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Feasibility of Scaling up the Cost-Competitive and Clean Electrolytic Hydrogen Supply in China

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engineering 2024年第8期39卷 154-165页

作者： Guangsheng Pan Wei Gu Zhongfan Gu Jin Lin Suyang Zhou Zhi Wu Shuai Lu school of Electrical engineering Southeast UniversityNanjing 210096China Department of Electrical engineering Tsinghua UniversityBeijing 100084China

Scaling up clean hydrogen supply in the near future is critical to achieving China’s hydrogen development *** study established an electrolytic hydrogen development mechanism considering the generation mix and operation optimization of power systems with access to *** on the incremental cost principle,we quantified the provincial and national clean hydrogen production cost performance levels in *** results indicated that this mechanism could effectively reduce the production cost of clean hydrogen in most provinces,with a national average value of less than 2 USD·kg^(-1) at the 40-megaton hydrogen supply *** cooperation via power transmission lines could further reduce the production cost to 1.72 USD·kg^(-1).However,performance is affected by the potential distribution of hydrogen *** the supply side,competitiveness of the mechanism is limited to clean hydrogen production,while from the demand side,it could help electrolytic hydrogen fulfil a more significant *** study could provide a solution for the ambitious development of renewables and the hydrogen economy in China.

关键词： Low-carbon energy system Electrolytic hydrogen Renewables Cost optimization and analysis

Bioinformatics and Biomedical Computing

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Fundamental Research 2024年第4期4卷 713-714页

作者： Hongmin Cai Jiazhou Chen Fa Zhang Jianxin Wang The school of Computer Science and engineering South China University of TechnologyGuangzhou 510006China The school of Medical Technology Bejing Institute of TechnologyBejing 100081China The school of Computer Science and engineering Central South UniversityChangsha 410083China

The rapid advancement of high-throughput sequencing technologies and the explosive growth of biological data have revolutionized the field of bioinformatics and biomedical computing[1-4].The generation of vast amounts of genomic,transcriptomic,proteomic,and metabolomic data has created unprecedented opportunities for understanding the complexities of biological systems and their implications for human health[5-6].Moreover,the emergence of spatial omics technologies,such as spatial transcriptomics and spatial proteomics,has added a new dimension to our understanding of the spatial organization and heterogeneity of biological *** cutting-edge technologies enable the mapping of molecular information at a high spatial resolution,providing valuable insights into the tissue microenvironment and the interplay between cells in various physiological and pathological conditions[7-10].

关键词： enable dimension insight

Recent progress in functional metal-organic frameworks for bio-medical application

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Regenerative Biomaterials 2024年第2期3卷 37-54页

作者： Wenwen Chai Xiaochen Chen Jing Liu Liyan Zhang Chunyu Liu Li Li John Robert Honiball Haobo Pan Xu Cui Deping Wang school of Materials Science and engineering Tongji UniversityShanghai 201804China Shenzhen Institute of Advanced Technology Chinese Academy of SciencesShenzhen 518055China Department of Orthopaedics&Traumatology School of Clinical MedicineLi Ka Shing Faculty of MedicineThe University of Hong KongHong KongChina

Metal-organic frameworks(MOFs)have a high specific surface area,adjustable pores and can be used to obtain functional porous materials with diverse and well-ordered structures through coordination and self-assembly,which has intrigued wide interest in a broad range of *** the arena of biomedical engineering,the functionalized modification of MOFs has produced drug carriers with excellent dispersion and functionalities such as target delivery and response release,with promising applications in bio-detection,disease therapy,tissue healing,and other *** review summa-rizes the present state of research on the functionalization of MOFs by physical binding or chemical cross-linking of small *** *** hvdrogels and evaluates the role and approach of MOFs functionalization in boosting the reactivity of *** this basis,research on the application of functionalized MOFs composites in biomedical engineering fields such as drug delivery,tissue repair,disease treatment,bio-detection and imaging is surveyed,and the development trend and application prospects of functionalized MOFs as an important new class of biomedical materials in the biomedical field are anticipated,which may provide some inspiration and reference for further development of MOF for bio-medical applications.

关键词： metal-organic frameworks porous functionalization tissue repair disease treatment

Ru(Ⅱ)-Catalyzed Selective C-H Alkynylation of Isoquinolones,Quinazolones and Phthalazinones with Bromoalkynes

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Chinese Journal of Chemistry 2024年第15期42卷 1686-1690页

作者： Quan-Jian Luo Han-Chi Wang Jing Zhang Jin-Heng Li Bo Sun State Key Laboratory Base of Eco-Chemical engineering College of Chemical EngineeringQingdao University of Science and TechnologyQingdaoShandong 266042China State Key Laboratory of Applied Organic Chemistry Lanzhou UniversityLanzhouGansu 730000China school of Chemistry and Chemical engineering Henan Normal UniversityXinxiangHenan 453007China

A new,selective Ru(Ⅱ)-catalyzed alkynylation reaction of isoquinolones,quinazolones and phthalazinones with readily available bromoalkynes has been *** reaction enables the selective construction of a new C(sp^(2))-C(sp)bond through C-H activation and C-Br functionalization,and offers an effective and selective route to synthesizing highly valuable alkynylated isoquinolone,quinazolone and phthalazinonederivatives with a wide substrate scope and highselectivity.

关键词： Ru(Ⅱ) Alkynylation Isoquinolones Bromoalkynes Heterocyclic compounds C-H activation C-C coupling Synthetic methods

A review of anode materials for sodium ion batteries

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新型炭材料（中英文） 2024年第5期39卷 743-769页

作者： Syed Ali Riza XU Ri-gan LIU Qi Muhammad Hassan YANG Qiang MU Dao-bin LI Li WU Feng CHEN Ren-jie Beijing Key Laboratory of Environment Science and engineering School of Material Science and EngineeringBeijing Institute of TechnologyBeijing 100081China

Lithium-ion batteries(LIBs)are used in electric vehicles and portable smart devices,but lithium resources are dwindling and there is an increasing demand which has to be catered *** ion batteries(SIBs),which are less costly,are a promising replacement for LIBs because of the abundant natural reserves of *** anode of a SIB is a necessary component of the battery but is less understood than the *** review outlines the development of various types of anodes,including carbonbased,metallic and organic,which operate using different reaction mechanisms such as intercalation,alloying and conversion,and considers their challenges and *** for modifying their structures by doping and coating,and also modifying the solid electrolyte interface are *** addition,this review also discusses the challenges encountered by the anode of SIBs and the solutions.

关键词： Sodium ion batteries Anode Carbon material Metallic compound Organic

Two-dimensional particle-in-cell modeling of blow-off impulse by X-ray irradiation

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Nuclear Science and Techniques 2024年第3期35卷 53-69页

作者： Ruibo Li Jin-Long Jiao Hui Luo Dezhi Zhang Dengwang Wang Kai Wang Graduate school of China Academy of engineering Physics Beijing 100193China Zhejiang Institute of Modern Physics Institute of AstronomySchool of PhysicsZhejiang UniversityHangzhou 310027China National Key Laboratory of Intense Pulsed Radiation Simulation and Effect Northwest Institute of Nuclear TechnologyXi’an 710024China

Space objects such as spacecraft or missiles may be exposed to intense X-rays in outer space,leading to severe *** reinforcement of these objects to reduce the damage caused by X-ray irradiation is a significant *** blow-off impulse(BOI)is a crucial physical quantity for investigating material damage induced by X-ray ***,the accurate calculation of BOI is challenging,particularly for large deformations of materials with complex *** this study,we develop a novel two-dimensional particle-in-cell code,Xablation2D,to calculate BOIs under far-field X-ray *** significantly reduces the dependence of the numerical simulation on the grid *** reliability of this code is verified by simulation results from open-source codes,and the calculated BOIs are consistent with the experimental and analytical results.

关键词： X-ray irradiation Energy deposition Blow-off impulse Particle in cells

Toward Trustworthy Decision-Making for Autonomous Vehicles:A Robust Reinforcement Learning Approach with Safety Guarantees

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engineering 2024年第2期33卷 77-89页

作者： Xiangkun He Wenhui Huang Chen Lv school of Mechanical and Aerospace engineering Nanyang Technological UniversitySingapore 639798Singapore

While autonomous vehicles are vital components of intelligent transportation systems,ensuring the trustworthiness of decision-making remains a substantial challenge in realizing autonomous ***,we present a novel robust reinforcement learning approach with safety guarantees to attain trustworthy decision-making for autonomous *** proposed technique ensures decision trustworthiness in terms of policy robustness and collision ***,an adversary model is learned online to simulate the worst-case uncertainty by approximating the optimal adversarial perturbations on the observed states and environmental *** addition,an adversarial robust actor-critic algorithm is developed to enable the agent to learn robust policies against perturbations in observations and ***,we devise a safety mask to guarantee the collision safety of the autonomous driving agent during both the training and testing processes using an interpretable knowledge model known as the Responsibility-Sensitive Safety ***,the proposed approach is evaluated through both simulations and *** results indicate that the autonomous driving agent can make trustworthy decisions and drastically reduce the number of collisions through robust safety policies.

关键词： Autonomous vehicle Decision-making Reinforcement learning Adversarial attack Safety guarantee

Research progress and prospect of low-carbon biological technology for nitrate removal in wastewater treatment

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Frontiers of Environmental Science & engineering 2024年第7期18卷 1-21页

作者： Ru Zheng Kuo Zhang Lingrui Kong Sitong Liu College of Environmental Sciences and engineering Peking UniversityBeijing 100871China Key Laboratory of Water and Sediment Sciences Ministry of Education of ChinaBeijing 100871China Eco-Environment and Resource Efficiency Research Laboratory School of Environment and EnergyPeking University Shenzhen Graduate SchoolShenzhen 518055China

Wastewater treatment plants are the major energy consumers and significant sources of greenhouse gas emissions,among which biological nitrogen removal of wastewater is an important contributor to carbon ***,traditional heterotrophic denitrification still has the problems of excessive residual sludge and the requirement of external carbon ***,the development of innovative low-carbon nitrate removal technologies is *** review outlines the key roles of sulfur autotrophic denitrification and hydrogen autotrophic denitrification in low-carbon wastewater *** discovered nitrate/nitrite dependent anaerobic methane oxidation enables sustainable methane emission reduction and nitrogen removal by utilizing available methane in *** microorganisms exhibited a promising potential to achieve carbon-negative nitrate ***,the algal-bacterial symbiosis system and photogranules offer effective and prospective low-carbon options for nitrogen ***,the emerging nitrate removal technology of photoelectrotrophic denitrification and the underlying,photoelectron transfer mechanisms are ***,we summarize and prospect these technologies,highlighting that solar-driven biological nitrogen removal technology is a promising area for future sustainable wastewater *** review has important guiding significance for the design of low-carbon wastewater treatment systems.

关键词： Carbon emissions Low-carbon Biological nitrogen removal Denitrification

Enhancing MXene-based supercapacitors:Role of synthesis and 3D architectures

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Journal of Energy Chemistry 2024年第4期91卷 1-26页

作者： Wen Siong Poh Wen Jie Yiang Wee-Jun Ong Pau Loke Show Chuan Yi Foo school of Energy and Chemical engineering Xiamen University MalaysiaSelangor Darul EhsanMalaysia&College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005FujianChina Kelip-kelip!Center of Excellence for Light Enabling Technologies Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia Center of Excellence for NaNo Energy&Catalysis Technology(CONNECT) Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia Department of Chemical engineering Khalifa UniversityShakhbout Bin Sultan St-Zone 1Abu DhabiUnited Arab Emirates Zhejiang Provincial Key Laboratory for Subtropical Water Environment and Marine Biological Resources Protection Wenzhou UniversityWenzhou 325035ZhejiangChina Department of Chemical and Environmental engineering Faculty of Science and EngineeringUniversity of Nottingham MalaysiaJalan Broga43500 SemenyihSelangor Darul EhsanMalaysia Department of Sustainable engineering Saveetha School of EngineeringSIMATSChennai 602105India

MXene has been the limelight for studies on electrode active materials,aiming at developing supercapacitors with boosted energy density to meet the emerging influx of wearable and portable electronic *** its various desirable properties including intrinsic flexibility,high specific surface area,excellent metallic conductivity and unique abundance of surface functionalities,its full potential for electrochemical performance is hindered by the notorious restacking phenomenon of MXene *** to its two-dimensional(2D)nature and surface functional groups,inevitable Van der Waals interactions drive the agglomeration of nanosheets,ultimately reducing the exposure of electrochemically active sites to the electrolyte,as well as severely lengthening electrolyte ion transport *** a result,energy and power density deteriorate,limiting the application versatility of MXene-based *** 3D architectures using 2D nanosheets presents as a straightforward yet ingenious approach to mitigate the fatal flaws of ***,the sheer number of distinct methodologies reported,thus far,calls for a systematic review that unravels the rationale behind such 3D MXene structural ***,this review aims to serve this purpose while also scrutinizing the structure–property relationship to correlate such structural modifications to their ensuing electrochemical performance ***,the physicochemical properties of MXene play fundamental roles in determining the effective charge storage capabilities of 3D MXene-based *** largely depends on different MXene synthesis techniques and synthesis condition variations,hence,elucidated in this review as ***,the challenges and perspectives for achieving viable commercialization of MXene-based supercapacitor electrodes are highlighted.

关键词： MXene 3D architectures Synthesis design Supercapacitor Energy storage