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Synthetic and Systems Biotechnology 2024年第1期9卷 127-133页

作者： Hu Li Wei Li Kaihui Song Yu Liu Guiyun Zhao Yi-Ling Du polytechnic institute Zhejiang UniversityHangzhou310022China Department of Microbiology Zhejiang University School of MedicineHangzhou310058China College of Life Sciences Zhejiang University310058HangzhouChina

The biological signaling molecule nitric oxide(NO)has recently emerged as a metabolic precursor for the creation of microbial natural products with diversified structures and biological *** the biosynthetic gene clusters(BGCs)of these compounds,genes associated with NO production pathways have been *** this study,we employ a nitric oxide synthase(NOS)-guided genome mining strategy for the targeted discovery of NO-derived bacterial natural products and NO-utilizing *** show that a conserved NOS-containing BGC,distributed across several actinobacterial genomes,is responsible for the biosynthesis of lajollamycin,a unique nitro-tetraene-containing antibiotic whose biosynthetic mechanism remains *** a combination of in vivo and in vitro studies,we unveil the first cytochrome P450 enzyme capable of catalyzing olefin nitration in natural product *** results not only expand the current knowledge about biosynthetic nitration processes but also offer an efficient way for targeted identification of NO-utilizing metabolic pathways and novel nitrating biocatalysts.

关键词： Nitric oxide Genome mining Biosynthesis Nitration Cytochrome P450

State estimation for delayed switched positive systems: delayed radius approach

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Science China(Information Sciences) 2024年第8期67卷 190-205页

作者： Weizhong CHEN Zhongyang FEI Xudong ZHAO Zheng-Guang WU School of Electronics and Information Xi'an Polytechnic University Research institute of Intelligent Control and Systems Harbin Institute of Technology Key Laboratory of Intelligent Control and Optimization for Industrial Equipment of Ministry of Education Dalian University of Technology School of Control Science and Engineering Dalian University of Technology State Key Laboratory of Industrial Control Technology Institute of Cyber-Systems and ControlZhejiang University

In this paper, an interval estimation scheme is developed for delayed switched positive systems（DSPS） with mode-dependent average dwell time switching. A lossless zonotopic estimation approach is proposed for the delayed intersection zonotope with the positive generator matrix. First, considering the existence of asynchronism between the system mode and the correction matrix mode, the mismatched intersection zonotope is constructed for DSPS to verify the consistency between the system model and ***, by utilizing the introduced radius definitions, the ?∞performance is addressed to optimize the size of delayed intersection zonotopes. Subsequently, we present a joint-design approach of switching signals and the mode-dependent correction matrix by constructing positive generator matrix-based delayed radius functions. Furthermore, guaranteed nonnegative state bounds are derived for the considered DSPS based on the proposed lossless zonotopic estimation criteria. Finally, detailed simulations are conducted to validate the feasibility and superiority of the developed methods.

关键词： delayed switched positive systems interval estimation asynchronous correction matrix zonotopes mode-dependent average dwell time

An inorganic liquid crystalline dispersion with 2D ferroelectric moieties

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National Science Review 2024年第5期11卷 254-263页

作者： Ziyang Huang Zehao Zhang Rongjie Zhang Baofu Ding Liu Yang Keyou Wu Youan Xu Gaokuo Zhong Chuanlai Ren Jiarong Liu Yugan Hao Menghao Wu Teng Ma Bilu Liu Shenzhen Graphene Centre Shenzhen Key Laboratory of Advanced Layered Materials for Value-added ApplicationsTsinghua-Berkeley Shenzhen Institute and Institute of Materials ResearchTsinghua Shenzhen International Graduate School Tsinghua University institute of Technology for Carbon Neutrality Faculty of Materials Science and Engineering Shenzhen Institute of Advanced Technology Chinese Academy of Sciences School of Physics and institute for Quantum Science and Engineering School of Chemistry and Institute of Theoretical ChemistryHuazhong University of Science and Technology Xi'an Research institute of High Technology Shenzhen institute of Advanced Technology Chinese Academy of Sciences Department of Applied Physics Hong Kong Polytechnic University

Electro-optical effect-based liquid crystal devices have been extensively used in optical modulation techniques, in which the Kerr coefficient reflects the sensitivity of the liquid crystals and determines the strength of the device's operational electric field. The Peterlin–Stuart theory and the O'Konski model jointly indicate that a giant Kerr coefficient could be obtained in a material with both a large geometrical anisotropy and an intrinsic polarization, but such a material is not yet reported. Here we reveal a ferroelectric effect in a monolayer two-dimensional mineral vermiculite. A large geometrical anisotropy factor and a large inherent electric dipole together raise the record value of Kerr coefficient by an order of magnitude, till 3.0 × 10-4mV-2. This finding enables an ultra-low operational electric field of10～2–10～4V m-1and the fabrication of electro-optical devices with an inch-level electrode separation, which has not previously been practical. Because of its high ultraviolet stability（decay <1% under ultraviolet exposure for 1000 hours）, large-scale production, and energy efficiency, prototypical displayable billboards have been fabricated for outdoor interactive scenes. This work provides new insights for both liquid crystal optics and two-dimensional ferroelectrics.

关键词： 2D materials layered minerals vermiculite ferroelectric inorganic liquid crystal Kerr coefficient

Editorial for Special Issue on Artificial Intelligence for Art

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Machine Intelligence Research 2024年第1期21卷 1-3页

作者： Luntian Mou Feng Gao Zijin Li Jiaying Liu Hongxun Yao Johan F.Hoorn Beijing University of Technology China Peking University China Central Conservatory of Music China Harbin institute of Technology China The Hong Kong polytechnic University China

As an innovative engine for digital content generation,AI-generated content(AIGC)has drawn more and more attention from academic fields as well as *** in the area of art creation,AI has demonstrated its great potential and gained increasing *** are greatly impressed by AI painting,composing,writing,virtual hosting,fashion,and ***,AI is also becoming capable of understanding art,evaluating the aesthetic value of art,and protecting the copyright of art as *** has not only exhibited creativity to some extent,but also served as an enabling tool to discover the principles underneath creativity and imagination,which are traditional challenges for neuroscience,cognitive science,and *** all these promising features of AI for art,we still have to face the many challenges such as the explainability of generative models and the copyright issues of AI art works.

关键词： gained becoming spite

Atomscopic of ripple origins for two-dimensional monolayer transition metal dichalcogenides

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Nano Research 2024年第3期17卷 2136-2144页

作者： Haitao Yu Mingzi Sun Xiao Wu Cheuk Hei Chan Bolong Huang Zhong Lin Wang CAS Center for Excellence in Nanoscience Beijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing 100049China Department of Applied Biology and Chemical Technology The Hong Kong Polytechnic UniversityKowloon 999077Hong KongChina Research Centre for Carbon-Strategic Catalysis The Hong Kong Polytechnic UniversityKowloon 999077Hong KongChina School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGeorgia 30332USA

During the development of ultrathin two-dimensional(2D)materials,the appearance of ripples has been widely ***,the formation mechanisms and their influences are still rarely investigated,especially their contributions to the electronic structures and optical *** compensate for the knowledge gap,we have carried out comprehensive theoretical studies on the monolayer WSe_(2) with a series of ripple structures from 0 to 12Åin different lattice *** sensitivity of the formation energy,band structures,electronic structures,and optical properties to the ripple structures have been performed systematically for the first *** formation of ripples in Armchair and zigzag simultaneously are more energetically favorable,leading to more flexible optimizations of the optoelectronic *** improved charge-locking effect and extension of absorption ranges indicate the significant role of ripple *** spontaneous formation of ripples is associated with orbital rearrangements and structural *** leads to the unique charge carrier correlate inversion between W-5d and Se-4p orbitals,resulting in the pinning of the Fermi *** work has supplied significant references to understand ultrathin 2D structures and benefit their future developments and applications in high-performance optoelectronic devices.

关键词： two-dimensional(2D)materials ripples strain effect charge carrier correlation inversion optoelectronic properties

Bioactive compounds in Hericium erinaceus and their biological properties:a review

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Food Science and Human Wellness 2024年第4期13卷 1825-1844页

作者： Yue Qiu Genglan Lin Weiming Liu Fuming Zhang Robert J.Linhardt Xingli Wang Anqiang Zhang College of Food Science and Engineering Zhejiang University of TechnologyHangzhou 310014China Zhejiang Biosan Biotech Co. Ltd.Hangzhou 310052China Department of Chemical and Biological Engineering Center for Biotechnology and Interdisciplinary StudiesRensselaer Polytechnic InstituteTroyNY 12180USA Departments of Chemistry and Chemical Biology and Biomedical Engineering Biological ScienceCenter for Biotechnology and Interdisciplinary StudiesRensselaer Polytechnic InstituteTroyNY 12180USA

Hericium erinaceus is a nutritious edible and medicinal fungi,rich in a variety of functional active ingredients,with various physiological functions such as antioxidation,anticancer,and enhancing *** is also effective in protecting the digestive system and preventing neurodegenerative *** this review paper,we summarize the sources,structures and efficacies of the main active components in *** fruiting body,mycelium,and culture media,and update the latest research progress on their biological activities and the related molecular *** on this information,we provide detailed challenges in current research,industrialization and information on the active ingredients of *** for future studies and new applications of *** are proposed.

关键词： Hericium erinaceus Bioactive compounds Biological activities Antioxidation Neuroprotection Immunoregulation

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Mitigating Lattice Distortion of High‑Voltage LiCoO_(2)via Core‑Shell Structure Induced by Cationic Heterogeneous Co‑Doping for Lithium‑Ion Batteries

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Nano-Micro Letters 2024年第3期16卷 169-182页

作者： Zezhou Lin Ke Fan Tiancheng Liu Zhihang Xu Gao Chen Honglei Zhang Hao Li Xuyun Guo Xi Zhang Ye Zhu Peiyu Hou Haitao Huang Department of Applied Physics and Research institute for Smart Energy The Hong Kong Polytechnic UniversityHong KongPeople’s Republic of China Department of Applied Physics The Hong Kong Polytechnic UniversityHong KongPeople’s Republic of China institute of Nanosurface Science and Engineering Guangdong Provincial Key Laboratory of Micro/Nano Optomechatronics EngineeringShenzhen UniversityShenzhenPeople’s Republic of China School of Physics and Technology University of JinanJinanShandongPeople’s Republic of China

Inactive elemental doping is commonly used to improve the structural stability of high-voltage layered transition-metal oxide ***,the one-step co-doping strategy usually results in small grain size since the low diffusivity ions such as Ti^(4+)will be concentrated on grain boundaries,which hinders the grain *** order to synthesize large single-crystal layered oxide cathodes,considering the different diffusivities of different dopant ions,we propose a simple two-step multi-element co-doping strategy to fabricate core–shell structured LiCoO_(2)(CS-LCO).In the current work,the high-diffusivity Al^(3+)/Mg^(2+)ions occupy the core of single-crystal grain while the low diffusivity Ti^(4+)ions enrich the shell *** Ti^(4+)-enriched shell layer(~12 nm)with Co/Ti substitution and stronger Ti–O bond gives rise to less oxygen ligand ***-situ XRD demonstrates the constrained contraction of c-axis lattice parameter and mitigated structural *** a high upper cut-off voltage of 4.6 V,the single-crystal CS-LCO maintains a reversible capacity of 159.8 mAh g^(−1)with a good retention of~89%after 300 cycles,and reaches a high specific capacity of 163.8 mAh g^(−1)at *** proposed strategy can be extended to other pairs of low-(Zr^(4+),Ta^(5+),and W6+,etc.)and high-diffusivity cations(Zn^(2+),Ni^(2+),and Fe^(3+),etc.)for rational design of advanced layered oxide core–shell structured cathodes for lithium-ion batteries.

关键词： Lithium-ion battery LiCoO_(2) Heterogeneous co-doping Core-shell structure High-voltage stability

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Heat source recognition sensor mimicking the thermosensation function of human skin

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The Innovation 2024年第5期5卷 84-90,83页

作者： Wenting Sun Pengxiang Zhang Xinyi Lin Yupeng Wang Shuaihua Wang Bin Yang Zijian Zheng Weishu Liu Department of Materials Science and Engineering Southern University and Science and TechnologyShenzhen 518055China Guangdong Provincial Key Laboratory of Functional Oxide Materials and Devices Southern University of Science and TechnologyShenzhen 518055China School of Fashion and Textiles The Hong Kong Polytechnic UniversityHong Kong SARChina Department of Applied Biology and Chemical Technology The Hong Kong Polytechnic UniversityHong Kong SAR 999077China Research institute for Intelligent Wearable Systems(RI-IWEAR) The Hong Kong Polytechnic UniversityHong Kong SAR 999077China Research institute for Smart Energy(RISE) The Hong Kong Polytechnic UniversityHong Kong SAR 999077China

The human skin maintains a comfortable and healthy somatosensory state by sensing different aspects of the thermal environment,including temperature value,heat source,energy level,and ***,state-of-the-art thermosensors only measure basic temperature values,not the full range of the thermosensation function of human ***,we propose a heat source recognition(hsr)sensor of poly(butyl acrylate)-lithium bis(n-fluoroalkylsulfonyl)imide(PBA-Li:nFSI;n=1,3,5),which enables response to temperature,pressure,and proximity stimulus signals based on the relaxation behavior of the ionic gel and distinguished between different types of heat sources(i.e.,radiation,convection,and conduction).The hsr sensor was integrated into a prosthetic limb covered by an e-skin with isothermal regulation,and experiments with a robot showed that it could achieve human-like thermosensation function,recognizing multidimensional information about thermal environments,such as temperature value,comfort level,and heat source *** work deeply mimics the human body’s thermosensation function and provides a reliable solution for the development of bionic e-skin for intelligent robots and prosthetics.

关键词： robot function source

Non-Linear Matrix Completion

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Journal of Data Analysis and Information Processing 2024年第1期12卷 115-137页

作者： Fengrui Zhang Randy C. Paffenroth David Worth Worcester polytechnic institute Worcester MA USA

Current methods for predicting missing values in datasets often rely on simplistic approaches such as taking median value of attributes, limiting their applicability. Real-world observations can be diverse, taking stock price as example, ranging from prices post-IPO to values before a company’s collapse, or instances where certain data points are missing due to stock suspension. In this paper, we propose a novel approach using Nonlinear Matrix Completion (NIMC) and Deep Matrix Completion (DIMC) to predict associations, and conduct experiment on financial data between dates and stocks. Our method leverages various types of stock observations to capture latent factors explaining the observed date-stock associations. Notably, our approach is nonlinear, making it suitable for datasets with nonlinear structures, such as the Russell 3000. Unlike traditional methods that may suffer from information loss, NIMC and DIMC maintain nearly complete information, especially in high-dimensional parameters. We compared our approach with state-of-the-art linear methods, including Inductive Matrix Completion, Nonlinear Inductive Matrix Completion, and Deep Inductive Matrix Completion. Our findings show that the nonlinear matrix completion method is particularly effective for handling nonlinear structured data, as exemplified by the Russell 3000. Additionally, we validate the information loss of the three methods across different dimensionalities.

关键词： Matrix Completion Data Pipeline Machine Learning

Free Vibration of Stiffened Plate with Cracked Stiffeners

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Advances in Applied Mathematics and Mechanics 2024年第1期16卷 253-278页

作者： Jian Xue Lihua Chen Yue Sun Wei Zhang Faculty of Materials and Manufacturing Beijing University of TechnologyBeijing 100124China Department of Mechanics School of ScienceHarbin Institute of TechnologyShenzhenGuangdong 518055China institute of Textiles and Clothing The Hong Kong Polytechnic UniversityHong KongChina

In this paper,a new cracked stiffener model for the stiffener with a partthrough and open crack is proposed,considering the compatibility condition of displacements between the plate and the *** on the first-order shear deformation theory,the free vibration of stiffened isotropic plates with cracked stiffeners are investigated for the first *** description of the crack parameters is based on the continuous equivalent bending stiffness and equivalent depth of the cracked beam,and it takes into consideration of shear deformation,bending-extensional coupling vibration,and eccentricity between the stiffeners and the *** stiffened plates with single or multiple cracked stiffeners are formulated and *** Ritz method with the modified characteristic functions is applied to demonstrate the effects of crack parameters(crack depth and location)coupling with the position and number of the cracked stiffeners on the vibration frequencies and modes of the stiffened *** validity and accuracy of the present solutions are verified through convergence studies and compared with the finite element results.

关键词： Free vibration stiffened plate cracked stiffener model crack Ritz method