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Science China(Information sciences) 2025年第1期68卷 400-401页

作者： Chenyu LIU Yibo WANG Wenhui XU Shuqi HUANG Chunxiao YU Zeyu YANG Xiaole JIA Xiaoxi LI Bochang LI Zhengdong LUO Cizhe FANG Yan LIU Tiangui YOU Xin OU Genquan HAN School of Microelectronics Xidian University Suzhou Institute of nano-Tech and nano-Bionics Chinese Academy of Sciences Shanghai Institute of Microsystem and Information Technology Chinese Academy of Sciences Hangzhou Institute of Technology Xidian University

Titanium/Gold （Ti/Au） metals have been widely employed as ohmic metal contacts on n+Ga2O3,exhibiting the specific contact resistance （ρc） of 10-5-10-6Ω·cm2[1].But previous studies have revealed the presence of a defective Ga2O3layer and reactive Ti-Ga2O3layer at the annealed Ti/*** an interfacial layer can afect the performance of ohmic contact,which may become more pronounced in power devices subjected to electrical stress and high-frequency ***,there have been no reports on the impact of bias stress effects and dynamic degradation of Ti/Au ohmic contacts on n+Ga2O3.

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Polymerized-ionic-liquid-based solid polymer electrolyte for ultra-stable lithium metal batteries enabled by structural design of monomer and crosslinked 3D network

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Materials Reports(Energy) 2025年第1期5卷 61-69页

作者： Lingwang Liu Jiangyan Xue Yiwen Gao Shiqi Zhang Haiyang Zhang Keyang Peng Xin Zhang Suwan Lu Shixiao Weng Haifeng Tu Yang Liu Zhicheng Wang Fengrui Zhang Daosong Fu Jingjing Xu Qun Luo Xiaodong Wu School of nano-Tech and nano-Bionics University of Science and Technology of ChinaHefei230026China i-Lab Suzhou Institute of Nano-Tech and Nano-Bionics(SINANO)Chinese Academy of SciencesSuzhou215123China School of Materials Science and Engineering Shanghai UniversityShanghai200444China Tianmu Lake Institute of Advanced Energy Storage Technologies Liyang213300China Institute of Physics Chinese Academy of sciences Beijing100190China College of Material Science and Engineering Hohai UniversityChangzhou213022China

Solid polymer electrolytes(SPEs)have attracted much attention for their safety,ease of packaging,costeffectiveness,excellent flexibility and ***-dioxolane(PDOL)is one of the most promising matrix materials of SPEs due to its remarkable compatibility with lithium metal anodes(LMAs)and suitability for in-situ ***,poor thermal stability,insufficient ionic conductivity and narrow electrochemical stability window(ESW)hinder its further application in lithium metal batteries(LMBs).To ameliorate these problems,we have successfully synthesized a polymerized-ionic-liquid(PIL)monomer named DIMTFSI by modifying DOL with imidazolium cation coupled with TFSI^(-)anion,which simultaneously inherits the lipophilicity of DOL,high ionic conductivity of imidazole,and excellent stability of *** the tridentate crosslinker trimethylolpropane tris[3-(2-methyl-1-aziridine)propionate](TTMAP)was introduced to regulate the excessive Li^(+)-O coordination and prepare a flame-retardant SPE(DT-SPE)with prominent thermal stability,wide ESW,high ionic conductivity and abundant Lit transference numbers(t_(Li+)).As a result,the LiFePO_(4)|DT-SPE|Li cell exhibits a high initial discharge specific capacity of 149.60 mAh g^(-1)at 0.2C and 30℃with a capacity retention rate of 98.68%after 500 *** work provides new insights into the structural design of PIL-based electrolytes for long-cycling LMBs with high safety and stability.

关键词： Polymerized ionic liquid Solid polymer electrolyte Structural design Crosslinked 3D network Lithium metal battery

Mixed-charge glycopolypeptides as antibacterial coatings with long-term activity

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Chinese Chemical Letters 2025年第2期36卷 270-278页

作者： Fangping Yang Jin Shi Yuansong Wei Qing Gao Jingrui Shen Lichen Yin Haoyu Tang Institute of Functional nano & Soft Materials(FUNSOM) Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow University

Planktonic bacteria adhere and subsequently form biofilms on implantable medical devices can cause severe infections that have become the major types of hospital-acquired infections. Traditional coatings for the implants are frequently lack of long-term antifouling and bactericidal activities. It is still a big challenge to simultaneously improve the antifouling and bactericidal activities of the coatings. Herein,we report that mixed-charge glycopolypeptide coatings are of long-term antibacterial activities to efficiently inhibit the biofilm growth. The glycosylation of mixed-charge polypeptides has led to a significant improvement of both antifouling and bactericidal activities. The cooperative effect of the saccharide residues and mixed-charge residues improved the resistance of the polypeptide coatings against protein adsorption. The saccharide and L-glutamic acid(E) residues collectively enhanced the bacterial membrane-disruption of cationic L-lysine(K) residues, leading to potent bactericidal activity. Meanwhile,the glycopolypeptide coatings showed superior biocompatibility, long-term antibiofilm and anti-infection properties in two types of mouse subcutaneous infection models and one type of mouse urinary tract infection model. This work provides a new strategy to achieve antibacterial coatings with long-term activities for preventing implantable medical device associated infections.

关键词： Antibacterial coating Bactericidal activity Biofilm Fouling Glycopolypeptide

Hybrid and enhanced electrokinetic system for soil remediation from heavy metals and organic matter

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Journal of Environmental sciences 2025年第1期147卷 424-450页

作者： Faris M.Hamdi Namuun Ganbat Ali Altaee Akshaya K.Samal Ibrar Ibrar John L.Zhou Adel O.Sharif Centre for Green Technology School of Civil and Environmental EngineeringThe University of Technology Sydney15 BroadwayNSW 2007Australia Department of Civil Engineering Jazan UniversityJazan 82822Saudi Arabia Centre for nano and Material sciences Jain UniversityRamanagaraBangaloreKarnataka 562112India School of Mechanical sciences Faculty of Engineering and Physical SciencesUniversity of SurreyAustralia

The electrokinetic(EK)process has been proposed for soil decontamination from heavy metals and organic *** advantages of the EK process include the low operating energy,suitability for fine-grained soil decontamination,and no need for *** the last three decades,enhanced and hybrid EK systems were developed and tested for improving the efficiency of contaminants removal from *** enhanced-EK processes exhibited excellent efficiency in removing contaminants by controlling the soil pH or the chemical reaction of *** hybrid systems were tested to overcome environmental hurdles or technical drawbacks of decontamination *** of the EK process with phytoremediation,bioremediation,or reactive filtermedia(RFM)improved the remediation process performance by capturing contaminants or facilitating biological agents’movement in the ***,EK process coupling with solar energy was proposed to treat off-grid contaminated soils or reduce the EK energy *** study reviews recent advancements in the enhancement and hybrid EK systems for soil remediation and the type of contaminants targeted by the *** study also covered the impact of operating parameters,imperfect pollution separation,and differences in the physicochemical characteristics and microstructure of soil/sediment on the EK ***,a comparison between various remediation processes was presented to highlight the pros and cons of these technologies.

关键词： Electrokinetic Soil remediation Reactive filter media Enhanced electrokinetic Contaminants

Regulating crystallization and retarding oxidation in Sn-Pb perovskite via 1D cation engineering for high performance all-perovskite tandem solar cells

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Journal of Energy Chemistry 2025年第1期100卷 646-652页

作者： Ranran Liu Xin Zheng Zaiwei Wang Miaomiao Zeng Chunxiang Lan Shaomin Yang Shangzhi Li Awen Wang Min Li Jing Guo Xuefei Weng Yaoguang Rong Xiong Li Michael Grätzel Center for Mesoscopic Solar Cells Wuhan National Laboratory for OptoelectronicsHuazhong University of Science and TechnologyWuhan 430074HubeiChina Institute of Technology for Carbon Neutrality Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055GuangdongChina School of Chemistry Chemical Engineering and Life SciencesState Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of Technology430070HubeiChina Suzhou Institute of nano-Tech and nano-Bionics(SInano) Chinese Academy of SciencesSuzhou 215123JiangsuChina School of Physics and Optoelectronic Engineering Hainan UniversityHaikou 570228HainanChina

All-perovskite tandem solar cells have the potential to surpass the theoretical efficiency limit of single junction solar cells by reducing thermalization ***,the challenges encompass the oxidation of Sn^(2+)to Sn^(4+)and uncontrolled crystallization kinetics in Sn-Pb perovskites,leading to nonradiative recombination and compositional heterogeneity to decrease photovoltaic efficiency and operational ***,we introduced an ionic liquid additive,1-ethyl-3-methylimidazolium iodide (EMIMI) into Sn-Pb perovskite precursor to form low-dimensional Sn-rich/pure-Sn perovskites at grain boundaries,which mitigates oxidation of Sn^(2+)to Sn^(4+)and regulates the film-forming dynamics of Sn/Pb-based perovskite *** optimized single-junction Sn-Pb perovskite devices incorporating EMIMI achieved a high efficiency of 22.87%.Furthermore,combined with wide-bandgap perovskite sub-cells in tandem device,we demonstrate 2-terminal all-perovskite tandem solar cells with a power conversion efficiency of 28.34%,achieving improved operational stability.

关键词： All-perovskite tandem solar cells Sn-Pb perovskite 1D Regulated crystallization Antioxidation

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Enhancing micro-scale SiOx anode durability:Electro-mechanical strengthening of binder networks via anchoring carbon nanotubes with carboxymethyl cellulose

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Journal of Energy Chemistry 2025年第2期101卷 23-33页

作者： Chaeyeon Ha Jin Kyo Koo Jun Myoung Sheem Young-Jun Kim SKKU Advanced Institute of nano Technology (SAINT) Sungkyunkwan University Department of nano Science and Technology Sungkyunkwan University Advanced Center for Convergence Energy Storage System Sungkyunkwan University SKKU Institute of Energy Science and Technology (SIEST) Sungkyunkwan University

With the increasing prevalence of lithium-ion batteries（LIBs） applications,the demand for high-capacity next-generation materials has also *** currently considered a promising anode material due to its exceptionally high capacity for ***,the significant volumetric changes of SiOxduring cycling and its initial Coulombic efficiency（ICE） complicate its use,whether alone or in combination with graphite *** this study,a three-dimensional conductive binder network with high electronic conductivity and robust elasticity for graphite/SiOxblended anodes was proposed by chemically anchoring carbon nanotubes and carboxymethyl cellulose binders using tannic acid as a chemical *** addition,a dehydrogenation-based prelithiation strategy employing lithium hydride was utilized to enhance the ICE of *** combination of these two strategies increased the CE of SiOxfrom 74% to87% and effectively mitigated its volume expansion in the graphite/SiOxblended electrode,resulting in an efficient electron-conductive binder *** led to a remarkable capacity retention of 94% after30 cycles,even under challenging conditions,with a high capacity of 550 mA h g-1and a current density of 4 mA ***,to validate the feasibility of utilizing prelithiated SiOxanode materials and the conductive binder network in LIBs,a full cell incorporating these materials and a single-crystalline Ni-rich cathode was *** cell demonstrated a～27.3% increase in discharge capacity of the first cycle(～185.7 mA h g-1) and exhibited a cycling stability of 300 ***,this study reports a simple,feasible,and insightful method for designing high-performance LIB electrodes.

关键词： Lithium-ion batteries SiO x anode Blended anode Carbon nanotubes Carboxymethyl cellulose Conductive binder network

Flat-band based high-temperature ferromagnetic semiconducting state in the graphitic C4N3 monolayer

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Fundamental Research 2025年第1期5卷 138-144页

作者： Chaoyu He Yujie Liao Tao Ouyang Huimin Zhang Hongjun Xiang Jianxin Zhong Laboratory for Quantum Engineering and Micro-nano Energy Technology and School of Physics and Optoelectronics Xiangtan UniversityXiangtan 411105China Key Laboratory of Computational Physical sciences(Ministry of Education) Institute of Computational Physical SciencesDepartment of PhysicsFudan UniversityShanghai 200433China

Half-filled isolated flat-band paves a new way to realize high-temperature ferromagnetic semiconductor for spintronics applications,but it is extremely rare in lattice models and lacking in realistic ***,the 2×2 super-cell of the honeycomb lattice with a single-hole defect is proposed as a new lattice model(HL-D-1/8)to realize nontrivial isolated *** further demonstrate that C_(4)N_(3)monolayer of the experimentally realized graphitic carbon nitride(***.,22,1004,2010;***.,9,3366,2018)is a perfect system holding such a lattice to host flat-bands.A new corrugated Pca21 configuration is proposed as the ground state for the free-standing C_(4)N_(3)monolayer,which is dynamically stable and energetically more favorable than the widely-used flat one without dynamical *** Pca21 configuration is found to be an intrinsic ferromagnetic half-semiconductor(T_(c)≈241 K)with one semiconducting spin-channel(1.75 eV)and one insulating spin-channel(3.64 eV),which is quite rare in two-dimensional *** ferromagnetic semiconducting property originates from the isolated pz-state flat-band as the corrugation shifts the flat-band upward to the Fermi ***,such a corrugated Pca21 C_(4)N_(3)monolayer is found to be both piezoelectric and ferroelectric,which makes it an unusual metal-free two-dimensional multiferroic.

关键词： Graphitic C_(4)N_(3) Isolated flat-band Ferromagnetic semiconductor Two-dimensional multiferroic First-principles calculation Tight-binding model

High-performance visible-infrared broadband transparent copper mesh conductor and applications for electromagnetic shielding and heating

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Science China Materials 2025年第2期68卷 421-431页

作者： Tengfei Li Xiaolian Chen Zhaohua Xu Shuhong Nie Wenya Xu Wei Yuan Su Xu Shuo Zhang Fangfang Pei Wenming Su Zheng Cui School of nano-Tech and nano-Bionics University of Science and Technology of ChinaHefei 230026China Printable Electronics Research Center Nano-Devices and Materials DivisionSuzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China

Transparent conductors(TCs)have widespread applications in the fields of modern photodetectors and smart *** TCs for visible wavelengths have seen significant advancements,the development of visible-infrared(vis-IR)broadband TCs for infrared is still a daunting challenge due to the trade-off between infrared transparency and ***,we present a vis-IR TC fabricated by using a damage-free indirect transfer *** method involves polymer-mediated bonding of a high-resolution,standalone copper(Cu)mesh onto infrared or visible substrates via a transfer *** obtained Cu mesh TC exhibits excellent conductivity with a sheet resistance as low as 0.06Ω/□,as well as 81%transmittance at a visible wavelength of 550 nm and 65%transmittance at an IR wavelength of 10μ***,a specially developed bonding strategy ensures the longterm reliability of the Cu mesh TC in harsh *** Cu mesh TC can be applied in both heating and electromagnetic(EM)*** a transparent heater,it reaches approximately 100℃ at an applied voltage of 1.2 V within 100 *** EM shielding,a demonstration using a stainlesssteel box with a transparent observation window which is integrated with the Cu mesh shows that while the window allows both optical and IR observations,the 4G signals(8.2 GHz)of a smartphone inside the box are effectively blocked.

关键词： infrared visible transparent conductors electromagnetic shielding Cu mesh

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Long-duration aqueous Zn-ion batteries achieved by dual-salt highly-concentrated electrolyte with low water activity

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Journal of Energy Chemistry 2025年第2期101卷 778-785页

作者： Lvzhang Jiang Lingbo Yao Gege Wang Chang Liu Xiaowei Chi Yu Liu Shanghai Institute of Ceramics Chinese Academy of Sciences University of Chinese Academy of sciences

Aqueous Zn-ion batteries have attracted much attention due to their unique high safety and low-cost ***,their practical applications are at a slow pace due to their short cycle life,which fundamentally results from the instability of the positive/negative electrode interface in the traditional dilute aqueous electrolytes with high water *** highly concentrated electrolyte（HCE）has been considered as an effective *** previous studies of single salt-based HCE（SSHCE）,herein,a new dual-salt HCE（15 m ZnCl2+10 m NH4NH2SO3DS-HCE） was proposed for the first ***-HCE was proven to simultaneously possess higher conductivity than traditional dilute electrolytes and ultralow water activity of SS-HCE by the regulation of dual high-concentration salts on the solvation structure,which renders the Zn‖Zn symmetric cell the record-long cycling life of 2200 h compared with those with SS-HCE（30 m ZnCl2,300 h） and other reported ***,the Zn‖NH4V4O10full cell with DS-HCE demonstrated impressed rate capability within a wide-range current densities from 0.1 to 10 A ***,at the high current density of 5 A g-1,the full cell shows almost100% capacity retention after 4000 cycles,which indicates the promising future of the DS-HCE system for long-duration aqueous Zn-ion batteries.

关键词： Ammonium vanadate Aqueous zinc battery Cycling stability Electrolyte

A cylindrical rod ultrasonic motor with 1 mm diameter and its application in endo-scopic OCT

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Chinese Science Bulletin 2005年第8期50卷 826-830页

作者： ZHOUTieying ZHANGKai CHENYu WANGHuan WUJigang JIANGKaili XUEPing departmentofphysicsandkeylaboratoryofatomicandmolecular-nano-sciences MinistryofEducationTsinghuaUniversityBeijing100084China

A tiny ultrasonic motor was constructed by using a piezoelectric ceramic cylindrical rod as a vibration generator of the stator. The fabricated tiny motor has a di- ameter of 1 mm, a length of 5 mm and a weight of 36 mg. The resonant frequency is 32 kHz with one fixed boundary or 83 kHz with two free boundaries. Four silver electrodes were deposited on the cylindrical surface. The spacing be- tween two adjacent electrodes was carefully designed. A method was developed for the polarization of the stator. By using the bending vibration mode of the stator, the motor shows a performance with a speed of 1800 rpm and a stalled torque of 4 μ Nm, and can bear a high driving voltage up to 350 Vpp. The motor was used to drive an optical prism for circular scanning in an endoscopic OCT system. The tomo- graphic images of the inner cavities of a plastic tube and a scallion were obtained, and the resolution was of the order of micrometer-scale.

关键词：圆柱杆超声波电机摆动弯度内窥镜检查循环扫描

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