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Preheating-assisted solid-state friction stir repair of Al-Mg-Si alloy plate at different rotational speeds

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International Journal of Minerals,Metallurgy and Materials 2024年第4期31卷 725-736页

作者： Hui Wang Yidi Li Ming Zhang Wei Gong Ruilin Lai Yunping Li state Key Laboratory of Powder Metallurgy Central South UniversityChangsha 410083China Research institute of Light Alloy Central South UniversityChangsha 410083China

Additive friction stir deposition(AFSD)is a novel structural repair and manufacturing technology has become a research hotspot at home and abroad in the past five *** this work,the microstructural evolution and mechanical performance of the Al-Mg-Si alloy plate repaired by the preheating-assisted AFSD process were *** evaluate the tool rotation speed and substrate preheating for repair quality,the AFSD technique was used to additively repair 5 mm depth blind holes on 6061 aluminum alloy *** results showed that preheat-assisted AFSD repair significantly improved joint bonding and joint strength compared to the control non-preheat substrate ***,increasing rotation speed was also beneficial to improve the metallurgical bonding of the interface and avoid volume *** preheating conditions,the UTS and elongation were positively correlated with rotation *** the process parameters of preheated substrate and tool rotation speed of 1000 r/min,defect-free specimens could be obtained accompanied by tensile fracture occurring in the substrate rather than the repaired *** UTS and elongation reached the maximum values of 164.2MPa and 13.4%,which are equivalent to 99.4%and 140%of the heated substrate,respectively.

关键词： additive friction stir deposition structural repair tool rotation speed Al alloy

Interfacial engineering for high-performance garnet-based solid-state lithium batteries

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SusMat 2024年第1期4卷 72-105页

作者： Lingchen Wang Jiaxin Wu Chengshuai Bao Zichang You Yan Lu Zhaoyin Wen state Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghaiChina

solid-state batteries represent the future of energy storage technology,offering improved safety and energy ***-type Li_(7)La_(3)Zr_(2)O_(12)(LLZO)solidstate electrolytes-based solid-state lithium batteries(SSLBs)stand out for their appealingmaterial properties and chemical ***,their successful deployment depends on conquering interfacial *** review article primarily focuses on the advancement of interfacial engineering for LLZO-based *** commence with a concise introduction to solid-state electrolytes and a discussion of the challenges tied to interfacial properties in LLZO-based *** deeply explore the correlations between structure and properties and the design principles vital for achieving an ideal electrode/electrolyte ***,we delve into the latest advancements and strategies dedicated to overcoming these challenges,with designated sections on cathode and anode interface *** the end,we share our insights into the advancements and opportunities for interface design in realizing the full potential of LLZO-based SSLBs,ultimately contributing to the development of safe and high-performance energy storage solutions.

关键词： anode interfaces cathode interfaces garnet-based electrolytes interfacial modifications solidstate lithium batteries

On-Chip Micro Temperature Controllers Based on Freestanding Thermoelectric Nano Films for Low-Power Electronics

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Nano-Micro Letters 2024年第7期16卷 98-108页

作者： Qun Jin Tianxiao Guo Nicolas Perez Nianjun Yang Xin Jiang Kornelius Nielsch Heiko Reith institute for Metallic Materials Leibniz Institute for Solid State and Materials Research01069 DresdenGermany institute of Materials Engineering University of Siegen57076 SiegenGermany institute of Applied Physics Technical University of Dresden01069 DresdenGermany institute of Materials Science Technical University of Dresden01069 DresdenGermany

Multidimensional integration and multifunctional com-ponent assembly have been greatly explored in recent years to extend Moore’s Law of modern ***,this inevitably exac-erbates the inhomogeneity of temperature distribution in microsystems,making precise temperature control for electronic components extremely ***,we report an on-chip micro temperature controller including a pair of thermoelectric legs with a total area of 50×50μm^(2),which are fabricated from dense and flat freestanding Bi2Te3-based ther-moelectric nano films deposited on a newly developed nano graphene oxide membrane *** tunable equivalent thermal resistance is controlled by electrical currents to achieve energy-efficient temperature control for low-power electronics.A large cooling temperature difference of 44.5 K at 380 K is achieved with a power consumption of only 445μW,resulting in an ultrahigh temperature control capability over 100 K mW^(-1).Moreover,an ultra-fast cooling rate exceeding 2000 K s^(-1) and excellent reliability of up to 1 million cycles are *** proposed on-chip temperature controller is expected to enable further miniaturization and multifunctional integration on a single chip for microelectronics.

关键词： Temperature control Low-power electronics On-chip micro temperature controller Freestanding thermoelectric nano films Temperature-sensitive components

Pion-photon and kaon-photon transition distribution amplitudes in the Nambu–Jona-Lasinio model

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Chinese Physics C 2024年第8期48卷 94-103页

作者： Jin-Li Zhang Jun Wu Department of Mathematics and Physics Nanjing Institute of TechnologyNanjing 211167China National Laboratory of solid state Microstructures Department of PhysicsNanjing UniversityNanjing 210093China

The Nambu–Jona-Lasinio model is utilized to investigate the pion-and kaon-photon leading-twist transition distribution amplitudes using proper time ***,the properties of the vector and axial vector pion-photon transition distribution amplitudes are examined,and the results meet the desired *** study involves sum rule and polynomiality *** vector and axial vector pion-photon transition form factors that are present in theπ^(+)→γe^(+)νprocess are the first Mellin moments of the pion-photon transition distribution *** vector transition form factor originates from the internal structure of hadrons,the axial current can be coupled to a pion,this pion is virtual,and its contribution will be present independently of the external *** kaon transition form factors are *** vector form factor's value at zero momentum transfer is determined by the axial anomaly,while this is not the case for the axial *** vector and axial form factors,as well as the neutral pion vector form factor F_(πγγ)(t),are *** to our findings,the pion axial transition form factor is harder than the vector transition form factor and harder than the electromagnetic form *** also discuss the link betweenπ−γandγ−πtransitions distribution amplitudes.

关键词： transition form factors NJL model transition distribution amplitudes

Achieving near-infrared-light-mediated switchable friction regulation on MXene-based double network hydrogels

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Friction 2024年第1期12卷 39-51页

作者： Pengxi WU Cheng ZENG Jinglun GUO Guoqiang LIU Feng ZHOU Weimin LIU Center of Advanced Lubrication and Sealing Materials State Key Laboratory of Solidification ProcessingNorthwestern Polytechnical UniversityXi’an 710072China state Key Laboratory of solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

MXene possesses great potential in enriching the functionalities of hydrogels due to its unique metallic conductivity,high aspect ratio,near-infrared light(NIR light)responsiveness,and wide tunability,however,the poor compatibility of MXene with hydrogels limits further *** this work,we report a uniformly dispersed MXene-functionalized poly-N-isopropylacrylamide(PNIPAM)/poly-2-acrylamido-2-methyl-1-propanesulfonic acid(PAMPS)double network hydrogel(M–DN hydrogel)that can achieve switchable friction regulation by using the NIR *** dispersity of MXene in hydrogels was significantly improved by incorporating the chitosan(CS)*** M–DN hydrogel showed much low coefficient of friction(COF)at 25℃ due to the presence of hydration layer on hydrogel *** illuminating with the NIR light,M–DN hydrogel with good photothermal effect rapidly raised the temperature to above the lower critical solution temperature(LCST),which led to an obvious increase of surface COF owing to the destruction of the hydration *** addition,M–DN friction control hydrogel showed good recyclability and controllability by tuning“on-off”of the NIR *** work highlights the construction of functional MXene hydrogels for intelligent lubrication,which provides insight for interface sensing,controlled transmission,and flexible robotic arms.

关键词： MXene dispersion photothermal hydrogel near-infrared(NIR)light friction modulation

Polyimide covalent organic frameworks as efficient solid-state Li^(+) electrolytes

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Science China Chemistry 2024年第5期67卷 1647-1652页

作者： Xu Liu Shi Wang Siqi Liu Chengfang Liu Xiangchun Li Jian Wu Dazhi Li Shihao Xu Chongyang Liu Wen-Yong Lai state Key Laboratory of Organic Electronics and Information Displays(SKLOEID) Institute of Advanced Materials(IAM)School of Chemistry and Life SciencesNanjing University of Posts&TelecommunicationsNanjing 210023China

Covalent organic frameworks(COFs) are attractive porous crystalline materials with extremely high stability, easy functionalization, and open channels, which are expected to be unique ion conductors/transporters in lithium ion batteries(LIBs). Despite recent advances, low ion conductivity and low transference number, resulting in low charging/discharging rate, low energy density, and short battery life, are the main issues that limit their direct application as solid electrolytes in LIBs. Here, we designed and synthesized a novel polyimide COF, namely, TAPA-PDI-COF, with abundant C=O groups, which has been successfully employed as high-performance solid electrolytes by doping TAPA-PDI-COF and succinonitrile(SN). Both the well-defined nanochannels of COFs and SN confined in the well-aligned channels restricted the free migration of anions, while C=O on COFs and CN groups of SN enhanced Li^(+) transport, thus achieving a high ion conductivity of 0.102 m S cm^(-1)at 80 °C and a high lithium-ion transference number of 0.855 at room temperature. According to density functional theory(DFT)calculations, Li-ion migration mainly adopted in-plane transport rather than the axial pathway, which may be due to the shorter hopping distances in the planar pathway. The results suggest an effective strategy for the design and development of all-solidstate ionic conductors for achieving high-performance LIBs.

关键词： lithium ion batteries(LIBs) covalent organic frameworks(COFs) solid-state ion conductors solid-state electrolytes ion conductivity

Modification of POSS and their tribological properties and resistant to space atomic oxygen irradiation as lubricant additive of multialkylated cyclopentanes

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Friction 2024年第5期12卷 884-896页

作者： Xingwei WANG Chaoyang ZHANG Chen ZHAO Yijing LIANG Ming ZHANG Wufang YANG Bo YU Qiangliang YU Meirong CAI Feng ZHOU Weimin LIU state Key Laboratory of solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou730000China Shandong Laboratory of Yantai Advanced Materials and Green Manufacturing Yantai264000China

Developing functional additive resistant to space atomic oxygen(AO)irradiation through simple molecular design and chemical synthesis to enhance the lubricating performance of multialkylated cyclopentanes(MACs)oil is a significant ***,sulfur-containing polyhedral oligomere silsesquioxane(POSS)were synthesize via a click-chemistry reaction of octavinyl polyhedral oligomeric with alkyl *** reduce-friction(RF),anti-wear(AW)properties and anti-AO irradiation of POSS-S-R as MACs base oil additives in atmospheric and simulated space environments were systematically investigated for the first *** demonstrate that POSS-S-R not only possesses outstanding anti-AO irradiation capacity but also effectively improves the RF and AW of MACs in atmospheric or simulated space *** improvement is due to the excellent anti-AO irradiation properties of the POSS structure itself and the high load-carrying ability of silicon-containing and sulfur-containing compounds generated by tribo-chemical reactions,which effectively separates the direct contact of the friction *** believe that this synthesized POSS-S-R is a promising additive for space lubricants.

关键词： POSS additive reduce-friction anti-wear multialkylated cyclopentanes(MACs) resistant atomic irradiation

Machine-learning-assisted efficient reconstruction of the quantum states generated from the Sagnac polarization-entangled photon source

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Chinese Physics B 2024年第8期33卷 50-54页

作者：毛梦辉周唯李新慧杨然龚彦晓祝世宁 National Laboratory of solid state Microstructures and School of Physics Nanjing UniversityNanjing 210093China Author notes

Neural networks are becoming ubiquitous in various areas of physics as a successful machine learning(ML)technique for addressing different *** on ML technique,we propose and experimentally demonstrate an efficient method for state reconstruction of the widely used Sagnac polarization-entangled photon *** properly modeling the target states,a multi-output fully connected neural network is well trained using only six of the sixteen measurement bases in standard tomography technique,and hence our method reduces the resource consumption without loss of *** demonstrate the ability of the neural network to predict state parameters with a high precision by using both simulated and experimental ***,the mean absolute error for all the parameters is below 0.05 for the simulated data and a mean fidelity of 0.99 is achieved for experimentally generated *** method could be generalized to estimate other kinds of states,as well as other quantum information tasks.

关键词： machine learning state estimation quantum state tomography polarization-entangled photon source

Recent advances in solving Li_(2)CO_(3) problems in garnet-based solid-state battery: A systematic review(2020-2023)

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Journal of Energy Chemistry 2024年第3期90卷 58-76,I0004页

作者： Shaoxiong Han Ziqi Wang Yue Ma Yanlan Zhang Yongzhen Wang Xiaomin Wang College of Materials Science and Engineering Taiyuan University of TechnologyTaiyuan 030024ShanxiChina Shanxi Joint Laboratory of Coal based solid Waste Resource Utilization and Green Ecological Development Taiyuan 030024ShanxiChina

Garnet solid electrolytes are one of the most promising electrolytes for solid-state ***,Li_(2)CO_(3) is a critical issue that hinders the practical application of garnet-based solid-state lithium-ion *** are two sources of Li_(2)CO_(3) *** main one is the aging of garnet electrolytes in the *** electrolytes can react with H_(2)O and CO_(2) in the air to form Li_(2)CO_(3),which reduces ion conductivity,increases electrode/garnet electrolyte interface resistance,and deteriorates the electrochemical performance of the *** strategies,such as elemental doping,grain boundary manipulation,and interface engineering,have been suggested to address these *** other is the passivation layer(Li_(2)CO_(3),Li_3N,LiOH,Li_(2)O) formed on the surface of the lithium foil after long-term storage,which is ignored by most *** better understand the current strategies and future trends to address the Li_(2)CO_(3) problem,this perspective provides a systematic review of journals published in this field from 2020-2023.

关键词： solid-state batteries Garnet electrolytes Air stability Interface engineering Lithium foil contamination