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Heterostructured Co_(3)Se_(4)/CoSe_(2)@C nanoparticles attached on three-dimensional reduced graphene oxide as a promising anode towards Li-ion batteries

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Frontiers of Materials Science 2024年第2期18卷 101-115页

作者： Mingjun Pang Zhaoyang Song Miaomiao Mao Shang Jiang Ruxia Zhang Runwei Wang Jianguo Zhao Engineering Research Center of Coal-based Ecological Carbon Sequestration Technology of the Ministry of Education Shanxi Datong UniversityDatong 037009China State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of ChemistryJilin UniversityChangchun 130012China

In situ carbon-coated Co_(3)Se_(4)/CoSe_(2)(Co_(x)Se_(y))nanoparticles(NPs)attached on three-dimensional(3D)reduced graphene oxide(rGO)sheets were skillfully developed in this work,which involved the environment-friendly hydrothermal method,freeze drying,and selenide *** the structure,the glucose-derived carbon layer exhibited significantly homogeneous dispersion under an argon *** structure not only has enhanced stability,but also can effectively mitigate the volume swell of Co_(x)Se_(y) *** resulted Co_(3)Sea/CoSe_(2)@C/rGO(CSe@C/rGO)exhibited a specific surface area(SSA)of 240.9 m^(2)·g^(-1),offering more electrochemically active sites for the storage of energy related to lithium *** rGO matrix held exceptional flexibility and functional structural rigidity,facilitating the swift ion intercalation and ensuring the high conductivity and recyclability of the *** applied to anodes designed for lithium-ion batteries(LiBs),this material demonstrated distinguished rate and ultra-high reversible capacity(872.98 mA·h·g^(-1) at 0.5 A·g^(-1)).Meanwhile,its capacity retention reached 119.5%after 500 cycles at 2 A·g^(-1),with a coulombic efficiency of 100%.This work potentially paves the way for generating fast and powerful metal selenide anodes and initiating LiBs with good performance.

关键词： CSe@C/rGO lithium-ion battery reduced graphene oxide electrochemicalperformance heterostructure

Potential of arbuscular mycorrhizal fungi for soil health:A review

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Pedosphere 2024年第2期34卷 279-288页

作者： Junling ZHANG Ruotong ZHAO Xia LI Jiangzhou ZHANG college of Resources and Environmental Sciences National Academy of Agriculture Green DevelopmentKey Laboratory of Plant-Soil InteractionsMinistry of EducationChina Agricultural UniversityBeijing 100193China college of Agronomy and Life Science Shanxi Datong UniversityDatong 037009China college of Resources and Environment/International Magnesium Institute Fujian Agriculture and Forestry UniversityFuzhou 350002China

Soil health is an important component of“One Health”.Soils provide habitat to diverse and abundant *** microbial diversity and functions is essential for building healthy soils towards sustainable *** mycorrhizal fungi(AMF)form potentially symbiotic associations with approximately 80%of land plant species that are well recognized for carbon flux and nutrient *** addition to disentangling the signaling pathways and regulatory mechanisms between the two partners,recent advances in hyphosphere research highlight some emerging roles of AMF and associated microbes in the delivery of soil *** paper reviews the contribution of AMF to soil health in agroecosystems,with a major focus on recent progress in the contribution of hyphosphere microbiome to nutrient cycling,carbon sequestration,and soil *** hyphosphere microbiome and fungal stimulants open avenues for developing new fertilizer formulas to promote AMF *** practice,developing AMF-friendly management strategies will have long-term positive effects on sustainable agriculture aiming at simultaneously providing food security,increasing resource use efficiency,and maintaining environment integrity.

关键词： arbuscular mycorrhizal fungi-friendly management strategies carbon sequestration hyphosphere microbiome nutrient cycling soil aggregation soilfunctions

Theoretical analysis of the double-differential cross-sections of neutron,proton,deuteron,^(3)He,andαfor the p+^(6) Li reaction

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Nuclear Science and Techniques 2024年第3期35卷 181-197页

作者： Fang-Lei Zou Xiao-Jun Sun Jing-Shang Zhang Hai-Rui Guo Yin-Lu Han Rui-Rui Xu Xi Tao Ji-Min Wang Xiao-Dong Sun Yuan Tian Tao Ye Yong-Li Xu Chun-Tian Liang college of Physics Guangxi Normal University541004 GuilinChina Guangxi Key Laboratory of Nuclear Physics and Nuclear Technology 541004 GuilinChina China Institute of Atomic Energy P.O.Box 275(41)102413 BeijingChina Institute of Applied Physics and Computational Mathematics 10094 BeijingChina college of Physics and Electronic Shanxi Datong University037009 DatongChina School of Science Tianjin Chengjian University300384 TianjinChina

Based on the unified Hauser–Feshbach and exciton model,which can describe the particle emission processes between discrete energy levels with energy,angular momentum,and parity conservations,a statistical theory of light nucleus reaction(STLN)is developed to calculate the double-differential cross-sections of the outgoing neutron and light charged particles for the proton-induced^(6) Li reaction.A significant difference is observed between the p+^(6) Li and p+^(7) Li reactions owing to the discrepancies in the energy-level structures of the *** reaction channels,including sequential and simultaneous emission processes,are analyzed in *** the double-differential cross-sections of the outgoing proton as an example,the influence of contaminations(such as^(1) H,^(7)Li,^(12)C,and^(16)O)on the target is identified in terms of the kinetic energy of the first emitted *** optical potential parameters of the proton are obtained by fitting the elastic scattering differential *** calculated total double-differential cross-sections of the outgoing proton and deuteron at E_(p)=14 MeV agree well with the experimental data for different outgoing ***,the mixed double differential cross-sections of^(3) He andαare in good agreement with the *** agreement between the measured data and calculated results indicates that the two-body and three-body breakup reactions need to be considered,and the pre-equilibrium reaction mechanism dominates the reaction *** on the STLN model,a PLUNF code for the p+^(6) Li reaction is developed to obtain an ENDF-6-formatted file of the double-differential cross-sections of the nucleon and light composite charged particles.

关键词： Statistical theory of light nucleus reaction p+^(6)Li reaction Light composite charged particle Double-differential cross-sections Two-body breakup Three-body breakup

Description of elastic scattering for 7Li-induced reactions on 1p-shell nuclei

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Chinese Physics C 2024年第2期48卷 153-161页

作者：徐永丽苏新武孙志豪韩银录孙小军张冬红蔡崇海 college of Physics and Electronic Science Shanxi Datong UniversityDatong 037009China Graduate School of China Academy of Engineering Physics Beijing 100088China Key Laboratory of Nuclear Data China Institute of Atomic EnergyBeijing 102413China college of Physics Guangxi Normal UniversityGuilin 541004China Department of Physics Nankai UniversityTianjin 300071China

The experimental data of elastic scattering angular distributions for 9Be,10B,11B,12C,13C,15N,and 16O targets from 4.5 to 131.8 MeV and 7Li target from 8.0 to 42.0 MeV are fitted to realize the global phenomenological optical potentials(GPOPs)for the 7Li-induced reactions on 1p-shell ***,the 7Li elastic scattering from the 1p-shell nuclei can be systematically described using the established *** elastic scattering angular distributions are also reanalyzed using a microscopic method within the framework of the new version of double folding S?o Paulo potential(SPP2).To better describe the elastic scattering at backward angles,the contribution of elastic transfer is further estimated by the distorted wave Born approximation(DWBA)*** on the obtained GPOPs,the inelastic scattering angular distributions are also obtained through the coupled channels(CC)method for the different excited states.

关键词： optical potential elastic scattering nuclear reaction mechanisms

Recent advances and trends of single-atom catalysts for proton exchange membrane fuel cell cathodes

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ChemPhysMater

ChemPhysMater 2024年第2期3卷 143-156页

作者： Zihao Wan Feng Liu Hongfei Xu Shuaili Zhao Zhen An Zizai Ma Zhonghua Zhang Yun Wu Xiaoguang Wang Laboratory of Advanced Materials and Energy Electrochemistry Institute of New Carbon MaterialsCollege of Material Science and EngineeringTaiyuan University of TechnologyTaiyuan 030024China datong Innoreagen Power Technology Co. LtdDatong 037000China college of Chemistry Taiyuan University of TechnologyTaiyuan 030024China Shanxi Key Laboratory of Gas Energy Efficient and Clean Utilization Taiyuan University of TechnologyTaiyuan 030024China Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials(Ministry of Education) School of Materials Science and EngineeringShandong UniversityJinan250061China Department of Materials Science and Engineering Guangdong University of Petrochemical TechnologyMaoming 525000China

Proton exchange membrane fuel cells(PEMFCs),which have the advantages of high-power density,zero emission,and low noise,are considered ideal electrochemical conversion systems for converting hydrogen(H2)and oxy-gen(O_(2))/air into ***,the oxygen reduction reaction(ORR),which is accompanied by multiple electrons,results in voltage loss and low conversion efficiency of ***,PEMFCs mainly use high-load precious platinum(Pt)to promote the ORR process;however,the high cost of Pt hinders the widespread commercialization of *** the past few years,metal-nitrogen-carbon single-atom catalysts(M-N-C SACs)have attracted considerable attention and have been recognized as potential Pt-based catalysts owing to their outstanding ORR *** review briefly introduces the components of ***,we discuss the catalytic mechanisms of the M-N-C SACs for the ***,the latest advances in noble,non-noble,and heteroatom-doped M-N-C SACs used as ORR and PEMFCs cathode catalysts are systematically *** sum-mary,we have outlined the current challenges and proposed a future perspective of M-N-C SACs for PEMFCs cathodes.

关键词： Proton exchange membrane fuel cells Oxygen reductionreaction Cathode Platinum-based catalysts Metal-nitrogen-carbon single-atom catalysts

Rearrangement of Hydrolysis Products of Tetrahydrofolate model compound

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Chinese Chemical Letters 1999年第9期10卷 727-728页

作者： Jian Xin CHENI Jun Sheng HAO Wei GUO Chi Zhong XIA(1datong medical college,datong,Shanxi 0370082Department of Chemistry. Shanxi University, Taiyuan 030006) datong medical college Department of Chemistry Shanxi University

The hydrolysis products of tetrahydrofolate model compound 4 were a mixture of 6 and 7 and the rearrangement reaction between 6 and 7 via 5 was in a state of equilibrium, confirmed by (HNMR)-H-1 and IR spectra.

关键词： tetrahydrofolate hydrolysis rearrangement

Buyang Huanwu decoction enhances cell membrane fluidity in rats with cerebral ischemia/reperfusion

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Neural Regeneration Research 2012年第21期7卷 1605-1610页

作者： Chenxu Li Institute of Brain Sciences Department of Physiology Medical College Datong University Datong 037009 Shanxi Province China

After bilateral carotid artery occlusion for 30 minutes and reperfusion for 2 hours, distinct pathological changes presented in the cerebral cortex and cerebellum of rats. Compared with normal rats, nerve cell membrane fluidity significantly decreased in ischemia/reperfusion rats as detected by spin-labeling electron spin resonance, consistent with order parameter S and rotational correlation time TC measurements. Brain nerve cells from rats with ischemia/reperfusion injury were cultured with 1-100 mg/mL Buyang Huanwu decoction. Results showed that Buyang Huanwu decoction gradually increased membrane fluidity dose-dependently to normal levels, and eliminated hydroxide （OH＇） and superoxide （O2＇） free radicals dose-dependenUy. These findings suggest that Buyang Huanwu decoction can protect against cell membrane fluidity changes in rats with ischemia/ reperfusion injury by scavenging free radicals.

关键词： Buyang Huanwu decoction ischemia/reperfusion electron spin resonance cell membrane fluidity free radical brain neural regeneration

Study on the Interferation of the Concentration of Free Calcium in Peripheral Human Lymphocyte by Low Dose Penicillin, Using Fura-2 as Fluorescent Probe

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Chinese Chemical Letters 2006年第5期17卷 665-666页

作者： Hai Yan WANG Dan Dan WANG Chun Gui ZHAO Ye Hong ZHOU Shao Min SHUANG Chuan DONG School of Chemistry and Chemical Engineering Shanxi University Taiyuan 030006 medical college of datong University Datong 037000

The effect of penicillin on the human peripheral lymphocytes was studied by steady fluorescent technique and ratiometric fluorescence dye, Fura-2, The change of the free calcium concentration in cytosol was examined under different conditions. A characterization of Fura-2-Ca interaction in an isotonic saline solution showed that Ca^2＋ formed a 1：1 Fura-2-Ca complex with the apparent dissociation constant 1.81×10^-7 mol/L. The mechanism, by which penicillin induced the decrease of [Ca^2＋]i , was discussed in detail. The low dose of penicillin might modify the lymphocytes＇ immunology response by interfering the increase in the intracellular free calcium concentration.

关键词： Penicillin lymphocytes Fura-2 Ca^2+ ouabain.

Decomposition of methylamine on Mo(100) surface: A DFT study

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Journal of Natural Gas Chemistry 2012年第2期21卷 132-137页

作者： Jianhong Liu Cunqin Lü Dongli Du Yong Guo college of Chemistry and Chemical Engineering Shanxi Datong UniversityDatong 037009ShanxiChina

The initial decomposition of methylamine on Mo（100） surface has been investigated by self-consistent （GGA-PW91） density functional theory combined with periodic slab model. The adsorption energies of possible species and the activation energies for possible elementary reactions involved are obtained in the present work. Our results indicate that the barriers decreased with the order of C-NN-HC-H. In addition, metastable adsorption of the abstracted hydrogen atom on the hollow site in the final state is also considered for the N-H and C-H bond breaking. For the C-H bond cleavage, the reaction barrier that the abstracted hydrogen located on the hollow site in the final state is lower than that on the bridge site. However, for the N H bond breaking, the barriers are alike for the abstracted hydrogen on both hollow and bridge sites in the final state.

关键词： methylamine decomposition Mo(100) DFT calculations slab model