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Visualized SERS Imaging of Single Molecule by Ag/ Black Phosphorus Nanosheets

Nano-Micro Letters 2022年第5期14卷 47-61页

作者： Chenglong Lin Shunshun Liang Yusi Peng Li Long Yanyan Li Zhengren Huang Nguyen Viet Long Xiaoying Luo Jianjun Liu Zhiyuan Li Yong Yang State Key Laboratory of High‑Performance Ceramics and Superfine Microstructures Shanghai Institute of CeramicsChinese Academy of Sciences1295 Dingxi RoadShanghai 200050People’s Republic of China Graduate School of the Chinese Academy of Sciences No.19(A)Yuquan RoadBeijing 100049People’s Republic of China Center of Materials Science and Optoelectronics engineering University of Chinese Academy of SciencesBeijing 100049People’s Republic of China State Key Laboratory of Oncogenes and Related Genes Shanghai Cancer InstituteRenji HospitalShanghai Jiaotong University School of Medicine200032 ShanghaiPeople’s Republic of China School of Physics and Optoelectronics South China University of TechnologyGuangzhou 510641People’s Republic of China department of electronics and telecommunications Saigon UniversityHochiminh CityVietnam

Single-molecule detection and imaging are of great value in chemical analysis,biomarker identification and other trace detection ***,the localization and visualization of single molecule are still quite a ***,we report a special-engineered nanostructure of Ag nanoparticles embedded in multi-layer black phosphorus nanosheets(Ag/BP-NS)synthesized by a unique photoreduction method as a surfaceenhanced Raman scattering(SERS)*** a SERS substrate features the lowest detection limit of 10^(–20) mol L^(−1) for R6G,which is due to the three synergistic resonance enhancement of molecular resonance,photoinduced charge transfer resonance and electromagnetic *** propose a polarization-mapping strategy to realize the detection and visualization of single *** addition,combined with machine learning,Ag/BP-NS substrates are capable of recognition of different tumor exosomes,which is meaningful for monitoring and early warning of the *** work provides a reliable strategy for the detection of single molecule and a potential candidate for the practical bio-application of SERS technology.

关键词： Black phosphorus Single molecule SERS Exosome Machine learning

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Synergetic analysis of springtime air pollution episodes over Gwangju,Korea

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Journal of Environmental Sciences 2017年第7期29卷 270-283页

作者： Sung-Kyun Shin Kwon-Ho Lee Seung-Shik Park Man Sing Wong Research Institute for Radiation-Satellite(RIRS) Gangneung-Wonju National University(GWNU)Gangneung 25457Republic of Korea department of Atmospheric and Environmental Sciences(DAES) Gangneung-Wonju National University(GWNU)Gangneung 25457Republic of Korea department of Environment and Energy engineering Chonnam National UniversityGwangju 61186Republic of Korea department of Land Surveying and Geo-Informatics The Hong Kong Polytech UniversityKowloonHong Kong

The characteristics of springtime aerosols,including their optical and microphysical properties,were analyzed for the months of March to May of 2009 in Gwangju（35.23°N,126.84°E）,Korea.A high Light Detection and Ranging（LIDAR）-derived aerosol depolarization ratio（δ） of 0.25 ± 0.04 was determined on dust particles during the observation ***？ngstr？m exponent values of the 440–870 nm wavelength pair（？_（440–870）） and single-scattering albedo at 675 nm（Ω_（675）） measured by a CIMEL sun/sky radiometer were 0.77 ± 0.19 and 0.95 ±0.01,*** elevated dust layers reached a maximum elevation of 4 km above sea ***/smoke particles that originated from highly populated/industrialized regions could be distinguished by their relatively smaller particle size（？_（440–870） ranged between1.33 and 1.36） and higher light-absorbing（Ω_（675） of 0.92 ± 0.01） *** aerosols are mostly distributed at altitudes 〈 1.2 *** root-mean-square deviation（RMSD） between the aerosol optical depth（AOD,τ） derived from LIDAR_（（τ_（LIDAR））） and from the CIMEL sun/sky radiometer_（（τ_（CIMEL））） varied with respect to the surface PM10 *** RMSD between τ_（LIDAR） and τ_（CIMEL） was as low as 13% under lower PM_（10） concentration levels（〈 100 μg/m^3）.In contrast,the RMSD between τ_（LIDAR） and τ_（CIMEL） increased three times（~31%） under high surface PM_（10） concentration levels（〉100 μg/m^3）.These results suggest that the accuracy of τ_（LIDAR） is influenced by specific atmospheric conditions,regardless of its uncertainty.

关键词： LIDAR Sun/sky radiometer MODIS Optical/microphysical properties Aerosol optical depth

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5G ENTERING INTO A NEW ERA

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China Communications 2017年第12期14卷 I0002-I0004页

作者： Feifei Gao Changle Li Jun Fang Kaizhi Huang Zhi Quan Chengwen Xing Jianhua Zhang Zhongshan Zhang Liqiang Zhao Yulong Zou department of Automation Tsinqhua UniversityBeiiingChina the State Key Laboratory of Integrated Services Networks Xidian university china communications ieee communications magazine ieee signal processing letters national digital switching system engineering&technological research center the college of information engineering shenzhen university the school of information and electronics beijing institute of technology bupt itu-r imt-2020 channel model ieee comm the school of computer and communication engineering in the university of science and technology beijing(ustb) state key lab.of integrated ser vice networks xidian university the nanjing university of posts and telecommunications(nupt)

The ever increasing wireless data services, such asimaging, video, audio, multimedia, etc., have de-mands for the very high speed wireless communicationsand network, which are unfortunately a bottleneck whencombining with the wireline core network. Users＇ arenow expecting high quality of experience with low-costdevices, ubiquitous connectivity, energy efficiency, highreliability, or even ultra-low latency if a vehicle terminalis applied.

关键词： 5G ENTERING A NEW ERA

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Advances in the Application of Perovskite Materials

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Nano-Micro Letters 2023年第10期15卷 334-381页

作者： Lixiu Zhang Luyao Mei Kaiyang Wang Yinhua Lv Shuai Zhang Yaxiao Lian Xiaoke Liu Zhiwei Ma Guanjun Xiao Qiang Liu Shuaibo Zhai Shengli Zhang Gengling Liu Ligang Yuan Bingbing Guo Ziming Chen Keyu Wei Aqiang Liu Shizhong Yue Guangda Niu Xiyan Pan Jie Sun Yong Hua Wu‑Qiang Wu Dawei Di Baodan Zhao Jianjun Tian Zhijie Wang Yang Yang Liang Chu Mingjian Yuan Haibo Zeng Hin‑Lap Yip Keyou Yan Wentao Xu Lu Zhu Wenhua Zhang Guichuan Xing Feng Gao Liming Ding Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190People’s Republic of China university of Chinese Academy of Sciences Beijing 100049People’s Republic of China department of Physics Link.ping University58183 Link.pingSweden Institute of Applied Physics and Materials engineering University of MacaoMacao 999078People’s Republic of China School of Materials Science and engineering Yunnan UniversityKunming 650091People’s Republic of China School of Microelectronics Science and Technology Sun Yat-sen UniversityZhuhai 519082People’s Republic of China College of Electronic Information and Optical engineering Nankai UniversityTianjin 300350People’s Republic of China Guangdong Provincial Key Laboratory of Semiconductor Optoelectronic Materials and Intelligent Photonic Systems Harbin Institute of TechnologyShenzhen 518055People’s Republic of China School of Materials Science and engineering Nanjing University of Science and TechnologyNanjing 210094People’s Republic of China College of Optical Science and engineering Zhejiang UniversityHangzhou 310027People’s Republic of China State Key Laboratory of Superhard Materials Jilin UniversityChangchun 130012People’s Republic of China College of Electronic and Optical engineering Nanjing University of Posts and TelecommunicationsNanjing 210023People’s Republic of China School of Chemistry Sun Yat-sen UniversityGuangzhou 510006People’s Republic of China School of Environment and Energy South China University of TechnologyGuangzhou 510000People’s Republic of China department of Chemistry Imperial College LondonLondon W120BZUK College of Chemistry Nankai UniversityTianjin 300071People’s Republic of China Institute for Advanced Materials and Technology University of Science and Technology BeijingBeijing 100083People’s Republic of China Institute of Semiconductors Chinese Academy of SciencesBeijing 100083People’s Republic of China School

Nowadays, the soar of photovoltaic performance of perovskite solar cells has set off a fever in the study of metal halide perovskite materials. The excellent optoelectronic properties and defect tolerance feature allow metal halide perovskite to be employed in a wide variety of applications. This article provides a holistic review over the current progress and future prospects of metal halide perovskite materials in representative promising applications, including traditional optoelectronic devices(solar cells, light-emitting diodes, photodetectors, lasers), and cutting-edge technologies in terms of neuromorphic devices(artificial synapses and memristors) and pressure-induced emission. This review highlights the fundamentals, the current progress and the remaining challenges for each application, aiming to provide a comprehensive overview of the development status and a navigation of future research for metal halide perovskite materials and devices.

关键词： Perovskites Optoelectronic devices Neuromorphic devices Pressure-induced emission

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Two-dimensional materials for future information technology: status and prospects

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Science China(Information Sciences) 2024年第6期67卷 1-147页

作者： Hao QIU Zhihao YU Tiange ZHAO Qi ZHANG Mingsheng XU Peifeng LI Taotao LI Wenzhong BAO Yang CHAI Shula CHEN Yiqi CHEN Hui-Ming CHENG Daoxin DAI Zengfeng DI Zhuo DONG Xidong DUAN Yuhan FENG Yu FU Jingshu GUO Pengwen GUO Yue HAO Jun HE Xiao HE Jingyi HU Weida HU Zehua HU Xinyue HUANG Ziyang HUANG Ali IMRAN Ziqiang KONG Jia LI Qian LI Weisheng LI Lei LIAO Bilu LIU Can LIU Chunsen LIU Guanyu LIU Kaihui LIU Liwei LIU Sheng LIU Yuan LIU Donglin LU Likuan MA Feng MIAO Zhenhua NI Jing NING Anlian PAN Tian-Ling REN Haowen SHU Litao SUN Yue SUN Quanyang TAO Zi-Ao TIAN Dong WANG Hao WANG Haomin WANG Jialong WANG Junyong WANG Wenhui WANG Xingjun WANG Yeliang WANG Yuwei WANG Zhenyu WANG Yao WE... School of Electronic Science and engineering Nanjing University School of Integrated Circuits Interdisciplinary Research Center for Future Intelligent Chips (Chip-X)Nanjing University School of Integrated Circuit Science and engineering Nanjing University of Posts and Telecommunications State Key Laboratory of Infrared Physics Shanghai Institute of Technical Physics Chinese Academy of Sciences School of Physics and Key Lab of Quantum Materials and Devices of the Ministry of Education School of Electronic Science & EngineeringSoutheast University College of Integrated Circuits State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University Suzhou Laboratory State Key Laboratory of Integrated Chips and Systems School of MicroelectronicsFudan University Shaoxin Laboratory department of Applied Physics The Hong Kong Polytechnic University Key Laboratory for Micro-Nano Physics and Technology of Hunan Province College of Materials Science and EngineeringHunan University College of Integrated Circuits Zhejiang University Shenzhen Geim Graphene Center Shenzhen Key Laboratory of Layered Materials for Value-Added ApplicationsTsinghua-Berkeley Shenzhen Institute & Institute of Materials ResearchTsinghua Shenzhen International Graduate SchoolTsinghua University State Key Laboratory of Extreme Photonics and Instrumentation College of Optical Science and EngineeringInternational Research Center for Advanced PhotonicsZijingang CampusZhejiang University National Key Laboratory of Materials for Integrated Circuits Shanghai Institute of Microsystem and Information TechnologyChinese Academy of Sciences CAS Key Laboratory of Nanophotonic Materials and Devices & Key Laboratory of Nanodevices and Applications i-LabSuzhou Institute of Nano-Tech and Nano-Bionics (SINANO)Chinese Academy of Sciences College of Chemistry and Chemical engineering Hunan University Key Laboratory of Quantum State Construction and Manipulation (Ministry of Education) Department of PhysicsRenmin University of China School

Over the past 70 years, the semiconductor industry has undergone transformative changes,largely driven by the miniaturization of devices and the integration of innovative structures and materials. Two-dimensional(2D) materials like transition metal dichalcogenides(TMDs) and graphene are pivotal in overcoming the limitations of silicon-based technologies, offering innovative approaches in transistor design and functionality, enabling atomic-thin channel transistors and monolithic 3D integration. We review the important progress in the application of 2D materials in future information technology, focusing in particular on microelectronics and optoelectronics. We comprehensively summarize the key advancements across material production, characterization metrology, electronic devices, optoelectronic devices, and heterogeneous integration on silicon. A strategic roadmap and key challenges for the transition of 2D materials from basic research to industrial development are outlined. To facilitate such a transition, key technologies and tools dedicated to 2D materials must be developed to meet industrial standards, and the employment of AI in material growth, characterizations, and circuit design will be essential. It is time for academia to actively engage with industry to drive the next 10 years of 2D material research.

关键词： two-dimensional (2D) materials information technology production technology standardization of characterization microelectronicdevices optoelectronic devices multi-functional integration

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Simulation and analysis of phase-sensitive surface plasmon resonance sensor based on enhanced optical transmission through arrays of nanoholes in silver films

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中国光学与应用光学 2010年第1期3卷 57-63页

作者： YANGT HO H p Jiangsu Key Laboratory for Organic electronics ＆ Information Displays Nanjing University of Posts and Telecommunications Nanjing （210000 ） China department of Electronic engineering Centre for Advanced ReSearch in Photonics The Chinese University of Hong KongShatinN. T. Hong Kong SAR China

A high spatial resolution, phase-sensitive Surface Plasmon Resonance(SPR) sensor based on Extraordinary Optical Transmission(EOT) is proposed to monitor the binding of organic and biological molecules to the silver surface. The 2D nanohole-array configuration is well suited for dense integration in a sensor chip. The optical geometry is collinear, which simplifies the alignment with respect to the traditional Kretschmann arrangement for SPR sensing. Various design parameters of the device have been studied by simulation. The heterodyne technique is used to improve the sensitivity. The optimization results indicate that the sensor has the advantages of achieving high resolution and a wide dynamic range simultaneously.

关键词：高分辨率等离子体生物传感器纳米孔

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Ultra compact and high resolution spectrometer based on optical transmission through submicron interferometer array

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中国光学与应用光学 2010年第1期3卷 38-44页

作者： YANG T LI C C HO H P Jiangsu Key Laboratory for Organic electronics ＆ Information Displays Nanjing University of Posts and Telecommunications Nanjing（ 210000 ） China department of Electronic engineering Centre for Advanced Research in Photonics The Chinese University of Hong Kong Shatin N. T. Hong Kong SAR China

We present an ultra compact and high resolution free space optical spectrometer and demonstrate it by using FDTD simulations. The miniature interferometer-based spectrometer is a series of submicron phase objects on a polymethyl methacrylate(PMMA) film with a CCD as the detector. The spectrum is obtained by solving a system of simultaneous linear equations. The Tikhonov regularization method is used to achieve a resolution at the picometer level. Compared with conventional spectrometers, the proposed device is low-cost and easy to fabricate due to its simple structure. Furthermore, its compact feature renders the device ideal for miniaturization and integration as the systems in microfluidics architectures and lab-on-chip designs.

关键词：光学材料高分辨率探测器光谱仪

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Femtosecond nonlinear losses in multimode optical fibers

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Photonics Research 2021年第12期9卷 2443-2453页

作者： MARIO FERRARO FABIO MANGINI MARIO ZITELLI ALESSANDRO TONELLO ANTONIO DE LUCA VINCENT COUDERC STEFAN WABNITZ department of Information engineering Electronicsand TelecommunicationsSapienza University of RomeVia Eudossiana 1800184 RomeItaly department of Information engineering University of BresciaVia Branze 3825123 BresciaItaly Universitéde Limoges XLIMUMR CNRS 7252123 Avenue A.Thomas87060 LimogesFrance Physics department University of CalabriaI-87036 Arcavacata di RendeCSItaly CNR Nanotec-Institute of Nanotechnology S.S.CosenzaI-87036 RendeCSItaly CNR-INO Istituto Nazionale di OtticaVia Campi Flegrei 34I-80078 PozzuoliNAItaly

Multimode optical fibers are attracting a growing interest for their capability to transport high-power laser beams,coupled with novel nonlinear optics-based ***,optical fiber breakdown occurs when beam intensities exceed a certain critical *** breakdown associated with irreversible modifications of the refractive index,triggered by multiphoton absorption,has been largely exploited for fiber material *** we show that,for light beam intensities slightly below the breakdown threshold,nonlinear absorption strongly affects the dynamics of a propagating beam as *** experimentally analyze this subthreshold regime and highlight the key role played by spatial self-imaging in graded-index fibers for enhancing nonlinear optical *** characterize the nonlinear power transmission properties of multimode fibers for femtosecond pulses propagating in the near-infrared spectral *** show that an effective N-photon absorption analytical model is able to describe the experimental data well.

关键词： breakdown Femto fibers

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Ultrafast laser processing of materials: from science to industry

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Light(Science & Applications) 2016年第1期5卷 548-561页

作者： Mangirdas Malinauskas Albertas Žukauskas Satoshi Hasegawa Yoshio Hayasaki Vygantas Mizeikis Ričardas Buividas Saulius Juodkazis Laser Research Centre Department of Quantum ElectronicsPhysics FacultyVilnius UniversitySaulėtekio Ave.10LT-10223 VilniusLithuania Center for Optical Research and Education(CORE) Utsunomiya University7-1-2 YotoUtsunomiya 321-8585Japan Research Institute of electronics Shizuoka University3-5-3-1 JohokuNaka-kuHamamatsu 432-8561Japan Centre for Micro-Photonics Faculty of ScienceEngineering and TechnologySwinburne University of TechnologyHawthornVIC 3122Australia Melbourne Centre for Nanofabrication ANFF151 Wellington RoadClaytonVIC 3168Australia Center of Nanotechnology King Abdulaziz UniversityJeddah 21589Saudi Arabia

Processing of materials by ultrashort laser pulses has evolved significantly over the last decade and is starting to reveal its scientific,technological and industrial *** ultrafast laser manufacturing,optical energy of tightly focused femtosecond or picosecond laser pulses can be delivered to precisely defined positions in the bulk of materials via two-/multi-photon excitation on a timescale much faster than thermal energy exchange between photoexcited electrons and lattice *** of photoionization and thermal processes with the highest precision,inducing local photomodification in sub-100-nm-sized regions has been ***-of-the-art ultrashort laser processing techniques exploit high 0.1–1μm spatial resolution and almost unrestricted three-dimensional structuring *** pulse duration,spatiotemporal chirp,phase front tilt and polarization allow control of photomodification via uniquely wide parameter *** opto-electrical/mechanical technologies have enabled laser processing speeds approaching meters-per-second,leading to a fast lab-to-fab *** key aspects and latest achievements are reviewed with an emphasis on the fundamental relation between spatial resolution and total fabrication *** biomedical applications implementing micrometer feature precision over centimeter-scale scaffolds and photonic wire bonding in telecommunications are highlighted.

关键词： biomedical applications direct laser writing functional microdevices material processing nonlinear light–matter interaction 3D structuring ultrashort laser pulses

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Recent Progress on Two-Dimensional Materials

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物理化学学报 2022年

作者： Cheng Chang Wei Chen Ye Chen Yonghua Chen Yu Chen Feng Ding Chunhai Fan Hongjin Fan Zhanxi Fan Cheng Gong Yongji Gong Qiyuan He Xun Hong Sheng Hu Weida Hu Wei Huang Yuan Huang Wei Ji Dehui Li Lain-Jong Li Qiang Li Li Lin Chongyi Ling Minghua Liu Nan Liu Zhuang Liu Kian Ping Loh Jianmin Ma Feng Miao Hailin Peng Mingfei Shao Li Song Shao Su Shuo Sun Chaoliang Tan Zhiyong Tang Dingsheng Wang Huan Wang Jinlan Wang Xin Wang Xinran Wang Andrew T. S. Wee Zhongming Wei Yuen Wu Zhongshuai Wu Jie Xiong Qihua Xiong Weigao Xu Peng Yin Haibo Zeng Zhiyuan Zeng Tianyou Zhai Han Zhang Hui Zhang Qichun Zhang Tierui Zhang Xiang Zhang Lidong Zhao Meiting Zhao Weijie Zhao Yunxuan Zhao Kaige Zhou Xing Zhou Yu Zhou Hongwei Zhu Hua Zhang Zhongfan Liu department of Electrical and Computer engineering and Quantum Technology Center， university of Maryland， College Park School of Materials Science and engineering， Beihang university department of Materials Science and engineering， City university of Hong Kong Center of Advanced Nanocatalysis (CAN)， Hefei National Laboratory for Physical Sciences at the Microscale， department of Applied Chemistry， university of Science and Technology of China College of Chemistry and Chemical engineering， State Key Laboratory of Physical Chemistry of Solid Surfaces， Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)， Xiamen university State Key Laboratory of Infrared Physics， Shanghai Institute of Technical Physics， Chinese Academy of Sciences Advanced Research Institute of Multidisciplinary Science， Beijing Institute of Technology Beijing Key Laboratory of Optoelectronic Functional Materials & Micro-Nano Devices， department of Physics， Renmin university of China School of Optical and Electronic Information， Wuhan National Laboratory for Optoelectronics， Huazhong university of Science and Technology department of Mechanical engineering， The university of Hong Kong Institute of Science and Technology Austria School of Physics， Southeast university department of Materials Science and engineering， National university of Singapore CAS Key Laboratory of Colloid， Interface and Chemical Thermodynamics， Institute of Chemistry， Chinese Academy of Sciences College of Chemistry， Beijing Normal university Institute of Functional Nano & Soft Materials (FUNSOM)， Jiangsu Key Laboratory for Carbon-based Functional Materials and Devices， Soochow university School of Materials and Energy， university of Electronic Science and Technology of China School of Physics， Nanjing university Center for Nanochemistry (CNC)， Beijing National Laboratory for Molecular Sciences， College of Chemistry and Molecular engineering， Beijing Graphene Institute (BGI)， Peking university State Key Laboratory of Chemical Resource engineering， Beijing

Research on two-dimensional (2D) materials has been explosively increasing in last seventeen years in varying subjects including condensed matter physics， electronic engineering， materials science， and chemistry since the mechanical exfoliation of graphene in 2004. Starting from graphene， 2D materials now have become a big family with numerous members and diverse categories. The unique structural features and physicochemical properties of 2D materials make them one class of the most appealing candidates for a wide range of potential applications. In particular， we have seen some major breakthroughs made in the field of 2D materials in last five years not only in developing novel synthetic methods and exploring new structures/properties but also in identifying innovative applications and pushing forward commercialisation. In this review， we provide a critical summary on the recent progress made in the field of 2D materials with a particular focus on last five years. After a brief background introduction， we first discuss the major synthetic methods for 2D materials， including the mechanical exfoliation， liquid exfoliation， vapor phase deposition， and wet-chemical synthesis as well as phase engineering of 2D materials belonging to the field of phase engineering of nanomaterials (PEN). We then introduce the superconducting/optical/magnetic properties and chirality of 2D materials along with newly emerging magic angle 2D superlattices. Following that， the promising applications of 2D materials in electronics， optoelectronics， catalysis， energy storage， solar cells， biomedicine， sensors， environments， etc. are described sequentially. Thereafter， we present the theoretic calculations and simulations of 2D materials. Finally， after concluding the current progress， we provide some personal discussions on the existing challenges and future outlooks in this rapidly developing field.

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