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Realize ultralow-energy-consumption photo-synaptic device based on a single(Al,Ga)N nanowire for neuromorphic computing

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nano Research 2024年第3期17卷 1933-1941页

作者： Xiushuo Gu Min Zhou Yukun Zhao Qianyi Zhang Jianya Zhang Yonglin Huang Shulong Lu College of Electronic and optical Engineering&College of Flexible Electronics(Future Technology) Nanjing University of Posts and TelecommunicationsNanjing 210023China Key Lab of nanodevices and Applications Suzhou Institute of Nano-Tech and Nano-Bionics(SINANO)Chinese Academy of Sciences(CAS)Suzhou 215123China School of nano-Tech and nano-Bionics University of Science and Technology of ChinaHefei 230026China Jiangsu Key Laboratory of Micro and nano Heat Fluid Flow Technology and Energy Application School of Physical Science and TechnologySuzhou University of Science and TechnologySuzhou 215009China

The rapid development of artificial intelligence poses an urgent need for low-energy-consumption and small-sized artificial photonic ***,it is pretty novel to demonstrate a light-stimulated synaptic device based on a single(Al,Ga)N nanowire *** to the presence of vacancy defects in the single nanowire,the artificial synaptic device can simulate multiple functions of biological synapses under stimulation of both 310 and 365 nm light photons,including paired-pulse facilitation,spike timing dependent plasticity,and memory learning *** energy consumption of artificial synaptic device can be reduced as little as 5.58×10^(-13) J,which is close to that of the biological synapse in human ***,the synaptic device is demonstrated to have the high stability for both long-time stimulation and long-time *** on the experimental conductance of long-term potentiation and long-term depression,the simulated three-layer neural network can achieve a high recognition rate of 92%after only 10 training *** a brain-like behavior,the single-nanowire-based synaptic devices can promote the development of visual neuromorphic computing technology and artificial intelligence systems requiring ultralow energy consumption.

关键词： single(Al Ga)N nanowire light-stimulated synaptic device low-energy-consumption neural network

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Effects of water molecules on luminescence in europium and terbium coordination polymers with p-fluorobenzoic acid as ligand

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Journal of Rare Earths 2024年第7期42卷 1258-1264,I0003页

作者： Xiaoqi Zhao Puyan Hao Yami Ling Mengzhen Jia Rui Zhu Jiawen Liu Qiang Xu Jianhong Zhou Collaborative Innovation Center of Rare-Earth optical Functional Materials and Devices Development Baoji Key Laboratory of Micro-Nano Optoelectronics and Terahertz TechnologySchool of Physics and Opto-Electronic TechnologyBaoji University of Arts and SciencesBaoji721016China

Our previous experimental observations show that the crystal structure of lanthanide luminescent complexes synthesized in aqueous solution usually contains a large number of coordination water molecules or free water *** order to probe the influence of water molecules on luminescent processes of lanthanide complexes,the photoluminescence properties of Ln-FBA(Ln=Eu and Tb,FBA=p-fluorobenzoic acid)coordination polymers at different ambient temperatures,in different solvents and aqueous DMSO solutions with different volume concentrations were systematically *** experiment results show that the presence of water molecules can promote the energy transfer from FBA ligand to Ln3+,at the same time,can cause luminescent non-radiation quenching of lanthanide *** addition,the variation of emission intensity ratio of 615 nm/591 nm peaks of Eu^(3+)with increasing the volume concentration of H_(2)O can be potentially used for the quantitatively detection of water traces in organic *** order to suppress the non-radiation quenching caused by the water molecules,Ln-FBA(Ln=Eu and Tb)coordination polymers were embedded into the PVP matrix to prepare Ln-FBA@PVP hybrid *** photoluminescence investigation indicates that PVP can not only block the quenching effect of water molecules on luminescence,but also effectively sensitize Eu^(3+)and Tb^(3+)*** experimental conclusions are useful for probing the influence of water molecules on luminescent processes of lanthanide complexes,quantitatively detecting water traces in organic solvents and enhancing the photoluminescence intensity in lanthanide complexes.

关键词： Lanthanide complexes Photoluminescence Luminescent quenching Rare earths

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Wideband chaos generation using a VCSEL with intensity modulation optical injection for random number generation

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Science China(Information Sciences) 2024年第6期67卷 457-458页

作者： Yu HUANG Shuangquan GU Yuhang FENG Yigong YANG Shuiying XIANG Pei ZHOU Nianqiang LI School of Optoelectronic Science and Engineering & Collaborative Innovation Center of Suzhou nano Science and Technology Soochow University State Key Laboratory of Integrated Service Networks Xidian University Key Lab of Advanced optical Manufacturing Technologies of Jiangsu Province & Key Lab of Modern optical Technologies of Education Ministry of China Soochow University

Physical random numbers have been widely used in modern network society,such as the generation of cryptographic keys for classical and quantum cryptography systems[1].Among the many sources of physical entropy,chaotic semiconductor lasers have attracted wide attention due to their desired characteristics including larger bandwidth,low cost,and monolithic integration[2].

关键词： optical signal processing

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Inversely engineered metasurfaces for independent manipulation of transmitted and reflected light fields

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Science China(Physics,Mechanics & Astronomy) 2024年第7期67卷 97-106页

作者： Yongjian Liu Yu Luo Fei Zhang Mingbo Pu Hanlin Bao Mingfeng Xu Yinghui Guo Lanting Li Xiong Li Xiaoliang Ma Xiangang Luo National Key Laboratory of optical Field Manipulation Science and Technology Chinese Academy of SciencesChengdu 610209China State Key Laboratory of optical Technologies on nano-Fabrication and Micro-Engineering Institute of Optics and ElectronicsChinese Academy of SciencesChengdu 610209China College of Materials Science and Opto-Electronic Technology University of Chinese Academy of SciencesBeijing 100049China Research Center on Vector optical Fields Institute of Optics and ElectronicsChinese Academy of SciencesChengdu 610209China Tianfu Xinglong Lake Laboratory Chengdu 610299China

Independent manipulation of transmitted and reflected light fields is a key technology for the realization of multifunctional optical applications,which can be implemented based on multilayered plasmonic or supercell subwavelength ***,the former is not suitable for the optical bands,while the latter is insufficient in generating large phase ***,an adjoint-optimization-based inverse design methodology is proposed,which utilizes the polarization-selective local interference between individual meta-atoms and enables monolayer dielectric metasurfaces to decouple the wavefront of transmitted and reflected optical ***,this methodology serves to mitigate the aperiodic electromagnetic crosstalk inherent between adjacent meta-atoms,consequently leading to a significant enhancement in the performance of *** analyzed the physical mechanism of adjoint optimization and proposed the concept of phase factors,highlighting their importance in the rapid inverse design of meta-devices—an aspect often overlooked in previous *** demonstrate the feasibility and robustness of our method,we optimize monolayer metasurfaces with different initial *** devices efficiently focus and deflect x-linearly and y-linearly polarized incident light in transmission and reflection spaces,***,this methodology holds immense potential for designing multifunctional,high-performing metasurfaces that meet multiple constraints,opening up broad prospects for applications.

关键词： full-space metasurfaces adjoint optimization inverse design

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3D nano-printed geometric phase metasurfaces for generating accelerating beams with complex amplitude manipulation

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Science China(Physics,Mechanics & Astronomy) 2024年第6期67卷 86-95页

作者： Tianchen Tang Saima Kanwal Yongzheng Lu Yuelong Li Shuangbao Wu Lei Chen Ziheng Qian Zhouyu Xie Jing Wen Dawei Zhang Research Center of optical Instrument and System Ministry of Education and Shanghai Key Lab of Modern Optical SystemUniversity of Shanghai for Science and TechnologyShanghai 200093China

Metasurface,a forefront in emerging optical devices,has demonstrated remarkable potential for complex amplitude manipulation of light ***,prevailing approaches face challenges in spatial resolution and complexities associated with integrating dynamic phases,impeding the simplified design and reproducible fabrication of ***,we introduce an innovative approach for complex amplitude modulation within 3D nano-printed geometric phase *** approach enables the generation of self-accelerating beams by encoding amplitude through phase-only manipulation,achieving high spatial ***,this method circumvents the conventional need to adjust the geometric parameters of metasurface unit structures for amplitude manipulation,offering a streamlined and efficient route for design and fabrication *** novel methodology holds promise for expedited and low-cost manufacturing of complex amplitude manipulation metasurfaces.

关键词： metasurface complex amplitude manipulation geometric phase 3D nano-printing Airy beam accelerating parabolic beam

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Towards the performance limit of catenary meta-optics via field-driven optimization

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Opto-Electronic Advances 2024年第5期7卷 33-42页

作者： Siran Chen Yingli Ha Fei Zhang Mingbo Pu Hanlin Bao Mingfeng Xu Yinghui Guo Yue Shen Xiaoliang Ma Xiong Li Xiangang Luo National Key Laboratory of optical Field Manipulation Science and Technology Chinese Academy of SciencesChengdu 610209China State Key Laboratory of optical Technologies on nano-Fabrication and Micro-Engineering Institute of Optics and ElectronicsChinese Academy of SciencesChengdu 610209China College of Materials Science and Opto-Electronic Technology University of Chinese Academy of SciencesBeijing 100049China Research Center on Vector optical Fields Institute of Optics and ElectronicsChinese Academy of SciencesChengdu 610209China Department of Electrical and Computer Engineering University of California Los Angeles(UCLA)Los AngelesCalifornia 90095USA

Catenary optics enables metasurfaces with higher efficiency and wider bandwidth,and is highly anticipated in the imaging system,super-resolution lithography,and broadband ***,the periodic boundary approximation without considering aperiodic electromagnetic crosstalk poses challenges for catenary optical devices to reach their performance ***,perfect control of both local geometric and propagation phases is realized through field-driven optimization,in which the field distribution is calculated under real boundary *** from other optimization methods requiring a mass of iterations,the proposed design method requires less than ten iterations to get the efficiency close to the optimal *** on the library of shape-optimized catenary structures,centimeter-scale devices can be designed in ten seconds,with the performance improved by ~15%.Furthermore,this method has the ability to extend catenary-like continuous structures to arbitrary polarization,including both linear and elliptical polarizations,which is difficult to achieve with traditional design *** provides a way for the development of catenary optics and serves as a potent tool for constructing high-performance optical devices.

关键词： catenary optics catenary structures field-driven optimization

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nano-sized stationary phase packings retained by single-particle frit for microchip liquid chromatography

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Chinese Chemical Letters 2024年第4期35卷 486-489页

作者： Wangyan Hu Ke Li Xiangnan Dou Ning Li Xiayan Wang Center Excellence for Environmental Safety and Biological Effects Beijing Key Laboratory for Green Catalysis and SeparationDepartment of ChemistryBeijing University of TechnologyBeijing 100124China Center for Environmental metrology National Institute of MetrologyBeijing 100029China

Modern chromatography is increasingly focused on miniaturization and integration. Compared to conventional liquid chromatography, microfluidic chip liquid chromatography(microchip-LC) has the potential due to its zero-dead volume connection and ease of integration. nano-sized packings have the potential to significantly enhance separation performance in microchip-LC. However, their application has been hindered by packing difficulties. This study presents a method for packing nano-sized silica particles into a microchannel as the stationary phase. The microchip-LC packed column was prepared by combining the weir and the porous silica single-particle as frit to retain the packing particles. A surface tensionbased single-particle picking technique was established to insert porous single-particle frit into glass microchannels. Additionally, we developed a slurry packing method that utilizes air pressure to inject nano-sized packing into the microchannel. Pressure-driven chromatographic separation was performed using this nano-packed column integrated into a glass microchip. The mixture of four PAHs was successfully separated within just 8 min using a 5 mm separation channel length, achieving high theoretical plates(10~6plates/m). Overall, these findings demonstrate the potential of utilizing nano-sized packings for enhancing chromatographic performance in microchip systems.

关键词： nano-size packing Single-particle frit Packed column Microchip LC Chromatographic separation

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Ultrafast laser state active controlling based on anisotropic quasi-1D material

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Light(Science & Applications) 2024年第4期13卷 717-726页

作者： Zixin Yang Qiang Yu Jian Wu Haiqin Deng Yan Zhang Wenchao Wang Tianhao Xian Luyi Huang Junrong Zhang Shuai Yuan Jinyong Leng Li Zhan Zongfu Jiang Junyong Wang Kai Zhang Pu Zhou College of Advanced Interdisciplinary Studies National University of Defense TechnologyChangsha 410073China. Nanhu Laser Laboratory National University of Defense TechnologyChangsha 410073China. i-Lab&Key Laboratory of nanodevices and Applications&Key Laboratory of nanophotonic Materials and Devices Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China. School of Applied and Engineering Physics Cornell UniversityIthacaNY 14853USA. State Key Laboratory of Advanced optical Communication Systems and Networks School of Physics and AstronomyShanghai Jiao Tong UniversityShanghai 200240China. Shanghai Key Lab of Modern optical System University of Shanghai for Science and TechnologyShanghai 200093China

Laser state active controlling is challenging under the influence of inherent loss and other nonlinear effects in ultrafast *** an extension of degree of freedom in optical devices based on low-dimensional materials may be a way ***,the anisotropic quasi-one-dimensional layered material Ta2PdS6 was utilized as a saturable absorber to modulate the nonlinear parameters effectively in an ultrafast system by polarization-dependent *** polarization-sensitive nonlinear optical response facilitates the Ta2PdS6-based mode-lock laser to sustain two types of laser states,i.e.,conventional soliton and noise-like *** laser state was switchable in the single fiber laser with a mechanism revealed by numerical *** coding was further demonstrated in this platform by employing the laser as a codable light *** work proposed an approach for ultrafast laser state active controlling with low-dimensional material,which offers a new avenue for constructing tunable on-fiber devices.

关键词： polarization fiber controlling

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Research on Fiber Optic Surface Plasmon R ***:A Review

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Photonic Sensors 2024年第2期14卷 1-30页

作者： Qi WANG Dianyun ZHANG Yizhuo QIAN Xiangyu YIN Lei WANG Shushuai ZHANG Yuyang WANG State Key Laboratory of Synthetical Automation for Process Industries Northeastern UniversityShenyang 110819China College of Information Science and Engineering Northeastern UniversiyShenyang 110819China Hebei Key Laboratory of Micro-nano Precision optical Sensing and Measurement Technology Qinhuangdao 066004China State Key Laboratory of Chemo/Biosensing and Chemometrics Hunan UniversityChangsha 410082China

Due to the benefits of the high sensitivity,real-time response,no labeling requirement,and good selectivity,fiber optic sensors based on surface plasmon resonance(SPR)have gained popularity in biochemical sensing in recent *** current research on such sensors is hot in enhancing sensitivity,improving detection accuracy,and achieving the detection of biochemical *** goal of this work is to present a thorough overview of recent developments in the optical fiber SPR biosensor ***,it explores the basic principles and sensing structures of optical fiber SPR biosensors,focusing on four ***,this paper introduces three fiber optic surface plasmon biosensors:SPR,localized surface plasmon resonance(LSPR),and long-range surface plasmon resonance(LRSPR).Each concept is explained from the perspective of the basic principles of fiber optic SPR ***,a classification of fiber optic SPR biosensors in health monitoring,food safety,environmental monitoring,marine detection,and other applications is introduced and ***,this paper summarizes the current research directions of SPR ***,it provides a prospective outlook on how fiber optic SPR sensors will develop in the future.

关键词： Surface plasmon resonance biosensors optical fiber sensors sensitivity

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Alcohol-dispersed polymer complex as an effective and durable interface modifier for n-i-p perovskite solar cells

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Journal of Energy Chemistry 2024年第6期93卷 243-252,I0007页

作者： Chang Shi Jiangling Li Shuping Xiao Ziyi Wang Wuchen Xiang Rui Wu Yang Liu Yinhua Zhou Weijun Ke Guojia Fang Pingli Qin Hubei Key Laboratory of optical Information and Pattern Recognition Wuhan Institute of TechnologyWuhan 430205HubeiChina Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074HubeiChina School of Physics and Technology Key Laboratory of Artificial Micro-and Nano-structures of the Ministry of Education and School of Physics and TechnologyWuhan UniversityWuhan 430072HubeiChina

Abundant interfacial defects remain a significant challenge that hampers both the efficiency and stability of perovskite solar cells(PSCs).Herein,an alcohol-dispersed conducting polymer complex,denoted as PEDOT:F(Poly(3,4-ethylene dioxythiophene):Perfluorinated sulfonic acid ionomers),is introduced into the interface between perovskite and hole transporting layer in regular-structured ***:F serves as a multi-functional interface layer(filling grain boundaries and covering perovskite's grain-surface)to achieve a robust interaction with organic groups within perovskites,which could induce a structural transformation of PEDOT to increase its conductivity for the efficient ***,the strong interaction between PEDOT and perovskites could promote an effective coupling of undercoordinated Pb~(2+)ions with the lone electron pairs near O&S atoms in PEDOT molecules,thereby enhancing defect ***,PEDOT:F with inherent hydrophobic properties prevents effectively moisture invasion into perovskites for the improved long-term stability of the ***,the PEDOT:F-based PSCs achieved a champion efficiency of 24.81%,and maintained ca.92%of their initial efficiency after 7680 h of storage in a dry air environment,accompanied by the enhanced photothermal stability.

关键词： Alcohol-dispersed conducting polymer complex Interface passivation Grain boundaries Device stability Perovskite solar cells

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