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Journal of Mountain Science 2023年第4期20卷 1061-1073页

作者： MA Jie SHEN Zhi-jie WANG Sheng-lan DENG Li SUN Jing LIU Ping SHE Ze-lei chongqing ecological and environmental monitoring center Chongqing401147China Key Laboratory of Organic Pollutants in environmental Chemical Behavior and ecological Toxicology of chongqing Chongqing401147China College of Resources and Environment Southwest UniversityChongqing400715China chongqing University of Arts and Sciences Chongqing402160China

This study studied the characteristics and source apportionment of heavy metal pollution in the agricultural soil surrounding a gangue coal heap in chongqing,China by using absolute principal component scores-multiple linear regression(APCSMLR)model and positive matrix factorization(PMF)*** applicability of the models was compared in the assessment of source *** results showed that the average contents of Cd,Hg,As,Pb,Cr,Cu,Ni,and Zn in the surface soil were 0.46,0.14,9.66,31.2,127,95.6,76.0,and 158 mg/kg,*** with the spatial distribution and correlation analyses,the results of source apportionment were consistent for both the APCSMLR and PMF ***,Hg,As,and Pb were mainly affected by the gangue heap accumulation,with respective contributions of 74.6%,79.4%,69.1%,and 67.2%based on the APCS-MLR model and respective contributions of 69.7%,60.7%,57.4%,and 41.9%based on the PMF *** and Zn were mainly affected by industrial and agricultural activities,while Cr and Cu were mainly affected by natural *** results of the source apportionment were approximately consistent between the APCS-MLR and PMF *** combined application of the two receptor models can make the results of source apportionment more comprehensive,accurate,and reliable.

关键词： Coal gangue heap Heavy metals Agricultural soil Source apportionment

Health risk assessment of trace metal(loid)s in agricultural soils based on Monte Carlo simulation coupled with positive matrix factorization model in chongqing, southwest China

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Journal of Mountain Science 2024年第1期21卷 100-112页

作者： MA Jie CHU Lijuan SUN Jing WANG Shenglan GE Miao DENG Li chongqing ecological and environmental monitoring center Chongqing 401147China Key Laboratory of Organic Pollutants in environmental Chemical Behavior and ecological Toxicology of chongqing Chongqing 401147China Department of Pediatrics Chongqing Health Center for Women and ChildrenChongqing 401147China Department of Pediatrics Women and Children’s Hospital of Chongqing Medical UniversityChongqing 401147China

This study aimed to investigate the pollution characteristics, source apportionment, and health risks associated with trace metal(loid)s(TMs) in the major agricultural producing areas in chongqing, China. We analyzed the source apportionment and assessed the health risk of TMs in agricultural soils by using positive matrix factorization(PMF) model and health risk assessment(HRA) model based on Monte Carlo simulation. Meanwhile, we combined PMF and HRA models to explore the health risks of TMs in agricultural soils by different pollution sources to determine the priority control factors. Results showed that the average contents of cadmium(Cd), arsenic (As), lead(Pb), chromium(Cr), copper(Cu), nickel(Ni), and zinc(Zn) in the soil were found to be 0.26, 5.93, 27.14, 61.32, 23.81, 32.45, and 78.65 mg/kg, respectively. Spatial analysis and source apportionment analysis revealed that urban and industrial sources, agricultural sources, and natural sources accounted for 33.0%, 27.7%, and 39.3% of TM accumulation in the soil, respectively. In the HRA model based on Monte Carlo simulation, noncarcinogenic risks were deemed negligible(hazard index <1), the carcinogenic risks were at acceptable level(10^(-6)

关键词： Monte Carlo simulation Health risk assessment Trace metal(loid)s Positive matrix factorization Agricultural soils

Exploration of the formation mechanism and source attribution of ambient ozone in chongqing with an observation-based model

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Science China Earth Sciences 2018年第1期61卷 23-32页

作者： SU Rong LU KeDing YU JiaYan TAN ZhaoFeng JIANG MeiQing LI Jing XIE ShaoDong WU YuSheng ZENG LiMin ZHAI ChongZhi ZHANG YuanHang State Key Joint Laboratory of environmental Simulation and Pollution Control College of Environmental Sciences and Engineering Peking University Beijing 100871 China ecological and environmental monitoring center ofchongqing Chongqing 401147 China

An intensive field campaign was conducted in chongqing during the summer of 2015 to explore the formation mechanisms of ozone pollution. The sources of ozone, the local production rates, and the controlling factors, as well as key species of volatile organic compounds(VOCs), were quantified by integrating a local ozone budget analysis, calculations of the relative incremental reactivity, and an empirical kinetic model approach. It was found that the potential for rapid local ozone formation exists in chongqing. During ozone pollution episodes, the ozone production rates were found to be high at the upwind station Nan Quan, the urban station Chao Zhan, and the downwind station Jin-Yun Shan. The average local ozone production rate was 30×10^(-9) V/V h^(-1) and the daily integration of the produced ozone was greater than 180×10^(-9) V/V. High ozone concentrations were associated with urban and downwind air masses. At most sites, the local ozone production was VOC-limited and the key species were aromatics and alkene, which originated mainly from vehicles and solvent usage. In addition, the air masses at the northwestern rural sites were NO_x-limited and the local ozone production rates were significantly higher during the pollution episodes due to the increased NOx concentrations. In summary, the ozone abatement strategies of chongqing should be focused on the mitigation of VOCs. Nevertheless, a reduction in NO_x is also beneficial for reducing the regional ozone peak values in chongqing and the surrounding areas.

关键词： Ozone chongqing Photochemistry NO_x VOCs Sensitivity analysis Relative incremental reactivity EKMA

Automatic mapping of gully from satellite images using asymmetric non-local LinkNet: A case study in Northeast China

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International Soil and Water Conservation Research 2024年第2期12卷 365-378页

作者： Panpan Zhu Hao Xu Ligang Zhou Peixin Yu Liqiang Zhang Suhong Liu College of Computer Sciences and Technology Chongqing University of Posts and TelecommunicationsChongqing Engineering Research Center for Spatial Big Data Intelligent TechnologyChongqing400065China College of Environment and Ecology Chongqing UniversityChongqing400044China chongqing Municipal ecological and environmental monitoring center Chongqing401120China Beijing Key Laboratory of environmental Remote Sensing and Digital Cities Faculty of Geographical ScienceBeijing Normal UniversityBeijing100875China China National environmental monitoring Centre Beijing100012China

Gully erosion can lead to the destruction of farmland and the reduction in crop *** mapping from remote sensing images is critical for quickly obtaining the distribution of gullies at regional scales and arranging corresponding prevention and control *** narrow and irregular shapes and similar colors to the surrounding farmland make mapping erosion gullies in sloping farmland from remote sensing images *** implement gully erosion mapping,we developed a small training samples-oriented lightweight deep leaning model,called asymmetric non-local LinkNet(ASNL-LinkNet).The ASNL-LinkNet integrates global context information through an asymmetric non-local operation and conducts multilayer feature fusion to improve the robustness of the extracted *** results show that the proposed ASNL-LinkNet achieves the best performance when compared with other deep learning *** quantitative evaluation results in the three test areas show that the F1-score of erosion gully recognition varies from 0.62 to *** study provides theoretical reference and practical guidance for monitoring erosion gullies on slope farmland in the black soil region of Northeast China.

关键词： Gully erosion mapping High-resolution satellite images Deep learning Black soil

Probabilistic ecological risk assessment of cadmium in the Bohai Sea using native saltwater species

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Acta Oceanologica Sinica 2014年第12期33卷 212-221页

作者： MU Jingli WANG Juying WANG Ying CONG Yi ZHANG Zhifeng Key Laboratory for ecological Environment in Coastal Areas State Oceanic Administration National Marine environmental monitoring center

Predicted no-effect concentration （PNEC） is often used in ecological risk assessment to determine low-risk concentrations for chemicals. In the present study, the chronic data from native saltwater species were used to calculated PNEC values using four methods： log-normal distribution （ETX 2.0）, log-triangle distribution （US EPA＇s water quality criteria procedure）, burr III distribution （BurrliOZ） and traditional assessment fac-tor （AF）. The PNECs that were calculated using four methods ranged from 0.08 μg/L to 1.8 μg/L. Three of the SSD-derived PNECs range from 0.94 to 1.8 μg/L, about a factor of two apart. To demonstrate the use of SSD-based PNEC values and comprehensively estimate the regional ecological risk for cadmium in surface water of the Bohai Sea, in the Liaodong Bay, Bohai Bay, and Laizhou Bay, China, the dissolved cadmium con-centrations were measured and obtained 753 valid data covering 190 stations from July 2006 to November 2007. Based on three ecological risk assessment approaches, namely hazard quotient （HQ）, probabilistic risk quotient and joint probability curve （JPC）, the potential ecological risk of cadmium in surface water of the Liaodong Bay, Bohai Bay, and Laizahou Bay were estimated. Overall, the ecological risk of cadmium to aquatic ecosystem in the whole Bohai Sea was at acceptable ecological risk level, the order of ecological risk was Liaodong Bay〉Bohai Bay〉Laizhou Bay. However, more concerns should be paid to aquatic ecological risk in the Liaodong Bay which is the home of many steel, metallurgy and petrochemical industrial in China.

关键词： Bohai Sea cadmium PNEC SSD probabilistic ecological risk assessment

Effects of shellfish culture on the community and mortality of zooplankton in a subtropical Bay

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Journal of Oceanology and Limnology 2023年第2期41卷 458-468页

作者： Bijian PANG Hongjun LI Mingmin LI Xin LUO Ying CHEN Tianshen LI Wenlu LAN Beibu Gulf Marine ecological Environment Field Observation and Research Station of Guangxi Marine Environmental Monitoring Center of GuangxiBeihai 536000China National Marine environmental monitoring center Dalian 116023China

Spatial and temporal distribution of abundance,community structure and succession,and mortality of zooplankton were examined in a subtropical bay—the Qinzhou Bay,Guangxi,South China,to evaluate the impact of oyster culture on *** on zooplankton abundance,phytoplankton biomass,and environmental parameters were collected in 12 routine samplings at four sites in the Qinzhou Bay in *** show that the hydrological environment in the estuary affected the temporal variation of zooplankton of the Qinzhou ***,the oyster culture affected the spatial distributions of *** abundance of zooplankton outside the oyster farm was higher than that inside,whereas the mortality outside the oyster farm,on the contrary,was lower than that *** culture in the Qinzhou Bay had built a significant impact on the abundance and community composition of zooplankton,and the food shortage caused by the ingestion of oyster might exacerbate the mortality of zooplankton in the Qinzhou *** addition,the large-scale oyster culture increased the spatial heterogeneity of the community structure of zooplankton inside and outside the oyster *** of this study provide a reference for future policy-making in aquaculture management.

关键词： zooplankton community structure mortality oyster culture Qinzhou Bay

Terrestrial input and nutrient change reflected by sediment records of the Changjiang River Estuary in recent 80 years

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Acta Oceanologica Sinica 2015年第2期34卷 27-35页

作者： LI Junlong ZHENG Binghui HU Xupeng WANG Yiming DING Ye LIU Fang College of Water Sciences Beijing Normal University State Key Laboratory of environmental Criteria and Risk Assessment Chinese Research Academy of Environmental Sciences State environmental Protection Key Laboratory of Quality Control in environmental monitoring China National Environmental Monitoring Center Zhoushan Marine ecological environmental monitoring Station

A variety of environmental problems have been observed in the Changjiang River Estuary and adjacent coastal area, including eutrophication, harmful algal blooms（HABs）, and hypoxia in recent decades. Application of sedimentary biogenic element indicators on the study of paleoenvironment can reconstruct environmental evolution history of waters. Two 210Pb-dated cores were collected from the Changjiang River Estuary（S3） and adjacent coastal area（Z13）, and total organic carbon（TOC）, total nitrogen（TN）, biogenic silicon（BSi）, total phosphorus（TP） and phosphorus（P） species were analyzed. Three stages of environmental changes are deduced by the nutrient sedimentary records. First, nutrient concentration increased rapidly since the 1950 s, which attributed to agriculture development and overused chemical fertilizers. Second, nutrient concentration kept high and primary production began to promote during the 1960 s to 1980 s, while diatom abundance and proportion began to decline since the 1970 s, accompanied by reduced 23 Si O- concentration and flux from the river. Third, due to several dams and bridges constructed, river runoff and coastal hydrodynamic conditions reduced to a certain extent since the 1990 s, which aggravated the unbalance in nutrient structure. Multi-nutrient proxies in sediment can reflect the natural environm-ental changes as well as influence of human activities.

关键词： biogenic elements phosphorus species sediment cores Changjiang River Estuary

Periodically hydrologic alterations decouple the relationships between physicochemical variables and chlorophyll-a in a dam-induced urban lake

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Journal of environmental Sciences 2021年第1期33卷 187-195页

作者： Tianyang Li Yuqi Zhang Binghui He Bing Yang Qi Huang College of Resources and Enuironment Southwest UniversityChongqing 400715China chongqing Eco-environmental monitoring center Chongqing 401147China Guiyang Engineering Corporation Limited Power ChinaGuiyang 550081China

Periodically hydrologic alterations driven by seasonal change and water storage capacity management strongly modify physicochemical properties and chlorophyll-a(Chl-a)and their interactions in dam-induced ***,the extent and magnitude of these changes still remain *** study aimed to determine the effects of periodically hydrologic alterations on physicochemical variables and Chl-a in the dam-induced urban Hanfeng Lake,upstream of Three Gorges *** in Chl-a and 13 physicochemical variables were recorded monthly in the lake from January 2013 to December ***-a was neither seasonal nor inter-annual differences while a few physical variables such as flow velocity(V)exhibited significantly seasonal variabilities,and chemical variables like total nitrogen(TN),nitrate-nitrogen(NO3-N),total phosphorus(TP),dissolved silica(DSi)were markedly inter-annual *** TN:TP(40:1)and lower NO3-N:DSi(0.8:1)relative to balanced stoichiometric ratios suggested changes in composition of phytoplankton communities and potentially increased proportion of diatom in Hanfeng ***-a was predicable by combination of dissolved oxygen(DO),TN and DSi in dry season,and by V alone in wet *** the whole study period,Chl-a was solely negatively correlated with TN:TP,indicating decline in N concentration and increase in P could therefore increase *** results highlight pronounced decoupling of linkages between Chl-a and physicochemical variables affected by periodically hydrologic alterations in dam-induced aquatic systems.

关键词： Chlorophyll-a Nutrients Dissolved silica Dam Hydrologic alterations

Web-system for processing and visualization of meteorological data for Siberian environment research

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International Journal of Digital Earth 2009年第S1期2卷 105-119页

作者： A.Titov E.Gordov I.Okladnikov T.Shulgina Institute of monitoring of Climatic and ecological Systems SB RAS TomskRussia Siberian center for environmental Research and Training TomskRussia

At present,mainly GIS software is used for exploration and visualization of spatially distributed *** the same time an approach based on the combination of advanced web technologies along with the standard rules of information-computational system development is more suitable for performing tasks requiring more sophisticated data *** this report,functional capabilities of the information-computational system created for meteorological and climatic data processing and online visualization are *** system represents a dedicated web-interface,which allows performing of mathematical and statistical operations on the diverse observational and model data and to determine characteristics of global and regional climate *** such datasets as NCEP/NCAR Reanalysis,ECMWF ERA-40 Reanalysis,*** available for *** particular,the system allows calculating of temporal average and extremum values,time trends,*** arbitrary spatial and temporal ranges for different meteorological *** possibility of online intercomparison of meteorological characteristics calculated for different datasets is also realized in the *** final version of the system being developed is supposed to find application in meteorological and climatological investigations and should help researchers to save time during performing routine analytical tasks by simplifying handling of huge arrays of spatially distributed meteorological data.

关键词： climate change geoinformatics global environmental change visualization

A novel method through solid phase extraction combined with gradient elution for concentration and separation of 66(ultra)trace persistent toxic pollutants in Antarctic waters

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Chinese Chemical Letters 2016年第3期27卷 405-411页

作者： Li Zhang Guang-Shui Na Chun-Xiang He Rui-Jing Li Hui Gao Lin-Ke Ge Yan-Jie Wang Yao Yao School of Chemistry and Chemical Engineering Liaoning Normal University Key Laboratory for ecological Environment in Coastal Areas (SOA) National Marine Environmental Monitoring Center

This study developed a method to perform the simultaneous concentration and selective separation of 66 （ultra） trace persistent toxic substances in Antarctic waters. The substances included 30 polychlorinated biphenyls, 17 organochlorine pesticides, 16 polycyclic aromatic hydrocarbons, 3 hexabromocyclododecanes. Solid phase extraction was performed using a C18 membrane and silica gel column. Gradient elution was conducted using organic solvents with different polarities; as a result, the efficiency of the C18 film is improved and the interferences from impurities and target compounds are eliminated. Extracts were subsequently analyzed through gas chromatography or liquid and gas chromatography coupled to tandem mass spectrometry. Method validation yielded the following values： recoveries of all target analytes in the Antarctic water ranged from 87.3% to 117.6% and reproducibility as percent relative standard deviation was lower than 5%. Quantification limits ranged from 0.004 μg L^-1 to 0.030 μg L^-1. The established method improved the recoveries and reduced the limits of detection. Results indicated the method exhibited good performance in the simultaneous concentration and selective separation of 66 （ultra） trace organic pollutants; Therefore, the proposed sample pretreatment can potentially eliminate the effects of various classes of impurities to some extent.

关键词： Polychlorinated biphenyls(PCBs) Organochlorine pesticides(OCPs) Polycyclic aromatic hydrocarbons(PAHs) Hexabromocyclododecanes(HBCDs) Solid phase extraction(SPE) Gradient elution