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Quantum synchronization with correlated baths

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Chinese Physics B 2024年第2期33卷 152-157页

作者：李磊王春辉尹洪浩王如泉刘伍明 school of Physical Science and Technology Inner Mongolia UniversityHohhot 010021China Beijing National Laboratory for Condensed matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China

We study quantum synchronization under the nonequilibrium *** consider a two-qubit XXZ chain coupled independently to their own reservoirs modeled by the collisional *** reservoir particles,initially prepared in a thermal state or a state with coherence,are correlated through a unitary transformation and afterward interact locally with the two quantum *** study the quantum effect of reservoir on synchronous dynamics of *** preparing different reservoir initial states or manipulating the reservoir particles coupling and the temperature gradient,we find that quantum entanglement of reservoir is the key to control quantum synchronization of system qubits.

关键词： quantum synchronization entanglement quantum coherence nonequilibrium reservoir

Controlling of coordination state of Ru_(x)N_(y) clusters for efficient oxygen reduction electrocatalysis

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Nano research 2024年第3期17卷 1035-1041页

作者： Weiyang Fu Yihuan Yu Tongtong Liu Yinliang Cao Zhengping Zhang Feng Wang State Key Laboratory of Chemical Resource Engineering Beijing Key Laboratory of Electrochemical Process and Technology for MaterialsBeijing University of Chemical TechnologyBeijing 100029China Beijing Advanced Innovation Center for soft matter Science and Engineering Beijing University of Chemical TechnologyBeijing 100029China Zhejiang Tianneng Hydrogen Energy Technology Co. Ltd.Huzhou 313100China

Ruthenium(Ru)is an attractive potential alternative to platinum as an electrocatalyst for the oxygen reduction reaction(ORR),in virtue of its high catalytic selectivity and relatively low *** this work,a series of well-dispersed nitrogen-coordinated Ru-clusters on carbon black(Ru_(x)N_(y)/C)were prepared by pyrolyzing different Ru-containing sandwich compounds as the Ru *** higher thermal stability of these complexed sandwich precursors(bis(1,2,3,4,5-pentamethylcyclopentadienyl)Ru(II)monomer,dichloro(p-cymene)Ru(II)dimer,and chloro(1,2,3,4,5-pentamethylcyclopentadienyl)Ru(II)tetramer)affords the control of coordinated state for the resulting Ru-clusters,in comparison of that derived from ruthenium *** the pyrolysis treatment,the Ru coordinated state in Ru_(x)N_(y)/C,with the Ru–N and Ru–Ru bonds,still showed the structural inheritance from the Ru(II)monomer,dimer,and tetramer,but using ruthenium chlorides as the Ru source resulted in the nanoscale Ru *** ORR testing exhibited that the Ru_(x)N_(y)/C sample derived from the Ru(II)tetramer(Ru_(x)N_(y)/C-T)presents the higher catalytic activity than the other obtained samples in either alkaline or acidic *** in the acidic electrolyte,Ru_(x)N_(y)/C-T shows the comparable ORR activity to that of Pt/C catalysts,and it shows the superior tolerance against methanol and *** X-ray absorption spectroscopy and density functional theory calculations demonstrate that these tetra-nuclear Ru-clusters could be the most active site due to their broadened d-orbital bands and lower energy d-band center than those of other subnano species and nanocrystals,and their favorable Yeager-type adsorption of O_(2)-molecules is also contributed to promoting O–O bond cleavage and accelerating the ORR process.

关键词： ruthenium clusters coordination environment sandwich compounds electrocatalysis oxygen reduction reaction

Purification of copper foils driven by single crystallization

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Chinese Physics B 2024年第2期33卷 506-511页

作者：寇金宗赵孟泽李兴光何梦林杨方友刘科海成庆秋任云龙刘灿付莹吴慕鸿刘开辉王恩哥 Songshan Lake Materials Laboratory Dongguan 523808China Beijing National Laboratory for Condensed matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials School of PhysicsSouth China Normal UniversityGuangzhou 510006China Guangdong–Hong Kong Joint Laboratory of Quantum matter Frontier Research Institute for PhysicsSouth China Normal UniversityGuangzhou 510006China State Key Laboratory for Mesoscopic Physics Frontiers Science Center for Nano-optoelectronicsSchool of PhysicsPeking UniversityBeijing 100871China Key Laboratory of Quantum State Construction and Manipulation(Ministry of Education) Department of PhysicsRenmin University of ChinaBeijing 100872China International Center for Quantum Materials Collaborative Innovation Center of Quantum MatterPeking UniversityBeijing 100871China school of Physics Liaoning UniversityShenyang 110036China

High-purity copper(Cu) with excellent thermal and electrical conductivity, is crucial in modern technological applications, including heat exchangers, integrated circuits, and superconducting magnets. The current purification process is mainly based on the zone/electrolytic refining or anion exchange, however, which excessively relies on specific integrated equipment with ultra-high vacuum or chemical solution environment, and is also bothered by external contaminants and energy consumption. Here we report a simple approach to purify the Cu foils from 99.9%(3N) to 99.99%(4N) by a temperature-gradient thermal annealing technique, accompanied by the kinetic evolution of single crystallization of *** success of purification mainly relies on(i) the segregation of elements with low effective distribution coefficient driven by grain-boundary movements and(ii) the high-temperature evaporation of elements with high saturated vapor *** purified Cu foils display higher flexibility(elongation of 70%) and electrical conductivity(104% IACS) than that of the original commercial rolled Cu foils(elongation of 10%, electrical conductivity of ~ 100% IACS). Our results provide an effective strategy to optimize the as-produced metal medium, and therefore will facilitate the potential applications of Cu foils in precision electronic products and high-frequency printed circuit boards.

关键词： purification copper foil thermal annealing technique single crystallization

Metamaterial terahertz device with temperature regulation function that can achieve perfect absorption and complete reflection conversion of ultrawideband

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Communications in Theoretical Physics 2024年第7期76卷 125-135页

作者： Hao Sun Zao Yi Can Ma Shubo Cheng Bin Tang Qingdong Zeng Sohail Ahmad school of Mathematics and Science Joint Laboratory for Extreme Conditions Matter Properties State Key Laboratory of Environment-Friendly Energy Materials Tianfu Institute of Research and InnovationSouthwest University of Science and Technology Department of Oncology Sichuan Science City Hospital school of Chemistry and Chemical Engineering Jishou University school of Physics and Optoelectronic Engineering Yangtze University school of Microelectronics and Control Engineering Changzhou University school of Physics and Electronic Information Engineering Hubei Engineering University Institute of Physics Bahauddin Zakariya University

The field of terahertz devices is important in terahertz technology. However, most of the current devices have limited functionality and poor performance. To improve device performance and achieve multifunctionality, we designed a terahertz device based on a combination of VO2and metamaterials. This device can be tuned using the phase-transition characteristics of VO2, which is included in the triple-layer structure of the device, along with SiO2and Au. The terahertz device exhibits various advantageous features, including broadband coverage, high absorption capability, dynamic tunability, simple structural design, polarization insensitivity, and incidentangle insensitivity. The simulation results showed that by controlling the temperature, the terahertz device achieved a thermal modulation range of spectral absorption from 0 to 0.99. At 313 K, the device exhibited complete reflection of terahertz waves. As the temperature increased,the absorption rate also increased. When the temperature reached 353 K, the device absorption rate exceeded 97.7% in the range of 5–8.55 THz. This study used the effective medium theory to elucidate the correlation between conductivity and temperature during the phase transition of VO2. Simultaneously, the variation in device performance was further elucidated by analyzing and depicting the intensity distribution of the electric field on the device surface at different temperatures. Furthermore, the impact of various structural parameters on device performance was examined, offering valuable insights and suggestions for selecting suitable parameter values in real-world applications. These characteristics render the device highly promising for applications in stealth technology, energy harvesting, modulation, and other related fields, thus showcasing its significant potential.

关键词： complete reflection perfect absorption smart device temperature regulation terahertz ultrawideband

Black holes as the source of dark energy:A stringent test with high-redshift JWST AGNs

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Science China(Physics,Mechanics & Astronomy) 2024年第2期67卷 181-188页

作者： Lei Lei Lei Zu Guan-Wen Yuan Zhao-Qiang Shen Yi-Ying Wang Yuan-Zhu Wang Zhen-Bo Su Wen-Ke Ren Shao-Peng Tang Hao Zhou Chi Zhang Zhi-Ping Jin Lei Feng Yi-Zhong Fan Da-Ming Wei Key Laboratory of Dark matter and Space Astronomy Purple Mountain ObservatoryChinese Academy of SciencesNanjing 210023China school of Astronomy and Space Science University of Science and Technology of ChinaHefei 230026China CAS Key Laboratory for research in Galaxies and Cosmology Department of AstronomyUniversity of Science and Technology of ChinaHefei 230026China

Studies have proposed that there is evidence for cosmological coupling of black holes(BHs)with an index of k≈3;hence,BHs serve as the astrophysical source of dark ***,the data sample is limited for the redshifts of≤*** recent years,the James Webb Space Telescope(JWST)has detected many high-redshift active galactic nuclei(AGNs)and *** the JWST NIRSpec-/NIRCam-resolved AGNs,three are determined to be in early-type host galaxies with a redshift of z~***,their M_(*)and MBH are in tension with the predicted cosmological coupling of black holes with k=3 at a confidence level of~2σ,which challenges the hypothesis that BHs serve as the origin of dark *** work on high-redshift AGNs using the JWST will further assess such a hypothesis by identifying more early-type host galaxies in the higher mass range.

关键词： dark energy supermassive black hole active galactic nuclei James Webb Space Telescope

Engineering Shewanella-re duce d graphene oxide aerogel biohybrid to efficiently synthesize Au nanoparticles

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Journal of Materials Science & Technology 2024年第1期168卷 50-61页

作者： Baocai Zhang Shulin Shao Huan Yu Qijing Liu Sicheng Shi Qingyuan Wu Zijie Wu Yiyu Feng Yifei Wang Xi Sun Deguang Wu Feng Li Hao Song Frontier Science Center for Synthetic Biology and Key Laboratory of Systems Bioengineering(Ministry of Education) Tianjin UniversityTianjin 300072China Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China Beijing Advanced Innovation Center for soft matter Science and Engineering Beijing University of Chemical TechnologyBeijing 100029China school of Materials Science and Engineering Tianjin UniversityTianjin 300350China College of Biological Engineering Tianjin Agricultural UniversityTianjin 300384China Department of Brewing Engineering Moutai InstituteLuban AveRenhuai 564507China

Biosynthesizing Au nanoparticles(AuNPs)from gold-bearing scraps provides a sustainable method to meet the urgent demand for ***,it remains challenging to efficiently biosynthesize AuNPs of which the diameter is less than 10 nm from a trace amount of Au^(3+)concentration at the level of tens ***,we constructed an exoelectrogenic cell(eCell)-conductive reduced-graphene-oxide aero-gel(rGA)biohybrid by assembling Shewanella sp.S1(SS1)as living biocatalyst and rGA as conductive ad-sorbent,in which Au^(3+)at trace concentrations would be enriched by the adsorption of rGA and reduced to AuNPs through the extracellular electron transfer(EET)of *** regulate the size of the synthe-sized AuNPs to 10 nm,the strain SS1 was engineered to enhance its EET,resulting in strain RS2(pYYD-P tac-ribADEHC&pHG13-P_(bad)-omcC in SS1).Strain RS2 was further assembled with rGA to construct the RS2-rGA biohybrid,which could synthesize AuNPs with the size of 7.62±2.82 nm from 60 ppm Au^(3+)*** eCell-rGA biohybrid integrated Au^(3+)adsorption and reduction,which enabled AuNPs biosyn-thesis from a trace amount of Au^(3+).Thus,the required Au^(3+)ions concentration was reduced by one or two orders of magnitude compared with conventional methods of AuNPs *** work devel-oped an AuNPs size regulation technology via engineering eCell’s EET with synthetic biology methods,providing a feasible approach to synthesize AuNPs with controllable size from trace level of gold ions.

关键词： Au nanoparticles Exoelectrogenic cell(e-Cell) Shewanella Synthesis biology Extracellular electron transfer Reduced graphene oxide aerogel

Dynamic asymmetric mechanical responsive carbon nanotube fiber for ionic logic gate

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Chinese Chemical Letters 2024年第6期35卷 249-253页

作者： Pei Cao Yilan Wang Lejian Yu Miao Wang Liming Zhao Xu Hou State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province(IKKEM) Xiamen 361005China The Higher Educational Key Laboratory for Biomedical Engineering of Fujian Province Department of BiomaterialsResearch Center of Biomedical Engineering of XiamenCollege of MaterialsXiamen UniversityXiamen 361005China Key Laboratory of Multifunctional Nanomaterials and Smart Systems Advanced Materials DivisionSuzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China Institute of Artificial Intelligence Xiamen UniversityXiamen 361005China Department of Physics Research Institute for Biomimetics and Soft MatterFujian Provincial Key Laboratory for Soft Functional Materials ResearchJiujiang Research InstituteCollege of Physical Science and TechnologyXiamen UniversityXiamen 361005China Engineering research Center of Electrochemical Technologies of Ministry of Education Xiamen UniversityXiamen 361005China

Inspired by biological ion channels,numerous artificial asymmetric ion channels have been synthesized to facilitate the fabrication of ionic ***,the creation of biomimetic asymmetric ion channels necessitates expensive scientific apparatus and intricate material processing procedures,which constrains its advancement within the realm of ionic *** this study,we have devised dynamic asymmetric ion channels with mechanical responsiveness by combining polymers of varying elastic modulus along the longitudinal axis of carbon nanotube fiber(CNTF).The ion rectification can be modulated via the disparate response of CNTF-based ion channels to mechanical *** have effectively employed these asymmetric ion channels with mechanical sensitivity in the design of a logic gate device,achieving logic operations such as“AND”and“OR”.The conception of these dynamic asymmetric ion channels with mechanical sensitivity offers a straightforward,cost-effective,and versatile approach for generating ion channels,highlighting their potential application in intricate,highly integrated ionic circuits.

关键词： Carbon nanotubes fibers Mechanical response Rectification effect Ionic logic gate

Implementation of integrated nonlocal sensing for object shape and rotational speed

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Science China(Physics,Mechanics & Astronomy) 2024年第7期67卷 6-12页

作者： Zhenyu Guo Yunlong Wang Zehong Chang Jiawei Wang Junliang Jia Pei Zhang Ministry of Education Key Laboratory for Nonequilibrium Synthesis and Modulation of Condensed matter Shaanxi Province Key Laboratory of Quantum Information and Quantum Optoelectronic DevicesSchool of PhysicsXi’an Jiaotong UniversityXi’an 710049China

The expeditious acquisition of information pertaining to objects through the utilization of quantum technology has been a perennial issue of *** far,the efficient utilization of information from dynamic objects with limited resources remains a significant ***,we realize a nonlocal integrated sensing of the object's amplitude and phase information by combining digital spiral imaging with the correlated orbital angular momentum *** amplitude information is utilized for object identification,while the phase information enables us to determine the rotational *** demonstrate the nonlocal identification of a rotating object's shape,irrespective of its rotational symmetry,and introduce the concept of the correlated rotational Doppler effect,establishing a fundamental connection between this effect and the classical rotational Doppler effect,i.e.,that both rely on extracting crucial information from the spiral spectrum of *** present study highlights a promising pathway towards the realization of quantum remote sensing and imaging.

关键词： digital spiral imaging orbital angular momentum correlated rotational Doppler effect

A layered multifunctional framework based on polyacrylonitrile and MOF derivatives for stable lithium metal anode

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Journal of Energy Chemistry 2024年第6期93卷 282-288,I0007页

作者： Fanfan Liu Peng Zuo Jing Li Pengcheng Shi Yu Shao Linwei Chen Yihong Tan Tao Ma Engineering research Center of High-frequency soft Magnetic Materials and Ceramic Powder Materials of Anhui Province School of Chemistry and Material EngineeringChaohu UniversityHefei 238024AnhuiChina Frontiers Science Center for Transformative Molecules School of Chemistry and Chemical EngineeringShanghai Jiao Tong UniversityShanghai 200240China school of Pharmacy Anhui University of Chinese MedicineHefei 230012AnhuiChina school of Materials and Energy Guangdong University of TechnologyGuangzhou 510006GuangdongChina Jiujiang DeFu Technology Co. Ltd.Jiujiang 332000JiangxiChina

Composite Li metal anodes based on three-dimensional(3D) porous frameworks have been considered as an effective material for achieving stable Li metal batteries with high energy ***,uneven Li deposition behavior still occurs at the top of 3D frameworks owing to the local accumulation of Li *** promote uniform Li deposition without top dendrite growth,herein,a layered multifunctional framework based on oxidation-treated polyacrylonitrile(OPAN) and metal-organic framework(MOF) derivatives was proposed for rationally regulating the distribution of Li ions flux,nucleation sites,and electrical *** from these merits,the OPAN/carbon nano fiber-MOF(CMOF) composite framework demonstrated a reversible Li plating/stripping behavior for 500 cycles with a stable Coulombic efficiency of around 99.0% at the current density of 2 mA/cm~***,such a Li composite anode exhibited a superior cycle lifespan of over 1300 h under a low polarized voltage of 18 mV in symmetrical *** the Li composite anode was paired with LiFePO_(4)(LFP) cathode,the obtained full cell exhibited a stable cycling over 500 ***,the COMSOL Multiphysics simulation was conducted to reveal the effects on homogeneous Li ions distribution derived from the above-mentioned OPAN/CMOF framework and electrical insulation/conduction *** electrochemical and simulated results shed light on the difficulties of designing stable and safe Li metal anode via optimizing the 3D frameworks.

关键词： Lithium metal anode Layered multifunctional framework Ions flux redistribution Electrical insulation/conduction structure Uniform Li deposition