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Magnetron sputtered nickel oxide with suppressed interfacial defect states for efficient inverted perovskite solar cells

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Journal of Energy Chemistry 2025年第1期100卷 348-355页

作者： Guoqiang Ma Qin Tan Zhaoning Li Jingwei Xiu Jiafeng Wang Tianle Cheng Dong He Qiang Sun Xuhang Ma Francesco Lamberti Zhubing He department of Materials Science and engineering Institute of Innovative Materials (I2M) Shenzhen Key Laboratory of Full Spectral Solar Electricity Generation (FSSEG)Southern University of Science and Technology (SUSTech) Core Research Facilities Southern University of Science and Technology department of Chemical Sciences Department of Industrial Engineering University of Padova

Widely used spin-coated nickle oxide （NiOx） based perovskite solar cells often suffer from severe interfacial reactions between the NiOxand adjacent perovskite layers due to surface defect states,which inherently impair device performance in a long-term view,even with surface molecule *** this study,we developed high-quality magnetron-sputtered NiOxthin films through detailed process optimization,and compared systematically sputtered and spin-coated NiOxthin film surfaces from materials to *** sputtered NiOxfilms exhibit improved crystallinity,smoother surfaces,and significantly reduced Ni3+or Ni vacancies compared to their spin-coated ***,the interface between the perovskite and sputtered NiOxfilm shows a substantially reduced density of defect *** solar cells （PSCs） fabricated with our optimally sputtered NiOxfilms achieved a high power conversion efficiency （PCE） of up to 19.93%and demonstrated enhanced stability,maintaining 86.2% efficiency during 500 h of maximum power point tracking under one standard sun ***,with the surface modification using (4-(2,7-dibromo-9,9-dimethylacridin-10（9H）-yl)butyl)p hosphonic acid （DMAcPA）,the device PCE was further promoted to 23.07%,which is the highest value reported for sputtered NiOxbased PSCs so far.

关键词： Nickle oxide Magnetron sputter Defect Stability Perovskite solar cell

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Maximizing biomass utilization: An integrated strategy for coproducing multiple chemicals

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Journal of Energy Chemistry 2025年第1期100卷 180-191页

作者： Byeongchan Ahn Sua Jo Jonggeol Na J.Jay Liu Young-Ju Kim Wangyun Won department of Chemical and Biological engineering Korea University department of Chemical engineering (Integrated process) Kyung Hee University department of Chemical engineering and Materials Science Ewha Womans University department of Chemical engineering Pukyong National University Resources engineering Plant Research department Korea Institute of Geoscience and Mineral Resources

Lignocellulosic biomass is one of the viable solutions to alleviate the global warming. However, the limited utilization of biomass majorly focused on cellulose and hemicellulose restricts the economic and environmental feasibilities. To cope with this issue, we proposed an integrated process of co-producing 1,6-hexanediol（1,6-HDO） with tetrahydrofuran and adipic acid from biomass, referred to as Strategy A. To compare the impacts of lignin upgrading and feedstock, Strategy B, which co-produces tetrahydrofuran alone, and Strategy C, which is the traditional route to produce 1,6-HDO from fossil fuels, were used. Heat networks are also designed to reduce operating costs and indirect carbon emissions due to energy consumption, saving 87% and 83% of the heat and cooling requirements, respectively, in Strategy A. The market competitiveness of Strategy A was evaluated by determining the minimum selling price through techno-economic analysis, and sustainability was thoroughly investigated by quantifying the environmental impacts through both midpoint and endpoint life-cycle assessments（LCAs）.Strategy A was found to be the most favorable both economically（USRDSCHARDOLLAR3,402/ton） and environmentally（-26.9 kg CO2eq.）. This indicates that lignin valorization is not only economically but also environmentally preferred. Finally, changes in economic and environmental feasibilities depending on economic, process, and environmental parameters were investigated using sensitivity and uncertainty analyses. The results of these analyses provide valuable insight into bio-based chemical production.

关键词： Biorefinery Carbon mitigation Climate change Global warming Lignin utilization Bioeconomy

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Optimized guided mode resonant structure as thermooptic sensor and liquid crystal tunable filter

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Chinese Optics Letters 2009年第8期7卷 667-670页

作者： I.Abdulhalim department of Electrooptic engineering Ben Gurion University of the Negev

Applicability of guided mode resonant structures to tunable optical filtering and sensing is demonstrated using nematic liquid crystals. As a sensor, a minimum refractive index detectivity of 10^-5 is demonstrated while as a tunable filter, tunability range of few tens of nanometers with 2-nm bandwidth is presented. The optimum design is achieved by maximizing the evanescent field region in the analyte which maximizes the overlap integral. The device can be operated in reflection or transmission modes at normal incidence. It can also be operated at a single wavelength by measuring the angular profile of the light beam.

关键词： mode Optimized guided mode resonant structure as thermooptic sensor and liquid crystal tunable filter

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On helical behavior of turbulence in the ship wake

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Journal of Hydrodynamics 2013年第1期25卷 83-90页

作者： GOLBRAIKH Ephim EIDELMAN Alexander SOLOVIEV Alex Physics department Ben-Gurion University of the Negev Mechanical engineering department Ben-Gurion University of the Negev Oceanographic Center NOVA South eastern University

Turbulent ship wake conservation at a long distance is among unsolved problems at present. It is well known that far wakes have a vortical structure and slowly expand with distance. As was obtained by Dubrovin et al., slow expansion of the wake may be related to the distribution of turbulent viscosity in it. In our work we study the effect of helicity in the wake on the behavior of turbulent viscosity. Taking into account the helical nature of the wake, we can clarify the difference between turbulence inside and outside the wake on the one hand and slowing down of its expansion with time on the other hand.

关键词： ship wake turbulent ship wake helical turbulence

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X-Ray Photoelectron Spectroscopy Study of the Metal/Cermet Interface

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Chinese Physics Letters 2001年第1期18卷 94-96页

作者： LU Hua SHEN Dian-Hong XUE Qi-Kun M.Polak N.Froumin department of Materials engineering Ben-Gurion University of the NegevIsrael

Interfacial reactions between aluminium and polycrystalline cermet TiC_(0.6) were investigated using x-ray photoelectron spectroscopy,Auger electron spectroscopy and x-ray *** was found that titanium exists in two chemical *** carbide and oxide of titanium can be detected simultaneously,and the atomic ratio of Ti:C:O is 5:3:*** suggests that TiC^(0.6) is a Ti-oxycarbide or oxygenated TiC composite:Ti_(5)C_(3)O_(2)(TiO_(2)+4TiC_(0.75)).When Al is deposited in vacuum on the Ti-oxycarbide surface,the active Al atoms react chemically only with TiO_(2) at room temperature,but not with Tico.75 in *** reaction products are Al2O3 and theintermetallic compound Als *** the Al/TiC_(0.6) interface at 750℃,Al reacts also with TiC_(0.75) to form a brittle Al_(4)C_(3) phase.

关键词： carbide diffraction. intermetallic

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Yaw stability control for a rear double-driven electric vehicle using LPV-H∞ methods

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Science China(Information Sciences) 2018年第7期61卷 82-94页

作者： Yonathan WEISS Liron I.ALLERHAND Shai AROGETI department of Mechanical engineering Ben-Gurion University of the Negev Bio Catch

This paper presents a new yaw stability controller for a rear double-driven electric vehicle. A linear parameter varying(LPV) model of the vehicle is formulated using longitudinal speed measurement and tire cornering stiffness estimation. The LPV model is then utilized to design a gain-scheduled H∞controller with guaranteed stability. Results from simulations, performed with Car Sim, show that the new controller improves the vehicle performance and handling even in extreme maneuvers and that it is robust to model parameter uncertainties.

关键词： yaw stability control electric vehicle torque vectoring H_∞ control gain-scheduling

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Ru/NiMnB spherical cluster pillar for highly proficient green hydrogen electrocatalyst at high current density

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Journal of Energy Chemistry 2025年第1期100卷 397-408页

作者： Md Ahasan Habib Shusen Lin Mehedi Hasan Joni Sumiya Akter Dristy Rutuja Mandavkar Jae-Hun Jeong Jihoon Lee department of Electronic engineering College of Electronics and Information Kwangwoon University

Advanced OER/HER electrocatalytic alternatives are crucial for the wide adaptation of green hydrogen ***,Ru/NiMnB spherical cluster pillar （SCP）,denoted as Ru/NiMnB,is synthesized using a combination of electro-deposition and hydrothermal *** investigation of Ru doping in the NiMnB matrix revealed significant improvements in electrocatalytic *** Ru/NiMnB SCPs demonstrate superior OER/HER activity with low overpotentials of 150 and 103 mV at 50mA/cm2in 1 M KOH,making them highly competitive with state-of-the-art ***,the Ru/NiMnB SCPs exhibit a low 2-E cell voltage of 2.80 V at ultra-high current density of 2,000 m A/cm2in 1 M KOH,outperforming the standard benchmark electrodes of RuO2||Pt/C,thereby positioning Ru/NiMnB as one of the best bifunctional *** SCPs exhibit exceptional high-current characteristics,stability and corrosion resistance,as evidenced by continuous operation at 1,000 mA/cm2high-current density for over 150 h in 6 M KOH at elevated temperatures under harsh industrial *** a small amount of Ru incorporation significantly enhances the electrocatalytic performances of NiMnB,attributed to increased active sites and improved intrinsic properties such as conductivity,adsorption/desorption capability and reaction ***,Ru/NiMnB SCPs present a promising bi-functional electrode concept for efficient green H2production.

关键词： Advanced electrocatalyst High current Corrosion resistance industrial requirement

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The detrimental effect of autofrettage on externally cracked modern tank gun barrels

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Defence Technology（防务技术） 2019年第2期15卷 146-153页

作者： M.Perl T.Saley Pearlstone Center for Aeronautical engineering Studies Department of Mechanical Engineering Ben-Gurion University of the Negev

Overstraining gun tubes has a twofold advantage. First, it enables the increase of the Safe Maximum Pressure(SMP) in the tube, resulting in a higher muzzle velocity which extends the gun's range and its projectile kinetic energy. Second, it reduces the tube's susceptibility to internal cracking which prolongs its fatigue life. Unfortunately, autofrettage also bears an inherent detrimental effect as it considerably increases the tensile hoop stress at the outer portion of the barrel's wall, which enhances external cracking of the tube by increasing the prevailing Stress Intensity Factor(SIF). In order to quantify this disadvantageous effect, 3-D Mode I SIFs distributions along the front of a single external radial semielliptical crack initiating from the outer surface of an autofrettaged modern gun barrel, overstrained by either the Swage or the Hydraulic autofrettage processes, are evaluated. The analysis is performed by the finite element(FE) method, using singular elements along the crack front. Innovative residual stress fields(RSFs), incorporating the Bauschinger effect for both types of autofrettage are applied to the ***'s [1] RSF is also applied to the tube for comparison reasons. All three RSFs are incorporated in the FE analysis, using equivalent temperature fields, Values for K_(IA)-the SIF resulting from the tensile residual stresses induced by autofrettage are evaluated for: a typical barrel of radii ratio R_o/R_i = 2, crack depth to wall-thickness ratios(a/t = 0.005-0.1),crack ellipticities(a/c = 0.2-1.0),and five levels of Swage,Hydraulic and Hill's autofrettage(e = 40%,60%,70%,80%,and 100%). In total,375 different 3-D cases are analyzed. The analysis demonstrates undoubtedly the detrimental effect of all types of autofrettage in increasing the prevailing effective stress intensity factor of external cracks, resulting in crack initiation enhancement and crack growth rate acceleration which considerably shortens the total fatigue life of the bar

关键词： Gun barrel Swage and hydraulic autofrettage External crack 3-D Finite element

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Three-dimensional single particle tracking using 4π self-interference of temporally phase-shifted fluorescence

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Light(Science & Applications) 2023年第3期12卷 415-424页

作者： Leanne Maurice Alberto Bilenca Biomedical engineering department Ben-Gurion University of the Negev1 Ben Gurion BlvdBe’er-Sheva84105Israel Ilse Katz Institute for Nanoscale Science and Technology Ben-Gurion University of the Negev1 Ben Gurion BlvdBe’er-Sheva84105Israel

Single particle tracking in three dimensions is an indispensable tool for studying dynamic processes in various disciplines,including material sciences,physics,and biology,but often shows anisotropic three-dimensional spatial localization precision,which restricts the tracking precision,and/or a limited number of particles that can be tracked simultaneously over extended *** we developed an interferometric,three-dimensional fluorescence single particle tracking method based on conventional widefield excitation and temporal phase-shift interference of the emitted,high-aperture-angle,fluorescence wavefronts in a greatly simplified,free-running,triangle interferometer that enables tracking of multiple particles at the same time with<10-nm spatial localization precision in all three dimensions over extended volumes(~35×35×2μm^(3))at video rate(25 Hz).We applied our method to characterize the microenvironment of living cells and up to~40μm deep in soft materials.

关键词： materials particle dimensions

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Graphene foam resonators:Fabrication and characterization

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Nano Research 2022年第1期15卷 225-229页

作者： Yahav ben-Shimon Siva KReddy Assaf Ya'akobovitz department of Mechanical engineering Faculty of Engineering SciencesBen-Gurion University of the NegevIsrael

Three-dimensional graphene foams(GFs)benefit from a large surface area and unique physical *** present here the first-ever miniaturized GF-based *** developed a simple yet reliable fabrication process,in which GFs are synthesized and assembled on a cavity to form suspended GF *** electrostatically excited these devices and analyzed their resonance and ring-down *** observed significant energy dissipation,as the quality factor of the devices was in the order of several ***,we investigated the influence of temperature on the operation of the devices and found that high temperatures mechanically soften the resonators but also considerably enhance energy ***,our devices demonstrated a mode-coupling of a resonance mode and a mode having twice its ***,this work paves the way toward the development of novel GF resonators that could be integrated into future devices,such as GF-based nano-electromechanical sensors,electrical circuits,and oscillators.

关键词： energy dissipation graphene foam micro/nano electromechanical systems three-dimensional graphene resonators

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