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Rare Metals 2024年第2期43卷 647-657页

作者： Chuan Ou Ming-Dong Tan Zhen-Bang Li Zhao-Jie Li Fei Tian Zheng-Ping Qiao Dan-Ni Lei Cheng-Xin Wang State Key Laboratory of Optoelectronic materials and Technologies School of Materials Science and EngineeringSun Yat-Sen UniversityGuangzhou510275China

Owing to its high theoretical capacity and low cost,Sn has attracted significant attention in sodium-ion ***,the slow kinetics of electrochemical reactions and the rapid decay of capacity resulting from drastic changes in the volume of Sn,as well as persistent side reactions between Sn and the organic electrolyte during the(de)sodium process,have limited its *** improve the electrochemical performance of Sn-based materials,the bottom-up method is normally used to prepare carbon-coated ***,its complex preparation processes and harsh conditions make it unsuitable for practical ***,a carbon-coated hybrid crystal composite(Sn/SnO_(x)@C)was prepared using an up-bottom method with commercial Sn/SnO *** effects accelerate the electrochemical kinetics and inhibit the coarsening of Sn *** Sn/SnO_(x)@C composite electrode exhibited capacity retention of 80.7%even after approximately 1000 cycles(360.4 mAh·g^(−1)) at a current density of 1 A·g^(−1).The high-load Na_(3)V_(2)(PO4)3||Sn/SnO_(x)@C full cell presents a capacity retention rate of 91.7%after 150 cycles at the current density of 0.5 A·g^(−1).This work may significantly accelerate the commercialization of the Sn/SnO_(x)@C composite in sodium-ion batteries with high energy density.

关键词： Sodium-ion batteries(SIBs) Sn-based anode Ultraviolet curing Up-bottom method

Enhanced piezoelectric performance of Cr/Ta non-equivalent co-doped Bi_(4)Ti_(3)O_(12)-based high-temperature piezoceramics

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Journal of Advanced Ceramics 2024年第3期13卷 263-271页

作者： Xuanyu Chen Ziqi Ma Bin Li Yejing Dai school of materials Sun Yat-sen UniversityShenzhen 518107China

In this study,(Cr_(1/3)/Ta_(2/3))non-equivalent co-doped Bi_(4)Ti_(3)O_(12)(BIT)ceramics were prepared to solve the problem that high piezoelectric performance,high Curie temperature,and high-temperature resistivity could not be achieved simultaneously in BIT-based ceramics.A series of Bi_(4)Ti_(3-x)(Cr_(1/3)Ta_(2/3))_(x)O_(12)(x=0-0.04)ceramics were synthesized by the solid-state reaction *** phase structure,microstructure,piezoelectric performance,and conductive mechanism of the samples were systematically *** B-site non-equivalent co-doping strategy combining high-valence Ta^(5+)and low-valence Cr^(3+)significantly enhances electrical properties due to a decrease in oxygen vacancy ***_(4)Ti_(2.97)(Cr_(1/3)Ta_(2/3))_(0.03)O_(12)ceramics exhibit a high piezoelectric coefficient(d_(33)=26 pC·N^(-1))and a high Curie temperature(TC=687℃).Moreover,the significantly increased resistivity(ρ=2.8×10^(6)Ω·cm at 500℃)and good piezoelectric stability up to 600℃are also obtained for this *** the results demonstrate that Cr/Ta co-doped BIT-based ceramics have great potential to be applied in high-temperature piezoelectric applications.

关键词： high temperature piezoelectricity co-doped Bi_(4)Ti_(3)O_(12)(BIT)

Research on Pulsar Time Steered Atomic Time Algorithm Based on DPLL

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Research in Astronomy and Astrophysics 2024年第3期24卷 237-248页

作者： Ze-Hao Zheng Yang Liu Dan Shen Fan Feng Jiu-Long Liu Yue-Xin Ma Xiang-Wei Zhu school of Electronic and Communication engineering Sun Yat-sen UniversityShenzhen 518107China school of Aeronautics and Astronautics Sun Yat-sen UniversityShenzhen 518107China school of Systems science and engineering Sun Yat-sen UniversityGuangzhou 510275China

In today’s society,there is a wide demand for high-precision and high-stability time service in the fields of electric power,communication,transportation and *** present,the time standard in various countries is mainly based on atomic clocks,but the frequency drift of atomic clocks will affect the long-term stability *** with atomic clocks,millisecond pulsars have better long-term stability and can complement with the excellent short-term stability of atomic *** order to improve the long-term stability of the atomic timescale,and then improve the timing accuracy,this paper proposes an algorithm for steering the atomic clock ensemble(ACE)by ensemble pulsar time(EPT)based on digital phase locked loop(DPLL).First,the ACE and EPT are generated by the ALGOS algorithm,then the ACE is steered by EPT based on DPLL to calibrate the long-term frequency drift of the atomic clock,so that the generated steered atomic time follows both the short-term stability characteristics of ACE and the long-term stability characteristics of EPT,and finally,the steered atomic time is used to calibrate the local cesium *** experimental results show that the long-term stability of atomic time after steering is improved by 2 orders of magnitude compared with that before steering,and the daily drift of a local cesium clock after calibration is less than 9.47 ns in 3 yr,3 orders of magnitude higher than that before calibration on accuracy.

关键词： (stars) pulsars general-time-methods data analysis-instabilities

HTDcr:a job execution framework for high-throughput computing on supercomputers

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science China(Information sciences) 2024年第1期67卷 69-85页

作者： Jiazhi JIANG Dan HUANG Hu CHEN Yutong LU Xiangke LIAO school of Computer science and engineering Sun Yat-sen University school of Software engineering South China University of Technology

High-throughput computing(HTC) is a computing paradigm that aims to accomplish jobs by easily breaking them into smaller,independent ***,it requires a large amount of computing power for a long *** existing HTC frameworks are job-oriented without support for coscheduling with hardware architecture and task-level ***,most of the frameworks reach a limited scale,and their usability needs further ***,we present HTDcr,a job execution framework for the HTC on *** study aims to improve the throughput,task dispatching,and usability of the *** detail,the throughput optimizations include a sophisticated designed task management system,a hierarchical scheduler,and the co-optimization of the task-scheduling strategy with the application and hardware *** optimizations for usability include a programable execution workflow,mechanisms for more robust and reliable service qualities,and a fine-grained resource allocation system for the colocation of multiple *** to our evaluations,HTDcr can achieve outstanding scalability and high throughput on large-scale clusters for the HTC *** evaluate HTDcr with several microbenchmarks and real-world applications on Tianhe-2 and sunway TaihuLight to demonstrate its effects on existing design *** instance,the task scheduling for two real-world applications integrated with the application and hardware characteristics achieves 1.7× and 1.9× speedups over the basic task-scheduling strategy.

关键词： high-throughput computing supercomputer task scheduling middleware password guessing

MIDNet:Deblurring Network for Material Microstructure Images

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Computers, materials & Continua 2024年第4期79卷 1187-1204页

作者： Jiaxiang Wang Zhengyi Li Peng Shi Hongying Yu Dongbai sun National Center for materials Service Safety University of Science and Technology BeijingBeijing100083China school of materials Sun Yat-Sen UniversityShenzhen518107China school of materials science and engineering Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai)Sun Yat-Sen UniversityGuangzhou510006China

Scanning electron microscopy(SEM)is a crucial tool in the field of materials science,providing valuable insightsinto the microstructural characteristics of ***,SEM images often suffer from blurrinesscaused by improper hardware calibration or imaging automation errors,which present challenges in analyzingand interpretingmaterial ***,rectifying the blurring of these images assumes paramountsignificance to enable subsequent *** address this issue,we introduce a Material Images DeblurringNetwork(MIDNet)built upon the foundation of the Nonlinear Activation Free Network(NAFNet).MIDNetis meticulously tailored to address the blurring in images capturing the microstructure of *** keycontributions include enhancing the NAFNet architecture for better feature extraction and representation,integratinga novel soft attention mechanism to uncover important correlations between encoder and decoder,andintroducing newmulti-loss functions to improve training effectiveness and overallmodel *** conducta comprehensive set of experiments utilizing the material blurry dataset and compare them to several state-of-theartdeblurring *** experimental results demonstrate the applicability and effectiveness of MIDNet in thedomain of deblurring material microstructure images,with a PSNR(Peak Signal-to-Noise Ratio)reaching 35.26 dBand an SSIM(Structural Similarity)of *** dataset is available at:https://***/woshigui/MIDNet.

关键词： Image deblurring material microstructure attention mechanism deep learning

Laser-Induced Methanol Decomposition for Ultrafast Hydrogen Production

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Research 2024年第1期2023卷 131-137页

作者： Weiwei Cao Yinwu Li Bo Yan Zhiping Zeng Pu Liu Zhuofeng Ke Guowei Yang State Key Laboratory of Optoelectronic materials and Technologies Nanotechnology Research CenterSun Yat-sen UniversityGuangzhou 510275P.R.China school of materials science and engineering Sun Yat-sen UniversityGuangzhou 510275P.R.China

Methanol(CH_(3)OH)is a liquid hydrogen(H_(2))source that effectively releases H_(2) and is convenient for *** thermocatalytic CH_(3)OH reforming reaction is used to produce H_(2),but this process needs to undergo high reaction temperature(e.g.,200℃)along with a catalyst and a large amount of carbon dioxide(CO_(2))*** photocatalysis and photothermal catalysis under mild conditions are proposed to replace the traditional thermal catalysis to produce H_(2) from CH_(3)OH,they still inevitably produce CO_(2) emissions that are detrimental to carbon ***,we,for the first time,report an ultrafast and highly selective production of H_(2) without any catalysts and no CO_(2) emission from CH_(3)OH by laser bubbling in liquid(LBL)at room temperature and atmospheric pressure.

关键词： catalysis reforming replace

Changes of nutrients and microbial communities in recovery process of abandoned rare earth tailings

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Pedosphere 2024年第4期34卷 826-836页

作者： Bing ZHANG Junli WU Mengyuan HUANG Yan ZHANG Jin ZHAO Chuntao HE Zhongyi YANG school of Environmental science and engineering Sun Yat-sen UniversityGuangzhou 510006China school of Life sciences Sun Yat-sen UniversityGuangzhou 510275China school of Agriculture State Key Laboratory for BiocontrolShenzhen Campus of Sun Yat-sen UniversitySun Yat-sen UniversityShenzhen 518107China

Rare earth element(REE)mining has wrought severe ecosystem destruction,particularly in the loss of carbon(C),nitrogen(N),and phosphorus(P).Furthermore,its effects on nutrient recovery characteristics and associated microbial abundance are still poorly *** this study,an investigation was conducted to determine C,N,and P recovery patterns and microbial communities in abandoned REE mining tailings with different abandoned durations of 1.5(1.5-Y),7(7-Y),10(10-Y),and 14(14-Y)years and at an unmined site(the control group)in Jiangxi Province,*** tailing delamination at each site was investigated in 0–15(layer 1)and 15–30(layer 2)cm tailing *** the abandoned duration of REE tailings,C and P in layer 1 continued to recover from 1.62 to 8.51 g kg^(-1) and from 0.71 to 1.94 g kg^(-1),respectively;N losses of 0.60 and 0.22 g kg^(-1) occurred at the 1.5-Y and 10-Y sites,while N in layer 1 slightly increased at the 14-Y ***,Methylosinus,Bradyrhizobium,Pseudomonas,and Azospirillum were dominant bacteria at the 14-Y site and in the *** relative abundances of N-fixing bacteria Mesorhizobium(32.94%),Sinorhizobium(0.24%),Frankia(0.71%),and Burkholderia(2.38%)at the 14-Y site were 1.33–3.97 times those in the control(24.19%,0.18%,0.32%and 0.60%,respectively),which was helpful for tailing N *** the 14-Y site,Tylospora(50.24%),Luellia(11.02%),Tomentella(6.94%),and Chaetomium(4.34%)were the dominant fungal genera,while Tylospora(56.93%),Suillus(11.45%),and Penicillium(6.78%)predominated in the *** relative abundance of the P-dissolving fungus Aspergillus at the 14-Y site(0.42%)was 4.2 times that in the control(0.1%),which may lead to the improved tailing P *** the 14-Y site,woody plants such as Pinus massoniana and native pioneering herbs and ferns such as Dicranopteris dichotoma and Nephrolepis auriculata probably invaded from adjacent *** study unraveled the natural restoration of plant and micro

关键词： abandoned duration mining tailing N-fixing bacteria nutrient recovery P-solubilizing fungi rare earth element

Multichannel microneedle dry electrode patches for minimally invasive transdermal recording of electrophysiological signals

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Microsystems & Nanoengineering 2024年第3期10卷 119-136页

作者： Zhengjie Liu Xingyuan Xu Shuang Huang Xinshuo Huang Zhibo Liu Chuanjie Yao Mengyi He Jiayi Chen Hui-jiuan Chen Jing Liu Xi Xie State Key Laboratory of Optoelectronic materials and Technologies School of Electronics and Information TechnologyGuangdong Province Key Laboratory of Display Material and TechnologySun Yat-Sen UniversityGuangzhouChina school of Biomedical engineering Sun Yat-Sen UniversityGuangzhouChina The First Affiliated Hospital of sun yat-sen university GuangzhouChina

The collection of multiple-channel electrophysiological signals enables a comprehensive understanding of the spatial distribution and temporal features of electrophysiological *** approach can help to distinguish the traits and patterns of different ailments to enhance diagnostic *** array electrodes,which can penetrate skin without pain,can lessen the impedance between the electrodes and skin;however,current microneedle methods are limited to single channels and cannot achieve multichannel collection in small ***,a multichannel(32 channels)microneedle dry electrode patch device was developed via a dimensionality reduction fabrication and integration approach and supported by a self-developed circuit system to record weak electrophysiological signals,including electroencephalography(EEG),electrocardiogram(ECG),and electromyography(EMG)*** microneedles reduced the electrode–skin contact impedance by penetrating the nonconducting stratum corneum in a painless *** multichannel microneedle array(MMA)enabled painless transdermal recording of multichannel electrophysiological signals from the subcutaneous space,with high temporal and spatial resolution,reaching the level of a single microneedle in terms of signal *** MMA demonstrated the detection of the spatial distribution of ECG,EMG and EEG signals in live rabbit models,and the microneedle electrode(MNE)achieved better signal quality in the transcutaneous detection of EEG signals than did the conventional flat dry electrode *** work offers a promising opportunity to develop advanced tools for neural interface technology and electrophysiological recording.

关键词： needle rabbit electrode

Structural transition,electric transport,and electronic structures in the compressed trilayer nickelate La4Ni3O10

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science China(Physics,Mechanics & Astronomy) 2024年第11期Mechanics & Astronomy) .卷 13-19页

作者： Jingyuan Li Cui-Qun Chen Chaoxin Huang Yifeng Han Mengwu Huo Xing Huang Peiyue Ma Zhengyang Qiu Junfeng Chen Xunwu Hu Lan Chen Tao Xie Bing Shen Hualei sun Dao-Xin Yao Meng Wang Center for Neutron science and Technology Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices School of Physics Sun Yat-sen University Center for materials of the Universe School of Molecular Sciences Arizona State University school of sciences Sun Yat-sen University

Atomic structure and electronic band structure are fundamental properties for understanding the mechanism of superconductivity. Motivated by the discovery of pressure-induced high-temperature superconductivity at 80 K in the bilayer Ruddlesden-Popper nickelate La3Ni2O7, the atomic structure and electronic band structure of the trilayer nickelate La4Ni3O10under pressure up to 44.3 GPa are investigated. A structural transition from the monoclinic P21/a space group to the tetragonal I4/mmm around 12.6-13.4 GPa is identified, accompanied by a drop of resistance below 7 K. Density functional theory calculations suggest that the bonding state of Ni 3dz2orbital rises and crosses the Fermi level at high pressures, which may give rise to possible superconductivity observed in resistance under pressure in La4Ni3O10. The trilayer nickelate La4Ni3O10shows some similarities with the bilayer La3Ni2O7and has unique properties, providing a new platform to investigate the underlying mechanism of superconductivity in nickelates.

关键词： La4Ni3O10 high pressure synchrotron X-ray diffraction structural transition DFT calculations

Boosting the cycling stability of all-solid-state lithium metal batteries through MOF-based polymeric protective layers

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Journal of Energy Chemistry 2024年第8期95卷 511-518,I0011页

作者： Hongfei Bao Diancheng Chen Jiaqi Cao Pengfeng Jiang Kaili Li Runtao Liu Yuling Zhao Yichun Zheng Beiqi Liao Yaming Zhang Xia Lu Yang sun school of materials Shenzhen Campus of Sun Yat-sen UniversityShenzhen 518107GuangdongChina

Solid-state electrolytes(SSEs)play a pivotal role in advancing next-generation lithium metal battery ***,they commonly encounter substantial interfacial resistance and poor stability when interfacing with lithium metal,hindering practical ***,we introduce a flexible metal-organic framework(MOF:NUS-6)-incorporated polymeric layer,denoted as NP,designed to protect the sodium superionic conductor(NASICON)-type Li_(1.3)Al_(0.3)Ti_(1.7)(PO_(4))_(3)(LATP)electrolyte from Li metal *** NP matrix establishes a soft interface with the LATP surface,effectively reducing voids and gaps that may arise between the LATP electrolyte and Li ***,the MOF component in NP enhances ionic conductivity,offers abundant Li^(+)transport sites,and provides hierarchical ion channels,ensuring a homogeneous Li^(+)flow and thus effectively inhibiting Li dendrite *** NP,we fabricate Li symmetrical cells cycled for over 1600 h at 0.2 mA cm^(-2)and all-solid-state LiINP-LATPI LiFePO_(4)batteries,achieving a remarkable 99.3%capacity retention after 200 cycles at 0.2 *** work outlines a general strategy for designing long-lasting and stable solid-state Li metal batteries.

关键词： All-solid-state Li metal battery MOF-based polymeric layer Li dendrite Interfacial contact LATP electrolyte stability