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Spin logic devices based on negative differential resistance -enhanced anomalous Hall effect

International Journal of Minerals,Metallurgy and Materials 2024年第6期31卷 1437-1448页

作者： Hongming Mou Ziyao Lu Yuchen Pu Zhaochu Luo Xiaozhong Zhang key laboratory of Advanced Materials(MOE) School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China state key laboratory of artificial microstructure and mesoscopic physics School of PhysicsPeking UniversityBeijing 100871China

Owing to rapid developments in spintronics,spin-based logic devices have emerged as promising tools for next-generation computing *** paper provides a comprehensive review of recent advancements in spin logic devices,particularly focusing on fundamental device concepts rooted in nanomagnets,magnetoresistive random access memory,spin–orbit torques,electric-field modu-lation,and magnetic domain *** operation principles of these devices are comprehensively analyzed,and recent progress in spin logic devices based on negative differential resistance-enhanced anomalous Hall effect is *** devices exhibit reconfigur-able logic capabilities and integrate nonvolatile data storage and computing *** current-driven spin logic devices,negative differential resistance elements are employed to nonlinearly enhance anomalous Hall effect signals from magnetic bits,enabling reconfig-urable Boolean logic ***,voltage-driven spin logic devices employ another type of negative differential resistance ele-ment to achieve logic functionalities with excellent cascading *** cascading several elementary logic gates,the logic circuit of a full adder can be obtained,and the potential of voltage-driven spin logic devices for implementing complex logic functions can be *** review contributes to the understanding of the evolving landscape of spin logic devices and underscores the promising pro-spects they offer for the future of emerging computing schemes.

关键词： spin logic spin–orbit torque negative differential resistance full-adder

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Half-integer Shapiro steps in MgB_(2) focused He ion beam Josephson junctions

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Chinese physics B 2024年第8期33卷 483-489页

作者：殷大利蔡欣炜徐铁权孙瑞宁韩颖张焱王越甘子钊 Applied Superconductivity Center State Key Laboratory for Mesoscopic PhysicsSchool of PhysicsPeking UniversityBeijing 100871China

Half-integer microwave induced steps(Shapiro steps)have been observed in many different Josephson junction systems,which have attracted a lot of attention because they signify the deviation of current phase relation(CPR)and uncover many unconventional physical *** this article,we first report the discovery of half-integer Shapiro steps in MgB_(2)focused He ion beam(He-FIB)Josephson *** half-integer steps'dependence on microwave frequency,temperature,microwave power,and magnetic field is also *** find that the existence of half-integer steps can be controlled by the magnetic field periodically,which is similar to that of high temperature superconductor(HTS)grain boundary junctions,and the similarity of the microstructures between gain boundary junctions and He-FIB junctions is *** a consequence,we mainly attribute the physical origin of half-integer steps in MgB_(2)He-FIB junctions to the model that a He-FIB junction is analogous to a parallel junctions'*** results show that He-FIB technology is a promising platform for researching CPR in junctions made of different superconductors.

关键词： Josephson junction half-integer Shapiro steps MgB_(2) focused helium ion beam

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Superhydrophobic Co/Fe sulfide nanoparticles and single-atoms doped carbon nanosheets composite air cathode for high-performance zinc-air batteries

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Journal of Energy Chemistry 2024年第9期96卷 568-577页

作者： Yan Tan Yijie Wang Aoshuang Li Xiucai Jiang Yuzhong Zhang Chuanwei Cheng Shanghai key laboratory of Special artificial microstructure Materials and Technology School of Physics Science and EngineeringTongji UniversityShanghai 200092China

Development of a high-performance bifunctional catalyst is essential for the actual implementation of zinc-air batteries in practical ***,a bifunctional cathode of Co_(3)S_(4)/FeS heterogeneous nanoparticles embedded in Co/Fe single-atom-loaded nitrogen-doped carbon nanosheets is ***-iron sulfides and single atomic sites with Co-N_(4)/Fe-N_(4)configurations are confirmed to coexist on the carbon matrix by EXAFS spectroscopy.3D self-supported super-hydrophobic multiphase composite cathode provides abundant active sites and facilitates gas–liquid-solid three-phase interface reactions,resulting in excellent electrocatalytic activity and batteries performance,i.e.,an OER overpotential(η_(10))of 260 mV,a half-wave potential(E_(1/2))of 0.872 V for ORR,aΔE of 0.618 V,and a discharge power density of 170 mW cm^(−2),a specific capacity of 816.3 mAh g^(−1).DFT analysis shows multiphase coupling of sulfide heterojunction through single-atomic metal doped carbon nanosheets reduces offset on center of electronic density of states before and after oxygen adsorption,and spin density of adsorbed oxygen with same spin orientation,leading to weakened charge/spin interactions between adsorbed oxygen and substrate,and a lowered oxygen adsorption energy to accelerate OER/ORR.

关键词： Zn-air battery Superhydrophobic interface Metal sulfide Heterostructure Spin density

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Co-doped BaFe_(2)As_(2) Josephson junction fabricated with a focused helium ion beam

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Chinese physics B 2024年第4期33卷 181-186页

作者：陈紫雯张焱马平徐中堂李宇龙王越路建明马衍伟甘子钊 Applied Superconductivity Research Center Peking UniversityBeijing 100871China state key laboratory for artificial microstructure and mesoscopic physics Peking UniversityBeijing 100871China Institute of Condensed Matter physics School of PhysicsPeking UniversityBeijing 100871China Yangtze Delta Institute of Optoelectronics Peking UniversityBeijing 100871China key laboratory of Applied Superconductivity Institute of Electrical EngineeringChinese Academy of SciencesBeijing 100190China

Josephson junction plays a key role not only in studying the basic physics of unconventional iron-based superconductors but also in realizing practical application of thin-film based devices,therefore the preparation of high-quality iron pnictide Josephson junctions is of great *** this work,we have successfully fabricated Josephson junctions from Co-doped BaFe_(2)As_(2)thin films using a direct junction fabrication technique which utilizes high energy focused helium ion beam(FHIB).The electrical transport properties were investigated for junctions fabricated with various He^(+)irradiation *** junctions show sharp superconducting transition around 24 K with a narrow transition width of 2.5 K,and a dose correlated foot-structure resistance which corresponds to the effective tuning of junction properties by He^(+)*** J_c suppression by more than two orders of magnitude can be achieved by increasing the He^(+)irradiation dose,which is advantageous for the realization of low noise ion pnictide thin film *** Shapiro steps are observed under 10 GHz microwave *** above results demonstrate the successful fabrication of high quality and controllable Co-doped BaFe_(2)As_(2)Josephson junction with high reproducibility using the FHIB technique,laying the foundation for future investigating the mechanism of iron-based superconductors,and also the further implementation in various superconducting electronic devices.

关键词： focused helium ion beam Co doped BaFe_(2)As_(2) Josephson junction

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Tunable artificial plasmonic nanolaser with wide spectrum emission operating at room temperature

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Chinese physics B 2024年第5期33卷 466-471页

作者：周鹏郭佳琦梁琨金磊梁熊玉李俊强邓绪彦秦建宇张家森于丽 state key laboratory of Information Photonics and Optical Communications School of ScienceBeijing University of Posts and TelecommunicationsBeijing 100876China state key laboratory for artificial microstructures and mesoscopic physics School of PhysicsPeking UniversityBeijing 100876China Peking University Yangtze Delta Institute of Optoelectronics Peking UniversityNantong 226010China

With the rapid development of information and communication technology,a key objective in the field of optoelectronic integrated devices is to reduce the nano-laser size and energy *** nanolasers are unable to exceed the diffraction limit and typically exhibit low modulation rates of several *** contrast,plasmonic nanolaser utilizes highly confined surface plasmon polariton(SPP)mode that can exceed diffraction limit and their strong Purcell effect can accelerate the modulation rates to several ***,we propose a parametrically tunable artificial plasmonic nanolasers based on metal–insulator–semiconductor–insulator–metal(MISIM)structure,which demonstrates its ability to compress the mode field volume toλ/*** the pump power increases,the proposed artificial plasmonic nanolaser exhibits 20-nm-wide output ***,we investigate the effects of various cavity parameters on the nanolaser’s output threshold,offering potentials for realizing low-threshold artificial plasmonic ***,we observe a blue shift in the center wavelength of the nanolaser output with thinner gain layer thickness,predominantly attributed to the increased exciton–photon coupling *** work brings inspiration to several areas,including spaser-based interconnects,nano-LEDs,spontaneous emission control,miniaturization of photon condensates,eigenmode engineering of plasmonic nanolasers,and optimal design driven by artificial intelligence(AI).

关键词： surface plasmon polaritons nanolaser ultrafast MISIM

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Low-thermal-budget synthesis of monolayer MoS2

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Science China Materials 2024年第1期67卷 372-374页

作者： Zongmeng Yang Shibo Fang Jing Lu state key laboratory for mesoscopic physics and School of physics Peking University Collaborative Innovation Center of Quantum Matter Beijing key laboratory for Magnetoelectric Materials and Devices (BKL-MEMD) Peking University Peking University Yangtze Delta Institute of Optoelectronics key laboratory for the physics and Chemistry of Nanodevices Peking University Beijing key laboratory of Quantum Devices Peking University

Two-dimensional (2D) materials, such as MoS2, have been considered as a competitive coordinate for future electronics due to their excellent electrostatics and high mobility [1–3]. Moreover, the potential integration of 2D materials with silicon circuits can present increased density and multifunction in future heterogeneously integrated circuits [4,5]. However, the high thermal-budget during Mo S2 synthesis exceeds the temperature requirement of direct integration with Si in the back-end-of-line (BEOL) fabrication process [6–8].

关键词： FILMS

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Progress in research on metal-based materials in stabilized Zn anodes

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Rare Metals 2024年第1期43卷 20-40页

作者： Le Li Shao-Feng Jia Ming-Hui Cao Yong-Qiang Ji Heng-Wei Qiu Dan Zhang Shaanxi key laboratory of Industrial Automation School of Mechanical EngineeringShaanxi University of TechnologyHanzhong 723001China School of Electronic and Information Engineering Qingdao UniversityQingdao 266071China state key laboratory for Artifcial microstructure and mesoscopic physics School of PhysicsPeking UniversityBeijing 100871China Department of Chemistry Key Laboratory of Bioorganic Phosphorus Chemistry and Chemical BiologyTsinghua UniversityBeijing 100084China Shaanxi key laboratory of Catalysis School of Chemistry and Environment ScienceShaanxi University of TechnologyHanzhong 723001China

Aqueous zinc-ion batteries(ZIBs) combine the benefits of metallic Zn anodes with those of aqueous electrolytes and are well suited for large-scale energy storage because of their inherent high safety, cost-effectiveness, and eco-friendliness. Currently, the practical application of such batteries is hindered by the poor cycling performance of Zn anodes due to uncontrolled dendrite formation and severe side reactions, although recent reports suggest that these problems can be mitigated through the modification of Zn anodes with metal-based *** that the mechanisms of improving Zn deposition and the structural evolution of metal-based materials have not been systematically reviewed, we herein systematically overview the metal-based materials used to stabilize Zn anodes, starting with a brief summary of the anode working mechanism and the challenges faced by stabilized Zn anodes. Subsequently, the design principles of Zn anodes stabilized by metal-based materials and the related recent progress are reviewed, and the key challenges and perspectives for the future development of such Zn anodes are proposed.

关键词： Zinc-ion batteries(ZIBs) Zn anode Metalbased materials Alloying metal Stabilized Zn anodes

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Buried Interface Molecular Hybrid Enables Efficient Perovskite Solar Cells

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Chinese physics Letters 2024年第9期 108-109页

作者：黄天宇朱瑞罗德映 state key laboratory for artificial microstructure and mesoscopic physics School of PhysicsFrontiers Science Center for Nano-optoelectronics & Collaborative Innovation Center of Quantum MatterPeking University Department of Chemical and Nano Engineering University of California San Diego

Perovskite solar cells（PSCs） with a positive-intrinsicnegative（p–i–n, commonly referred to as “inverted”）structure are becoming commercially attractive due to their superior power conversion efficiency（PCE） and better operational stability as compared to the “normal” structure device.[1–5]Nonetheless, further improvements in the device performance of inverted PSCs are hampered by interface losses, particularly where the buried interfaces are responsible for perovskite crystallization and chargecarrier extraction.[6–9]

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基于低浓度掺杂TTF-HLCT一体化分子提供的多重激子循环通道增强深蓝光OLED的稳定性

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Science China Materials 2024年第7期67卷 2161-2168页

作者：唐振宇龚乐帆郭浩清杨爽罗骏唐荣肖静张震曲波陈志坚肖立新 state key laboratory of artificial microstructure and mesoscopic physics School of PhysicsPeking UniversityBeijing 100871China College of physics and Electronic Engineering Taishan UniversityTaian 271000China key laboratory of Advanced Display and System Applications Ministry of EducationShanghai UniversityShanghai 200072China

目前,商用的深蓝有机发光二极管(OLED)使用的三重态-三重态融合(TTF)型发光材料只能捕获50%的三重态(T_(1))激子,导致其器件效率较低.基于窄带蓝色发射体的热激活延迟荧光(TADF)和超荧光策略可以实现接近100%的激子利用率,然而,在发射层... 详细信息

目前,商用的深蓝有机发光二极管(OLED)使用的三重态-三重态融合(TTF)型发光材料只能捕获50%的三重态(T_(1))激子,导致其器件效率较低.基于窄带蓝色发射体的热激活延迟荧光(TADF)和超荧光策略可以实现接近100%的激子利用率,然而,在发射层(EML)中停留的高能量T_(1)激子通常会导致不可避免的分子降解,从而限制了器件的使用寿命.为了解决这一问题,本文研究了一种TTF-杂化局域-电荷转移态(HLCT)一体化分子,旨在通过多个激子回收通道降低EML内T_(1)激子的密度,从而提高高效深蓝OLED的稳定性.通过TTF过程回收T_(1)激子,通过HLCT过程利用高能三重态(Tn)激子,可以提高EML中三重态激子的利用率.此外,低浓度掺杂的TTF-HLCT分子在TADF体系中可以减轻T_(1)激子猝灭造成的效率损失.最后,实现了外量子效率(EQE)为25.9%、CIE为(0.131,0.050)、蓝光指数(CE由CIEy校准)为312 cd A^(−1) CIE_(y)^(−1)的顶发射OLED,并且其寿命T90@1000 cd m^(−2)从0.5小时延长到6.1小时.本工作揭示了低浓度TTF-HLCT分子掺杂的潜力,作为一种可行的解决方案,可以最大限度地减少效率猝灭,并解决蓝光OLED的稳定性问题.

关键词： organic light-emitting diode stability multiple ex-citon recycling channels deep blue emission TTF-HLCT

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Dynamically enhanced Autler–Townes splitting by orthogonal XUV fields

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Chinese physics B 2024年第7期33卷 344-350页

作者：吴立龙姜维超彭良友 Institute of Quantum Precision Measurement College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China state key laboratory for mesoscopic physics and Frontiers Science Center for Nano-optoelectronics School of PhysicsPeking UniversityBeijing 100871China

Based on numerical solutions of the time-dependent Schr ¨odinger equation, we theoretically investigate the photoelectron spectrum of hydrogen atoms ionized by a pair of ultrashort, intense, and orthogonally polarized laser pulses with a relative time delay in a pump–probe configuration. The pump pulse resonantly excites electrons from the 1s and 2p levels,inducing Rabi oscillations. The resulting dynamically enhanced Autler–Townes(AT) splitting is observed in the photoelectron energy spectrum upon interaction with the second probe pulse. In contrast to the previous parallel-polarization scheme, the proposed orthogonal-polarization configuration enables the resolution of dynamically enhanced AT splitting over a considerably wider range of probe photon energies.

关键词： Autler–Townes splitting orthogonal XUV fields photoelectron spectra Rabi frequency

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