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Removal and fluorescence detection of antibiotics from wastewater by layered double oxides/metal-organic frameworks with different topological configurations

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Chinese Chemical Letters 2024年第8期35卷 401-405页

作者： Zhiqiang Liu Qiang Gao Wei Shen Meifeng Xu Yunxin Li Weilin Hou Hai-Wei Shi Yaozuo Yuan Erwin Adams Hian Kee Lee Sheng Tang School of environmental and Chemical engineering Jiangsu University of Science and TechnologyZhenjiang 212003China National Medical Products Administration Key Laboratory for Impurity Profile of Chemical Drugs Nanjing 210019China Chemical Drug Inspection Laboratory 2 Jiangsu Institute for Food and Drug ControlNanjing 210019China Department of Pharmaceutical and Pharmacological sciences Pharmaceutical AnalysisKU LeuvenHerestraat 49O&N2PB 923Leuven B-3000Belgium Department of Chemistry National University of Singapore3 Science Drive 3Singapore 117543Singapore

Owing to the serious potential side-effects on the environment and human health,the rapid detection and removal of antibiotics have become an important research *** this work,four zinc-based metal-organic frameworks(MOFs)with different functional groups,i.e.,Zn-MOF,Zn-MOF-CH_(3),Zn-MOF-NO_(2),Zn-MOF-COOH,were utilized for the construction of LDO/MOF composite materials with a nickel-iron-cobalt-based layered double oxide,*** results showed that the LDO/MOF composites not only had high sensitivity in detecting sulfonamide and quinolone antibiotics,but also had an appreciable ability to adsorb them from *** maximum adsorption capacities of all the four types of LDO@Zn-MOFs to all antibiotics can at least reach 150 mg/g,and the limits of detection in relation to all four antibiotics were at least as low as 100μg/*** work suggested the dual-function extraction performance can be attributed to the synergistic effects between the LDO and the ***,the strong ferromagnetism derived from the LDO provided great convenience for the separation and regeneration of the LDO/MOF composites.

关键词： Light-emitting metal-organic frameworks Layered double oxides Antibiotics Topological configurations Fluorescence detection

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Fabricating bio-inspired high impact resistance carbon nanotube network films for multi-protection under an extreme environment

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Nano Research 2024年第9期17卷 7793-7802页

作者： Mingquan Zhu Kailu Xiao Wei Zhang Xudong Lei Yunxiang Bai Shijun Wang Peng Zhang Feng Gao Congying Wang Wenqiang Xu Huiyong Li Xianqian Wu Chao Wang Hui Zhang Luqi Liu Zhong Zhang CAS Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190China University of Chinese Academy of sciences Beijing 100049China Department of Materials science and engineering Texas A&M UniversityCollege StationTexas 77840USA Institute of Mechanics Chinese Academy of SciencesBeijing 100190China School of Astronautics Harbin Institute of TechnologyHarbin150001China CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Modern MechanicsUniversity of Science and Technology of ChinaHefei 230027China

The fabrication of light-weight,highly impact-resistant,and energy-absorbent materials is urgently demanded in many facets of the society from body armor to aerospace engineering,especially under an extreme *** nanotubes(CNTs),one of the strongest and toughest materials ever found,also have good conductivity,chemical stability,and thermal stability,etc,making them a competitive candidate as building blocks to help achieve the above *** this work,a kind of CNT network was prepared by using chlorosulfonic acid(CSA)to release the internal stress of super-aligned carbon nanotube films(SA-CNTF)and dendritic polyamide amine(PAMAM)to further introduce multiple hydrogen bonds and interlocking *** fabricated bioinspired carbon nanotube network films(PAMAM@C-CNTF)have a high toughness of 45.97 MJ/m3,showing an increase of 420%compared to neat *** importantly,the anti-impact performance of the films(e.g.,with a maximum specific energy absorption of 1.40 MJ/kg under 80-100 m/s projectile impact)is superior to that of conventional protective materials from steel and Kevlar fiber,and also exceeds that of any other reported carbon-based *** hierarchical energy dissipation mechanism was further revealed through experiment and *** functions including intelligent heating/anti-icing,ultraviolet protection,as well as electromagnetic interference shielding properties make these network films have great potential in practical multi-protection applications,especially under an extreme environment.

关键词： carbon nanotubes composites mechanical properties multi-function

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Measuring Impact of Lean Manufacturing Tools for Continuous Improvement on Economic Sustainability

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Journal of Systems science and Systems engineering 2024年第4期33卷 452-474页

作者： Luis Javier Márquez Figueroa Jorge Luis García-Alcaraz Ahmed I.Osman Alfonso Jesús Gil López Yashar Aryanfar Mika Sillanpää Mamdouh El Haj Assad Department of Electrical engineering and Computer science Universidad Autónoma de Ciudad JuárezCiudad JuárezChihuahuaMéxico Department of Industrial engineering and Manufacturing Universidad Autónoma de Ciudad JuárezCiudad JuárezChihuahuaMéxico School of Chemistry and Chemical engineering Queens UniversityBelfastNorthern IrelandUK Department of Economic and Managerial sciences University of La RiojaLa RiojaSpain Department of Chemical engineering University of JohannesburgJohannesburgSouth Africa Department of Sustainable and Renewable Energy engineering University of SharjahSharjahUAE

Using Lean Manufacturing(LM)tools in production processes is crucial for companies’economic,environmental,and social sustainability *** study shows a structural equation model(SEM)that shows the relationship between LM Tools like Kaizen(KAI),Gemba(GEM),Value Stream Mapping(VSM)and Key Performance Indicator(KPI)with Economic Sustainability(ECS).Seven hypotheses were evaluated with data from 179 responses to a questionnaire about the Mexican maquiladora industry,showing that these variables are *** a 95%confidence level,the model was evaluated using the partial least squares *** findings indicate that the relationships between KAI and GEM and KAI and VSM have the strongest relationship,followed by VSM and ECS;however,VSM has the strongest effect on *** on these findings,it is recommended that managers adopt a continuous improvement(KAI)approach based on working directly on the shop floor(GEM and VSM)to support their decisions regarding economic growth(ECS).

关键词： Lean manufacturing economic sustainability structural equation model quality improvement

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二氧化碳静态爆破的边坡振动场地效应和能量分析

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Journal of Central South University 2024年第1期31卷 210-224页

作者：王小飞胡少斌王恩元 School of Safety engineering China University of Mining and TechnologyXuzhou 221116China Tunnel and Underground engineering Institute College of Civil and Transportation EngineeringHohai UniversityNanjing 210098China

进行真三轴CO_(2)静态爆破压裂实验和现场测试,获得压力曲线、试样裂隙分布、现场振动曲线和岩体破坏特征,并通过分析压力曲线和裂缝扩展特征来研究致裂原理,同时还利用窗函数傅里叶变换提取振动特征,以评估破岩现场边坡的结构安全。研... 详细信息

进行真三轴CO_(2)静态爆破压裂实验和现场测试,获得压力曲线、试样裂隙分布、现场振动曲线和岩体破坏特征,并通过分析压力曲线和裂缝扩展特征来研究致裂原理,同时还利用窗函数傅里叶变换提取振动特征,以评估破岩现场边坡的结构安全。研究结果表明:(1)CO_(2)静态爆破的峰值振动速度在8 m处衰减至满足建筑物保护要求,比传统的钻爆法更安全;(2)CO_(2)静态爆破引起的振动波形的主频高于钻爆法的,且随着距离的加长,振动能量的分布逐渐分散;(3)钻爆法的振动速度预测公式适用于CO_(2)静态爆破的,且带高程的预测公式更为准确。根据压力曲线、试样裂隙分布和现场岩体损伤,提出CO_(2)静态爆破的HIG破岩模型,为新技术的研究提供了基础框架。在实验中没有采集到温度数据,今后迫切需要对聚能剂的瞬时放热特性和温度对CO_(2)状态的影响进行研究。

关键词：破岩技术二氧化碳静态爆破振动速度致裂机理能量计算

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Complex interplay between formation routes and natural organic matter modification controls capabilities of C_(60)nanoparticles(nC_(60)) to accumulate organic contaminants

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Journal of environmental sciences 2017年第1期29卷 315-323页

作者： Lei Hou John D.Fortner Ximeng Wang Chengdong Zhang Lilin Wang Wei Chen college of environmental science and engineering Southwest Forestry University college of environmental science and engineering Nankai University Department of Energy Environmental and Chemical EngineeringWashington University in St.Louis

Accumulation of organic contaminants on fullerene nanoparticles（nC（60）） may significantly affect the risks of C（60） in the *** objective of this study was to further understand how the interplay of nC（60） formation routes and humic acid modification affects contaminant adsorption of nC（60）.Specifically,adsorption of 1,2,4,5-tetrachlorobenzene（a model nonionic,hydrophobic organic contaminant） on nC（60） was greatly affected by nC（60）formation route- the formation route significantly affected the aggregation properties of nC（60）,thus affecting the available surface area and the extent of adsorption via the pore-filling *** on whether nC（60） was formed via the ＂top-down＂ route（i.e.,sonicating C（60） powder in aqueous solution） or ＂bottom-up＂ route（i.e.,phase transfer from an organic solvent） and the type of solvent involved（toluene versus tetrahydrofuran）,modification of nC（60） with Suwannee River humic acid（SRHA） could either enhance or inhibit the adsorption affinity of nC（60）.The net effect depended on the specific way in which SRHA interacted with C（60） monomers and/or C（60） aggregates of different sizes and morphology,which determined the relative importance of enhanced adsorption from SRHA modification via preventing C（60） aggregation and inhibited adsorption through blocking available adsorption *** findings further demonstrate the complex mechanisms controlling interactions between nC（60） and organic contaminants,and may have significant implications for the life-cycle analysis and risk assessment of C（60）.

关键词： Fullerene nanoparticles Aggregation Natural organic matter Organic contaminants Adsorption

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Carbon nanotubes-reinforced polylactic acid/hydroxyapatite porous scaffolds for bone tissue engineering

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Frontiers of Materials science 2024年第1期18卷 59-69页

作者： Weiwei Lan Mingbo Wang Zhenjun Lv Jun Li Fuying Chen Ziwei Liang Di Huang Xiaochun Wei Weiyi Chen Research Center for Nano-Biomaterials&Regenerative Medicine Department of Biomedical EngineeringCollege of Biomedical EngineeringTaiyuan University of TechnologyTaiyuan 030024China Guangdong engineering Technology Research Center of Implantable Medical Polymer Shenzhen Lando Biomaterials Co.Ltd.Shenzhen 518107China Shanxi-Zheda Institute of Advanced Materials and Chemical engineering Taiyuan 030060China Department of Orthopaedics The Second Hospital of Shanxi Medical UniversityTaiyuan 030001China

In the field of bone defect repair,critical requirements for favorable cytocompatibility and optimal mechanical properties have propelled research efforts towards the development of composite *** this study,carbon nanotubes/polylactic acid/hydroxyapatite(CNTs/PLA/HA)scaffolds with different contents(0.5,1,1.5 and 2 wt.%)of CNTs were prepared by the thermally induced phase separation(TIPS)*** results revealed that the composite scaffolds had uniform pores with high porosities over 68%and high through *** addition of CNTs significantly enhanced the mechanical properties of resulted PLA/HA,in which the 1.5 wt.%CNTs/PLA/HA composite scaffold demonstrated the optimum mechanical behaviors with the bending elastic modulus of(868.5±12.34)MPa,the tensile elastic modulus of(209.51±12.73)MPa,and the tensile strength of(3.26±0.61)***,L929 cells on the 1.5 wt.%CNTs/PLA/HA scaffold displayed good spreading performance and favorable ***,it is expected that the 1.5 wt.%CNTs/PLA/HA scaffold has potential applications in bone tissue engineering.

关键词： CNTs/PLA/HA scaffold TIPS method mechanical property bone tissue engineering

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NaBSOwith unprecedented[BSO]double chains and largest birefringence among borosulfates induced by the uniform arrangement of[BO] units

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science China Chemistry 2024年

作者： Jinbin Fan Ziting Yan Zilong Chen Huimin Li Zhihua Yang Fangfang Zhang Shilie Pan Research Center for Crystal Materials State Key Laboratory of Functional Materials and Devices for Special Environmental ConditionsXinjiang Key Laboratory of Functional Crystal Materials Xinjiang Technical Institute of Physics and Chemistry Chinese Academy of Sciences Center of Materials science and Optoelectronics engineering University of Chinese Academy of Sciences

Birefringence is crucial for birefringent crystals to modulate polarized light and nonlinear optical crystals to enable *** is closely related to the arrangement of advantageous functional groups with large microcosmic polarizability anisotropy in the ***,designing crystals with large birefringence by modulating the arrangement of advantageous functional groups is still a *** this work,the arrangement of the advantageous[B3O7]groups is optimized by introducing rigid tetrahedral[SO4]groups,resulting in a novel boron-rich borosulfate,Na2B6SO13,which exhibits unprecedented[B6SO13]∞double chain and an enhanced birefringence （Δn=0.07 at 589.3 nm） against the borate parent *** calculations confirm that the birefringence is mainly attributable to the uniform alignment of[B3O7]***2B6SO13also possesses a deep ultraviolet （DUV） cutoff edge （λ<185 nm）.This work provides a feasible method to design DUV birefringent crystals with large birefringence by inducing the arrangement of advantageous functional groups.

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Facile Semiconductor p-n Homojunction Nanowires with Strategic p-Type Doping engineering Combined with Surface Reconstruction for Biosensing Applications

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Nano-Micro Letters 2024年第10期16卷 15-30页

作者： Liuan Li Shi Fang Wei Chen Yueyue Li Mohammad Fazel Vafadar Danhao Wang Yang Kang Xin Liu Yuanmin Luo Kun Liang Yiping Dang Lei Zhao Songrui Zhao Zongzhi Yin Haiding Sun iGaN Laboratory School of MicroelectronicsUniversity of Science and Technology of ChinaHefei 230026People's Republic of China Department of Obstetrics and Gynecology The First Affiliated Hospital of Anhui Medical UniversityNo 218 Jixi RoadHefei 230022People's Republic of China Department of Electrical and Computer engineering McGill University3480 University StreetMontrealQC H3A 0E9Canada Union Hospital Tongji Medical CollegeHuazhong University of Science and TechnologyNo 1277 Jiefang Ave.Wuhan 430022People's Republic of China

Photosensors with versatile functionalities have emerged as a cornerstone for breakthroughs in the future optoelectronic systems across a wide range of *** particular,emerging photoelectrochemical(PEC)-type devices have recently attracted extensive interest in liquid-based biosensing applications due to their natural electrolyte-assisted operating ***,a PEC-type photosensor was carefully designed and constructed by employing gallium nitride(GaN)p-n homojunction semiconductor nanowires on silicon,with the p-GaN segment strategically doped and then decorated with cobalt-nickel oxide(CoNiO_(x)).Essentially,the p-n homojunction configuration with facile p-doping engineering improves carrier separation efficiency and facilitates carrier transfer to the nanowire surface,while CoNiO_(x)decoration further boosts PEC reaction activity and carrier dynamics at the nanowire/electrolyte ***,the constructed photosensor achieves a high responsivity of 247.8 mA W^(-1)while simultaneously exhibiting excellent operating ***,based on the remarkable stability and high responsivity of the device,a glucose sensing system was established with a demonstration of glucose level determination in real human *** work offers a feasible and universal approach in the pursuit of high-performance bio-related sensing applications via a rational design of PEC devices in the form of nanostructured architecture with strategic doping engineering.

关键词： p-n GaN nanowires Strategic p-doping Surface decoration Photoelectrochemical sensor Glucose sensing

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具有UCST行为和UV/温度诱导多色荧光的水凝胶用于协同编码和加密（英文）

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science China Materials 2024年

作者：刘川郝康安俞润昊李蓉黄安荣吴翀郑凯杨吟野左晓玲 college of Physics and Mechatronic engineering Guizhou Minzu University college of Materials science and engineering Guizhou Minzu University National engineering Research Center for Compounding and Modification of Polymeric Materials college of Pharmacy Guizhou University of Traditional Chinese Medicine School of Materials and Energy engineering Guizhou Institute of Technology

开发能够发射多色荧光的水凝胶为解决信息泄漏和敏感数据失真等问题提供了一条有希望的途径.将多因素诱导可调荧光与水凝胶中独特的上临界溶液温度(UCST)行为相结合,有助于开发既能动态显示信息,又能提供高水平信息安全与保护的多维和...

开发能够发射多色荧光的水凝胶为解决信息泄漏和敏感数据失真等问题提供了一条有希望的途径.将多因素诱导可调荧光与水凝胶中独特的上临界溶液温度(UCST)行为相结合,有助于开发既能动态显示信息,又能提供高水平信息安全与保护的多维和多级信息存储材料.然而,将这些优势特性融合到水凝胶中,并用于信息存储和显示仍然是一个相当大的挑战.在此背景下,我们通过光固化3D打印技术—一种可持续的和高效的材料制造方法,制备了一种新型三维荧光编码水凝胶阵列.该阵列结合了上述特性,并且需要两个不同步骤依次解密隐藏的信息,也即:i)温度诱导的相变,以及ii)紫外光和温度在特定条件下(即特定的紫外光照射时长、加热时长和辐照波长)触发的多色荧光.这些水凝胶具有可逆透明性和可编程荧光发射特性,有望显著增强信息加密和防伪过程.这一进步有望为信息安全领域带来革命性变化.

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Injectable“cocktail”hydrogel with dual-stimuli-responsive drug release,photothermal ablation,and drug-antibody synergistic effect

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SmartMat 2024年第2期5卷 43-53页

作者： Li Zhao Jiawen Xu Yao Tong Pengyu Gong Fucheng Gao Hui Li Yanyan Jiang Key Laboratory for Liquid-Solid Structural Evolution&Processing of Materials(Ministry of Education) School of Materials Science and EngineeringShandong UniversityJinanChina Department of Pathology Shandong Provincial Hospital Affiliated to Shandong First Medical UniversityJinanChina Department of Clinical Laboratory The Second HospitalCheeloo College of MedicineShandong UniversityJinanChina

The combination of the first-line standard chemotherapeutic drug doxorubicin hydrochloride(DOX)and the molecular-targeted drug Herceptin(HCT)has emerged as a promising strategy for human epidermal growth receptor 2(HER-2)overexpressing breast cancer ***,insufficient drug accumulation and severe cardiotoxicity are two major challenges that limit its clinical ***,an in situ forming gold nanorods(AuNRs)-sodium alginate(ALG)hybrid hydrogel encapsulating DOX and HCT was engineered for tumor synergistic therapy involving injectable,dual-stimuli-responsive drug release,photothermal ablation,and drug-antibody synergistic *** photothermal agent AuNRs,anticancer drug DOX,and anticancer antibody HCT were mixed in ALG solution,and after injection,the soluble ALG was quickly transformed into a hydrogel in the presence of Ca^(2+)in the ***,the hybrid hydrogel exhibits an extremely high photothermal conversion efficiency of 70%under 808 nm laser *** thermal effect can also provide photothermal stimulation to trigger the drug release from the gel *** addition,the drug release rate and the releasing degree are also sensitive to the *** vitro studies demonstrated that the PEI-AuNR/DOX/HCT/ALG hydrogel has facilitated the therapeutic efficiency of each payload and demonstrated a strong synergistic killing effect on SK-BR-3 *** vivo imaging results showed that the local drug delivery system can effectively reduce the nonspecific distribution in normal tissues and increase drug concentration at tumor *** proposed hydrogel system shows significant clinical implications by easily introducing a sustainable photothermal therapy and a potential universal carrier for the local delivery of multiple drugs to overcome the challenges faced in HER-2 overexpressing cancer therapy.

关键词： dual-stimuli-responsive drug release HER-2 overexpressing breast cancer injectable hydrogel photothermal therapy synergistic effect

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