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半导体学报:英文版 2023年第9期44卷 1-2页

作者： Hoi-Sing Kwok Zhiyong Fan Department of Electronic and Computer Engineering The Hong Kong University of Science and TechnologyClear Water BayKowloonHong Kong SARChina state key laboratory of advanced displays and optoelectronics technologies HKUSTClear Water BayKowloonHong Kong SARChina

This year marks the tenth anniversary of the state key laboratory of advanced displays and optoelectronics technologies(SKLADOT)at the Hong Kong University of Science and Technology(HKUST).The predecessor of SKLADOT w... 详细信息

关键词： ADO key UST

Multicolor emission from lanthanide ions doped lead-free Cs_(3)Sb_(2)Cl_(9) perovskite nanocrystals

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Journal of Rare Earths 2024年第5期42卷 940-946,I0005页

作者： He Shao Lifang Li Xiufeng Wu Lin Xu Biao Dong Donglei Zhou Xue Bai Hongwei Song state key laboratory of Organic Electronics and Information displays&Institute of advanced Materials College of Materials Science and EngineeringNanjing University of Posts&TelecommunicationsNanjing210023China state key laboratory of Integrated optoelectronics College of Electronic Science and Engineering Jilin UniversityChangchun130012China

The toxicity of lead ions has become the severe challenge for the all-inorganic lead halide p erovskite materials,although some works have rep orted the lead-free perovskite nanocrystals(NCs),the photoluminescence quantum yield(PLQY)of these materials is still ***,because the halogen ions can be easily exchanged,the controllable multicolor emission in perovskite NCs is difficult to realize in current *** this work,we introduced lanthanide ions into lead-free Cs_(3)Sb_(2)Cl_(9) perovskite *** from the energy transfer between Cs_(3)Sb_(2)Cl_(9) perovskite NC host and lanthanide ions,the multicolor emission was *** on controlling the doping concentration of Tb^(3+)and Eu^(3+)ions,the white light emission under UV excitation would be turned easily in the Tb^(3+)/Eu^(3+)codoped *** addition,efficient energy transfer from perovskite NCs to Tb^(3+)or Eu^(3+)ions is beneficial to improving the optical properties of lead-free perovskite NCs,resulting in maximum PLQYs of red,green and white light emission of 22.6%,19.7%and 28.5%,***,a white light emitting device(WLED)was fabricated with a power efficiency of 18.5 lm/W,which presents the Commission Internationale de l'Eclairage(CIE)of(0.33,0.35).

关键词： Perovskite nanocrystals Lead free Lanthanide ions Energy transfer White light emitting device Rare earths

High-performance ultrathin Ag electrodes by chemical bond anchoring Ag atoms for stretchable organic light-emitting devices

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Nano Research 2024年第8期17卷 7614-7620页

作者： Yue Qin Yawei Wang Xinxin Wang Yaqi Zhang Jiahao Xu Kanchi Dong Yuehua Chen Wenyong Lai Xinwen Zhang state key laboratory of Organic Electronics and Information displays and Institute of advanced Materials(IAM) Nanjing University of Posts and TelecommunicationsNanjing 210023China

The progress of stretchable organic light-emitting devices(OLEDs)has brought about new possibilities for highly functional wearable ***,the efficiency and durability of stretchable OLEDs have been limited by the performance of stretchable transparent ***,we proposed an interface engineering strategy that involves anchoring the growth of silver(Ag)atoms with amine-enriched biomaterials for high-quality stretchable transparent *** strong interactions between the Ag atom and the amine group enable the uniform Ag electrodes at an ultralow thickness of 7 nm,and provide remarkable mechanical flexibility and strain endurance to the Ag *** distinct effects of different amino acids were investigated,and a deep understanding of their unique contributions to the film formation process was *** resulting ultrathin Ag electrodes exhibit outstanding optoelectrical properties(transmittance of~98% and sheet resistance of~8.7Ω/sq)and excellent stretchability during 500 stretching cycles at 100%*** green phosphorescent OLEDs based on the Ag electrodes have been demonstrated with a current efficiency of up to~70.4 cd/***,the devices show excellent stretching stability,retaining~89% of the original luminance and~78% of the original current efficiency after 200 stretching cycles at 100%*** work opens up new possibilities for stretchable transparent electrodes,fostering advancements in wearable displays and other innovative flexible devices.

关键词： transparent flexible electrodes ultrathin metal film interface mechanical stability

Rational design of biodegradable semiconducting polymer nanoparticles for NIR-II fluorescence imaging-guided photodynamic therapy

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Nano Research 2024年第6期17卷 5399-5408页

作者： Xuxuan Gu Jinlong Shen Zhiwei Xu Wenqi Wang Ying Wu Wen Zhou Chen Xie Quli Fan state key laboratory of Organic Electronics and Information displays&Institute of advanced Materials(IAM) Nanjing University of Posts&Telecommunications9 Wenyuan RoadNanjing 210023China

Semiconducting polymer nanoparticles(SPNs)have shown great promise in second near-infrared window(NIR-II)***,the issue of long metabolic time significantly restricts the clinical application of *** this study,we rationally designed a biodegradable SPN(BSPN50)for NIR-II fluorescence imaging-guided photodynamic therapy(PDT).BSPN50 is prepared by encapsulating a biodegradable SP(BSP50)with an amphiphilic copolymer ***50 is composed of NIR-II fluorescent diketopyrrolopyrrole(DPP)segment and degradable poly(phenylenevinylene)(PPV)segment with the ratio of 50/***50 has both satisfactory degradability under myeloperoxidase(MPO)/hydrogen peroxide(H_(2)O_(2))and NIR-II fluorescence emission upon 808 nm laser ***,BSPN50 shows good photodynamic efficacy under 808 nm laser ***50 shows a faster degradation rate than BSPN100 which has no PPV segment both in vitro and in *** addition,BSPN50 can effectively diagnose tumor via NIR-II fluorescence imaging and inhibit the tumor growth by ***,our study provides a rational approach to construct biodegradable nanoplatforms for efficient tumor NIR-II phototheranostics.

关键词： near-infrared(NIR)-II fluorescence imaging semiconducting polymer nanoparticles photodynamic therapy tumor imaging

Polyimide covalent organic frameworks as efficient solid-state Li^(+) electrolytes

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Science China Chemistry 2024年第5期67卷 1647-1652页

作者： Xu Liu Shi Wang Siqi Liu Chengfang Liu Xiangchun Li Jian Wu Dazhi Li Shihao Xu Chongyang Liu Wen-Yong Lai state key laboratory of Organic Electronics and Information displays(SKLOEID) Institute of Advanced Materials(IAM)School of Chemistry and Life SciencesNanjing University of Posts&TelecommunicationsNanjing 210023China

Covalent organic frameworks(COFs) are attractive porous crystalline materials with extremely high stability, easy functionalization, and open channels, which are expected to be unique ion conductors/transporters in lithium ion batteries(LIBs). Despite recent advances, low ion conductivity and low transference number, resulting in low charging/discharging rate, low energy density, and short battery life, are the main issues that limit their direct application as solid electrolytes in LIBs. Here, we designed and synthesized a novel polyimide COF, namely, TAPA-PDI-COF, with abundant C=O groups, which has been successfully employed as high-performance solid electrolytes by doping TAPA-PDI-COF and succinonitrile(SN). Both the well-defined nanochannels of COFs and SN confined in the well-aligned channels restricted the free migration of anions, while C=O on COFs and CN groups of SN enhanced Li^(+) transport, thus achieving a high ion conductivity of 0.102 m S cm^(-1)at 80 °C and a high lithium-ion transference number of 0.855 at room temperature. According to density functional theory(DFT)calculations, Li-ion migration mainly adopted in-plane transport rather than the axial pathway, which may be due to the shorter hopping distances in the planar pathway. The results suggest an effective strategy for the design and development of all-solidstate ionic conductors for achieving high-performance LIBs.

关键词： lithium ion batteries(LIBs) covalent organic frameworks(COFs) solid-state ion conductors solid-state electrolytes ion conductivity

Hydrogen bond-induced elastic polyzwitterion electrolytes constructed by mussel-inspired autopolymerization for zinc-ion battery

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Science China Chemistry 2024年第10期67卷 3438-3449页

作者： Shi Wang Xinyi Wu Chao Liu Lingjun He Shuanghan Li Yuqi Miao Mingrui Cai Yi Li Zheng-Dong Huang Wen-Yong Lai state key laboratory of Organic Electronics and Information displays(SKLOEID) Institute of Advanced Materials(IAM)School of Chemistry and Life SciencesNanjing University of Posts&TelecommunicationsNanjing 210023China

Aqueous zinc-ion batteries(ZIBs)have attracted much interest to realize safe rechargeable batteries with high safety and high energy ***,it is still challenging to address dendrite growth and parasitic reactions in zinc *** propose herein the design concept of hydrogen bond-induced elastic polyzwitterion electrolytes with zincophilic groups for achieving robust ***-inspired autopolymerization has been developed to construct the polyzwitterion electrolytes at room temperature by inducing electron density delocalization atα-position of C=C bond in zwitterion monomer by Zn^(2+).Specifically,the zwitterionic functional groups construct ion transport channels,and the unique–NH–and SO_(3)^(-)groups co-compete with H_(2)O for coordination with Zn^(2+)and promote the desolvation of hydrated Zn^(2+),thus achieving a high room temperature ionic conductivity(6.7 mS cm^(-1))and an increased Zn^(2+)migration number(0.65)for the polyzwitterion *** addition,various interactions such as hydrogen bonding and electrostatic interactions between electrolyte ions and zwitterionic groups impart high stretchability and strength to the polyzwitterion electrolytes,which,combined with SO_(3)^(-)philic(002)crystallographic properties,effectively inhibit the growth of zinc *** a result,rigid/wearable solid-state ZIBs exhibit excellent cycling and C-rate *** believe that the strategy of constructing polyzwitterionic electrolytes with zincophilic groups and ion transport channels opens up a new direction in polymer electrolyte engineering towards safe and high energy batteries.

关键词： flexible electronics wearable electronics polyzwitterion electrolytes self-polymerization zinc-ion batteries

Effects of longitudinal magnetic field on primary dendrite spacing and segregation of directionally solidified single crystal superalloy

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Progress in Natural Science:Materials International 2024年第1期34卷 26-36页

作者： Congjiang Zhang Yilin Zhou Chen Shen Weili Ren Xiaotan Yuan Biao Ding Haibiao Lu Zuosheng Lei Yunbo Zhong Ang Zhang state key laboratory of advanced Special Steel College of Materials Science and Engineering Shanghai University National Engineering Research Center for Magnesium Alloys Natural Key Laboratory of Advanced Casting Technologies College of Materials Science and EngineeringChongqing University

The primary dendrite spacing(PDS) and segregation of directionally solidified single crystal(SC) superalloy under the longitudinal magnetic field(LMF) were investigated based on the analysis of the whole cross-sectional microstructure at different solidification distances. The results show that the PDS under the LMF remains basically unchanged at different solidification distances, and it is greater than that under no LMF. With the increase of magnetic field intensity, the PDS increases and the macrosegregation decreases. The increasing PDS and reducing segregation under the LMF can be attributed to the increase of solute boundary layer, which expands the non-equilibrium freezing temperature range and brings the effective partition coefficient closer to 1. The increase of the solute enrichment layer thickness could be caused by the downward secondary circulation generated by the thermoelectric magnetic convection(TEMC) near the interface, which drives the migration of solutes towards the interdendritic region. This work not only clarifies the mechanism of LMF controlling PDS and reducing segregation by TEMC, but also provides theoretical guidance for producing high-quality SC superalloys using magnetic fields.

关键词： Primary dendrite spacing Segregation Single crystal superalloy Directional solidification Magnetic field Thermoelectric magnetic convection

Nitrogen and fluorine co-doped graphene for ultra-stable lithium metal anodes

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Nano Research 2024年第8期17卷 7212-7220页

作者： Pan Li Yifan Liu Xujian Bao Jinghao Xie Zhao Li Hongcheng Li Qiang Ren Xiaomiao Feng Yue Hu Yanwen Ma state key laboratory for Organic Electronics and Information displays(KLOEID)and Jiangsu key laboratory for Biosensors Institute of Advanced Materials(IAM)Nanjing University of Posts and TelecommunicationsNanjing 210023China key laboratory of Carbon Materials of Zhejiang Province College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325000China

The heteroatom doping strategies have been utilized to effectively improve the performance of the carbon-based hosts,such as graphene,for lithium(Li)metal in high energy density lithium metal ***,solely doped graphene hosts often need the assistance of other materials with either better lithiophilicity or electronic conductance to achieve smooth and efficient deposition of Li,which adds extra weight or ***,graphene co-doped by nitrogen and fluorine(NFG)is employed as a stable host for Li,where the N-doping provides lithiophilicity and electronic conductivity lacked by F-doping and the F-doping facilitates fast formation of solid electrolyte interphase(SEI)retarded by *** well regulation of Li plating/stripping and SEI formation is verified by quickly stabilized and small-magnitude voltage hysteresis,which stands out in Li hosts based on doped graphene and leads to excellent long-term cycling performance of NFG based electrodes.A voltage hysteresis of 20 mV is observed for more than 850 h in the symmetrical *** remarkable efficiency of lithium usage is confirmed by the highcapacity retention of a full cell paired with LiFePO_(4)(LFP),which exceeds 70%after 500 *** work presents an innovative perspective on the control of Li plating/stripping by simultaneously introducing two kinds of dopants into graphene and paving the way for exploring practical Li metal batteries.

关键词： Co-doped graphene lithium metal anode dendrite suppression lithiophilic skeleton solid electrolyte interphase(SEI)formation

Interfacial modification using the cross-linkable tannic acid for highly-efficient perovskite solar cells with excellent stability

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Journal of Energy Chemistry 2024年第4期91卷 236-244页

作者： Xing Gao Lirong Rong Fei Wu Yen-Hung Lin Ye Zeng Junhong Tan Rongxing He Cheng Zhong Linna Zhu Chongqing key laboratory for advanced Materials and technologies of Clean Energy School of Materials&EnergySouthwest UniversityChongqing 400715China Hubei key Lab on Organic and Polymeric Optoelectronic Materials Department of ChemistryWuhan UniversityWuhan 430072HubeiChina key laboratory of Luminescence Analysis and Molecular Sensing Ministry of EducationSchool of Chemistry and Chemical EngineeringSouthwest UniversityChongqing 400715China Department of Electronic and Computer Engineering The Hong Kong University of Science and TechnologyClear Water BayKowloon 999077Hong KongChina state key laboratory of advanced displays and optoelectronics technologies The Hong Kong University of Science and TechnologyClear Water BayKowloon 999077Hong KongChina

Although the performance of perovskite solar cells(PSCs)has been dramatically increased in recent years,stability is still the main obstacle preventing the PSCs from being *** device instability can be caused by a variety of reasons,including ions diffusion,surface and grain boundary defects,*** this work,the cross-linkable tannic acid(TA)is introduced to modify perovskite film through post-treatment *** numerous organic functional groups(–OH and C=O)in TA can interact with the uncoordinated Pb^(2+)and I^(-)ions in perovskite,thus passivating defects and inhibiting ions *** addition,the formed TA network can absorb a small amount of the residual moisture inside the device to protect the perovskite ***,TA modification regulates the energy level of perovskite,and reduces interfacial charge ***,following TA treatment,the device efficiency is increased significantly from 21.31%to 23.11%,with a decreased hysteresis ***,the treated device shows excellent air,thermal,and operational *** light of this,the readily available,inexpensive TA has the potential to operate as a multipurpose interfacial modifier to increase device efficiency while also enhancing device stability.

关键词： Tannic acid Defect passivation lons diffusion Hydrophilic Stability Perovskite solar cells

Cross-Modal Graph Semantic Communication Assisted by Generative AI in the Metaverse for 6G

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Research 2024年第2期2024卷 19-27页

作者： Mingkai Chen Minghao Liu Congyan Wang Xingnuo Song Zhe Zhang Yannan Xie Lei Wang key laboratory of Broadband Wireless Communication and Sensor Network Technology Nanjing University of Posts and TelecommunicationsNanjng 210003China state key laboratory of Organic Electronics and Information displays&Institute of advanced Materials(IAM) Nanjing University of Posts and TelecommunicationsNanjing 210023China

Recently, the development of the Metaverse has become a frontier spotlight, which is an important demonstration of the integration innovation of advanced technologies in the Internet. Moreover, artificial intelligence (AI) and 6G communications will be widely used in our daily lives. However, the effective interactions with the representations of multimodal data among users via 6G communications is the main challenge in the Metaverse. In this work, we introduce an intelligent cross-modal graph semantic communication approach based on generative AI and 3-dimensional (3D) point clouds to improve the diversity of multimodal representations in the Metaverse. Using a graph neural network, multimodal data can be recorded by key semantic features related to the real scenarios. Then, we compress the semantic features using a graph transformer encoder at the transmitter, which can extract the semantic representations through the cross-modal attention mechanisms. Next, we leverage a graph semantic validation mechanism to guarantee the exactness of the overall data at the receiver. Furthermore, we adopt generative AI to regenerate multimodal data in virtual scenarios. Simultaneously, a novel 3D generative reconstruction network is constructed from the 3D point clouds, which can transfer the data from images to 3D models, and we infer the multimodal data into the 3D models to increase realism in virtual scenarios. Finally, the experiment results demonstrate that cross-modal graph semantic communication, assisted by generative AI, has substantial potential for enhancing user interactions in the 6G communications and Metaverse.

关键词： modal frontier guarantee