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Toward implantable devices for angle-sensitive,lens-less,multifluorescent,single-photon lifetime imaging in the brain using Fabry-Perot and absorptive color filters

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Light(Science & Applications) 2022年第2期11卷 197-211页

作者： Adriaan J.Taal Changhyuk Lee Jaebin Choi Björn Hellenkamp Kenneth L.Shepard Columbia University-Department of Electrical Engineering 500W.120th St.Mudd 1310New York 10027 NYUSA Korea Institute of Science and Technology-Brain Science Institute 5 Hwarang-ro 14-gilSeongbuk-guSeoul 02792Republic of Korea

Implantable image sensors have the potential to revolutionize *** to their small form factor requirements;however,conventional filters and optics cannot be *** limitations obstruct highresolution imaging of large neural *** advances in angle-sensitive image sensors and single-photon avalanche diodes have provided a path toward ultrathin lens-less fluorescence imaging,enabling plenoptic sensing by extending sensing capabilities to include photon arrival time and incident angle,thereby providing the opportunity for separability of fluorescence point sources within the context of light-field microscopy(LFM).However,the addition of spectral sensitivity to angle-sensitive LFM reduces imager resolution because each wavelength requires a separate pixel ***,we present a 1024-pixel,50μm thick implantable shank-based neural imager with color-filtergrating-based angle-sensitive *** angular-spectral sensitive front end combines a metal–insulator–metal(MIM)Fabry–Perot color filter and diffractive optics to produce the measurement of orthogonal light-field information from two distinct colors within a single *** result is the ability to add independent color sensing to LFM while doubling the effective pixel *** implantable imager combines angular-spectral and temporal information to demix and localize multispectral fluorescent *** this initial prototype,this is demonstrated with 45μm diameter fluorescently labeled beads in scattering *** lifetime imaging is exploited to further aid source separation,in addition to detecting pH through lifetime changes in fluorescent *** these initial fluorescent targets are considerably brighter than fluorescently labeled neurons,further improvements will allow the application of these techniques to in-vivo multifluorescent structural and functional neural imaging.

关键词： filters lifetime angle

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SnO_(2)/Graphene Composite with High Lithium Storage Capability for Lithium Rechargeable Batteries

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Nano Research 2010年第11期3卷 813-821页

作者： Haegyeom Kim Sung-Wook Kim Young-Uk Park Hyeokjo Gwon Dong-Hwa Seo Yuhee Kim Kisuk Kang Graduate School of Energy EnvironmentWaterand SustainabilityKorea Advanced Instituteof Science and Technology(KAIST)335 GwahangnoYuseong-guDaejeon 305-701Republic of Korea Department of Materials Science and Engineering KAIST335 GwahangnoYuseong-guDaejeon 305-701Republic of Korea KAIST Institute for Eco-energy NanocenturyKAIST335 GwahangnoYuseong-guDaejeon 305-701Republic of Korea Korea Institute of Science and Technology(KIST) 39-1 Hawolgok-dongWolsong-gil 5Seongbuk-guSeoul 136-791Republic of Korea

SnO_(2)/graphene nanocomposites have been fabricated by a simple chemical *** the fabrication process,the control of surface charge causes echinoid-like SnO_(2)nanoparticles to be formed and uniformly decorated on the *** electrostatic attraction between a graphene nanosheet(GNS)and the echinoid-like SnO_(2)particles under controlled pH creates a unique nanostructure in which extremely small SnO_(2)particles are uniformly dispersed on the *** SnO_(2)/graphene nanocomposite has been shown to perform as a high capacity anode with good cycling behavior in lithium rechargeable *** anode retained a reversible capacity of 634 mA·h·g^(–1)with a coulombic efficiency of 98%after 50 *** high reversibility can be attributed to the mechanical buffering by the GNS against the large volume change of SnO_(2)during delithiation/lithiation ***,the power capability is significantly enhanced due to the nanostructure,which enables facile electron transport through the GNS and fast delithiation/lithiation reactions within the echinoid-like nano-SnO_(2).The route suggested here for the fabrication of SnO_(2)/graphene hybrid materials is a simple economical route for the preparation of other graphene-based hybrid materials which can be employed in many different fields.

关键词： Graphene SnO_(2) surface charge nanocomposite rechargeable batteries lithium

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Numerical characterization of heat transfer in closed-loop vertical ground heat exchanger

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Science China(Technological Sciences) 2010年第1期53卷 111-116页

作者： Chulho LEE Hujeong GIL Hangseok CHOI Shin-Hyung KANG School of Civil Environmental and Architectural EngineeringKorea University5-GaAnam-DongSeongbuk-GuSeoul 136-713Republic of Korea Pyungsan SI Co. Ltd.1337-31 Seocho-DongSeocho-GuSeoul 137-860Republic of Korea Department of Mechanical Engineering Konyang University119Deahak-RoNonsanChungnam 320-711Republic of Korea

A series of numerical analyses has been performed on the characteristics of heat transfer in a closed-loop vertical ground heat exchanger(U-loop).A 2-D finite element analysis was conducted to evaluate the temperature distribution over the cross section of the U-loop system involving high-density polyethylene(HDPE) pipe/grout/soil to compare the sectional efficiency between the conventional U-loop and a new latticed HDPE pipe system,which is equipped with a thermally insulating lattice in order to reduce thermal interference between the inlet and outlet *** addition,a 3-D finite volume analysis(FLUENT) was adopted to simulate the operation of the closed-loop vertical ground heat exchanger with the consideration of the effect of a distance between the inlet and outlet pipes,grout's thermal properties,the effectiveness of the latticed HDPE pipe system,and the rate of circulation *** was observed that the thermal interference between the two strands of U-loop is of importance in enhancing efficiency of the ground heat ***,it is recommended to modify the configuration of the conventional U-loop system by equipping the thermally insulating lattice between the two pipe strands.

关键词： ground heat exchanger HDPE pipe latticed pipe sectional efficiency

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Compensating the impurities on the Cu surface by MOFs for enhanced hydrocarbon production in the electrochemical reduction of carbon dioxide

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Journal of Energy Chemistry 2022年第3期31卷 68-73,I0003页

作者： Shin Joon Kang Jong Ho Won Hansaem Choi Woohyeong Sim Mun Kyoung Kim Siraj Sultan Youngkook Kwon Hyung Mo Jeong School of Mechanical Engineering and Department of Smart Fab.Technology Sungkyunkwan University2066 Seobu-roJangan-guSuwon 16419Republic of Korea Department of Chemistry Kookmin University77 Jeongneung-roSeongbuk-guSeoul 02707Republic of Korea School of Energy and Chemical Engineering Emergent Hydrogen Technology R&D CenterUlsan National Institute of Science and Technology50 UNIST-gilUlsan 44919Republic of Korea

Copper(Cu)provides a cost-effective means of producing value-added fuels through the electrochemical reduction of carbon dioxide(CO_(2)RR).However,we observed the production of hydrocarbons via CO_(2)RR on commercial Cu films is less efficient because of the surface impurities,i.e.,*** monoxide(CO),a reaction intermediate of CO_(2)RR to hydrocarbons,binds strongly to the Fe sites and interrupts the production of hydrocarbons,resulting in an active hydrogen evolution reaction(HER).Herein,we report a method of blocking the effect of Fe impurities on the Cu surface through the preferential growth of nano-sized metal-organic frameworks(MOFs)on Fe *** zirconium(Zr)-based MOFs(UiO-66)forms a compensating layer on Cu film via the terephthalic acid(TPA)-Fe coordination bond,the Ui O-66 coated Cu film(UiO-66@Cu)presents significantly improved hydrocarbon Faradaic efficiency(FE)of 37.59%compared to 14.68%FE on commercial Cu film(99.9%purity)by suppressing *** to X-ray photoelectron spectroscopy(XPS)analysis,the UiO-66 ligand binds to entire metallic Fe site on the Cu surface,while metallic Cu is ***,UiO-66@Cu provides active sites of Cu for CO_(2)RR and leads to highly efficient and selective production of hydrocarbons.

关键词： Impurity on Cu film Zr-based MOFs Electrocatalysts CO_(2)reduction Hydrocarbon

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Micro Manipulation Using Magnetic Microrobots

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Journal of Bionic Engineering 2016年第4期13卷 515-524页

作者： Hoyeon Kim Jamel Ali U Kei Cheang Jinwoo Jeong din Seok Kim Min dun Kim Department of Mechanical Engineering Southern Methodist University Dallas TX75272 USA Department of MechanicaI Engineering and Mechanics Drexel University Philadelphia PA 19104 USA Center for Bionics Korea Institute of Science and Technology 5 Hwarang-ro 14-gil Seongbuk-gu Seou102792 Republic of Korea

When developing microscale robotic systems it is desired that they are capable of performing microscale tasks such as small scale manipulation and transport. In this paper, we demonstrate the transport of microscale objects using single or multiple microrobots in low Reynolds number fluidic environment. The microrobot is composed of a ‘U＇ shaped SU-8 body, coated on one side with nickel. Once the nickel coating is magnetized, the motion of the microrobots can be driven by external magnetic fields. To invoke different responses from two microrobots under a global magnetic field, two batches of microrobots were fabricated with different thicknesses of nickel coating as a way to promote heterogeneity within the microrobot population. The heterogeneity in magnetic content induces different spatial and temporal responses under the same control input, resulting in differences in movement speed. The nickel coated microstructure is manually controlled through a user interface developed using C＋＋. This paper presents a control strategy to navigate the microrobots by controlling the direction and strength of ex- ternally applied magnetic field, as well as orientation of the microrobots based on their polarity. In addition, multiple micro- robots are used to perform transport tasks.

关键词： microrobot magnetic control microtransport magnetic polarity micromanipulation

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Improved photocatalytic activity of surface charge functionalized ZnO nanoparticles using aniline

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Journal of Materials Science & Technology 2021年第17期76卷 1-10页

作者： Chatchai Rodwihok Korakot Charoensri Duangmanee Wongratanaphisan Won Mook Choi Seung Hyun Hur Hyun Jin Park Jin Suk Chung School of Chemical Engineering University of Ulsan680-749.South ICorea Department of Biotechnology College of Life Sciences andBiotechnologyKorea University145 Anam-roSeongbuk-guSeoul02841South Korea Research Center in Physics andAstronomy Faculty of ScienceChiang Mai UniversityChiang Mai50200Thailand

Functionalization of aniline molecules on zinc oxide(ZnO)nanoparticles is reported using a simple impregnation *** ZnO samples were systematically characterized based on morphology,surface and optical properties,and photocatalytic performance towards methyl orange(MO).Aniline functionalization increased the surface charge of the modified *** to pristine ZnO,the aniline-functionalized ZnO yielded faster photodegradation of MO,degrading 98.29%of MO in 60 min and superoxide radicals were the major species during the MO photodegradation *** results indicate that the improvement of photocatalytic degradation could be attributed to opposite charge-induced surface ***,protonated amine as a positively charged molecule was expected to increase the surface adsorption of MO(as an anionic dye)on ZnO nanoparticles surfaces,thereby increasing their photocatalytic degradation performance.

关键词： Photocatalysts Surface charge ZnO Aniline Methyl orange

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Investigation of the sodium storage mechanism of iron fluoride hydrate cathodes using X-ray absorption spectroscopy and mossbauer spectroscopy

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Journal of Energy Chemistry 2023年第2期77卷 535-542,I0014页

作者： Ghulam Ali Muhammad Akbar Faiza Jan Iftikhar Qamar Wali Beata Kalska Szostko Dariusz Satuła Kyung Yoon Chung Energy Storage Research Center Korea Institute of Science and TechnologyHwarang-ro 14 gil 5Seongbuk-guSeoul 02792South Korea USPCAS-E National University of Sciences and Technology(NUST)H-12Islamabad 44000Pakistan Division of Energy&Environment Technology KIST SchoolKorea University of Science and Technology(UST)Hwarang-ro 14-gil-5Seongbuk-guSeoul 02792South Korea NUTECH School of Applied Sciences and Humanities National University of TechnologyIslamabad 44000Pakistan University of Białystok Faculty of ChemistryCiołkowskiego 1K15-424 BiałystokPoland University of Białystok Faculty of PhysicsCiołkowskiego 1L15-424 BiałystokPoland

Elucidation of a reaction mechanism is the most critical aspect for designing electrodes for highperformance secondary ***,we investigate the sodium insertion/extraction into an iron fluoride hydrate(FeF_(3)·0.5H_(2)O)electrode for sodium-ion batteries(SIBs).The electrode material is prepared by employing an ionic liquid 1-butyl-3-methylimidazolium-tetrafluoroborate,which serves as a reaction medium and precursor for F^(-)*** crystal structure of FeF_(3)·0.5H_(2)O is observed as pyrochlore type with large open 3-D tunnels and a unit cell volume of 1129A^(3).The morphology of FeF_(3)·0.5H_(2)O is spherical shape with a mesoporous *** microstructure analysis reveals primary particle size of around 10 *** FeF_(3)·0.5H_(2)O cathode exhibits stable discharge capacities of 158,210,and 284 mA h g^(-1) in three different potential ranges of 1.5-4.5,1.2-4.5,and 1.0-4.5 V,respectively at 0.05 C *** specific capacities remained stable in over 50 cycles in all three potential ranges,while the rate capability was best in the potential range of 1.5-4.5 *** electrochemical sodium storage mechanism is studied using X-ray absorption spectroscopy,indicating higher conversion at a more discharged ***-situ M?ssbauer spectroscopy strengthens the results for reversible reduction/oxidation of *** results will be favorable to establish high-performance cathode materials with selective voltage window for SIBs.

关键词： Iron fluoride Sodium-ion batteries Pyrochlore X-ray absorption spectroscopy Mössbauer spectroscopy

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Evaluation of model fidelity for solar analysis in the context of distributed PV integration at urban scale

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Building Simulation 2022年第1期15卷 3-16页

作者： Wei Liao Shen Xu Yeonsook Heo School of Architecture South China University of Technology381 Wushan RoadGuangzhou510640China School of Architecture and Urban Planning Huazhong University of Science and Technology1037 Luoyu RoadWuhan430074China School of Civil Environmental and Architectural EngineeringKorea University145 Anam-roSeongbuk-guSeoul 02841Republic of Korea

This paper examines the level of model fidelity required to support design phases in the urban solar planning *** two modelling features crucial to the fidelity of the photovoltaic(PV)yield prediction on urban surfaces are(1)a level of fidelity for modelling urban shading and solar reflection and(2)a level of fidelity for modelling PV system *** paper compares three different models for predicting urban shading and reflection and two different PV models for predicting PV system *** relevance of the model fidelities is investigated through a case study of an urban area in Wuhan,China under three decision-making contexts:setting a solar target,place-making,and economic assessment for urban-scale distributed PV *** for the decision-makings are generated using the selected models through computational simulation under the same annual weather *** results show that the relatively less accurate canyon-based method tends to overpredict with 57 buildings identified as suitable for PV installation for walls in the studied urban area;the more accurate vector-based model predicts only 14 suitable *** results predicted with additional consideration of dynamic PV system operation exhibit differences from those predicted by the static PV system model,with a difference of roughly 13 buildings on average within each payback-time *** differences are noticeable but can be regarded as incremental for urban-scale economic assessment compared with the significant difference due to the fidelity level of modelling urban shading and reflection.

关键词： urban-scale solar analysis distributedPVintegration urban shading prediction PV system model

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Impacts of low-intensity prescribed fire on microbial and chemical soil properties in a Quercus frainetto forest

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Journal of Forestry Research 2018年第3期29卷 683-692页

作者： Serdar Akburak Yowhan Son Ender Makineci Meric Cakir Faculty of Forestry Soil Science and Ecology DepartmentIstanbul University34473 BahcekoySariyerIstanbulTurkey Division of Environmental Science and Ecological Engineering Korea University145 Anam-roSeongbuk-guSeoul 136-713Korea Faculty of Forestry Soil Science and Ecology DepartmentCankiri Karatekin University18100 CankkiriTurkey

Prescribed fire is a common economical and effective forestry practice, and therefore it is important to understand the effects of fire on soil properties for better soil management. We investigated the impacts of low-intensity prescribed fire on the microbial and chemical properties of the top soil in a Hungarian oak(Quercus frainetto Ten.) forest. The research focused on microbial soil parameters(microbial soil respiration(RSM), soil microbial biomass carbon(Cmic) and metabolic quotient(qCO2) and chemical topsoil properties(soil acidity(pH),electrical conductivity(EC), carbon(C), nitrogen(N), C/N ratio and exchangeable cations). Mean annual comparisons show significant differences in four parameters(C/N ratio,soil pH, Cmic and qCO2) while monthly comparisons do not reveal any significant differences. Soil pH increased slightly in the burned plots and had a significantly positive correlation with exchangeable cations Mg, Ca, Mn and *** mean annual C/N ratio was significantly higher in the burned plots(28.5:1) than in the control plots(27.0:1). The mean annual Cmic(0.6 mg g-1) was significantly lower although qCO2(2.5 lg CO2–C mg Cmic h-1) was significantly higher, likely resulting from the microbial response to fire-induced environmental stress. Low-intensity prescribed fire caused very short-lived changes. The annual mean values of C/N ratio, pH, Cmic and qCO2showed significant differences.

关键词： C/N Exchangeable cations Microbial biomass carbon qCO_2 Soil pH

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High-performance solid-solution potassium-ion intercalation mechanism of multilayered turbostratic graphene nanosheets

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Journal of Energy Chemistry 2022年第4期31卷 814-823页

作者： Jiae Um Seung Uk Yoon Hoseong Kim Beom Sik Youn Hyoung-Joon Jin Hyung-Kyu Lim Young Soo Yun Program in Environmental and Polymer Engineering Inha Universityncheon 22212 South Korea Department of Polymer Science and Engineering Inha UniversityIncheon 22212South Korea Division of Chemical Engineering and Bioengineering Kangwon National University Chuncheon Gangwon-do 24341 South Korea KU-KIST Graduate School of Converging Science and Technologyea University 145 Anam-roSeongbuk-guSoul02841 South Korea Department of Integrative Energy Engineering 145 Anam-roSongbuk-guKorea UniversitySeoul 02841 South Korea

The solid-solution reaction between an alkali cation and an active host material is known as a singlephase redox mechanism,and it is typically accompanied by a continuous voltage *** is distinct from the typical alkali cation intercalation reaction at an equivalent site of the active host material,which exhibits a voltage ***,we report an unusual solid-solution potassium-ion intercalation mechanism with a low-voltage plateau capacity on multilayered turbostratic graphene nanosheets(T-GNSs).Despite the disordered graphitic structure with a broad range of d-spacings(3.65–4.18À),the T-GNSs showed a reversible plateau capacity of~200 m A h g^(-1),which is higher than that of a well-ordered graphite nanoplate(~120 m A h g^(-1)).In addition,a sloping capacity of~220 m A h g^(-1)was delivered with the plateau capacity,and higher rate capabilities,better reversibility,and a more stable cycling performance were confirmed on the turbostratic ***-principles calculations suggest that the multitudinous lattice domains of the T-GNSs contain diverse intercalation sites with strong binding energies,which could be the origin of the high-performance solid-solution potassium-ion intercalation behavior when the turbostratic graphene stacks have a d-spacing smaller than that of equilibrium potassium–graphite intercalation compounds(5.35À).

关键词： Turbostratic graphite Graphene nanosheet Defective carbon Anode Potassium-ion batteries

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