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Accelerated reconstruction of ZIF-67 with significantly enhanced glucose detection sensitivity

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Nano research 2024年第6期17卷 4737-4743页

作者： Huihui Jin Weihao Zeng Wei Qian Lun Li Pengxia Ji Zhengying Li Daping He School of Information engineering Wuhan University of TechnologyWuhan 430070China hubei engineering research center of rf-microwave technology and application Wuhan University of TechnologyWuhan 430070China State Key Laboratory of Advanced technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China

research on metal-organic framework(MOF)-based non-enzymatic glucose sensors usually ignores the impact of the surface reconstruction degree of MOF on the activity of catalyzing glucose *** this work,we choose zeolitic imidazolate framework-67(ZIF-67),which is commonly used in glucose sensing,as a representative to investigate the influence of reconstruction degree on its structure and glucose catalytic *** employing the electrochemical activation strategy,the activity of ZIF-67 in catalyzing glucose gradually increased with the prolongation of the activation time,reaching the optimum after 2 h *** detection sensitivity of the activated ZIF-67 was 19 times higher than that of the initial ZIF-67,and the limit of detection(LOD)was lowered from 7 to 0.4μ*** findings demonstrate that the oxidation degree of ZIF-67 deepened rapidly with continuously activation and was basically reconstructed to CoOOH after 2 h activation,accompanied by a morphological change from cuboctahedral to ***,theoretical investigation revealed that ZIF-67 is not suitable as a stable glucose sensor electrode since the adsorbed glucose molecules hasten the dissociation of ligands and the breaking of Co-N bond in ***,our work has important implications for the rational design of next-generation MOF-based glucose sensors.

关键词： zeolitic imidazolate framework-67(ZIF-67) glucose oxidation electrochemical activation reconstruction CoOOH

Highly Flexible Graphene-Film-Based Rectenna for Wireless Energy Harvesting

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Energy & Environmental Materials 2024年第2期7卷 320-325页

作者： Jingwei Zhang Yuchao Wang Rongguo Song Zongkui Kou Daping He hubei engineering research center of rf-microwave technology and application School of ScienceWuhan University of TechnologyWuhan 430070China Sanya Science and Education Innovation Park of Wuhan University of technology Sanya 572000China State Key Laboratory of Advanced technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China

Herein,we report the design,fabrication,and performance of two wireless energy harvesting devices based on highly flexible graphene macroscopic films(FGMFs).We first demonstrate that benefiting from the high conductivity of up to 1×10^(6)S m^(-1)and good resistive stability of FGMFs even under extensive bending,the FGMFs-based rectifying circuit(GRC)exhibits good flexibility and rf-to-DC efficiency of 53%at 2.1 ***,we further expand the application of FGMFs to a flexible wideband monopole rectenna and a 2.45 GHz wearable rectenna for harvesting wireless *** wideband rectenna at various bending conditions produces a maximum conversion efficiency of 52%,46%,and 44%at the 5th Generation(5G)2.1 GHz,Industrial Long-Term Evolution(LTE)2.3 GHz,and Scientific Medical(ISM)2.45 GHz,respectively.A 2.45 GHz GRC is optimized and integrated with an AMC-backed wearable *** proposed 2.45 GHz wearable rectenna shows a maximum conversion efficiency of 55.7%.All the results indicate that the highly flexible graphene-film-based rectennas have great potential as a wireless power supplier for smart Internet of Things(loT)applications.

关键词： flexible rectennas highly flexible graphene-based films wireless energy harvesting

Controlling electrodeposited Ni layers by different-sized graphene oxides enables conductive e-textiles for the highly sensitive electrochemical detection of glucose

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Nano research 2024年第7期17卷 6258-6264页

作者： Zhen Li Zibo Chen Xiaodong Ji Huihui Jin Yunfa Si Jingwei Zhang Cheng Chen Daping He Sanya Science and Education Innovation Park of Wuhan University of technology Sanya 572000China School of Science Wuhan University of TechnologyWuhan 430070China State Key Laboratory of Advanced technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China hubei engineering research center of rf-microwave technology and application Wuhan University of TechnologyWuhan 430070China

With the increasing popularity of wearable electronic devices,there is an urgent demand to develop electronic textiles(e-textiles)for device ***,the difficulty in reconciliation between conductivity and manufacturing costs hinders their large-scale practical ***,we reported a facile and economic method for preparing conductive ***,nonconductive polypropylene(PP)was wrapped by reduced graphene oxide(rGO),followed by the electrodeposition of Ni nanoparticles(NPs).Notably,modulating the sheet size of graphene oxide(GO)resulted in controllable deposition of Ni NPs with adjustable size,allowing for controlled manipulations over the structures,morphologies,and conductivity of the obtained e-textiles,which influenced their performance in electrochemical glucose detection *** optimal material,denoted as Ni/rGO+(0.2)/PP,exhibited an impressive conductivity of 7.94×10^(4)S·m^(−1).With regard to the excellent conductivity of the as-prepared e-textiles and the high electrocatalytic activity of Ni for glucose oxidation,the asprepared e-textiles were subjected to glucose *** was worth emphasizing that the Ni/rGO_(0.2)/PP-based electrode demonstrated promising performance for nonenzymatic/label-free glucose detection,with a detection limit of 0.36μM and a linear response range of 0.5μM to 1 *** study paves the way for further development and application prospects of conductive etextiles.

关键词： conductive e-textiles nonenzymatic/label-free glucose detection controllable Ni deposition graphene oxides sizedependent effect

Scalable graphene foam with ultrahigh conductivity for stabilizing Pt towards efficient hydrogen evolution

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Nano research 2024年第8期17卷 6968-6976页

作者： Ming Zhao Meng Huang Huihui Jin Dayin He Wei Qian Zixin Zhang Daping He State Key Laboratory of Advanced technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China hubei engineering research center of rf-microwave technology and application Wuhan University of TechnologyWuhan 430070China School of Information engineering Wuhan University of TechnologyWuhan 430070China School of Chemistry and Materials Science University of Science and Technology of ChinaHefei 230026China Sanya Science and Education Innovation Park of Wuhan University of technology Sanya 572000China

For the carbon-based catalyst to be active and stable,especially in harsh electrochemical environments,the key is to decrease the concentration of defects and raise the degree of graphitization of the carbon ***,we develop a highly graphitized graphene foam with multiplicated structure to fabricate self-supporting Pt-based catalysts for efficient and stable hydrogen evolution reaction(HER)*** foam(GO-2850)is obtained through an ultra-high temperature treatment at 2850℃,with perfect graphene structure and extremely low defect,ensuring high electrical conductivity and corrosion ***,its multiplicated structure provides an inherently favorable environment for the dispersion of Pt nanoparticles(Pt NPs)and offers abundant channels for electrolyte infiltration during the catalytic *** a result,the as-prepared Pt/GO-2850 is far active and stable than the Pt NPs supported on commercial carbon paper(Pt/CP)counterpart toward catalyzing HER,exhibiting an outstanding activity and long-term durability(300 h@10 mA·cm^(−2))in acidic/alkaline/seawater *** can be attributed to the stronger interaction between the lower-defect GO-2850 substrate and Pt,as evidenced by characterization and theoretical *** work extends further insight into the design self-supporting catalysts of high activity and stability with promising prominent application toward green energy devices.

关键词： graphene foam high graphitization Pt nanoparticles hydrogen evolution reaction long-term stability

Hybrid ionic/electronic interphase enabling uniform nucleation and fast diffusion kinetics for stable lithium metal anode

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Chinese Chemical Letters 2024年第2期35卷 626-633页

作者： Lun Li Pengxia Ji Meng Huang Zixin Zhang Hong Wang Francis Verpoort Jinlong Yang Daping He State Key Laboratory of Advanced technology for Materials Synthesis and Processing School of Materials Science and EngineeringWuhan University of TechnologyWuhan 430070China Guangdong research center for Interfacial engineering of Functional Materials College of Materials Science and EngineeringShenzhen UniversityShenzhen 518060China Sanya Science and Education Innovation Park of Wuhan University of technology Sanya 572000China hubei engineering research center of rf-microwave technology and application Wuhan University of TechnologyWuhan 430070China State Key Laboratory of Silicate Materials for Architectures Wuhan University of TechnologyWuhan 430070China

Lithium(Li)dendrite issue,which is usually caused by inhomogeneous Li nucleation and fragile solid electrolyte interphase(SEI),impedes the further development of high-energy Li metal ***,the integrated construction of a high-stable SEI layer that can regulate uniform nucleation and facilitate fast Li-ion diffusion kinetics for Li metal anode still falls ***,we designed an artificial SEI with hybrid ionic/electronic interphase to regulate Li deposition by in-situ constructing metal Co clusters embedded in LiF *** generated Co and LiF both enable fast Li-ion diffusion kinetics,meanwhile,the lithiophilic properties of Co clusters can serve as Li-ion nucleation sites,thereby contributing to uniform Li nucleation and non-dendritic *** a result,a dendrite-free Li deposition with a low overpotential(16.1 mV)is achieved,which enables an extended lifespan over 750 h under strict *** full cells with high-mass-loading LiFePO_(4)(11.5 mg/cm^(2))as cathodes exhibit a remarkable rate capacity of 84.1 mAh/g at 5 C and an improved cycling performance with a capacity retention of 96.4%after undergoing 180 cycles.

关键词： Lithium metal anode Hybrid ionic/electronic interphase Solid electrolyte interphase Fast diffusion kinetics Dendritic growth of lithium

Enhanced resonance frequency in Co2FeAl thin film with different thicknesses grown on flexible graphene substrate

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Chinese Physics B 2024年第3期33卷 618-622页

作者：周偲袁少康朱登玉白宇明王韬刘福福潘禄禄冯存芳张博涵何大平汪胜祥 hubei engineering and technology research center for Functional Fiber Fabrication and Testing Wuhan Textile UniversityWuhan 430200China School of Electronic and Electrical engineering Wuhan Textile UniversityWuhan 430200China School of Mathematical and Physical Sciences Wuhan Textile UniversityWuhan 430200China School of Integrated Circuits Huazhong University of Science and TechnologyWuhan 430074China Key Laboratory for Magnetism and Magnetic Materials Ministry of EducationLanzhou UniversityLanzhou 730000China Beijing National center for Condensed Matter Physics and Institute of Physics Chinese Academy of SciencesBeijing 100190China hubei engineering research center of rf-microwave technology and application Wuhan University of TechnologyWuhan 430070China

The flexible materials exhibit more favorable properties than most rigid substrates in flexibility,weight saving,mechanical reliability,and excellent environmental ***,flexible graphene film with unique mechanical properties was extensively explored in high frequency ***,we report the characteristics of structure and magnetic properties at high frequency of Co2FeAl thin film with different thicknesses grown on flexible graphene substrate at room *** exciting finding for the columnar structure of Co2FeAl thin film lays the foundation for excellent high frequency property of Co2FeAl/flexible graphene ***-plane magnetic anisotropy field varying with increasing thickness of Co2FeAl thin film can be obtained by measurement of ferromagnetic resonance,which can be ascribed to the enhancement of crystallinity and the increase of grain ***,the resonance frequency which can be achieved by the measurement of vector network analyzer with the microstrip method increases with increasing thickness of Co2FeAl thin ***,in our case with graphene film,the resonance magnetic field is quite stable though folded for twenty cycles,which demonstrates that good flexibility of graphene film and the stability of high frequency magnetic property of Co2FeAl thin film grown on flexible graphene *** results are promising for the design of microwave devices and wireless communication equipment.

关键词： enhanced resonance frequency magnetic resonance field flexible graphene substrate

Robust textile-based spoof plasmonic frequency scanning antenna for on-body IoT applications

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Science China(Information Sciences) 2024年第8期67卷 269-284页

作者： Zhao-Min CHEN Jun-Lin ZHAN Hao CHEN Ya LI Hongjun HE Wu YANG Zhen-Guo LIU Wei-Bing LU State Key Lab of Millimeter Waves School of Information Science and EngineeringSoutheast University center for Flexible rf technology Frontiers Science Center for Mobile Information Communication and SecuritySoutheast University Future research Laboratory China Mobile Research Institute Purple Mountain Laboratories

Securing a comfortable, wearable compact frequency beam scanning antenna(FBSA) with robustness to deformation, low specific absorption rate(SAR), and good coverage of the surrounding environment for Internet of Things(IoT) applications, such as on-body navigation and wireless communication is an emerging challenge. In this work, a robust textile-based spoof plasmonic frequency scanning antenna utilizing higher-order modes is presented, which is also robust to deformation caused by the activities of the human body. The innovative design of the element ensures the high-efficiency transmission of the fundamental mode of spoof surface plasmon polaritons(SSPP) structure, providing the potential of being a multifunctional composite device in the compact on-body network. Besides, an artificial magnetic conductor(AMC) is designed underneath the SSPP structure, obtaining a low SAR value(0.113 W/kg), which ensures the safety of users. As a practical realization of this concept, a textile-based spoof plasmonic antenna was fabricated in the microwave regime and the performed experimental results show the proposed antenna has a single-beam radiation characteristic with a 70° beam scanning angle range when the frequency is 4.7–6.0 GHz with a high average realized gain of 13.15 dBi. And it still maintains a steady performance when faced with structure deformation, which proves its robustness. Wireless communication quality experiments are performed to demonstrate the proposed antenna can measure the angles of targets and realize wireless signal transmission to specific targets as the frequency varies, it may find great potential in the field of on-body IoT applications.

关键词： frequency beam scanning antenna (FBSA) Internet of Things (IoT) on-body communication spoof surface plasmon polaritons (SSPP) textile-based antenna

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Physical mechanism of secondary-electron emission in Si wafers

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Chinese Physics B 2024年第4期33卷 677-681页

作者：赵亚楠孟祥兆彭淑婷苗光辉高玉强彭斌崔万照胡忠强 State Key Laboratory for Manufacturing Systems engineering Electronic Materials Research LaboratoryKey Laboratory of the Ministry of EducationEngineering Research Center of Spin Quantum Sensor ChipsUniversities of Shaanxi ProvinceSchool of Electronic Science and EngineeringXi'an Jiaotong UniversityXi'an 710049China College of Aeronautics Nanjing University of Aeronautics and AstronauticsNanjing 210016China National Key Laboratory of Science and technology on Space microwave China Academy of Space TechnologyXi'an 710100China Department of Physics School of Physics and Electronic InformationAnhui Normal UniversityWuhu 241000China

CMOS-compatible rf/microwave devices,such as filters and amplifiers,have been widely used in wireless communication ***,secondary-electron emission phenomena often occur in rf/microwave devices based on silicon(Si)wafers,especially in the high-frequency *** this paper,we have studied the major factors that influence the secondary-electron yield(SEY)in commercial Si wafers with different doping *** show that the SEY is suppressed as the doping concentration increases,corresponding to a relatively short effective escape depthλ.Meanwhile,the reduced narrow band gap is beneficial in suppressing the SEY,in which the absence of a shallow energy band below the conduction band will easily capture electrons,as revealed by first-principles ***,the new physical mechanism combined with the effective escape depth and band gap can provide useful guidance for the design of integrated rf/microwave devices based on Si wafers.

关键词： secondary-electron yield doping concentration escape depth Si wafer

Wide Stopband Substrate Integrated Waveguide Filter Using Bisection and Trisection Coupling in Multilayer

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Chinese Journal of Electronics 2024年第2期33卷 436-442页

作者： Peng CHU Jianguo FENG Peng ZHU Lei GUO Long ZHANG Leilei LIU Guoqing LUO Ke WU College of Electronic and Optical engineering Nanjing University of Posts and Telecommunications National and Local Joint engineering Laboratory of rf Integration and Micro-Assembly technology School of Information and Communication engineering Dalian University of Technology Guangdong Provincial Key Laboratory of Optoelectronic Information Processing Chips and Systems Sun Yat-sen University College of Electronics and Information engineering Shenzhen University School of Electronics and Information Hangzhou Dianzi University Poly-Grames research center Polytechnique Montreal

This article presents a highly efficient method for substrate-integrated-waveguide（SIW） filters to achieve very wide stopbands. By employing the proposed trisection slots in addition to the bisection slots as the inter-coupling structures, all spurious modes below TE505 of a SIW filter working in the fundamental mode TE101（f0）can be eliminated without requiring additional structure or complex theoretical analysis, without affecting the design of the fundamental passbands, and without degrading the performance of the filters. For verification, two prototype filters are designed, fabricated, and measured with wide stopbands up to 4.15f0 and 4.83f0, respectively. The proposed technique could facilitate the development of high-performance wide-stopband SIW filters for microwave/wireless circuits and systems.

关键词： microwave measurement Couplings Filters Prototypes Nonhomogeneous media microwave theory and techniques microwave circuits