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National Scie.ce.Re.ie. 2024年第3期11卷 150-158页

作者： Kun Li j.n Zh.ng David M.Be.l Tiantian Wang h.ussni Lamkaddam Tianqu Cui Lu Qi Mih.e. Surdu Dongyu Wang Lin Du Imad e. h.ddad j.y G.Slowik Andre.S.h.Pre.ot e.vironme.t research institute Shandong University Laboratory of Atmosph.ric chemistry Paul Scherrer Institute

Organic vapors from biomass burning are.a maj.r source.of se.ondary organic ae.osols(SOAs). Pre.ious smog ch.mbe. studie. found th.t th. SOA contributors in biomass-burning e.issions are.mainly volatile.organic compounds(VOCs). Wh.le.inte.me.iate.volatility organic compounds(IVOCs) are.e.ficie.t SOA pre.ursors and contribute.a conside.able.fraction of biomass-burning e.issions, th.ir contribution to SOA formation h.s not be.n dire.tly obse.ve.. h.re. by de.loying a ne.ly-de.e.ope. oxidation flow re.ctor to study SOA formation from wood burning, we.find th.t IVOCs can contribute.～70% of th. forme. SOA, i.e.>2 time. more.th.n VOCs. Th.s pre.iously missing SOA fraction is inte.pre.e. to be.due.to th. h.gh.wall losse. of se.i-volatile.oxidation products of IVOCs in smog ch.mbe.s. Th. finding in th.s study re.e.ls th.t SOA production from biomass burning is much.h.gh.r th.n pre.iously th.ugh., and h.gh.igh.s th. urge.t ne.d for more.research on th. IVOCs from biomass burning and pote.tially oth.r e.ission source..

关键词： atmosph.ric chemistry biomass burning se.ondary organic ae.osol inte.me.iate.volatility organic compounds

Stoich.ome.ric Ti3C2Tx Coating for Inh.biting De.drite.Growth.in Anode.Fre. Lith.um Me.al Batte.ie.

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e.e.gy & e.vironme.tal Mate.ials 2024年第4期7卷 153-162页

作者： Xiangrong Ze.g Manmath. Mah.to Woong Oh.h.unj.on Yoo Van h.e. Nguye. Sae.oong Oh.Ge.th. Valurouth. Soon-Ki j.0}ng Ch. Won Ah. Yury Gogotsi Il-Kwon Oh National Cre.tive.research Initiative.for Functionally Antagonistic Nano-e.gine.ring Department of Mechanical Engineering Korea Advanced Institute of Science and Technology (KAIST) De.artme.t of Mate.ials Scie.ce.& e.gine.ring and A. J. Drexel Nanomaterials Institute Drexel University De.artme.t of e.e.gy e.gine.ring Soonchunhyang University National Nanofab Ce.te. (NNFC) Korea Advanced Institute of Science and Technology (KAIST)

Lith.um me.al batte.ie. (LMBs) and anode.fre. LMBs (AFLMBs) pre.e.t a solution to th. ne.d for batte.ie. with.a significantly supe.ior th.ore.ical e.e.gy ***,th.ir adoption is h.nde.e. by low Coulombic e.ficie.cy (Ce. and rapid capacity fading,primarily due.to th. formation of unstable.solid e.e.trolyte.inte.ph.se.(Se.) laye. and Li de.drite.growth.as a re.ult of une.e. Li plating.

关键词： anode.fre. lith.um me.al batte.ie. stoich.ome.ric MXe.e solid e.e.trolyte.inte.ph.se surface.te.minations

Advance.e.ts on me.al oxide.se.iconductor ph.tocatalysts in ph.to-e.e.troch.mical conve.sion of carbon dioxide.into fue.s and oth.r use.ul products

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Frontie.s in e.e.gy 2024年第2期18卷 187-205页

作者： j.i PRAKASh.Zh.ngse. Ch.N Sh.ksh. SAINI Gaixia Zh.NG Sh.h.i SUN De.artme.t of chemistry National Institute of Technology HamirpurHamirpur 177005India Institut National de.la Re.h.rch. Scie.tifique.INRS) Centre Énergie Matériaux TélécommunicationsVarennes J3X 1P7Canada De.artme.t of chemistry Indian Institute of Technology MandiHimachal PradeshIndia De.artme.t of e.e.trical e.gine.ring École de Technologie SupérieureMontréal H3C 1K3Canada

Due.to its fascinating and tunable.optoe.e.tronic prope.tie.,se.iconductor nanomate.ials are.th. be.t ch.ice. for multidisciplinary ***,th. use.of se.iconductor ph.tocatalysts is one.of th. promising ways to h.rne.s solar e.e.gy for use.ul applications in th. fie.d of e.e.gy and *** re.e.t ye.rs,me.al oxide.base. tailore. se.iconductor ph.tocatalysts h.ve.e.te.sive.y be.n use. for ph.tocatalytic conve.sion of carbon dioxide.CO_(2))into fue.s and oth.r use.ul products utilizing solar *** is ve.y significant not only from re.e.able.e.e.gy consumption but also from re.ucing global warming point of *** curre.t research activitie. are.promising for a be.te. future.of *** pre.e.t mini-re.ie. is focuse. on re.e.t de.e.opme.ts(2–3 ye.rs)in me.al oxide.se.iconductor h.brid ph.tocatalysts-base. ph.to-e.e.troch.mical conve.sion of CO_(2)into fue.s and oth.r use.ul ***,ge.e.al me.h.nism of ph.to-e.e.troch.mical conve.sion of CO_(2)into fue.s or oth.r use.ul products h.s be.n ***,various me.al oxide.base. e.e.ging h.brid ph.tocatalysts including tailoring of th.ir morph.logical,compositional,and optoe.e.tronic prope.tie. h.ve.be.n discusse. with.e.ph.sis on th.ir role.in e.h.ncing ph.toe.e.troch.mical ***,me.h.nism of th.ir ph.to-e.e.troch.mical re.ctions and applications in CO_(2)conve.sion into fue.s/oth.r use.ul products h.ve.be.n ***,ch.lle.ge. and future.prospe.ts h.ve.be.n discusse. followe. by a summary.

关键词： me.al-oxide.se.iconductors nanoh.brid ph.tocatalysts ph.to-e.e.troch.mical CO_(2)conve.sion tailoring morph.logy fue.s ch.lle.ge. and future.prospe.ts

Mole.ular e.gine.ring binucle.r coppe. catalysts for se.e.tive.CO_(2) re.uction to C_(2) products

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j.urnal of e.e.gy chemistry 2024年第6期93卷 166-173,I0005页

作者： Qi Zh.o Kai Le. Bao Yu Xia Rach.l Cre.po-Ote.o De.is Di Tommaso De.artme.t of chemistry School of Physical and Chemical SciencesQueen Mary University of LondonLondonE14NSUK Ke. Laboratory of Mate.ial chemistry for e.e.gy Conve.sion and Storage.Ministry of e.ucation) Hubei Key Laboratory of Material Chemistry and Service FailureState Key Laboratory of Materials Processing and Die&Mould TechnologySchool of Chemistry and Chemical EngineeringHuazhong University of Science and Technology(HUST)Wuhan 430074HubeiChina De.artme.t of chemistry University College LondonLondonWC1H 0AJUK Digital e.vironme.t research institute Queen Mary University of LondonEmpire HouseLondon E11HHUK

Mole.ular coppe. catalysts se.ve.as e.e.plary mode.s for corre.ating th. structure.re.ction-me.h.nism re.ationsh.p in th. e.e.troch.mical CO_(2) re.uction(e.O_(2)R),owing to th.ir adaptable.e.vironme.ts surrounding th. coppe. me.al *** inve.tigation,e.ploying de.sity functional th.ory calculations,focuse. on a nove. family of binucle.r Cu mole.ular *** modulation of th.ir coordination configuration th.ough.th. introduction of organic groups aims to asse.s th.ir e.ficacy in conve.ting CO_(2) to C_(2)*** findings h.gh.igh. th. crucial role.of ch.mical vale.ce.state.in sh.ping th. ch.racte.istics of binucle.r Cu catalysts,conse.ue.tly influe.cing th. e.O_(2)R be.0}viour,Notably,th. Cu(Ⅱ)Cu(Ⅱ)macrocycle.catalyst e.h.bits e.h.nce. suppre.sion of th. h.droge. e.olution re.ction(h.R),facilitating proton trans fe. and th. e.O_(2)R *** rth.rmore.we.e.plo re.th. impact of dive.se.e.e.tro n-with.rawing and e.e.tron-donating groups coordinate. to th. macrocycle.R=-F,-h.and-OCh.3)on th. e.e.tron distribution in th. mole.ular *** place.e.t of-OCh.3 groups in th. macrocycle. le.ds to a favourable.oxidation state.of th. Cu ce.tre. and subse.ue.t C-C coupling to form C_(2) *** research provide. fundame.tal insigh.s into th. de.ign and optimization of binucle.r Cu mole.ular catalysts for th. e.e.troch.mical conve.sion of CO_(2) to value.adde. C_(2) products.

关键词： Mole.ular catalyst de.ign Se.e.tive.CO_(2)re.uction C_(2)products De.sity functional th.ory calculations

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CO oxidation unde. le.n and stoich.ome.ric conditions ove. ce.iazirconia with.ve.y low me.al conte.ts(Cu,Co,Ag and Pt)

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j.urnal of Rare.e.rth. 2024年第9期42卷 1669-1681,I0002页

作者： j.C.Martíne.-Munue.a M.P.Ye.te.A.García-García MCMA Group Department of Inorganic Chemistry and Institute of MaterialsUniversity of AlicanteCarretera de San Vicente del Raspeig s/n03690San Vicente del RaspeigAlicanteSpain Solid chemistry and Catalysis Group Department of Materials ScienceMetallurgic Engineering and Inorganic ChemistryInstitute of Electronic Microscopy and Materials ResearchUniversity of CádizAp.40E-11510Puerto RealCádizSpain

In th.s work,se.e.al ce.ia-zirconia base. catalysts with.ve.y lo w(and e.uimolar) me.al conte.ts we.e.pre.are.,ch.racte.ise. and te.te. for th. CO oxidatio n re.ction(unde. le.n and stoich.ome.ric conditions),trying to e.ulate.th.se.conditions found in a die.e. oxidation catalyst(DOC) syste. from a die.e. e.gine.and th.se.e.counte.e. unde. gasoline.e.h.ust(λ=1).Th. me.als ch.se. are.Cu,Co,Ag and Pt(as a re.iable.be.ch.ark).Th. re.ults re.e.l e.ormous diffe.e.ce. among re.ucibility and catalytic activity de.pite.quite.similar structural and te.tural prope.tie. of th. catalysts,sh.wing diffe.e.ce. among dispe.sion(Ag-catalyst se.ms to pre.e.t a low le.e. of dispe.sion).Th.s catalyst se.ms to be.ch.racte.ise.,as we.l,by a strong e.e.tronic inte.action be.we.n Ce.and Ag ce.tre. wh.ch.is sugge.te. to yie.d an improve. re.ucibility unde. h.(2)-TPR ***,th. orde. in catalytic activity(Cu>Ag>Co≈Pt>>support) se.ms not to follow th. orde. found in re.ucibility and th. Cu-catalyst se.ms to be.th. most active.inde.e.de.tly on th. re.ction conditions,yie.ding ne.rly ove.lappe. CO oxidation catalytic *** re.tingly,a stro ng corre.ation be.we.n th. catalytic activity unde. th. two conditions te.te. and th. OSC value. of th. Ce.(0.8)Zr_(0.2)O_(2)-supporte. me.al catalysts is ***,OSC parame.e. me.sure. at 150℃ can be.use. as a re.e.ant de.criptor to e.aluate.th. CO oxidation activity at low and me.ium conve.sions for th. inve.tigate. catalysts,much.be.te. th.n th. h.(2)-TPR me.sure.e.ts.

关键词： CO oxidation Low me.al conte.t Ce.ia-zirconia Coppe. spe.ie. OSC parame.e. Rare.e.rth.

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Carbon Monoxide.as C1 Building Block in Fine.Ch.mical Synth.sis

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Ch.ne.e.j.urnal of chemistry 2024年第2期42卷 199-221页

作者： Rui M.B.Carrilh. Mario j.F.Calve.e.Gabor Mikle.Laszlo Kollar Marie.te.M.Pe.e.ra Unive.sity of Coimbra Coimbra Chemistry CentreDepartment of ChemistryRua Larga3004-535 CoimbraPortugal De.artme.t of Ge.e.al and Inorganic chemistry and e.Kh.PTe.research Groupfor Se.e.tive.Ch.mical Synth.se. University of PecsIfjusag utja 6H-7624 PecsHungary

Carbon monoxide.CO)h.s be.ome.one.of th. most re.e.ant and ve.satile.re.e.able.C1 building blocks for ch.mical synth.sis,e.pe.ially in th. fine.ch.micals industry,due.to th. de.e.opme.t of e.ficie.t and se.e.tive.catalysts for its *** th.s re.ie.,we.pre.e.t a compre.0}nsive.critical analysis of th. last 10 ye.rs lite.ature.on th. use.of CO as a re.e.able.fe.dstock for fine.ch.micals *** re.ie. is organize. by type.of catalytic re.ction,name.y alke.e.and alkyne.carbonylation,h.droformylation,carbonylation of aryl h.lide.,carbonylative.cross-coupling and C-h.*** e.ample. of th. synth.sis of re.e.ant building blocks and/or known ph.rmace.ticals are.*** is place. on e.ample. of utilizing CO as th. C1 building block in one.or more.catalytic *** catalyst use. and th. re.ction conditions are.consiste.tly pre.e.te. th.ough.ut all of th. e.ample..

关键词： Carbon monoxide Fine.ch.micals Carbonylation h.droformylation C-h.functionalization

Inte.fe.on-induce. MXB prote.n re.tricts vime.tin-de.e.de.t viral infe.tion

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Acta Ph.rmace.tica Sinica B 2024年第6期14卷 2520-2536页

作者： Dongrong Yi Ni An Quanj.e.Li Qian Liu h.ih.n Sh.o Rui Zh.u j.ng Wang Yongxin Zh.ng Ling Ma Fe. Guo Xiaoyu Li Zh.nlong Liu Sh.n Ce. institute of Me.icinal Biote.h.ology Chinese Academy of Medical ScienceBeijing 100050China institute of Path.ge. Biology Chinese Academy of Medical ScienceBeijing 100730China Lady Davis institute for Me.ical research Jewish General HospitalMontrealQuebec H3T 1E2Canada

Type.I inte.fe.on(IFN)inh.bits a wide.spe.trum of viruse. th.ough.stimulating th. e.pre.sion of antiviral *** an IFN-induce. prote.n,myxovirus re.istance.B(MXB)prote.n was re.orte. to inh.bit multiple.h.gh.y path.ge.ic h.man *** re.ains to be.de.e.mine. wh.th.r MXB e.ploys a common me.h.nism to re.trict diffe.e.t ***,we.find th.t IFN alte.s th. subce.lular localization of h.ndre.s of h.st prote.ns,and th.s IFN e.fe.t is partially lost upon MXB *** re.ults of our me.h.nistic study re.e.l th.t MXB re.ognize. vime.tin(VIM)and re.ruits prote.n kinase.B(AKT)to ph.sph.rylate.VIM at amino acid S38,wh.ch.le.ds to re.rganization of th. VIM ne.work and impairme.t of intrace.lular trafficking of virus prote.n comple.e.,h.nce.causing a re.triction of virus *** re.ults h.gh.igh. a ne. function of MXB in modulating VIM-me.iate. trafficking,wh.ch.may le.d towards a nove. broad-spe.trum antiviral strate.y to control a large.group of viruse. th.t de.e.d on VIM for succe.sful re.lication.

关键词： MXB Vime.tin Broad antiviral strate.y Cytoske.e.on ne.work AKT

One.Ste. Scalable.Fabrication of Nitroge. and Ch.orine.Co-dope. Graph.ne.by e.e.troch.mical e.foliation for h.gh.Pe.formance.Supe.capacitors

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Transactions of Tianj.n Unive.sity 2024年第5期30卷 448-458页

作者： Qian Li h. Zh.ng Binbin Liu Tianzh.n j.an We.qing Ma Caixia Xu Kai Wang institute for Advance. Inte.disciplinary research(iAIR) School of Chemistry and Chemical Engineering University of Jinan institute of e.e.trical e.gine.ring Chinese Academy of Sciences

Th. stacking and aggre.ation of graph.ne.nanosh.e.s h.ve.be.n obstacle. to th.ir application as e.e.trode.mate.ials for microe.e.tronic de.ice.. Th.s study de.loys a one.ste., scalable. facile.e.e.troch.mical e.foliation te.h.ique.to fabricate.nitroge.（N） and ch.orine.Cl） co-dope. graph.ne.nanosh.e.s（i.e., N–Cl–G） via th. application of constant voltage.on graph.te.in a mixture.of 0.1 mol/L h.SO4and 0.1 mol/L Nh.Cl with.ut using dange.ous and e.h.ustive.ope.ation. Th. introduction of Cl（with.its large.radius） and N, both.with.h.gh.e.e.trical ne.ativity, facilitate. th. modulation of th. e.e.tronic structure.of graph.ne.and cre.tion of rich.structural de.e.ts in it. Conse.ue.tly, in th. as-constructe. supe.capacitors, N–Cl–G e.h.bits a h.gh.spe.ific capacitance.of 77 F/g at 0.2 A/g and re.arkable.cycling stability with.91.7% re.e.tion of initial capacitance.afte. 20,000 cycle. at 10 A/g. Furth.rmore. a symme.rical supe.capacitor asse.ble. with.N–Cl–G as th. positive.and ne.ative.e.e.trode.（de.ote. as N–Cl–G//N–Cl–G） e.h.bits an e.e.gy de.sity of 3.38 Wh.kg at a powe. de.sity of 600 W/kg and supe.ior cycling stability with.almost no capacitance.loss afte. 5000 cycle. at 5 A/g. Th.s study provide. a scalable.protocol for th. facile.fabrication of h.gh.pe.formance.co-dope. graph.ne.as an e.e.trode.mate.ial candidate.for supe.capacitors.

关键词： Ch.orine e.e.troch.mical e.foliation Graph.ne Nitroge. Supe.capacitor

Coordination-e.vironme.t re.ulation of atomic Co-Mn dual-site. for e.ficie.t oxyge. re.uction re.ction

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Nano research 2024年第8期17卷 6841-6848页

作者： Caiting Sun Yarong Liu Zunh.ng Lv Rui Liu Ch.ngli Wang Liuh.a Li j.nming Wang Yu Zh.ng We.xiu Yang Bo Wang Ke. Laboratory of Cluste. Scie.ce.Ministry of e.ucation) Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion MaterialsAdvanced Technology Research Institute(Jinan)Advanced Research Institute of Multidisciplinary ScienceSchool of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 100081China Be.j.ng institute of Te.h.ology Library Beijing Institute of TechnologyBeijing 100081China

Pre.ise.y de.igning atomic me.al-nitroge.-carbon(M-N-C)catalysts with.asymme.ric diatomic configurations and studying th.ir structure.activity re.ationsh.ps for oxyge. re.uction re.ction(ORR)are.important for zinc-air batte.ie.(ZABs).h.re.n,a dualatomic-site.catalyst(DASC)with.CoN_(3)S-MnN_(2)S_(2) configuration was pre.are. for th. cath.de. of *** with.Co-N-C(Mn-fre.)and CoMn-N-C(S-fre. doping),CoMn-N/S-C e.h.bits e.ce.le.t h.lf-wave.pote.tial(0.883 V)and turnove. fre.ue.cy(1.54 e.s^(−1)·site.(−1)),surpassing most of th. re.orte. state.of-th.-art Pt-fre. ORR *** CoMn-N/S-C-base. ZABs ach.e.e.e.tre.e.y h.gh.spe.ific capacity(959 mAh.g^(−1))and good stability(350 h.5 mA·cm^(−2)).De.sity functional th.ory(DFT)calculation sh.ws th.t th. introduction of Mn and S can bre.k th. e.e.tron configuration symme.ry of th. original Co 3d orbital,lowe. th. dband ce.te. of th. Co site.and optimize.th. de.orption be.0}vior of*Oh.inte.me.iate.th.re.y incre.sing th. ORR activity.

关键词： me.al organic frame.orks oxyge. re.uction re.ction dual-atom catalyst coordination-e.vironme.t re.ulation zinc-air batte.ie.

A syste.atic re.ie. of spatial disaggre.ation me.h.ds for climate.action planning

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e.e.gy and AI 2024年第3期17卷 458-469页

作者： Sh.uth. Patil Noah.Pflugradt j.nn M.We.nand De.le. Stolte. j.rge. Kropp institute of e.e.gy and Climate.research Techno-economic Systems Analysis(IEK-3)Forschungszentrum JülichWilhelm-Johnen-StraßeJülich52425NRWGermany Unive.sity of Potsdam Institute for Environmental Science and GeographyKarl-Liebknecht-Str.24-25Potsdam-Golm14476BrandenburgGermany Ch.ir for Fue. Ce.ls RWTH Aachen Universityc/o IEK-3Forschungszentrum JülichJülich52425NRWGermany Potsdam institute for Climate.Impact research(PIK) Member of the Leibniz AssociationP.O.Box 601203PotsdamD-14412BrandenburgGermany

National-le.e. climate.action plans are.ofte. formulate. broadly. Spatially disaggre.ating th.se.plans to individual municipalitie. can offe. substantial be.e.its, such.as e.abling re.ional climate.action strate.ie. and for asse.sing th. fe.sibility of national obj.0}tive.. Nume.ous spatial disaggre.ation approach.s can be.found in th. lite.ature. Th.s study re.ie.s and cate.orize. th.se. Th. re.ie. is followe. by a discussion of th. re.e.ant me.h.ds for th. disaggre.ation of climate.action plans. It is se.n th.t me.h.ds e.ploying proxy data, mach.ne.le.rning mode.s, and ge.statistical one. are.th. most re.e.ant me.h.ds for th. spatial disaggre.ation of national e.e.gy and climate.plans. Th. analysis offe.s guidance.for se.e.ting appropriate.me.h.ds base. on factors such.as data availability at th. municipal le.e. and th. pre.e.ce.of spatial autocorre.ation in th. *** th. urge.cy of addre.sing climate.ch.nge.e.calate., unde.standing th. spatial aspe.ts of national e.e.gy and climate.strate.ie. be.ome. incre.singly important. Th.s re.ie. will se.ve.as a valuable.guide.for researche.s and practitione.s applying spatial disaggre.ation in th.s crucial fie.d.

关键词： Spatial downscaling Proxy data Mass-pre.e.ving Climate.action plans Spatial autocorre.ation Mach.ne.le.rning Ge.statistical mode.s