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Evaluation of arsenic pollution in field-contaminated soil at the soil’s actual pH

Journal of environmental Sciences 2024年第10期144卷 137-147页

作者： Tiancong Gao Haixia Tian Huimin Niu Mallavarapu Megharaj Wenxiang He College of Natural Resources and environment Northwest A&F UniversityKey Laboratory of Plant Nutrition and Agro-environment in Northwest ChinaMinistry of AgricultureYanglingShaanxi 712100China global centre for environmental Remediation College of EngineeringScience and EnvironmentUniversity of NewcastleCallaghanNSW 2308Australia

The pollution and ecological risks posed by arsenic(As)entering the soil are the major environmental challenges faced by human *** phosphatase can serve as a useful indicator for assessing As contamination under specific soil pH ***,the study of phosphatase kinetics in long-term field As-contaminated soil remains unclear,presenting a significant obstacle to the monitoring and evaluation of As pollution and *** purpose of this study was to determine phosphatase activity and explore enzyme kinetics in soils subjected to long-term field As *** revealed that the soil phosphatase activity varied among the tested soil samples,depending on the concentrations of *** relationship between total As,As fractions and phosphatase activity was found to be significant through negative exponential function *** parameters,including maximum reaction velocity(Vmax),Michaelis constant(Km)and catalytic efficiency(V_(max)/K_(m)),ranged from 3.14×10^(−2)–53.88×10^(−2) mmol/(L·hr),0.61–7.92 mmol/L,and 0.46×10^(−2)–11.20×10^(−2) hr−1,*** and Vmax/Km of phosphatase decreased with increasing As pollution,while Km was less ***,Vmax/Km showed a significant negative correlationwith all As fractions and total *** ecological doses(ED10)for the complete inhibition and partial inhibition models ranged from0.22–70.33 mg/kg and 0.001–55.27 mg/kg,respectively,indicating that V_(max)/K_(m) can be used as an index for assessing As pollution in field-contaminated *** study demonstrated that the phosphatase kinetics parameters in the soil’s pH system were better indicators than the optimal pH for evaluating the field ecotoxicity of As.

关键词： Arsenic pollution Ecological risk Soil phosphatase Enzyme kinetics Catalytic efficiency(V_(max)/K_(m))

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Heterogeneous integration of 2D materials on Si charge-coupled devices as optical memory

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Science China(Information Sciences) 2024年第6期67卷 190-197页

作者： Zheng BIAN Feng TIAN Zongwen LI Xiangwei SU Tianjiao ZHANG Jialei MIAO Bin YU Yang XU Yuda ZHAO College of Integrated Circuits Hangzhou Global Scientific and Technological Innovation CentreZhejiang University

Optical memory integrates the function of optical sensing in memory devices, remarkably promoting the interconnection between sensory and memory terminals. Silicon charge-coupled photodetectors and floating gate memory have been widely used in imaging and storage technologies, respectively. However,the heterogeneous integration of the two devices requires technological innovation and complex electrical connections. In this work, we adopt a three-dimensional layer stacking method to design a novel optical memory device. On the top of Si charge-coupled photodetectors, we successively deposit two-dimensional graphene,hexagonal boron nitride, and molybdenum disulfide as a floating gate layer, a tunneling layer, and a readout layer, respectively. By applying a gate bias on lightly doped Si, a deep depletion layer is formed with a high voltage potential drop. Under dark conditions, the depletion layer cannot be filled, and the electric field across the h-BN tunnel barrier is relatively small. Under light irradiation, the deep depletion layer is gradually filled, and the h-BN tunneling layer withstands the increasing electric field, resulting in charge storage in the floating gate layer. Based on this mechanism, the device exhibits a gate voltage-dependent operation mode, including an integrated optical sensing-memory mode and an electrically driven storage mode. Under moderate gate voltage, the device can effectively detect the optical information with varied intensity and store the optical information in the floating gate, displaying optically controlled memory characteristics. Our work demonstrates a compact device structure for optical memory and displays excellent optically controlled memory performance, which can be applied in artificial vision systems.

关键词： heterogeneous integration charge-coupled device floating gate optical memory molybdenum disulfide lightly doped silicon

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Assessment of spongy moth infestation impacts on forest productivity and carbon loss using the Sentinel-2 satellite remote sensing and eddy covariance flux data

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Ecological Processes 2024年第2期13卷 231-245页

作者： Nur Hussain Alemu Gonsamo Shusen Wang M.Altaf Arain School of Earth Environment and Society and McMaster Centre for Climate Change Mc Master University Canada centre for Remote Sensing Natural Resources Canada

Background Deciduous forests in eastern North America experienced a widespread and intense spongy moth（Lymantria dispar） infestation in 2021. This study quantified the impact of this spongy moth infestation on carbon（C） cycle in forests across the Great Lakes region in Canada, utilizing high-resolution（10 × 10 m2） Sentinel-2 satellite remote sensing images and eddy covariance（EC） flux data. Study results showed a significant reduction in leaf area index（LAI） and gross primary productivity（GPP） values in deciduous and mixed forests in the region in *** Remote sensing derived, growing season mean LAI values of deciduous（mixed） forests were 3.66（3.18）, 2.74（2.64）, and 3.53（2.94） m2m-2in 2020, 2021 and 2022, respectively, indicating about 24（14）% reduction in LAI, as compared to pre-and post-infestation years. Similarly, growing season GPP values in deciduous（mixed） forests were 1338（1208）, 868（932）, and 1367（1175） g C m-2, respectively in 2020, 2021 and 2022, showing about 35（22）% reduction in GPP in 2021 as compared to pre-and post-infestation years. This infestation induced reduction in GPP of deciduous and mixed forests, when upscaled to whole study area（178,000 km2）, resulted in 21.1（21.4） Mt of C loss as compared to 2020（2022）, respectively. It shows the large scale of C losses caused by this infestation in Canadian Great Lakes *** The methods developed in this study offer valuable tools to assess and quantify natural disturbance impacts on the regional C balance of forest ecosystems by integrating field observations, high-resolution remote sensing data and models. Study results will also help in developing sustainable forest management practices to achieve net-zero C emission goals through nature-based climate change solutions.

关键词： Spongy moth Infestation Carbon Gross ecosystem productivity Leaf area index Temperate forest Remote sensing Sentinel-2 Eddy covariance

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Self-templating synthesis of biomass-based porous carbon nanotubes for energy storage and catalytic degradation applications

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Green Energy & environment 2024年第3期9卷 584-595页

作者： Manman Xu Shiqi Fu Yukai Wen Wei Li Qiongfang Zhuo Haida Zhu Zhikeng Zheng Yuwen Chen Anqi Wang Kai Yan Research centre for Eco-environmental Engineering School of Environment and Civil EngineeringDongguan University of TechnologyDongguan523808China School of environmental Science and Engineering Sun Yat-sen UniversityGuangzhou510275China

Dwindling energy sources and a worsening environment are huge global problems,and biomass wastes are an under-exploited source of material for both energy and material ***,self-template decoction dregs of Ganoderma lucidum-derived porous carbon nanotubes(ST-DDLGCs)were synthesized via a facile and scalable strategy in response to these ***-DDLGCs exhibited a large surface area(1731.51 m^(2)g^(-1))and high pore volume(0.76 cm^(3)g^(-1)),due to the interlacing tubular structures of precursors and extra-hierarchical porous structures on tube *** the ST-DDLGC/PMS system,the degradation efficiency of capecitabine(CAP)reached~97.3%within 120 ***,ST-DDLGCs displayed high catalytic activity over a wide pH range of 3–9,and strong anti-interference to these typical and ubiquitous anions in wastewater and natural water bodies(i.e.,H_(2)PO_(4)^(-),NO_(3)^(-),Cl^(-) and HCO_(3)^(-)),in which a ^(1)O_(2)-dominated oxidation was identified and non-radical mechanisms were ***,ST-DDLGC-based coin-type symmetrical supercapacitors exhibited outstanding electrochemical performance,with specific capacitances of up to 328.1 F g^(-1)at 0.5 A g^(-1),and cycling stability of up to 98.6%after 10,000 cycles at a current density of 2 A g^(-1).The superior properties of ST-DDLGCs could be attributed to the unique porous tubular structure,which facilitated mass transfer and presented numerous active *** results highlight ST-DDLGCs as a potential candidate for constructing inexpensive and advanced environmentally functional materials and energy storage devices.

关键词： Ganoderma lucidum residue Porous carbon nanotubes Self-template method Wastewater treatment Supercapacitor electrode

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A Systematic Analysis of Systems Approach and Flood Risk Management Research:Trends,Gaps,and Opportunities

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International Journal of Disaster Risk Science 2024年第1期15卷 45-57页

作者： Lum Sonita Awah Johanes Amate Belle Yong Sebastian Nyam Israel Ropo Orimoloye Disaster Management Training and Education centre for Africa University of the Free StateBloemfontein 9300South Africa School of environment Geographyand SustainabilityWestern Michigan UniversityKalamazooMI 49008USA

Flooding is a global threat,necessitating a comprehensive management *** to the complexity of managing flood hazards and risks,researchers have advocated for holistic,comprehensive,and integrated *** study,employing a systems thinking perspective,assessed global flood risk management research trends,gaps,and opportunities using132 published documents in BibTeX format.A systematic review of downloaded documents from the Scopus and Web of Science databases revealed slow progress of approximately 11.61% annual growth in applying systems thinking and its concomitant approaches to understanding global flood risk management over the past two decades compared to other fields like water resource management and business management systems.A significant gap exists in the application of systems thinking methodologies to flood risk management research between developed and developing countries,particularly in Africa,highlighting the urgency of reoriented research and policy *** application gaps of the study methodology are linked to challenges outlined in existing literature,such as issues related to technical expertise and resource *** study advocates a shift from linear to holistic approaches in flood risk management,aligned with the Sendai Framework for Disaster Risk Reduction 2015-2023 and the Sustainable Development *** among researchers,institutions,and countries is essential to address this global challenge effectively.

关键词： Flood risk management research Gaps and opportunities global trends in flood research Systematic review.Systems thinking

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Exploring the Roles of Single Atom in Hydrogen Peroxide Photosynthesis

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Nano-Micro Letters 2024年第2期16卷 32-67页

作者： Kelin He Zimo Huang Chao Chen Chuntian Qiu Yu Lin Zhong Qitao Zhang International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education Institute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518000China Queensland Micro‑and Nanotechnology centre School of Environment and ScienceGriffith UniversityNathanQLD 4222Australia Institute for Sustainable Transformation School of Chemical Engineering and Light IndustryGuangdong University of TechnologyGuangzhou 51006China ZJU‑Hangzhou global Scientific and Technological Innovation Center Zhejiang UniversityHangzhou 311215China

This comprehensive review provides a deep exploration of the unique roles of single atom catalysts(SACs)in photocatalytic hydrogen peroxide(H_(2)O_(2))*** offer multiple benefits over traditional catalysts such as improved efficiency,selectivity,and flexibility due to their distinct electronic structure and unique *** review discusses the critical elements in the design of SACs,including the choice of metal atom,host material,and coordination environment,and how these elements impact the catalytic *** role of single atoms in photocatalytic H_(2)O_(2)production is also analysed,focusing on enhancing light absorption and charge generation,improving the migration and separation of charge carriers,and lowering the energy barrier of adsorption and activation of *** these advantages,several challenges,including H_(2)O_(2)decomposition,stability of SACs,unclear mechanism,and low selectivity,need to be *** towards the future,the review suggests promising research directions such as direct utilization of H_(2)O_(2),high-throughput synthesis and screening,the creation of dual active sites,and employing density functional theory for investigating the mechanisms of SACs in H_(2)O_(2)*** review provides valuable insights into the potential of single atom catalysts for advancing the field of photocatalytic H_(2)O_(2)production.

关键词： Single atom catalysts H_(2)O_(2)photosynthesis Catalyst design and optimization

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A CFD study on the hydrodynamic response of a small-scale ice floe induced by a passing ship

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Journal of Hydrodynamics 2024年第2期36卷 290-299页

作者： Zongyu Jiang Spyros Hirdaris Sasan Tavakoli Mikko Suominen Pentti Kujala Marine and Arctic Technology Department of Mechanical EngineeringAalto UniversityEspooFinland global Ship Systems centre ABS Hellenic SM LLC.AthensGreece Department of Infrastructure Engineering The University of MelbourneMelbourneAustralia

A Reynolds averaged Navier-Stokes(RANS)computational fluid dynamics(CFD)model is built to investigate the hydrodynamic response of a circular ice floe under the influence of a passing ship in calm *** ship,mirroring the KRISO Container Ship’s hull design,progresses near an ice floe whose diameter is 30%of the ship’s length and its thickness is 3 *** ship advances at a constant speed,which is handled by using the overset mesh *** study focuses on the ice floe’s motions and the hydrodynamic forces induced by three speeds and three transverse distances of the passing *** reveal that ship-generated wakes notably influence the ice floe’s motions,with a greater influence on sway than ***,the ship’s speed and proximity distinctly affect the ice floe’s motions.

关键词： Hydrodynamics ship-ice interactions ice floe Reynolds averaged Navier-Stokes(RANS)computational fluid dynamics(CFD)

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Variations in Column Concentration of Greenhouse Gases in China and Their Response to the 2015-2016 El Niño Event

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Journal of Meteorological Research 2024年第3期38卷 608-619页

作者： Ningwei LIU Lingjun XIA Youjun DOU Shaorou DONG Jing WEN Ying WANG Rui FENG Ruonan WANG Yuhe LI Institute of Atmospheric environment China Meteorological AdministrationShenyang110166China Jiangxi Ecological Meteorology centre Nanchang330096China Beijing Xiangyuan Academy of Meteorological Observing Technology Beijing100081China Climate centre of Guangdong Province Guangzhou510641China Guangdong Meteorological Service Guangzhou510062China Liaoning Provincial Meteorological Equipment Support centre Shenyang110166China Meteorological centre of Northeast Air Traffic Administration of Civil Aviation of China Shenyang110161China

Since the industrial revolution,enhancement of atmospheric greenhouse gas concentrations as a result of human activities has been the primary cause of global *** monitoring and evaluation of greenhouse gases are significant prerequisites for carbon emission *** monthly data of global atmospheric carbon dioxide(CO_(2))and methane(CH4)column concentrations(hereinafter XCO_(2) and XCH_(4),respectively)retrieved by the Greenhouse Gas Observation Satellite(GOSAT),we analyzed the variations in XCO_(2)and XCH_(4)in China during 2010-2022 after confirming the reliability of the ***,the influence of a strong El Niño event in 2015-2016 on XCO_(2) and XCH_(4) variations in China was further *** results show that the retrieved XCO_(2) and XCH_(4) from GOSAT have similar temporal variation trends and significant correlations with the ground observation and emission inventory data of an atmospheric background station,which could be used to assess the variations in XCO_(2) and XCH_(4) in ***_(2) is high in spring and winter while XCH_(4) is high in *** XCO_(2) and XCH_(4) gradually declined from Southeast China to Northwest and Northeast China,with variation ranges of 401-406 and 1.81-1.88 ppmv,respectively;and the high value areas are located in the middle-lower Yangtze River ***_(2) and XCH_(4) in China increased as a whole during 2010-2022,with rapid enhancement and high levels of XCO_(2) and XCH_(4) in several *** significant increases in XCO_(2) and XCH_(4) over China in 2016 might be closely related to the strong El Niño-Southern Oscillation(ENSO)event during *** a global warming background in 2015,XCO_(2) and XCH_(4) increased by 0.768%and 0.657%in 2016 in *** analysis reveals that both the XCO_(2) and XCH_(4) variations might reflect the significant impact of the ENSO event on glacier melting in the Tibetan Plateau.

关键词： greenhouse gases column concentration CO_(2) CH4 El Niño-Southern Oscillation(ENSO) El Niño

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One-pot synthesis of N-doped petroleum coke-based microporous carbon for high-performance CO_(2) adsorption and supercapacitors

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Journal of environmental Sciences 2024年第5期139卷 93-104页

作者： Wenfu Zhu Yuqin Wang Fan Yao Xiaohong Wang Haoming Zheng Guangzheng Ye Hairong Cheng Junliang Wu Haomin Huang Daiqi Ye School of environment and Energy South China University of TechnologyGuangzhou 510006China National Engineering Laboratory for VOCs Pollution Control Technology and Equipment Guangzhou 510006China Guangdong Provincial Key Laboratory of Atmospheric environment and Pollution Control(SCUT) Guangzhou 510006China Guangdong Provincial Engineering and Technology Research centre for environmental Risk Prevention and Emergency Disposal South China University of TechnologyGuangzhou 510006China

Waste resource utilization of petroleum coke is crucial for achieving global carbon emission ***,a series of N-doped microporous carbons were fabricated from petroleum coke using a one-pot synthesis *** as-prepared samples had a large specific surface area(up to 2512 m^(2)/g),a moderate-high N content(up to 4.82 at.%),and high population(55%)of ultra-micropores(<0.7 nm).Regulating the N content and ultra-microporosity led to efficient CO_(2)adsorption and *** ambient pressure,the optimal N-doped petroleum coke-based microporous carbon exhibited the highest CO_(2)uptake of 4.25 mmol/g at 25℃ and 6.57 mmol/g at 0℃.These values are comparable or even better than those of numerous previously reported adsorbents prepared by multistep synthesis,primarily due to the existence of *** sample exhibited excellent CO_(2)/N_(2)selectivity at 25℃ owing to the abundant basic pyridinic and pyrrolic N species;and showed superior CO_(2)adsorption-desorption cycling performance,which was maintained at 97% after 10 cycles at 25℃.Moreover,petroleum coke-based microporous carbon,with a considerably high specific surface area and hierarchical pore structure,exhibited excellent electrochemical performance over the N-doped sample,maintaining a favorable specific capacitance of 233.25F/g at 0.5 A/g in 6 mol/L KOH aqueous *** study provides insight into the influence of N-doping on the porous properties of petroleum coke-based ***,the as-prepared carbons were found to be promising adsorbents for CO_(2)adsorption,CO_(2)/N_(2)separation and electrochemical application.

关键词： One-pot synthesis N-doped microporous carbon CO_(2)adsorption CO_(2)/N_(2)selectivity Electrochemical performance

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Reply to “Beyond microbial carbon use efficiency”

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National Science Review 2024年第4期11卷 35-37页

作者： Feng Tao Johannes Lehmann Ying-Ping Wang Lifen Jiang Bernhard Ahrens Kostiantyn Viatkin Stefano Manzoni Benjamin Z.Houlton Yuanyuan Huang Xiaomeng Huang Yiqi Luo Department of Ecology and Evolutionary Biology Cornell University Soil and Crop Sciences Section School of Integrative Plant ScienceCornell University CSIRO environment Max Planck Institute for Biogeochemistry Department of Physical Geography and Bolin centre for Climate Research Stockholm University Department of global Development Cornell University Key Laboratory of Ecosystem Network Observation and Modeling Institute of Geographic Sciences and Natural Resources Research Chinese Academy of Sciences Department of Earth System Science Ministry of Education Key Laboratory for Earth System Modelling Institute for Global Change Studies Tsinghua University

In their commentary, Xiao et al.[1]cautioned that the conclusions on the critical role of microbial carbon use efficiency (CUE) in global soil organic carbon (SOC) storage in the paper by Tao et al.[2] might be too *** claimed that Tao et al.’s study lacked mechanistic consideration of SOC formation and excluded important data *** et al. brought up important points,which can be largely reconciled with our findings by understanding the differences in expressing processes in empirical studies and in models.

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