN Yue HAO state key laboratory of Integrated Service Networks Xidian University state key discipline laboratory of wide bandgap semiconductor technology School of MicroelectronicsXidian University

A modified supervised learning rule which is suitable for training photonic spiking neural networks(SNN) is proposed for the first time. The proposed learning rule is independent of the time intervals between actual spike and desired spike or between presynaptic spike and postsynaptic spike. Based on the proposed supervised learning rule, 10 digital images are learned in photonic neural network which consists of 30 presynaptic neurons and 10 postsynaptic neurons. Presynaptic and postsynaptic neurons are photonic neurons based on vertical-cavity surface-emitting lasers with an embedded saturable absorber(VCSEL-SA).The results show that 10 digital images are recognized correctly in photonic SNN after enough ***, the effects of learning rate, the jitters of learning rate, initial weights distribution of SNN and bias current of postsynaptic neurons(VCSELs-SA) on the recognized error are examined carefully based on the proposed learning rule. To the best of our knowledge, such modified supervised learning rule has not yet been reported, which would contribute to training photonic neural networks, and hence is interesting for neuromorphic photonic systems and pattern recognition.

关键词： vertical-cavity surface-emitting laser modified supervised learning rule optical spiking neural networks learning system pattern recognition

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Promoted monolithic perovskite/organic tandem solar cells through elaborate manipulation of light transmission and carrier tunneling in interconnect junction

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Science China Chemistry 2024年第9期67卷 3131-3139页

作者： Rongbo Wang Jiawei Zhang Juntao Zhao Ya Wang Yi Ding Ying Zhao Xiaodan Zhang Guofu Hou Institute of Photoelectronic Thin Film Devices and technology Renewable Energy Conversion and Storage CenterSolar Energy Conversion CenterNankai UniversityTianjin 300350China key laboratory of Photoelectronic Thin Film Devices and technology of Tianjin Tianjin 300350China Engineering Research Center of Thin Film Photoelectronic technology of Ministry of Education Tianjin 300350China state key laboratory of Photovoltaic Materials and Solar Cells Tianjin 300350China

Monolithic perovskite/organic tandem solar cells(TSCs)have emerged as promising thin film solar *** is recognized that interconnect junction plays a pivotal role in tandem ***,wide bandgap Cs_(0.25)FA_(0.75)Pb(I_(0.6)Br_(0.4))_(3)perovskite top-cell and narrow bandgap PM6:Y6:PC_(61)BM ternary organic bottom-cell were integrated in this study with several kinds of thin metal interconnect layers,which provides feasibility to elaborately manipulate light transmission and carrier tunneling process in interconnect *** is confirmed that,in comparison with Au,employing an Ag interconnect layer elevates integrated transmittance of light in longer wavelength regions,mainly because of the alleviated screening effect with a lower free electron concentration,which offers sufficient light harvest for the ***,established energy barriers with moderate height afford convenient extraction and recombination for both holes and ***,the performance of TSCs is promoted ***,an innovative Ag/Au double interconnect layer is proposed accordingly,which can preserve exceptional conductivity and light transmission and further reduce barrier height,especially for hole tunneling,by optimizing the band alignment between the interconnect layer and ***,the monolithic perovskite/organic TSC with a striking efficiency of 23.26% is *** a word,this study can pave a general approach toward high-performance TSCs integration.

关键词： tandem solar cells band alignment perovskite organic solar cells interconnect junction

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Enhanced memory capacity of a neuromorphic reservoir computing system based on a VCSEL with double optical feedbacks

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Science China(Information Sciences) 2020年第6期63卷 164-175页

作者： Xingxing GUO Shuiying XIANG Yahui ZHANG Aijun WEN Yue HAO state key laboratory of Integrated Service Networks Xidian University state key discipline laboratory of wide bandgap semiconductor technology School of Microelectronics Xidian University

In this paper, a neuromorphic reservoir computing(RC) system with enhanced memory capacity(MC) based on a vertical-cavity surface-emitting laser(VCSEL) subject to double optical feedbacks(DOF)is proposed and investigated numerically. The aim of this study is to explore the MC of the proposed *** the purpose of comparison, the MC of the VCSEL-based RC system with single optical feedback(SOF)is also taken into account. It is found that, compared with the VCSEL-based RC system subject to SOF,enhanced MC can be obtained for the VCSEL-based RC system with DOF. Besides, the effects of feedback strength, injected strength, frequency detuning as well as injection current on the MC of the VCSEL-based RC system with DOF are considered. Moreover, the influence of feedback delays is also carefully ***, such proposed VCSEL-based RC system with DOF provides a prospect for the further development of the neuromorphic photonic system based on RC.

关键词： vertical-cavity surface-emitting laser nanophotonic reservoir computing memory capacity double feedback information processing

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Real-time optical spike-timing dependent plasticity in a single VCSEL with dual-polarized pulsed optical injection

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Science China(Information Sciences) 2020年第6期63卷 143-154页

作者： Shuiying XIANG Yanan HAN Xingxing GUO Aijun WEN Genquan HAN Yue HAO state key laboratory of Integrated Service Networks Xidian University state key discipline laboratory of wide bandgap semiconductor technology School of MicroelectronicsXidian University

We propose and numerically realize an optical spike-timing dependent plasticity(STDP) scheme by using a single vertical-cavity surface-emitting laser(VCSEL). In the scheme, the VCSEL is subjected to an orthogonally-polarized continuous-wave optical injection(OPCWOI) and dual-polarized pulsed optical injections(DPPOI). Based on the widely used spin-flip model, the response spiking dynamics of VCSEL is numerically studied, and then the optical STDP in a single VCSEL is explored. The roles of bias current, the strength of OPCWOI and DPPOI, and the frequency detuning on the optical STDP curve are numerically analyzed. It is found that, by simultaneously utilizing the response spiking dynamics in two orthogonal polarization modes, an optical STDP could be achieved by using a single VCSEL. Furthermore, the weight update of STDP curve can be calculated in real-time. Additionally, the STDP curves can also be controlled by adjusting some controllable parameters. The real-time optical STDP based on a single VCSEL is numerically realized for the first time, which paves the way towards fully VCSELs-based photonic neuromorphic systems with low power consumption.

关键词： vertical-cavity surface-emitting laser optical spike-timing dependent plasticity neuromorphic photonic system dual polarized pulsed optical injections artificial intelligent systems

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Optical and electrical anisotropy regulation engineering of low-dimensional materials toward polarized detection and imaging applications

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Rare Metals 2024年第7期43卷 2968-2993页

作者： Jian-Bin Zhang Nan Zhou Li-Hui Zhang Cong-Hui Shang Jia-Xuan Li Yi Zhao Guo-Hui Jia Ru-Sen Yang Hua Xu Xiao-Bo Li Shaanxi Joint key laboratory of Graphene Shaanxi Key Laboratory of High-Orbits-Electron Materials and Protection Technology for AerospaceShaanxi Joint Key Laboratory of GrapheneSchool of Advanced Materials and NanotechnologyXidian UniversityXi'an710126China Guangzhou Institute of technology Xidian UniversityGuangzhou 710068China Xi'an Thermal Power Research Institute Co. LtdXi'an 710054China key laboratory of Applied Surface and Colloid Chemistry Ministry of EducationShaanxi Key Laboratory for Advanced Energy DevicesShaanxi Engineering Lab for Advanced Energy TechnologySchool of Materials Science and EngineeringShaanxi Normal UniversityXi'an Xi'an 710119China

Polarized-sensitive image sensors are a kind of photodetector with great development potential due to their enhanced ability to detect and identify the target objects from the aspect of spatial,spectral and polarized ***,low-dimensional anisotropic materials with inherent anisotropic properties,ultrathin thickness,tunable bandgap and feasible integration with complementary metal oxide semiconductor(CMOS)fabrication processes have attracted great interest for their facilitation of polarized photodetector devices *** the polarized detection performance of low-dimensional materials to satisfy realistic needs stimulates the exploration of modulation of anisotropic *** this review,we comprehensively introduce the latest research progress in modulating the optical and optoelectronic anisotropy characteristics of low-dimensional *** strategy of anisotropy regulation through crystal structure engineering and coupling system is discussed ***,the latest progress in image recognition applications using anisotropic low-dimensional materials is reviewed in ***,we summarize the challenge and propose future opportunities in the practical application of polarized-sensitive imaging photodetectors based on low-dimensional anisotropic materials.

关键词： Anisotropy Polarized detection Image recognition Low-dimensional materials

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Carbon nanotube integrated circuit technology:purification,assembly and integration

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International Journal of Extreme Manufacturing 2024年第3期6卷 120-138页

作者： Jianlei Cui Fengqi Wei Xuesong Mei state key laboratory for Manufacturing Systems Engineering Xi’an Jiaotong UniversityXi’an 710049People’s Republic of China

As the manufacturing process of silicon-based integrated circuits(ICs)approaches its physical limit,the quantum effect of silicon-based field-effect transistors(FETs)has become increasingly *** the burgeoning carbon-based semiconductor technology has become one of the most disruptive technologies in the post-Moore *** one-dimensional nanomaterials,carbon nanotubes(CNTs)are far superior to silicon at the same technology nodes of FETs because of their excellent electrical transport and scaling properties,rendering them the most competitive material in the next-generation ICs ***,certain challenges impede the industrialization of CNTs,particularly in terms of material preparation,which significantly hinders the development of CNT-based *** on CNT-based ICs technology,this review summarizes its main technical status,development trends,existing challenges,and future development directions.

关键词： carbon nanotubes integrated circuits field-effect transistors post-Moore

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Surface repair of wide-bandgap perovskites for high-performance all-perovskite tandem solar cells

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Journal of Energy Chemistry 2024年第6期93卷 64-70,I0003页

作者： Xiaojing Lv Weisheng Li Jin Zhang Yujie Yang Xuefei Jia Yitong Ji Qianqian Lin Wenchao Huang Tongle Bu Zhiwei Ren Canglang Yao Fuzhi Huang Yi-Bing Cheng Jinhui Tong state key laboratory of Advanced technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070HubeiChina key Lab of Artificial Micro-and Nano-Structures of Ministry of Education of China School of Physics and TechnologyWuhan UniversityWuhan 430072HubeiChina Department of Electrical and Electronic Engineering Photonics Research Institute(PRI)Research Institute for Intelligent Wearable Systems(iWEAR)The Hong Kong Polytechnic University999077Hong KongChina laboratory of Advanced Materials Fudan UniversityShanghai 200438China Xianhu laboratory of the Advanced Energy Science and technology Guangdong laboratory Foshan 528200GuangdongChina

wide-bandgap(WBG)perovskite solar cells(PSCs)play a fundamental role in perovskite-based tandem solar ***,the efficiency of WBG PSCs is limited by significant open-circuit voltage losses,which are primarily caused by surface *** this study,we present a novel method for modifying surfaces using the multifunctional S-ethylisothiourea hydrobromide(SEBr),which can passivate both Pb^(-1)and FA^(-1)terminated surfaces,Moreover,the SEBr upshifted the Fermi level at the perovskite interface,thereby promoting carrier *** proposed method was effective for both 1.67 and 1.77 eV WBG PSCs,achieving power conversion efficiencies(PCEs)of 22.47%and 19.90%,respectively,with V_(OC)values of 1.28 and 1.33 V,along with improved film and device *** this advancement,we were able to fabricate monolithic all-perovskite tandem solar cells with a champion PCE of 27.10%,This research offers valuable insights for passivating the surface trap states of WBG perovskite through rational multifunctional molecular engineering.

关键词： wide-bandgap perovskite Surface defect Multifunctional molecule All-perovskite tandem solar cells

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