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Spatially confined synthesis of TiNb_(2)O_(7)quantum dots onto mesoporous carbon and Ti_(3)C_(2)T_(X)MXene for boosting lithium storage

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Green Energy & Environment 2025年第2期10卷 358-366页

作者： Daoguang Sun Cheng Tang Haitao Li Xinlin Zhang Guanjia Zhu Zhen-Dong Huang Aijun Du Haijiao Zhang Institute of Nanochemistry and Nanobiology School of Environmental and Chemical EngineeringShanghai UniversityShanghai200444China School of Chemistry and Physics and Centre for Materials Science Queensland University of TechnologyBrisbaneQLD4001Australia State Key Laboratory for Organic Electronics and Information Displays&Jiangsu Key Laboratory for Biosensors Institute of Advanced Materials(IAM)Jiangsu National Synergetic Innovation Center for Advanced Materials(SICAM)Nanjing University of Posts and Telecommunications9 Wenyuan RoadNanjing210023China

TiNb_(2)O_(7)has been emerged as one of the most promising electrode materials for high-energy lithium-ion ***,limited by the slow electron/ion transport kinetics,and insufficient active sites in the bulk structure,the TiNb_(2)O_(7)electrode still suffers from unsatisfactory lithium storage ***,we demonstrate a spatially confined strategy toward a novel TiNb_(2)O_(7)-NMC/MXene composite through a triblock copolymer-directed one-pot solvothermal route,where TiNb_(2)O_(7)quantum dots with a particle size of 2-3 nm are evenly embedded into N-doped mesoporous carbon(NMC)and Ti_(3)C_(2)T_(X)***,the as-prepared TiNb_(2)O_(7)-NMC/MXene anode exhibits a high reversible capacity(486.2 mAh g^(-1)at 0.1 A g^(-1)after 100 cycles)and long cycle lifespan(363.4 mAh g^(-1)at ss1 A g^(-1)after 500 cycles).Both experimental and theorical results further demonstrate that such a superior lithium storage performance is mainly ascribed to the synergistic effect among 0D TiNb_(2)O_(7)quantum dots,2D Ti_(3)C_(2)T_(X)MXene nanosheets,and N-doped mesoporous *** strategy presented also opens up new horizon for space-confined preparation of high-performance electrode materials.

关键词： TiNb_(2)O_(7)quantum dots Ti_(3)C_(2)T_(X)MXene Mesoporous carbon Confined synthesis Lithium-ion batteries

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Peripheral mitochondrial DNA as a neuroinflammatory biomarker for major depressive disorder

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Neural Regeneration Research 2025年第6期20卷 1541-1554页

作者： Jinmei Ye Cong Duan Jiaxin Han Jinrong Chen Ning Sun Yuan Li Tifei Yuan Daihui Peng Division of Mood Disorder Shanghai Mental Health CenterShanghai Jiao Tong University School of MedicineShanghaiChina Department of Psychiatry First Hospital of Shanxi Medical UniversityTaiyuanShanxi ProvinceChina Shanghai Key Laboratory of Psychotic Disorders Brain Health InstituteNational Center for Mental DisordersShanghai Mental Health CenterShanghai Jiao Tong University School of MedicineShanghaiChina Co-innovation center of Neuroregeneration Nantong UniversityNantongJiangsu ProvinceChina

In the pathogenesis of major depressive disorder, chronic stress-related neuroinflammation hinders favorable prognosis and antidepressant response. Mitochondrial DNA may be an inflammatory trigger, after its release from stress-induced dysfunctional central nervous system mitochondria into peripheral circulation. This evidence supports the potential use of peripheral mitochondrial DNA as a neuroinflammatory biomarker for the diagnosis and treatment of major depressive disorder. Herein, we critically review the neuroinflammation theory in major depressive disorder, providing compelling evidence that mitochondrial DNA release acts as a critical biological substrate, and that it constitutes the neuroinflammatory disease pathway. After its release, mitochondrial DNA can be carried in the exosomes and transported to extracellular spaces in the central nervous system and peripheral circulation. Detectable exosomes render encaged mitochondrial DNA relatively stable. This mitochondrial DNA in peripheral circulation can thus be directly detected in clinical practice. These characteristics illustrate the potential for mitochondrial DNA to serve as an innovative clinical biomarker and molecular treatment target for major depressive disorder. This review also highlights the future potential value of clinical applications combining mitochondrial DNA with a panel of other biomarkers, to improve diagnostic precision in major depressive disorder.

关键词： biomarker cytokine exosomes inflammasome major depressive disorder microglia mitochondrial DNA mitochondrial dysfunction neuroinflammation Toll-like receptor

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Highly sensitive and specific uranyl ion detection by a fluorescent sensor containing uranyl-specific recognition sites

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Science Bulletin 2025年第1期70卷 70-77页

作者： Tiantian Feng Shilei Zhao Meng Cao Xinfeng Du Hui Wang Xuewen Cao Lijuan Feng Yihui Yuan Ning Wang State Key Laboratory of Marine Resource Utilization in South China Sea Collaborative Innovation Center of Marine Science and TechnologyHainan UniversityHaikou 570228China

Uranium pollution has become a serious threat to human health and environmental safety,making the detection of environmental uranium contamination of great *** sensitive and specific detection of uranyl ions,which are the dominant form of uranium in the environment,depends on the specific recognition of uranyl ions by chemical *** this study,a novel fluorescent sensor containing a highly specific uranyl ion recognition group is synthesized via the reaction of 1-ethyl-3-(3-dimethylaminopropyl)carbodiimide(EDC)and 1,1,2,2-tetra(4-carboxylphenyl)ethylene(TPE-(COOH)4).Owing to the effects of aggregation-induced emission(AIE)and intramolecular charge transfer(ICT),the fluorescent sensor,named TPE-EDC,exhibits significant fluorescent properties in aqueous *** binding of uranyl ions by specific recognition groups in TPE-EDC leads to a decrease in the ICT effect,thus causing a significant reduction in the emission intensity of *** attenuation of the fluorescence intensity of TPE-EDC shows an excellent linear relationship with an increase in uranyl ion ***-EDC exhibits ultra-sensitive and ultra-selective detection ability for uranyl ions with an ultra-low detection limit of 69 pmol/L and an ultrashort response time of 30 *** high detection performances render the fluorescent sensor TPE-EDC a promising candidate for early warning of uranium pollution.

关键词： Uranium Detection Specificity Recognition Intramolecular charge transfer

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Impacts of Land–Atmosphere Coupling on Summer Extreme Hot-Humid Compound Events over Southern Eurasia under Different Sea Surface Temperature Backgrounds

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Advances in Atmospheric Sciences 2025年第4期42卷 744-760页

作者： Yajing QI Haishan CHEN Siguang ZHU State Key Laboratory of Climate System Prediction and Risk Management/Key Laboratory of Meteorological Disaster Ministry of Education/Collaborative Innovation Center on Forecast and Evaluation of Meteorological DisastersNanjing University of Information Science and TechnologyNanjing 210044China School of Atmospheric Sciences Nanjing University of Information Science and TechnologyNanjing 210044China

Land–atmosphere coupling and sea surface temperature(SST)anomalies both have essential impacts on weather and climate *** on the ERA5 reanalysis dataset and the CESM1.2.2 model,this study investigates the influence of land–atmosphere coupling on summer extreme hot-humid events(EHHE)over southern Eurasia under different SST *** results suggest that coupling causes near-surface air temperature increases that exceed 0.5℃.From 1961 to 2020,the frequency of EHHE has continuously increased,and is closely related to soil moisture anomalies in the northern Indian Peninsula(IDP)and the middle and lower reaches of the Yangtze River(YRB).Numerical simulations further demonstrate that land–atmosphere coupling raises the risk of EHHE by 25.4%.In a typical El Niño SST background state,intensified land–atmosphere coupling tends to produce notable increases in the frequency of *** dominant processes that land–atmosphere coupling affects the EHHE variations are evidently different between these two *** surface thermal anomalies predominate in the IDP,while moisture conditions are more critical in the *** warm SST anomalies exist,dry soil anomalies in the IDP are prominent,and evaporation is constrained,increasing sensible heat *** geopotential height anomalies are significant,combined with adiabatic warming induced by descending motion and a noticeable warm center in the near-surface *** southward shift of the westerly jet enhances divergence over *** anticyclonic circulation anomalies over the western Pacific are conducive to guiding moisture transport to the YRB,providing a favorable circulation background for the development of summer EHHE.

关键词： land-atmosphere coupling sea surface temperature extreme hot-humid events southern Eurasia

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High-precision magnetic field measurement system based on a coherent population trapping magnetometer onboard the SATech-01 satellite

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Science China(Technological Sciences) 2025年第2期68卷 227-242页

作者： Hongbo XUE Wei SONG Haoran ZHAO Yiteng ZHANG Shanzhi YE Jindong WANG Ran TAO Peng SANG Keli CHEN Xingzi BI Bingjun CHENG Bin ZHOU Yongliang XUE Yingying TANG Liu LIU Jinsong LI Xiaocheng ZHU Baoquan LI Jinguo LIU Wen CHEN Xiaofeng ZHANG Yonghe ZHANG Lei LI State Key Laboratory of Space Weather National Space Science CenterChinese Academy of SciencesBeijing 100190China Key Laboratory of Solar Activity and Space Weather National Space Science CenterChinese Academy of SciencesBeijing 100190China Key Laboratory of Electronics and Information technology for Space Systems National Space Science CenterChinese Academy of SciencesBeijing 100190China State Key Laboratory of Robotics Shenyang Institute of AutomationChinese Academy of SciencesShenyang 110016China innovation Academy for Microsatellites Chinese Academy of SciencesShanghai 201304China

On July 27,2022,a high-precision system for measuring the magnetic field based on a coherent population trapping magnetometer(referred to as the CPT system)was launched onboard the Space Advanced technology demonstration satellite(SATech-01)by a ZK-1A *** payload comprises a scalar coherent population trapping magnetometer(CPTM),triaxial anisotropic magnetoresistance magnetometer(AMRM),and nano star tracker mounted on a non-magnetic telescopic tubular *** configuration enables synchronized measurement of scalar and vector geomagnetic fields,as well as the attitude,making the payload with its compact sensors suitable for applications on miniature satellite *** November 7,2022,the novel telescopic tubular mast was deployed in orbit,extending to a length of 5.28 *** CPTM,an absolute scalar magnetometer with an omnidirectional sensor,is the first China-developed quantum/atomic magnetometer successfully operating in *** orbit,the CPTM has sensitivity of~10 pT/Hz^(1/2) and can automatically operate under complex magnetic field *** difference between the scalar fields obtained using the CPTM and CHAOS model has a mean deviation of -3.73 nT and a standard deviation of 26.11 nT(1σ),without on-orbit calibration or *** miniaturized AMRM has a sensitivity of~0.3 nT/Hz^(1/2) and maintains stable and reliable operation in *** low-power and miniaturized nano star tracker has a measurement uncertainty of 14.23″(1σ)in *** mission has realized the on-orbit technical verification of the integrated and synchronized detection of the vector magnetic field and attitude and fully validated the system’s performance,automation level,and reliability.

关键词： magnetic field measurement system coherent population trapping magnetometer anisotropic magnetoresistance magnetometer nano star tracker non-magnetic telescopic tubular mast satellite

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A low redox potential and long life organic anode material for sodium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 557-564页

作者： Zhi Li Yang Wei Kang Zhou Xin Huang Xing Zhou Jie Xu Taoyi Kong Junwei Lucas Bao Xiaoli Dong Yonggang Wang Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials Institute of New EnergyCollaborative Innovation Center of Chemistry for Energy Materials(iChEM)Fudan UniversityShanghai 200433China Department of Chemistry Boston CollegeChestnut HillMA 02467USA School of Materials Science and Engineering Anhui University of TechnologyMa’anshan 243002AnhuiChina

Sodium-ion batteries (SIBs) with organic electrodes are an emerging research direction due to the sustainability of organic materials based on elements like C,H,O,and sodium ***,organic electrode materials for SIBs are mainly used as cathodes because of their relatively high redox potentials(>1 V).Organic electrodes with low redox potential that can be used as anode are ***,a novel organic anode material (tetrasodium 1,4,5,8-naphthalenetetracarboxylate,Na_(4)TDC) has been developed with low redox potential (<0.7 V) and excellent cyclic *** three-sodium storage mechanism was demonstrated with various in-situ/ex-situ spectroscopy and theoretical calculations,showing a high capacity of 208 mAh/g and an average decay rate of merely 0.022%per ***,the Na_(4)TDC-hard carbon composite can further acquire improved capacity and cycling stability for 1200 cycles even with a high mass loading of up to 20 mg cm^(-2).By pairing with a thick Na_(3)V_(2)(PO_(4))_(3)cathode (20.6 mg cm^(-2)),the as-fabricated full cell exhibited high operating voltage (2.8 V),excellent rate performance and cycling stability with a high capacity retention of 88.7% after 200 cycles,well highlighting the Na_(4)TDC anode material for SIBs.

关键词： Organic anode material Low redox potential Composite anode Sodium-ion batteries

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Axial coordinated iron-nitrogen-carbon as efficient electrocatalysts for hydrogen evolution and oxygen redox reactions

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Chinese Chemical Letters 2025年第1期36卷 637-642页

作者： Yanan Zhou Li Sheng Lanlan Chen Wenhua Zhang Jinlong Yang School of Material Science and Chemical Engineering Institute of Mass SpectrometryNingbo UniversityNingbo 315211China Department of Chemical Physics University of Science and Technology of ChinaHefei 230026China Department of Material Science and Engineering University of Science and Technology of ChinaHefei 230026China Hefei national Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Materials for Energy Conversion and Synergetic Innovation Centre of Quantum Information and Quantum PhysicsUniversity of Science and Technology of ChinaHefei 230026China

Designing highly active electrocatalysts for the hydrogen evolution reaction(HER)and oxygen evolution and reduction reactions(OER and ORR)is pivotal to renewable energy ***,based on density functional theory(DFT)calculations,we systematically investigate the catalytic activity of iron-nitrogen-carbon based covalent organic frameworks(COF)monolayers with axially coordinated ligands(denotes as Fe N_(4)-X@COF,X refers to axial ligand,X=-SCN,-I,-H,-SH,-NO_(2),-Br,-ClO,-Cl,-HCO_(3),-NO,-ClO_(2),-OH,-CN and-F).The calculated results demonstrate that all the catalysts possess good thermodynamic and electrochemical *** different ligands axially ligated to the Fe active center could induce changes in the charge of the Fe center,which further regulates the interaction strength between intermediates and catalysts that governs the catalytic ***,FeN_(4)-SH@COF and Fe N_(4)-OH@COF are efficient bifunctional catalysts for HER and OER,FeN_(4)-OH@COF and FeN_(4)-I@COF are promising bifunctional catalysts for OER and *** findings not only reveal promising bifunctional HER/OER and OER/ORR catalysts but also provide theoretical guidance for designing optimum ironnitrogen-carbon based catalysts.

关键词： Axial coordinated ligands DFT calculation Hydrogen evolution reaction Oxygen evolution reaction Oxygen reduction reaction

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A robust statistical prediction model for late-summer heavy precipitation days in North China

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Science China Earth Sciences 2025年第1期68卷 158-171页

作者： Shunli JIANG Tingting HAN Xin ZHOU Huijun WANG Zhicong YIN Xiaolei SONG Collaborative innovation center on Forecast and Evaluation of Meteorological Disasters/Key Laboratory of Meteorological Disaster Ministry of EducationNanjing University for Information Science and TechnologyNanjing210044China Nansen-Zhu International Research Centre Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing100029China Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai) Zhuhai519080China

Recently,heavy precipitation(HP)events have occurred frequently in North China(NC),causing devastating economic losses and human ***,the short-term climate prediction of HP is quite *** year-to-year increment(DY)method and sliding correlations,we developed a robust seasonal prediction model for late-summer HP days(HPDs)in NC during 1982–2022,utilizing three independent predictors—February sea surface temperature(SST)in the Indian Ocean(SST_IO),February snow depth over North Asia(SDE_NA),and May melted snow depth in NC(MSDE_NC).The SST_IO anomalies affect NC's precipitation through the Pacific-Japan *** SDE_NA anomalies are associated with East Asian anomalous anticyclone by southeastern propagation of Rossby wave at *** MSDE_NC anomalies are followed by vertical motion and moisture anomalies in situ and thereby cause precipitation *** prediction model can well simulate the variations of the HPDs,with a correlation coefficient(CC)of 0.81(0.65)between the observed and predicted HPDs_DY(HPDs_anomaly).The percentage with the same sign for 15 extreme HPDs_anomaly years(PSSE)is 100%.Moreover,in the cross-validation test during 1982–2022,the PSSE for HPDs_anomaly is as high as 100%,along with a low rootmean-square error of *** independent hindcasts during 2013–2022,the CC between the observed and predicted HPDs_DY(HPDs_anomaly)is 0.93(0.83),together with high Nash-Sutcliffe efficiency(0.82)and agreement index(0.89).Specifically,the predictions are broadly consistent with the observations for 2015,2016,2017,2021,and 2022,reflecting excellent performance of this prediction model of HPDs in NC.

关键词： Heavy precipitation at North China Year-to-year increment approach Robust seasonal prediction Sea surface temperature Snow depth

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Artificial intelligence advances drug delivery system and its clinical transition

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Science Bulletin 2025年第3期70卷 305-308页

作者： Hui Wang Xiao-Yan You Guo-Ping Zhao Master Lab for Innovative Application of Nature Products National Center of Technology Innovation for Synthetic BiologyTianjin Institute of Industrial BiotechnologyChinese Academy of Sciences(CAS)Tianjin 300308China Henan Engineering Research center of Food Microbiology College of Food and BioengineeringHenan University of Science and TechnologyLuoyang 471023China Haihe Laboratory of Synthetic Biology Tianjin 300308China CAS-Key Laboratory of Synthetic Biology CAS Center for Excellence in Molecular Plant SciencesShanghai Institute of Plant Physiology and EcologyChinese Academy of SciencesShanghai 200032China CAS Key Laboratory of Quantitative Engineering Biology Shenzhen Institute of Synthetic BiologyShenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China

Since November 2022,ChatGPT,an artificial intelligence(AI)chatbot,has rapidly captured global attention for its detailed responses and articulated answers across a broad spectrum of knowledge domains[1],[2].All industries will reorient around it,prompting a reevaluation of how this technology could further promote scientifical research and its clinical applications.

关键词： system transition spectrum

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24.4 THz·V fT ×BV figure-of-merit AlN/GaN/AlN MISHEMTs with thin AlN buffer layer

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Science China(Information Sciences) 2025年

作者： Chaoqun ZHANG Hong ZHOU Sami ALGHAMDI Kun ZHANG Zhihong LIU Yue HAO Jingcheng ZHANG State Key Laboratory of Wide-Bandgap Semiconductor Devices and Integrated technology Xidian University Guangzhou Wide Bandgap Semiconductor innovation center Guangzhou Institute of TechnologyXidian University Electrical and Computer Engineering Department King Abdulaziz University

Gallium nitride-based high-electron-mobility-transistors(HEMTs) have gained widespread interest and become primary candidates for next-generation high-frequency and high-power RF electronics, due to their wide bandgap,high breakdown field, and strong polarization-induced highdensity 2-dimensional electron gas (2DEG) at the heterojunction interface. AlGaN-based barriers and GaN-based buffers have become the dominant commercialized device structures for radar, satellite, and 5G communications [1, 2].

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