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Boosting bidirectional sulfur conversion enabled by introducing boron-doped atoms and phosphorus vacancies in Ni2P for lithium-sulfur batteries

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Journal of Energy Chemistry 2025年第1期100卷 760-769页

作者： Lin Peng Yu Bai Hang Li Meixiu Qu Zhenhua Wang Kening Sun Advanced Research institute of Multidisciplinary Science Beijing Institute of Technology Beijing Key Laboratory of Chemical Power Source and Green Catalysis School of Chemistry and Chemical Engineering Beijing Institute of Technology

Lithium-sulfur （Li-S） batteries have gained great attention due to the high theoretical energy density and low cost,yet their further commercialization has been obstructed by the notorious shuttle effect and sluggish redox ***,we supply a strategy to optimize the electron structure of Ni2P by concurrently introducing B-doped atoms and P vacancies in Ni2P （Vp-B-Ni2P）,thereby enhancing the bidirectional sulfur *** study indicates that the simultaneous introduction of B-doped atoms and P vacancies in Ni2P causes the redistribution of electron around Ni atoms,bringing about the upward shift of d-band center of Ni atoms and effective d-p orbital hybridization between Ni atoms and sulfur species,thus strengthening the chemical anchoring for lithium polysulfides （LiPSs） as well as expediting the bidirectional conversion kinetics of sulfur ***,theoretical calculations reveal that the incorporation of B-doped atoms and P vacancies in Ni2P selectively promotes Li2S dissolution and nucleation ***,the Li-S batteries with Vp-B-Ni2P-separators present outstanding rate ability of 777 m A h g-1at 5 C and high areal capacity of 8.03 mA h cm-2under E/S of 5μL mg-1and sulfur loading of 7.20 mg *** work elucidates that introducing heteroatom and vacancy in metal phosphide collaboratively regulates the electron structure to accelerate bidirectional sulfur conversion.

关键词： Lithium sulfur batteries

High-energy-density lithium manganese iron phosphate for lithium-ion batteries: Progresses, challenges, and prospects

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Journal of Energy Chemistry 2025年第1期100卷 1-17页

作者： Bokun Zhang Xiaoyun Wang Shuai Wang Yan Li Libo Chen Handong Jiao Zhijing Yu Jiguo Tu State Key Laboratory of Advanced Metallurgy University of Science and Technology Beijing Research institute for Intelligent Wearable Systems The Hong Kong Polytechnic University institute of Advanced Structure Technology Beijing Institute of Technology

The soaring demand for smart portable electronics and electric vehicles is propelling the advancements in high-energy–density lithium-ion *** manganese iron phosphate (LiMnxFe1-xPO4) has garnered significant attention as a promising positive electrode material for lithium-ion batteries due to its advantages of low cost,high safety,long cycle life,high voltage,good high-temperature performance,and high energy *** LiMnxFe1-xPO4has made significant breakthroughs in the past few decades,there are still facing great challenges in poor electronic conductivity and Li-ion diffusion,manganese dissolution affecting battery cycling performance,as well as low tap *** review systematically summarizes the reaction mechanisms,various synthesis methods,and electrochemical properties of LiMnxFe1-xPO4to analyze reaction processes accurately and guide material ***,the main challenges currently faced are concluded,and the corresponding various modification strategies are discussed to enhance the reaction kinetics and electrochemical performance of LiMnxFe1-xPO4,including multi-scale particle regulation,heteroatom doping,surface coating,as well as microscopic morphology ***,in view of the current research challenges faced by intrinsic reaction processes,kinetics,and energy storage applications,the promising research directions are *** importantly,it is expected to provide key insights into the development of high-performance and stable LiMnxFe1-xPO4materials,to achieve practical energy storage requirements.

关键词： Lithium manganese iron phosphate High energy density Lithium-ion batteries Reaction mechanism Tap density

Ecological Devastation in Lake Victoria: Part A: Thermal Structure and Anoxia

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Open Journal of Ecology 2015年第7期5卷 287-298页

作者： Moshe Gophen migal-scientific institute Kiryat Shemone Israel

Lake Victoria is the second (excl. Caspian Sea) largest lake in the world by surface area and 7th by Volume. The lake and catchment territories are shared between three countries, Kenya, Uganda and Tanzania. A research was carried out during 1990-1992 exploring the changes of the thermo-chemical structure occurred after the invasion of Nile Perch. Results of changes of physico-chemical (Temperature, DO and pH) conditions are summarized in this paper. The anoxic conditions by space and time were enhanced. Enhancement of pollutant supply from anthropogenic developments of terrestrial sources and atmospheric dust deposition accompanied by the deleterious effects of the Nile Perch invasion caused enhancement of anoxia in the lake in space and time. The combination of bottom-up nutrient supply and strong mixing conditions, expressed as low RTR values accelerate phytoplankton growth rate and production. The surplus of organic matter originated from algal biomass, enhanced anoxia.

关键词： Lake Victoria Kenya Nile Perch Anoxia Thermal Stability

The Impact of Climate Change on Zooplankton Biodiversity Index (ZBDI) in Lake Kinneret, Israel

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Open Journal of Ecology 2020年第12期10卷 822-828页

作者： Moshe Gophen migal Scientific Research Institute Kiryat Shmone Israel

Climate change conditions were indicated in the watershed of Lake Kinneret: air and consequently water temperature increase, decline in rainfall, and diminish river discharges accompanied by a reduction in Epilimnetic nitrogen and a slight increase in phosphorus. It is suggested that warming trend of the Kinneret Epilimnion enhanced decline of Zooplankton Biodiversity Index (ZBDI).

关键词： Climate Change Kinneret Zooplankton Biodiversity

Population Dynamics of Cyclopoid Copepods in Lake Kinneret (Israel)

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Open Journal of Modern Hydrology 2016年第4期6卷 212-221页

作者： Moshe Gophen migal-scientific Research institute Kiryat Shmone Israel

Reports on the Kinneret zooplankton in general and particularly on copepods are dealing recently with numerical densities of feeding habit classes. Nevertheless, for the evaluation of the integrated role of copepod assemblages in the entire lake ecosystem, their life cycle stages fluctuations are essential. It was not done in previous reports. Therefore, long term analysis of the cyclopoid copepods life stages dynamics in Lake Kinneret was carried out. Due to information availability, two complementary methods of density concentrations were evaluated for two consecutive data sets: 1) 1969-1985 numerical (No/L) documentation of life cycle stages of nauplii (I - III and III - V), copepodites (I, II, III, IV, V) and adults;2) 1969-2002 monthly averages of wet biomass density (g/m2) of zooplankton major groups combined with metabolic rates. nauplii densities represent June-August peaks and older stages spring decline and high levels during summer-early winter. Polynomial Regressions between Numerical annual averages of predator and Herbivore stages as well as young vs. older life stages indicate significant relations. During winter-spring season, temperatures are optimal for cyclopoid growth as a result of the high efficiency of metabolic activity and the low pressure of fish predation. The high rate of metabolism and intensive fish predation in summer enhance low densities of adult cyclopoids.

关键词： Kinneret Cyclopoida Population Dynamics Metabolism

On The Biology of Tilapia zillii (Gervais1848) in Lake Kinneret (Israel)

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Open Journal of Ecology 2016年第4期6卷 167-175页

作者： Moshe Gophen migal-scientific Research institute Kiryat Shmone Israel

Fish (mostly Tilapia zillii), (TZ), mass mortality in Lake Kinneret initiated a study of the biology of TZ in Lake Kinneret. The study included several aspects: spawning and nesting behavior, feeding habits, the status of TZ in the Kinneret fishery and temperature tolerance. The merit of TZ to commercial landing fishery is negligible, but this specimen is one of the most common fishes in the lake. Several environmental factors are considered as promoters of the epilimnetic temperature decline: Jordan water inputs in winter season as a heat source parameter. ENSO (EL-NIÑO/Southern Oscillation) acts as a cooling enhancement factor. Supportive data on the impact of ENSO were found in two terrestrial agricultural monitors in the northern and southern parts of the drainage basin. Gut content analysis of young fingerlings and an adult TZ specimen, indicated the significant contribution of benthic sources which are common in the shallows. The great adaptive capabilities of breeding TZ with various bottom habitats are demonstrated.

关键词： T. zillii Kinneret Breeding Temperature ENSO River Jordan

Thermal Preference by <i>Mesocyclops ogunnus</i>(Onabamiro, 1957)

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Open Journal of Ecology 2015年第2期5卷 15-21页

作者： M. Gophen migal scientific Research institute Kiryat Shmone Israel

In this work, the thermal response of Mesocyclops ogunnus was experimentally studied. Temperature was the only one parameter that was tested. Other parameters, such as food quality and availability, light conditions, predation pressure, and water mass motions were not included in the study. Organisms were collected in Lake Kinneret and the experiments were carried out under diffused light, 12/12 hours light/dark conditions. In the experimental system, the organisms were exposed to different temperatures of 15℃, 25℃, 27℃, and 30℃ with open pathway to migrate according to temperature preference. The preference of upper thermal range (25℃, 27℃, 30℃) by copepodite and adult stages was documented.

关键词： Mesocyclops Ogunnus Thermal Preference

Chemical, Hydrological and Climatological Properties of Lake Agmon, Hula Valley (Israel), (1994-2006)

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Open Journal of Modern Hydrology 2016年第1期6卷 8-18页

作者： Moshe Gophen Moshe Meron Yosef Tsipris Valerie Orlov-Levin Mordechay Peres migal Scientific Research Institute Kiryat Shmone Israel

The first decade of monitoring program in Lake Agmon (Hula Valley, Northern Israel) is summarized. The presented part of the program include: water discharges, physico-chemical (pH, EC, Temperature) and chemical parameters (TP, TN, TDN, TDP, NO3, NH4, SO4, TDS, TSS,). It was found that Nitrogen concentrations decline from north to south and the opposite for Phosphorus. Resulting of re-suspension by wind direction of western-southern-eastern and averaged maximal velocities of 9 - 10 m/s is suggested. De-nitrification and particles sedimentation emphasize Lake Agmon as a sink for Nitrogen. Sulfate-Carbonates association and the production of precipitated Gypsum (CaSO4) highlight the sink property of Lake Agmon. Nevertheless Sulfate removal by the Lake Agmon hydrological system is significant.

关键词： Agmon Hula Chemical Hydrological Climatological Properties

Ecophysiology of Lake Kinneret (Israel) Zooplankton

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Open Journal of Ecology 2015年第5期5卷 187-198页

作者： Moshe Gophen migal-scientific Research institute Kiryat Shmone Israel

A summary of a long-term research of Lake Kinneret zooplankton distribution is presented. During 1969-2002 several prominent changes have been recorded in the Kinneret ecosystem. This paper is an attempt aimed at analyzing the impact of these ecological changes on the zooplankton communities. The impacts of Phytoplankton, Bacteria, Protozoa, Temperature, Nutrient composition and fish predation on zooplankton dynamics are analyzed. It was found that periodical fluctuations of zooplankton density were mostly affected by fish predation as well as by temperature increase and food availability. Ecological conditions in Lake Kinneret have been modified since early 1990’s and the new conditions were consequently accompanied by zooplankton Homeostatic response. Moreover, as a result of the ecological changes fish intensified their pressure on zoo-plankton. The flexibility of food resource preference by zooplankton enabled its existence but fish predation predominantly controlled their density.

关键词： Kinneret Zooplankton Ecophysiology Food-Web