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Coupling N-doping and confined Co3O4 on carbon nanotubes by polydopamine coating strategy for pleiotropic water purification

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Rare Metals 2024年第7期43卷 3146-3160页

作者： Wen-Long Tu Gang Wang Yue Zhang Hong-Yang Zhu Rong-Rong Du Hong-Yao Zhao Sheng Tang Zeng-Jing Guo Jun Yang Fu Yang Cheng-Zhang Zhu school of Environmental and Chemical engineering Jiangsu University of Science and Technology school of Chemistry and Chemical engineering Liaocheng University school of Material Science and engineering Jiangsu University of Science and Technology school of Environmental Science and engineering Nanjing Tech University

The development of effective and sustainable solutions for pleiotropic water purification becomes urgent and *** Fenton-like catalysts for activation of peroxymonosulfate（PMS） to purify organic wastewater show great *** this work,by tuning metal loading with an in-situ polydopamine coating strategy,oxygen vacancy-enriched Co3O4loading on N-doped carbon nanotubes（CNTs） were constructed to enhance PMS activation efficiency for pollutants ***,the obtained modified CNTs afford a well-developed N-containing network structure,which is further endowed with abundant Co（Ⅱ）/Co（Ⅲ） redox cycles and significant metal-carbon *** particular,the surface N doping in CNTs might induce the oriented enrichment of pollutants around the catalyst,which reduces the migration distance and correspondingly improves the utilization of reactive oxidative *** electron transfer efficiency of the catalyst can be further improved by incorporating oxygen vacancy-enriched *** performance results show that the optimal NC/Co-1 could mineralize 20 × 10-6of bisphenol A（BPA） by almost 98% in 8 min.A low reaction activation energy(26.05 kJ·mol-1) in BPA degradation was demonstrated by the NC/*** importantly,NC/Co-1 can inherit excellent degradation performance towards oxytetracycline,2,4-dichlorophenol,and tetracycline,showing wide practical *** addition,by virtue of the photothermal conversion property,NC/Co-1 achieves an additive function for interfacial solar water evaporation(1.84 kg·m-2·h-1,112.51%),showing impressive potential for clean water recovery under complicated environmental pollution conditions.

关键词： Carbon nanotube Advanced oxidation process Co 3 O 4 Photothermal conversion Solar water evaporation

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Cooperative control for heterogeneous multi-agent systems: progress, applications, and challenges

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Science China(Information Sciences) 2024年第5期67卷 318-320页

作者： Bing YAN Peng SHI Jonathon CHAMBERS school of Electrical and Mechanical engineering Faculty of Science Engineering and TechnologyThe University of Adelaide school of engineering College of Science and Engineering University of Leicester

Cooperative control for heterogeneous multi-agent systems(MASs) is a critical and rapidly evolving field in modern automation and robotics. Characterized by the integration of agents with diverse capabilities and func... 详细信息

关键词： Multi agent systems

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One-step growth of ultrathin CoSe_(2)nanobelts on N-doped MXene nanosheets for dendrite-inhibited and kinetic-accelerated lithium-sulfur chemistry

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Science Bulletin 2024年第13期69卷 2059-2070页

作者： Chuanliang Wei Zhengran Wang Peng Wang Xinlu Zhang Xuguang An Jinkui Feng Baojuan Xi Shenglin Xiong school of Chemistry and Chemical engineering School of Materials Science and EngineeringShandong UniversityJinan 250100China school of Mechanical engineering Chengdu UniversityChengdu 610106China

The practical application of lithium–sulfur(Li–S)batteries is inhibited by the shuttle effect of lithium polysulfides(LiPSs)and slow polysulfide redox kinetics on the S cathode as well as the uncontrollable growth of dendrites on the Li metal ***,both cathode and anode sides must be considered when modifying LiS ***,two-dimensional(2D)ultrathin CoSe_(2)nanobelts are in situ grown on 2D N-doped MXene nanosheets(CoSe_(2)@N-MXene)via one-step solvothermal process for the first *** to its unique 2D/2D structure,CoSe_(2)@N-MXene can be processed to crumpled nanosheets by freeze-drying and flexible and freestanding films by vacuum *** crumpled CoSe_(2)@NMXene nanosheets with abundant active sites and inner spaces can act as S hosts to accelerate polysulfide redox kinetics and suppress the shuttle effect of LiPSs owing to their strong adsorption ability and catalytic conversion effect with ***,the CoSe_(2)@N-MXene film(CoSe_(2)@NMF)can act as a current collector to promote uniform Li deposition because it contains lithiophilic CoSe_(2)and N *** the systematic effect of CoSe_(2)@N-MXene on S cathode and Li metal anode,the electrochemical and safety performance of Li–S batteries are ***_(2)@NMF also shows excellent storage performances in flexible energy storage devices.

关键词： Ultrathin CoSe_(2)nanobelts N-doped MXene nanosheets In situ growth Flexible MXene-based films Li-S batteries

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Rapid Phase Ambiguity Elimination Methods for DOA Estimator via Hybrid Massive MIMO Receive Array

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Chinese Journal of Electronics 2024年第1期33卷 175-184页

作者： Xichao ZHAN Zhongwen SUN Feng SHU Yiwen CHEN Xin CHENG Yuanyuan WU Qi ZHANG Yifan LI Peng ZHANG school of Information and Communication engineering Hainan University school of Electronic and Optical engineering Nanjing University of Science and Technology

For a sub-connected hybrid multiple-input multiple-output(MIMO) receiver with K subarrays and N antennas, there exists a challenging problem of how to rapidly remove phase ambiguity in only single time-slot. A direction of arrival(DOA) estimator of maximizing received power(Max-RP) is proposed to find the maximum value of K-subarray output powers, where each subarray is in charge of one sector, and the center angle of the sector corresponding to the maximum output is the estimated true DOA. To make an enhancement on precision, Max-RP plus quadratic interpolation(Max-RP-QI) method is designed. In the proposed Max-RP-QI, a quadratic interpolation scheme is adopted to interpolate the three DOA values corresponding to the largest three receive powers of *** achieve the Cramer Rao lower bound, a Root-MUSIC plus Max-RP-QI scheme is developed. Simulation results show that the proposed three methods eliminate the phase ambiguity during one time-slot and also show low computational complexities. The proposed Root-MUSIC plus Max-RP-QI scheme can reach the Cramer Rao lower bound,and the proposed Max-RP and Max-RP-QI are still some performance losses 2–4 d B compared to the Cramer Rao lower bound.

关键词： Phased arrays Interpolation Wireless sensor networks Direction-of-arrival estimation Simulation Receiving antennas Massive MIMO

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An unexpected approach to enhance specific surface area and mesopore amount of polyaniline by Zn doping

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Rare Metals 2024年第9期43卷 4585-4594页

作者： Zhi-Da Zhu Yu-Zhe Han Xiao-Bi Jing school of Mechanical engineering Yangzhou University school of Chemistry and Chemical engineering Yangzhou University

Poly-p-anisidine could be easily fabricated via the oxidative polymerization reaction of p-anisidine using H2O2as the green oxidant. It was unexpectedly found that zinc doping could significantly improve the adsorption ability of the material versus heavy metals such as Pb, Cu,Pd, Ag and Hg. Results of nitrogen adsorption–desorption experiments demonstrated that Zn doping could enhance the specific surface area and mesopore amount of the prepared material, which might facilitate its absorption to metals. This work not only provides a novel material for the treatment of heavy metal-polluted water but also leads to a nice mesoporous catalyst support for environment protection and organic synthesis, i.e. the Zn-doped poly-panisidine can be employed as the catalyst support to prepare Cu@PANI-OMe/Zn or Pd@PANI-OMe/Zn for the oxidative degradation reaction of phenol or Suzuki–Miyaura coupling reactions, respectively. It discloses a new strategy for fabricating the mesoporous polyaniline materials with profound application potential.

关键词： Adsorption Catalysis Porous materials Rare metal concentration Surfaces

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Structural uncertainty quantification of Reynolds-Averaged Navier–Stokes closures for various shock-wave/boundary layer interaction flows

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Chinese Journal of Aeronautics 2024年第3期37卷 34-48页

作者： Fanzhi ZENG Tianxin ZHANG Denggao TANG Jinping LI Chao YAN school of Aeronautic Science and engineering Beihang UniversityBeijing 100191China school of Aeronautical engineering Air Force Engineering UniversityXi’an 710038China

Accurate prediction of Shock-Wave/Boundary Layer Interaction(SWBLI)flows has been a persistent challenge for linear eddy viscosity models.A major limitation lies in the isotropic representation of the Reynolds stress,as assumed under the Boussinesq *** studies have shown promise in improving the prediction capability for incompressible separation flows by perturbing the Reynolds-stress anisotropy ***,it remains uncertain whether this approach is effective for SWBLI flows,which involve compressibility and *** address this issue,this study systematically quantifies the structural uncertainty of the anisotropy for oblique SWBLI *** eigenspace perturbation method is applied to perturb the anisotropy tensor predicted by the Menter Shear–Stress Transport(SST)model and reveal the impacts of anisotropy on the prediction of quantities of interest,such as separation and reattachment positions,wall static pressure,skin friction,and heat *** results demonstrate the potential and reveal the challenges of eigenspace perturbation in improving the SST ***,a detailed analysis of turbulent characteristics is performed to identify the source of *** findings indicate that eigenspace perturbation primarily affects turbulent shear stress,while the prediction error of the SST model is more related to turbulent kinetic energy.

关键词： Shock-wave/boundary layer interaction(SWBLI) Turbulence models Uncertainty analysis Eigenspace perturbation Anisotropy

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Numerical and experimental investigation on hydraulic-electric rock fragmentation of heterogeneous granite

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International Journal of Mining Science and Technology 2024年第1期34卷 15-29页

作者： Xiaohua Zhu Ling He Weiji Liu Yunxu Luo Youjian Zhang Wuji Tang school of Mechatronic engineering Southwest Petroleum UniversityChengdu 610500China school of Mechanical engineering Sichuan University of Science and EngineeringYibin 643002China

Hydraulic-electric rock fragmentation(HERF)plays a significant role in improving the efficiency of high voltage pulse rock ***,the underlying mechanism of HERF remains *** this study,considering the heterogeneity of the rock,microscopic thermodynamic properties,and shockwave time domain waveforms,based on the shockwave model,digital imaging technology and the discrete element method,the cyclic loading numerical simulations of HERF is achieved by coupling electrical,thermal,and solid mechanics under different formation temperatures,confining pressure,initial peak voltage,electrode bit diameter,and loading ***,the HERF discharge system is conducive to the laboratory experiments with various electrical parameters and the resulting broken pits are numerically reconstructed to obtain the geometric *** results show that,the completely broken area consists of powdery rock *** the pre-broken zone,the mineral cementation of the rock determines the transition of type CⅠcracks to type CⅡand type CⅢ***,the peak pressure of the shockwave increased with initial peak voltage but decreased with electrode bit diameter,while the wave front time ***,increasing well depth,formation temperature and confining pressure augment and inhibit HERF,but once confining pressure surpassed the threshold of 60 MPa for 152.40,215.90,and 228.60 mm electrode bits,and 40 MPa for 309.88 mm electrode bits,HERF is ***,for the same kind of rock,the volume and width of the broken pit increase with higher initial peak voltage and rock fissures will promote ***,the electrode drill bit with a 215.90 mm diameter is more suitable for drilling pink *** research contributes to a better microscopic understanding of HERF and provides valuable insights for electrode bit selection,as well as the optimization of circuit parameters for HERF technology.

关键词： Hydraulic-electric rock fragmentation Shockwave Thermodynamics Microcracks Weak Linear Parallel Bond Model

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Resilient sliding mode control for 2D CPSs under denial-of-service attacks

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Science China(Information Sciences) 2024年第6期67卷 262-278页

作者： Lingling LI Rongni YANG Zhiguang FENG Ligang WU College of Intelligent Systems Science and engineering Harbin Engineering University school of Control Science and engineering Shandong University school of Astronautics Harbin Institute of Technology

This study addresses the resilient sliding mode control(SMC) problem for two-dimensional cyber-physical systems(2D CPSs) characterized by the Roesser model under denial-of-service attack(DoSA), which can interfere with signal transmission over the communication network. First, the DoS-A model is established by introducing constraints on the Do S frequency and duration. Then, based on active or silent attack situations, the considered system is described as a switched mode. Furthermore, together with Lyapunov theory, the average dwell time technique is employed to deduce sufficient criteria that assure the existence of the desired sliding mode controller. Finally, verification examples are provided to show the validity of the established SMC scheme.

关键词： two-dimensional systems cyber-physical systems denial-of-service attack resilient sliding mode control

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HTDcr:a job execution framework for high-throughput computing on supercomputers

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Science China(Information Sciences) 2024年第1期67卷 69-85页

作者： Jiazhi JIANG Dan HUANG Hu CHEN Yutong LU Xiangke LIAO school of Computer Science and engineering Sun Yat-sen University school of Software engineering South China University of Technology

High-throughput computing(HTC) is a computing paradigm that aims to accomplish jobs by easily breaking them into smaller,independent ***,it requires a large amount of computing power for a long *** existing HTC frameworks are job-oriented without support for coscheduling with hardware architecture and task-level ***,most of the frameworks reach a limited scale,and their usability needs further ***,we present HTDcr,a job execution framework for the HTC on *** study aims to improve the throughput,task dispatching,and usability of the *** detail,the throughput optimizations include a sophisticated designed task management system,a hierarchical scheduler,and the co-optimization of the task-scheduling strategy with the application and hardware *** optimizations for usability include a programable execution workflow,mechanisms for more robust and reliable service qualities,and a fine-grained resource allocation system for the colocation of multiple *** to our evaluations,HTDcr can achieve outstanding scalability and high throughput on large-scale clusters for the HTC *** evaluate HTDcr with several microbenchmarks and real-world applications on Tianhe-2 and Sunway TaihuLight to demonstrate its effects on existing design *** instance,the task scheduling for two real-world applications integrated with the application and hardware characteristics achieves 1.7× and 1.9× speedups over the basic task-scheduling strategy.

关键词： high-throughput computing supercomputer task scheduling middleware password guessing

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Heterogeneous engineering of MnSe@NC@ReS2 core-shell nanowires for advanced sodium-/potassium-ion batteries

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Rare Metals 2024年第8期43卷 3713-3723页

作者： Sheng-Jun Lu Jin-Yi Lin Cai-Hong Wang Yu-Fei Zhang Yi Zhang Hao-Sen Fan College of Materials Science and Metallurgy engineering Guizhou University school of Energy Science and engineering Nanjing Tech University school of Chemistry and Chemical engineering Guangzhou University

Sodium-ion batteries（SIBs） and potassium-ion batteries（PIBs） have been attracting great attentions and widely been exploited due to the abundant sodium/potassium ***,the preparation of high-powered anode materials for SIBs/PIBs plays a decisive role for the commercial applications of SIBs/PIBs in the *** selenides are a class of potential anode materials for SIBs/PIBs because of their small band gap and high electrical *** this work,MnSe and ReS2core-shell nanowires connecting by polydopamine derived carbon nanotube（MnSe@NC@ReS2） have been successfully synthesized from growing ReS2nanosheets array on the surface of MnSe@NC nano wires,which present excellent Na+/K+storage *** applied as SIBs anode,the specific capacity of 300 mAh·g-1was maintwined after 400 cycles at the current density of 1.0 A·***,it could also keep 120 mAh·g-1specific capacity after 900 cycles at 1.0 A·g-1for the anode of *** heterogeneous engineering and one-dimensional-two-dimensional（1D-2D） hybrid strategies could provide an ideal strategy for the synthesis of new hetero-structured anode materials with outstanding battery performance for SIBs and PIBs.

关键词： Heterogeneous engineering Core–shell nanowires MnSe@NC@ReS 2 nanowires Na + batteries K + batteries

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