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Oil-soluble polymer brushes-functionalized nanoMOFs for highly efficient friction and wear reduction

Friction 2024年第7期12卷 1499-1511页

作者： Jianxi LIU Yong QIAN Dongsheng LI Wei WU Mengchen ZHANG Jie YAN Bin LI Feng ZHOU State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi'an 710072China shaanxi engineering research center of special sealing technology Xi'an Aerospace Propulsion InstituteXi'an 710100China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

Nanomaterials as lubricating oil additives have attracted significant attention because of their designable composition and structure,suitable mechanical property,and tunable surface ***,the poor compatibility between nanomaterials and base oil limits their further *** this work,we demonstrated oil-soluble poly(lauryl methacrylate)(PLMA)brushes-grafted metal-organic frameworks nanoparticles(nanoMOFs)as lubricating oil additives that can achieve efficient friction reduction and anti-wear *** were synthesized by free-radical polymerization,which was coordinatively grafted onto the surface of the UiO-67 ***,PLMA brushes were grown on the macroinitiator-modified UiO-67 by surface-initiated atom transfer radical polymerization,which greatly improved the lipophilic property of the UiO-67 nanoparticles and significantly enhanced the colloidal stability and long-term dispersity in both non-polar solvent and base *** adding UiO-67@PLMA nanoparticles into the 500 SN base oil,coefficient of friction and wear volume reductions of 45.3%and 75.5%were achieved due to their excellent mechanical properties and oil ***,the load-carrying capacity of 500 SN was greatly increased from 100 to 500 N by the UiO-67@PLMA additives,and their excellent tribological performance was demonstrated even at a high friction frequency of 65 Hz and high temperature of 120℃.Our work highlights oil-soluble polymer brushes-functionalized nanoMOFs for highly efficient lubricating additives.

关键词： MOFs polymer brushes surface modification tribological properties friction reduction anti-wear

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Adaptive observer-based integral event-triggered antivibration control of a full aircraft active landing gear system with irregular runway excitations

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Science China(Information Sciences) 2024年第6期67卷 248-261页

作者： Wenxiao HU Chenglong DU Fanbiao LI Xinmin CHEN Chunhua YANG Weihua GUI School of Automation Central South University research center in System engineering for special Aircrafts Ningbo Institute of Materials Technology and EngineeringChinese Academy of Sciences

This study addresses the antivibration issue of a full aircraft active landing gear system(LGS)under landing impact and runway excitations via a novel adaptive observer-based integral event-triggered control method. First, a full aircraft active LGS comprising a front gear and two synchronized main left and right gears with active suspensions is established, where the information exchange among them is not implemented directly. Second, two adaptive observers are designed separately for the front and main LGSs to identify the varying damping parameters and estimate the system states simultaneously. Third, estimated states are transmitted to a shared network through a novel integral event-triggered mechanism(I-ETM);thus, the front and main LGSs are interconnected, and a networked control scheme for the aircraft LGS is constructed. Additionally, the integrated active control law is designed with the aid of the transmitted states of the front and main LGSs, enhancing the robustness against the pitch vibration of the ***, the L2-stability of the hybrid system is guaranteed to depress the vertical vibration effect of the landing impact and irregular runway excitations, thus improving passenger safety and comfort. Moreover,a codesign method is provided to obtain feasible solutions to the gain matrices of the observers and controllers simultaneously. Simulation and comparison results are presented to illustrate the effectiveness and superiority of the proposed control scheme in antivibration and saving communication resources.

关键词： aircraft active landing gear antivibration control integral event-triggered mechanism adaptive observer ${\mathcal{L}}_2$-stability

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On the Application of Mixed Models of Probability and Convex Set for Time-Variant Reliability Analysis

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Computer Modeling in engineering & Sciences 2024年第5期139卷 1981-1999页

作者： Fangyi Li Dachang Zhu Huimin Shi center for research on Leading technology of special Equipment School of Mechanical and Electric EngineeringGuangzhou UniversityGuangzhou510006China

In time-variant reliability problems,there are a lot of uncertain variables from different ***,it is important to consider these uncertainties in *** addition,time-variant reliability problems typically involve a complexmultilevel nested optimization problem,which can result in an enormous amount of *** this end,this paper studies the time-variant reliability evaluation of structures with stochastic and bounded uncertainties using a mixed probability and convex set *** this method,the stochastic process of a limit-state function with mixed uncertain parameters is first discretized and then converted into a timeindependent reliability ***,to solve the double nested optimization problem in hybrid reliability calculation,an efficient iterative scheme is designed in standard uncertainty space to determine the most probable point(MPP).The limit state function is linearized at these points,and an innovative random variable is defined to solve the equivalent static reliability analysis *** effectiveness of the proposed method is verified by two benchmark numerical examples and a practical engineering problem.

关键词： Mixed uncertainty probability model convex model time-variant reliability analysis

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A review on surface coating strategies for anti-hygroscopic of high energy oxidizer ammonium dinitramide

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Defence technology（防务技术） 2024年第3期33卷 237-269页

作者： Hongyu Yang Fuyao Chen Yiwen Hu Qiangqiang Lu Lei Xiao Yinglei Wang Fengqi Zhao Wei Jiang Gazi Hao National special Superfine Powder engineering research center of China School of Chemistry and Chemical EngineeringNanjing University of Science and TechnologyNanjing 210094China Xi’an Modern Chemistry research Institute Xi’an 710065China

Ammonium dinitramide(ADN),which has the advantages of high energy density,no halogen and low characteristic signal,is not only considered as a new high-energy oxidizer that is expected to replace the traditional oxidizer ammonium perchlorate(AP)in solid propellants,but also a good performance explosive in ***,due to the strong hygroscopicity of ADN,its application in solid propellants and explosives is greatly *** the hygroscopicity of ADN is the key to realize the wide application of *** this paper,we systematically review the research progress of anti-hygroscopic strategies of ADN *** surface coating methods are focusing on solvent volatilization,solvent-non-solvent,melt crystallization and atomic layer deposition *** characteristics of the different methods are compared and analyzed,and the basis for the classification and selection of the coating materials are introduced in *** addition,the feasibility of material for surface coating of ADN is evaluated by several compatibility analysis *** is highly expected that the liquid phase method(solvent volatilization method,solvent-non-solvent method)would be the promising method for future ADN coating because of its effective,safety and facile ***,polymer materials,are the preferred coating materials due to their high viscosity,easy adhesion,good anti-hygroscopic effect,and heat resistance,which make ADN weak hygroscopicity,less sensitive,easier to preserve and good compatibility.

关键词： Ammonium dinitramide(ADN) Energetic materials Anti-hygroscopic Surface coating Compatibility analysis

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Pressure Pulse Response of High Temperature Molten Salt Check Valve Hit by Crystal Particles

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Journal of Shanghai Jiaotong university(Science) 2024年第2期29卷 271-279页

作者：李树勋沈恒云刘斌才胡迎港马廷前 School of Petrochemical engineering Lanzhou University of TechnologyLanzhou 730050China Machinery Industry Pump and special Valve engineering research center Lanzhou 730050China

In view of the problem that crystalline particles cause wall vibration at a low temperature,based on two-phase flow model,computational fuid dynamics is used to conduct the numerical simulation of internal flows when the valve openings are 20%,60%and 100%*** molten salt fow may be changed under strict conditions and produce forced vibration of the inner parts of molten salt particle shock valve *** two-phase flow model is used for different molten salt sizes to extract temporal pressure pulse information and conduct statistical data processing *** influence of the molten salt crystallization of molten salt particles on the fow and pressure pulse strength is *** results show that the crystallization of molten salt has a serious impact on the vibration of the valve body,especially in the throttle *** valve oscillation caused by the pressure pulsation mostly occurs from the small opening *** the opening increases,the pressure pulse threshold and its change trend decrease.

关键词： molten salt valve numerical simulation pressure pulsation two-phase flow crystal frozen blocking

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A healable, mechanically robust and ultrastretchable ionic conductive elastomer for durably wearable sensor

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Nano research 2024年第4期17卷 3369-3378页

作者： Guoxian Zhang Chunmei Li JiaoJun Tan Mingqi Wang Yafeng Ren Feijie Ge Qiuyu Zhang Key Laboratory of special Functional and Smart Polymer Materials of Ministry of Industry and Information technology School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi'an 710072China College of Bioresources Chemical and Materials engineering National Demonstration Center for Experimental Light Chemistry Engineering EducationShaanxi University of Science&TechnologyXi’an 710021China

The ionic conductive elastomers show great promise in multifunctional wearable electronics,but they currently suffer from liquid leakage/evaporation or mechanical *** ionic conductive elastomers integrating non-volatility,mechanical robustness,superior ionic conductivity,and ultra-stretchability remains urgent and ***,we developed a healable,robust,and conductive elastomer via impregnating free ionic liquids(ILs)into the ILs-multigrafted poly(urethane-urea)(PUU)elastomer networks.A crucial strategy in the molecular design is that imidazolium cations are largely introduced by double-modification of PUU and centipede-like structures are obtained,which can lock the impregnated ILs through strong ionic *** this system,the PUU matrix contributes outstanding mechanical properties,while the hydrogen bonds and ionic interactions endow the elastomer with self-healing ability,conductivity,as well as non-volatility and *** fabricated ionic conductive elastomers show good conductivity(3.8×10^(-6) S·cm^(-1)),high mechanical properties,including tensile stress(4.64 MPa),elongation(1470%),and excellent healing ability(repairing efficiency of 90%after healing at room temperature for 12 h).Significantly,the conductive elastomers have excellent antifatigue properties,and demonstrate a highly reproducible response after 1000 uninterrupted extension-release *** work provides a promising strategy to prepare ionic conductive elastomers with excellent mechanical properties and stable sensing capacity,and further promote the development of mechanically adaptable intelligent sensors.

关键词： ionic conductive elastomers poly(urethane-urea)(PUU) ionic interactions centipede-like self-healing

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Complementary multicolor electrochromic devices with excellent stability based on porous tin oxide nanosheet scaffold

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Nano research 2024年第4期17卷 3035-3042页

作者： Chenchen Bian Jinhui Wang Huanhuan Liu Yin Yan Ping Zhang Weilong Yang Sensen Jia Xiaodan Guo Guofa Cai Key Laboratory for special Functional Materials of Ministry of Education National&Local Joint Engineering Research Center for High-Efficiency Display and Lighting TechnologySchool of Materials and Engineeringand Collaborative Innovation Center of Nano Functional Materials and ApplicationsHenan UniversityKaifeng 475004China

Electrochromic devices(ECDs)have been extensively investigated as promising candidates in broad cutting-edge applications,such as smart windows,electronic labels,adaptive camouflage,***,they have suffered from either inadequate color variations or poor cycling stability for a long ***,we developed a general strategy to boost the cyclic stability and enrich the color variations of ECDs by scrupulous design of the composition and nanostructure of electrodes,in which porous tin oxide(SnO_(2))nanosheets serve as the scaffold and typical metal oxides or conducting polymers as the active electrochromic *** electrochromic composite materials,including polyaniline(PANI)@SnO_(2),V2O5@SnO_(2),and WO_(3)@SnO_(2) heterostructured nanoarrays were prepared by the facile wet-chemical *** composite electrodes exhibit remarkable electrochromic performances,e.g.,superior cycling stability(more than 2000 cycles),rich color variations(more than 5 colors for PANI@SnO_(2)),and enlarged optical *** excellent performances account for the heterogenous porous nanoarrays,which not only facilitate the intercalation/extraction of ions but also relieve the stress generated during the electrochemical *** addition,diverse prototypes of complementary multicolor ECD with excellent cycling stability(over thousands of cycles)and rich color variations(8 colors)were realized for the first *** believe that our work put forward a general strategy for developing high-quality multicolor complementary electrochromic devices.

关键词： electrochromism tin oxide metal oxide cycling stability multicolor complementary device

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Characterizing the complete mitochondrial genome of Psephenothrips eriobotryae Dang&Qiao(Thysanoptera:Phlaeothripidae)with massive gene arrangement in Phlaeothripidae

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Zoological Systematics 2024年第2期49卷 116-128页

作者： Lihong Dang Chengwen Li Dongxue Wang Yuxin Gao Linpeng Zhao Bin Zhang School of Biological Science&engineering Shaanxi University of TechnologyHanzhong 723000China engineering research center of Quality Improvement and Safety Control of Qinba special Meat Products Universities of Shaanxi ProvinceHanzhong 723000China shaanxi Changqing National Nature Reserve Changqing JiayuanNo.176Hanzhong 723000China College of Life Sciences&technology Inner Mongolia Normal UniversityHohhot 010022China

Each species within the order Thysanoptera has a distinct mitochondrial gene order displaying a high level of gene rearrangement,particularly massive in *** understand the evolutionary patterns of rearrangement in this family,we sequenced the complete mitochondrial genome of Psephenothrips eriobotryae,a notable potential pest of loquat *** mitogenome is a circular DNA molecule(15,413 bp in size)composed of 37 genes:13 PCGs,22 tRNAs,two rRNAs,and two putative control regions(CRs).By comparing with the ancestral mitogenome of arthropods,*** exhibits notable gene rearrangement ***,it shares four conserved gene blocks with three closely related species in *** the phylogenetic tree,*** was clustered with these three leaffeeding Phlaeothripinae *** presence of more similar conserved gene blocks probably indicates a strong correlation between gene rearrangements and the phylogeny within ***,the mitogenome of *** shows some characteristics:(a)two putative CRs in which CR2 is the copy of partial CR1 with 99.62%sequence similarity,and CR1 consists of two 237 bp repeat unites;(b)high A+T content of 82.6%in overall base composition;(c)trn S1 lacking a complete dihydrouridine(DHU)arm;(d)the protein coding gene,atp8 started with TTG instead of the more common ATN,while nad3 terminated by TAG rather than TAA;(e)translocations and inversions observed in fifteen of the 37 genes.

关键词： Mitogenome structure phylogenetic relationships Liothrips-lineage repeat regions

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Mechanism of high-energy pulsed current-assisted rolling of 08AL carbon steel ultra-thin strip

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Journal of Iron and Steel research(International) 2024年第2期31卷 416-427页

作者： Zhong-kai Ren Ya-nan Xu Jia-zhao Chen He Li Rui-lin Yuan Zhen-hua Wang Tao Wang Xiao Liu College of Mechanical and Vehicle engineering Taiyuan University of TechnologyTaiyuan030024ShanxiChina engineering research center of Advanced Metal Composites Forming technology and Equipment(Ministry of Education) Taiyuan University of TechnologyTaiyuan030024ShanxiChina National Key Laboratory of Metal Forming technology and Heavy Equipment China National Heavy Machinery Research Institute Co.Ltd.Xi’an710016ShaanxiChina

To improve the plastic deformation performance of a 08AL carbon steel ultra-thin strip,a pulsed electric field was integrated into the plastic processing of the ultra-thin strip,and the effects of high-energy current on its deformation ability were ***-assisted tensile tests were employed,and the results clarified that the pulsed current could reduce the activation energy of faults and promoted dislocation slip within grains and at grain boundaries,leading to a decrease in the deformation resistance of the metal and an increase in its plastic *** the current density of 2.0 A/mm2,the yield strength,tensile strength,and elongation of the rolled sample reached 425 MPa,467 MPa,and 12.5%,*** the rolling process,it was found that the pulsed current promoted the dynamic recrystallization of the ultra-thin strip,reduced its dislocation density and deformation resistance,and promoted the coordinated deformation of the metal.

关键词： 08AL ultra-thin strip High-energy pulsed current Mechanical property Dislocation density Dynamic recrystallization

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New insights in nano-copper chromite catalyzing ultrafine AP:Evaluation of dispersity and mixing uniformity

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Defence technology（防务技术） 2024年第2期32卷 120-133页

作者： Yong Kou Peng Luo Lei Xiao Yanping Xin Guangpu Zhang Yubing Hu Junqing Yang Hongxu Gao Fengqi Zhao Wei Jiang Gazi Hao National special Superfine Powder engineering research center of China School of Chemistry and Chemical EngineeringNanjing University of Science and TechnologyNanjing210094China Xi'an North Huian Chemical Industry Co.Ltd Xi'an710302China Xi'an Modern Chemistry research Institute Xi'an710065China

Improving the application of nanomaterials has always been a research hotspot in the field of energetic materials(EMs)due to their obvious catalytic effect on the EMs,especially the uniformly dispersed ***,few studies have reported the dispersion of *** this study,the dispersity and mixing uniformity of nano-CuCr_(2)O_(4)was evaluated based on the difference of solid UV light absorption between the nano-catalytic materials and *** nano-CuCr_(2)O_(4)/ultrafine AP composites with different dispersity of nano-CuCr_(2)O_(4)were prepared by manual grinding and mechanical grinding with different grinding strength and griding *** then,the absorbance of different samples at 212 nm was obtained by solid UV testing due to the high repeatability of the absorbance at 210-214 nm for three parallel experiments,and the dispersity of different samples was calculated through the established difference ***,the samples were characterized by XRD,IR,SEM,EDS,DSC and TG-MS,which confirmed that different mixing methods did not change the structure of the samples(XRD and IR),and the mixing uniformity improved with the increase of grinding strength and grinding time(SEM and EDS).The scientificity and feasibility of the difference equation were further verified by *** dispersity of nano-CuCr_(2)O_(4)exhibits a positive intrinsic relationship with its catalytic performance,and the uniformly dispersed nano-CuCr_(2)O_(4)significantly reduces the thermal decomposition temperature of ultrafine AP from 367.7 to 338.8℃.The TG-MS patterns show that the dispersed nano-CuCr_(2)O_(4)advanced the thermal decomposition process of ultrafine AP by about 700 s,especially in the high temperature decomposition stage,and the more concentrated energy release characteristic is beneficial to further enhance the energy performance of AP-based *** above conclusions show that the evaluation method of dispersity based on solid UV curves could pro

关键词： Nano-CuCr_(2)O_(4) Ultrafine AP Dispersity UVeVis diffuse reflectance spectroscopy Thermal decomposition

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