检索结果-南通市图书馆

Breakthrough of Carbon-Ash Recalcitrance in Hydrochar via Molten Carbonate:engineering Mineral-Rich Biowaste Toward Sustainable Platform Carbon Materials

引用

engineering 2024年第5期36卷 167-177页

作者： Zihan Wang Leli Zhang Yuanhui Zhang Zhidan Liu Laboratory of environment-Enhancing Energy(E2E) Key Laboratory of Agricultural Engineering in Structure and EnvironmentMinistry of AgricultureCollege of Water Resources and Civil EngineeringChina Agricultural UniversityBeijing 100083China department of agricultural and Biological engineering University of Illinois at Urbana-ChampaignUrbanaIL 61801USA

The function-led design of porous hydrochar from mineral-rich biowaste for environmental applications inevitably suffers from carbon-ash ***,a method to alter the original carbon skeleton with ash remains elusive and hinders the availability of ***,we propose a facile strategy for breaking the rigid structure of carbon-ash coupled hydrochar using phase-tunable molten carbonates.A case system was designed in which livestock manure and NaHCO3 were used to prepare the activated hydrochar,and NH3 served as the target *** to the redox effect,we found that organic fractions significantly advanced the melting temperature of Na2CO3 below 800℃.The Na species steadily broke the carbon-ash interaction as the thermal intensity increased and transformed inorganic constituents to facilitate ash dissolution,rebuilding the hydrochar skeleton with abundant hierarchical channels and active defect *** surface polarity and mesopore distribution collectively governed the five cycles NH3 adsorption attenuation *** hydrochar delivered favorable potential for application with a maximum overall adsorption capacity of 100.49 mg·g^(-1).Integrated spectroscopic characterization and theoretical computations revealed that incorporating NH3 on the carbon surface could transfer electrons to chemisorbed oxygen,which promoted the oxidation of pyridine-N during *** work offers deep insight into the structure function correlation of hydrochar and inspires a more rational design of engineered hydrochar from high-ash biowaste.

关键词： Hydrochar Livestock manure Ammonia adsorption Deashing Oxygen activation

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Patterns of crop-specific fertilizer-nitrogen losses and opportunities for sustainable mitigation:A quantitative overview of 15N-tracing studies

引用

Soil Ecology Letters 2024年第2期6卷 71-81页

作者： Cong Xu Hanshen Zhu Haokuang Liu Cheng Ji Jie Yuan Guanlin Li Jidong Wang Yongchun Zhang National agricultural Experimental Station for agricultural environment LuheInstitute of Agricultural Resources and EnvironmentJiangsu Academy of Agricultural SciencesNanjing210014China School of the environment and Safety engineering Jiangsu UniversityZhenjiang212013China

Pattern and mitigation potential of crop-specific fertilizer-N losses were *** showed high fertilizer-N losses due to high N application rates and low ***,SOC,and soil pH are key parameters affecting fertilizer-N *** a given application rate,soils with higher SOC have lower fertilizer-N *** N rate combined with SOC improvement could cut 34.8%-59.6%of N losses.

关键词： fertilizer-nitrogen loss crop-specific 15N tracing soil organic carbon meta-analysis

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Bicarbonate used as a buffer for controlling nutrient solution pH value during the growth of hydroponic lettuce

引用

International Journal of agricultural and Biological engineering 2024年第3期17卷 59-67页

作者： Mengxue Zhang Wenxin Wang Luming Zhong Fang Ji Dongxian He Key Laboratory of agricultural engineering in Structure and environment of MARA College of Water Resources&Civil EngineeringChina Agricultural UniversityBeijing 100083China

Unstable pH of nutrient solution in hydroponic systems is a major obstacle to *** simplify the management of nutrient solution pH and attenuate negative effects of pH on plant growth,this study investigated the effect of different buffer salt additions on nutrient solution pH,ion uptake,growth and photosynthesis of Yamazaki lettuce,with the equivalent concentrations of macro-element *** results indicated that the pH of nutrient solution was buffered to varying degrees by the 2 mol/L HCO_(3)^(-),1 mol/L HCO_(3)^(-),and 0.33 mol/L HPO_(4)^(2-)The 0.33 mol/L HPO_(4)^(2-)treatment fluctuated most with a pH of 1.74 units,while the addition of HCO_(3)^(-)buffered nutrient solution pH was better,with higher pH values(7.2-7.7).The CK-pH control solution,1 mol/L HCO_(3)^(-)and 0.33 mol/L HPO_(4)^(2-)treatments all promoted the uptake of ion and then the growth of lettuce was better in comparison with the CK-pH no adjustment treatment,while the 2 mol/L HCO_(3)^(-)treatment inhibited K uptake and reduced the availability of Fe,the shoot and root fresh weight of lettuce decreased by 21.3%and 10.1%,*** addition,although the chlorophyll content and net photosynthetic rate under 1 mol/L HCO_(3)^(-)and 0.33 mol/L HPO_(4)^(2-)treatments were significantly lower than the CK-pH control solution treatment,there were no significant differences in leaf length and leaf number of lettuce among them,and shoot fresh weight per plant was 83.09,82.95,and 78.92 g,*** conclusion,adding 1 mol/L HCO_(3)^(-)to the nutrient solution in a single dosage not only buffered the pH of nutrient solution better but also promoted ion uptake,it had no negative effects on the growth,photosynthesis and ion uptake of hydroponic lettuce in comparison with the CK-pH control solution ***,1 mol/L HCO_(3)^(-)can be used as a buffer during the growth of hydroponic lettuce and reduce frequent addition of acids or alkalis,and then simplify the management of nut

关键词： pH buffer nutrient solution hydroponic lettuce growth ion uptake

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

熔融碳酸盐突破水热炭中碳-灰刚性屏障——从高灰分生物质废弃物到可持续平台碳材料（英文）

引用

engineering 2024年第5期 167-177页

作者：王子涵张乐礼张源辉刘志丹 Laboratory of environment-Enhancing Energy (E25) Key Laboratory of Agricultural Engineering in Structure and Environment Ministry of Agriculture College of Water Resources and Civil Engineering China Agricultural University department of agricultural and Biological engineering University of Illinois at Urbana-Champaign

The function-led design of porous hydrochar from mineral-rich biowaste for environmental applications inevitably suffers from carbon–ash recalcitrance. However, a method to alter the original carbon skeleton with ash remains elusive and hinders the availability of hydrochar. Herein, we propose a facile strategy for breaking the rigid structure of carbon–ash coupled hydrochar using phase-tunable molten carbonates.A case system was designed in which livestock manure and Na HCO3were used to prepare the activated hydrochar, and NH3served as the target contaminant. Due to the redox effect, we found that organic fractions significantly advanced the melting temperature of Na2CO3below 800.C. The Na species steadily broke the carbon–ash interaction as the thermal intensity increased and transformed inorganic constituents to facilitate ash dissolution, rebuilding the hydrochar skeleton with abundant hierarchical channels and active defect edges. The surface polarity and mesopore distribution collectively governed the five cycles NH3adsorption attenuation process. Manure hydrochar delivered favorable potential for application with a maximum overall adsorption capacity of 100.49 mg.g-1. Integrated spectroscopic characterization and theoretical computations revealed that incorporating NH3on the carbon surface could transfer electrons to chemisorbed oxygen, which promoted the oxidation of pyridine-N during adsorption. This work offers deep insight into the structure function correlation of hydrochar and inspires a more rational design of engineered hydrochar from high-ash biowaste.

关键词：

来源：

同方期刊数据库评论

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Are gender inclusiveness and rural transformation interlinked?The case of Bangladesh

引用

Journal of Integrative Agriculture 2024年第6期23卷 2112-2126页

作者： Maria Fay Rola-Rubzen Mohammad Jahangir Alam Jon Marx Sarmiento Ismat Ara Begum Al Amin Al Abbasi Subrata Saha UWA School of Agriculture and environment The University of Western AustraliaPerth 6009Australia department of Agribusiness and Marketing Bangladesh Agricultural UniversityMymensingh-2202Bangladesh department of agricultural Economics Bangladesh Agricultural UniversityMymensingh-2202Bangladesh

Gender inclusiveness is important in the rural transformation process of Bangladesh as rural women play key roles in both agricultural and non-agricultural *** inclusiveness also leads to gender *** empirically evaluate relationships between rural transformation and gender inclusiveness in *** consider three rural transformation indicators:high-value commodities’share in agricultural output values,non-farm employment’s share in rural labor employment,and non-agricultural GDP’s share in total *** capturing gender inclusiveness include the per capita rural income of males and females,ratio of investments into gender programs,female access to education,access to healthcare,employment participation,land ownership,and asset *** test the effect of the difference in per capita rural income of males and females and the ratio of their incomes and check for the robustness of the gender variables across different model *** 128 district-level observations from 32 districts of Bangladesh across four time periods(2000,2005,2010 and 2016),we use both ordinary least squares and fixed effects panel regression *** find that female land and asset ownership and access to education and healthcare are robust determinants of various stages of rural ***,our results suggest that improving women’s ownership of land and assets and investing in women’s education and healthcare will likely contribute to a more inclusive rural transformation.

关键词： rural transformation Bangladesh gender inclusiveness investments on women

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Co-incorporation of Chinese milk vetch(Astragalus sinicus L.)and chemical fertilizers alters microbial functional genes supporting short-time scale positive nitrogen priming effects in paddy soils

引用

Pedosphere 2024年第3期34卷 567-576页

作者： Limin WANG Chunmei HE Dongfeng HUANG Juhua YU Cailing LIU Qinghua LI Yibin HUANG Juan LI Fei WANG Institute of Resources Environment and Soil FertilizerSoil and Fertilizer InstituteFujian Academy of Agricultural SciencesFuzhou 350012(China) School of Resources and environment engineering Anhui UniversityHefei 230601(China)

Nitrogen(N)priming is a microbially mediated biochemical process as affected by different incorporation ***,little information is known about the microbial mechanisms driving the response of N priming to co-operation of Chinese milk vetch(CMV,Astragalus sinicus L.)and different rates of chemical fertilizers in paddy soils in South ***,an anaerobic incubation experiment was conducted to study N priming effects(PE)and their relationships with soil microbial functional genes after CMV incorporation alone(M),co-incorporation of CMV with 100%(normal dosage)chemical fertilizers(MC100),and co-incorporation of CMV with 80% chemical fertilizers(MC80).Co-incorporation of CMV and chemical fertilizers enhanced the short-time scale(the first 20 d of incubation)positive PE of N,while no significant differences existed among the three treatments on day 60 or 90 of incubation(P>0.05).Compared with the M treatment,gross priming effect(GPE)in the MC100 and MC80 treatments significantly increased by 34.0% and 31.3%,respectively,and net priming effect(NPE)increased by 47.7% and 47.8%,respectively,during the first 20 d of incubation(P<0.05).This was likely attributed to soil nutrient availability and added substrate *** MC100 and MC80 treatments increased the gdhA gene abundance by 5.0% and 9.8%,increased the gdh2 gene abundance by 12.7% and 45.7%,and increased the nasB gene abundance by 9.5% and 41.4%,respectively,in comparison with the M treatment on day 20 of *** analyses indicated that soil microbial functional genes involved in N mineralization(gdhA and gdh2),assimilatory nitrate reduction(nasB),and nitrification(amoB)were significantly correlated with N priming under different incorporation practices during the incubation period(P<0.05).Thus,co-incorporation of CMV and chemical fertilizers can regulate soil microbial community functional gene structure,which may accelerate mineralization and assimilatory nitrate reduction and inhibit

关键词： green manure gross priming effect incorporation practice microbial mechanism net priming effect rice field soil

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Nitrogen rhizodeposition from corn and soybean,and its contribution to the subsequent wheat crops

引用

Journal of Integrative Agriculture 2024年第7期23卷 2446-2457页

作者： Sainan Geng Lantao Li Yuhong Miao Yinjie Zhang Xiaona Yu Duo Zhang Qirui Yang Xiao Zhang Yilun Wang College of Resources and environment Henan Agricultural UniversityZhengzhou 450002China

Nitrogen(N)is a key factor in the positive response of cereal crops that follow leguminous crops when compared to gramineous crops in rotations,with the nonrecyclable rhizosphere-derived N playing an important ***,quantitative assessments of differences in the N derived from rhizodeposition(NdfR)between legumes and gramineous crops are lacking,and comparative studies on their contributions to the subsequent cereals are *** this study,we conducted a meta-analysis of NdfR from leguminous and gramineous crops based on 34 observations published *** addition,pot experiments were conducted to study the differences in the NdfR amounts,distributions and subsequent effects of two major wheat(Triticum aestivum L.)-preceding crops,corn(Zea mays L.)and soybean(Glycine max L.),by the cotton wick-labelling method in the main wheat-producing areas of *** meta-analysis results showed that the NdfR of legumes was significantly greater by 138.93%compared to gramineous *** our pot experiment,the NdfR values from corn and soybean were 502.32 and 944.12 mg/pot,respectively,and soybean was also significantly higher than corn,accounting for 76.91 and 84.15%of the total belowground nitrogen of the plants,***,in different soil particle sizes,NdfR was mainly enriched in the large macro-aggregates(>2 mm),followed by the small macro-aggregates(2–0.25 mm).The amount and proportion of NdfR in the macro-aggregates(>0.25 mm)of soybean were 3.48 and 1.66 times higher than those of corn,respectively,indicating the high utilization potential of soybean *** the N accumulation of subsequent wheat,the contribution of soybean NdfR to wheat was approximately 3 times that of corn,accounting for 8.37 and 4.04%of the total N uptake of wheat,*** conclusion,soybean NdfR is superior to corn in terms of the quantity and distribution ratio of soil *** future field production,legume NdfR should be included in the nitrogen p

关键词： crop rotation nitrogen rhizodeposition meta-analysis soil aggregates nitrogen transfer

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Acetylacetone effectively controlled the secondary metabolites of Microcystis aeruginosa under simulated sunlight irradiation

引用

Journal of environmental Sciences 2024年第1期135卷 285-295页

作者： Xiaomeng Wang Yixin Luo Shujuan Zhang Lixiang Zhou department of environmental engineering College of Resources and Environmental SciencesNanjing Agricultural UniversityNanjing 210095China The State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China

Inactivation of cyanobacterial cells and simultaneous control of secondary metabolites is of significant necessity for the treatment of cyanobacteria-laden ***(AcAc)has been reported a specific algicide to inactivate Microcystis aeruginosa(***)and an effective light activator to degrade *** study systematically investigated the photodegradation ability of AcAc under xenon(Xe)irradiation on the secondary metabolites of ***,mainly algal organic matter(AOM),especially toxic microcystin-LR(MC-LR).Results showed that AcAc outperformed H_(2)O_(2)in destructing the protein-like substances,humic acid-like matters,aromatic proteins and fulvic-like substances of *** MC-LR(250μg/L),0.05 mmol/L AcAc attained the same degradation efficiency(87.0%)as 0.1mmol/L H_(2)O_(2).The degradation mechanism of Xe/AcAc might involve photo-induced energy/electron transfer and formation of carbon center *** conditions(pH>9.0)were detrimental to the photoactivity of AcAc,corresponding to the observed degradation rate constant(k_(1)value)of MC-LR drastically decreasing to 0.0013 min^(-1)as solution pH exceeded *** PO_(4)^(3-)and HCO_(3)^(-)ions had obvious inhibition effects,whereas NO_(3)^(-)slightly improved k_(1)value from 0.0277 min^(-1)to 0.0321 min^(-1).The presence of AOM did not significantly inhibit MC-LR degradation in Xe/AcAc *** addition,the biological toxicity of MC-LR was greatly reduced after *** results demonstrated that AcAc was an alternative algicidal agent to effectively inactivate algal cells and simultaneously control the secondary metabolites after cell ***,the concentration and irradiation conditions should be further optimized in practical application.

关键词： Microcystis aeruginosa Photodegradation Acetylacetone Secondary metabolites Microcystin

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Antibiotic ciprofloxacin removal from aqueous solutions by electrochemically activated persulfate process:Optimization,degradation pathways,and toxicology assessment

引用

Journal of environmental Sciences 2024年第9期143卷 85-98页

作者： Elif Yakamercan Ahmet Aygün Halis Simsek environmental engineering department Bursa Technical UniversityBursaTurkey agricultural and Biological engineering department Purdue UniversityWest LafayetteINUSA

Ciprofloxacin(CIP)is a commonly used antibiotic in the fluoroquinolone group and is widely used in medical and veterinary medicine disciplines to treat bacterial *** CIP is discharged into the sewage system,it cannot be removed by a conventional wastewater treatment plant because of its recalcitrant *** this study,boron-doped diamond anode and persulfate were used to degrade CIP in an aquatic solution by creating an electrochemically activated persulfate(EAP)*** added to the system as a coactivator and the process was called EAP+*** effects of independent variables,including pH,Fe^(2+),persulfate concentration,and electrolysis time on the systemwere optimized using the response surface *** results showed that the EAP+Fe process removed 94%of CIP under the following optimum conditions:A pH of 3,persulfate/Fe^(2+)concentration of 0.4 mmol/L,initial CIP concentration 30 mg/L,and electrolysis time of 12.64 *** removal efficiency was increased from 65.10%to 94.35%by adding Fe^(2+)as a transition *** degradation products,7 pathways,and 78 intermediates of CIP were studied,and three of those intermediates(m/z 298,498,and 505)were *** toxicological analysis based on toxicity estimation software results indicated that some degradation products of CIP were toxic to targeted animals,including fathead minnow,Daphnia magna,Tetrahymena pyriformis,and *** optimumoperation costswere similar in EAP and EAP+Fe processes,approximately 0.54€/m^(3).

关键词： Ciprofloxacin Response surface methodology Electrochemically activated persulfate Electrooxidation

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Annual growth of Fagus orientalis is limited by spring drought conditions in Iran’s Golestan Province

引用

Journal of Forestry Research 2024年第1期35卷 128-142页

作者： Khalil Ghorbani Jahangir Mohammadi Laleh Rezaei Ghaleh department of Water engineering Faculty of Water and Soil EngineeringGorgan University of Agricultural Sciences and Natural ResourcesGorganIran department of Forestry Gorgan University of Agricultural Sciences and Natural ResourcesGorganIran department of Water engineering Faculty of AgricultureUrmia UniversityUrmiaIran

Due to the lack of a uniform and accurate defi-nition of‘drought’,several indicators have been introduced based on different variables and methods,and the efficiency of each of these is determined according to their relationship with *** relationship between two drought indices,SPI(standardized precipitation index)and SPEI(standard-ized precipitation-evapotranspiration index)in different sea-sons was investigated using annual rings of 15 tree samples to determine the effect of drought on the growth of oriental beech(Fagus orientalis Lipsky)in the Hyrcanian forests of northern *** different evapotranspiration calcula-tion methods were evaluated on SPEI efficiency based on Hargreaves-Samani,Thornthwaite,and Penman-Monteith methods using the step-by-step M5 decision tree regression *** results show that SPEI based on the Penman-Monteith in a three-month time scale(spring)had similar temporal changes and a better relationship with annual tree rings(R^(2)=0.81)at a 0.05 significant *** change and a decreasing trend in the time series of annual tree rings are similar to the variation in the SPEI based on the Penman-Monteith *** affecting evapotranspiration,temperature,wind speed,and sunshine hours(used in the Penman-Monteith method),increased but precipitation *** non-linear modeling methods,SPEI based on Penman-Monteith best illustrated climate changes affecting tree growth.

关键词： Climate change Drought index Hyrcanian forests SPEI'Annual growth rings Fagus orientalis

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：