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生物启发膜在水系镁离子电池阴极的界面工程

Science China Materials 2024年第8期67卷 2558-2566页

作者：洛古子呷苟倩志罗号燃陈昭宇邓江斌王凯鑫何玉婷李英芳王磊张奔郑玉杰李猛 National Innovation center for Industry-Education Integration of Energy Storage Technology Xuefeng Mountain Energy Equipment Safety National Observation and Research StationMOE Key Laboratory of Low-Grade Energy Utilization Technologies and SystemsCQU-NUS Renewable Energy Materials&Devices Joint LaboratoryCollege of Energy&Power EngineeringChongqing UniversityChongqing 400044China Chongqing Windmagics Weichu Energy Co. Ltd.Chongqing 401121China Southwest Technology and engineering Research Institute Chongqing 400039China

受到水合镁离子的高脱溶能垒和不良界面水分解行为的限制,水系镁离子电池通常受制于缓慢的离子传输动力学和严重的阴极溶解.为了克服这些障碍,受细胞膜两亲性结构的启发,我们成功构建了一种由疏水性聚(3,4-乙二氧基噻吩)(PEDOT)和亲水性... 详细信息

受到水合镁离子的高脱溶能垒和不良界面水分解行为的限制,水系镁离子电池通常受制于缓慢的离子传输动力学和严重的阴极溶解.为了克服这些障碍,受细胞膜两亲性结构的启发,我们成功构建了一种由疏水性聚(3,4-乙二氧基噻吩)(PEDOT)和亲水性α-MnO_(2)基底组成的MnO_(2)碳基阴极.结合实验和理论计算结果分析,PEDOT层可以有效提高整体电极的导电性,降低水合Mg^(2+)的脱溶能垒,并抑制阴极溶解,从而提高复合电极的性能.因此,本文所制备的复合电极表现出优越的速率性能(58.4mA hg^(-1),3Ag^(-1))和增强的长期循环稳定性(1000个循环后85.92mA hg^(-1),2Ag^(-1)),优于原始的α-MnO_(2)阴极.这项基于生物启发设计理念的工作将为水合镁离子电池的发展提供创新方向.

关键词：镁离子电池复合电极生物启发传输动力学循环稳定性界面工程脱溶能垒

Numerical simulations of faraday waves in cylindrical and hexagonal tanks based on MPS method

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Journal of Hydrodynamics 2023年第2期35卷 278-286页

作者： Cong-yi Huang Wei-wen Zhao De-cheng Wan computational Marine Hydrodynamics Lab(CMHL) School of Naval ArchitectureOcean and Civil EngineeringShanghai Jiao Tong UniversityShanghai200240China

When a partially loaded liquid container vibrates along the vertical direction,the liquid inside will oscillate regularly,which is called Faraday *** some cases,the wave form of the Faraday wave is stable and smooth,and sometimes there is violent wave breaking and liquid *** this paper,the Faraday waves inside the cylindrical tank and the hexagonal tanks are simulated by the in-house solver MLParticle-SJTU base on the moving particle semi-implicit(MPS)*** surface tension model is used to better model the free surfaces with large *** such as wave breaking and liquid splashing are well captured and *** results show that the waveforms are significantly different at different excitation *** the tank shape also has an obvious effect on the waveform.

关键词： Faraday wave moving particle semi-implicit(MPS)method wave breaking liquid splash surface tension

Research progress on the hydrodynamic performance of water-air-bubble mixed flows around a ship

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Journal of Hydrodynamics 2022年第2期34卷 171-188页

作者： Zheng Li Xiao-song Zhang De-cheng Wan computational Marine Hydrodynamics Lab(CMHL) School of Naval ArchitectureOcean and Civil EngineeringShanghai Jiao Tong UniversityShanghai 200240China

The interaction between ship and surrounding fluids generates the water-air-bubble mixed flow laden with numerous droplets and *** water-air-bubble mixed flow is a complex multi-phase flow phenomenon,which involves intense air-water mixture,complex evolution of interface shape,interactions between multi-scale flow structures and strong turbulent *** on the field observations at sea,a large range of white water-air-bubble flow exists widely around a large-scale sailing ship,and directly affects the hydrodynamic performance of ship from various *** paper reviews the research progress of water-air-bubble mixed flow around a *** knowledge about the formation and evolution mechanism are introduced ***,the effects of the water-air-bubble mixed flow on ship performance are further reviewed,the main concerns are ship resistance,propulsion performance,slamming and ***,the future research prospects are summarized.

关键词： Water-air-bubble mixed flow ship resistance propulsion performance ship slamming characteristics maneuverability

Numerical simulations of sloshing waves in vertically excited square tank by improved MPS method

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Journal of Hydrodynamics 2022年第1期34卷 76-84页

作者： Guan-yu Zhang Wei-wen Zhao De-cheng Wan computational Marine Hydrodynamics Lab(CMHL) School of Naval ArchitectureOcean and Civil EngineeringShanghai Jiao Tong UniversityShanghai200240China

Faraday wave is a phenomenon of sloshing due to a heave motion of a partially filled tank,which is also called parametric instability or parametric *** the present paper,the phenomenon of faraday wave in a pure heave excited square tank is numerically simulated through the moving particle semi-implicit(MPS)*** surface tension effect and a new Dirichlet boundary condition for the pressure Poisson equation are considered to avert unphysical fragmentation and clustering of particles in splash *** the numerical simulation,the evolution of wave motion,and the non-linearity together with breaking phenomenon of faraday wave can be *** agreement is good in general,both amplitude and ***,the parameter studies including the excitation frequency and the forcing amplitude are carried out to analyses the mechanism of resonances response.

关键词： Liquid sloshing faraday wave moving particle semi-implicit(MPS)method surface tension MLParticle-SJTU solver

High-precision parallel computing model of solute transport based on GPU acceleration

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Journal of Hydrodynamics 2024年第1期36卷 202-212页

作者： Shang-hong Zhang Rong-qi Zhang Wen-da Li Xi-yan Yang Yang Zhou School of Water Resources and Hydropower engineering North China Electric Power UniversityBeijing102206China Hubei Key Laboratory of Intelligent Yangtze and Hydroelectric Science China Yangtze Power Co.Ltd.Yichang443133China

The scenario simulation analysis of water environmental emergencies is very important for risk prevention and control,and emergency *** quickly and accurately simulate the transport and diffusion process of high-intensity pollutants during sudden environmental water pollution events,in this study,a high-precision pollution transport and diffusion model for unstructured grids based on Compute Unified Device Architecture(CUDA)is *** finite volume method of a total variation diminishing limiter with the Kong proposed r-factor is used to reduce numerical diffusion and oscillation errors in the simulation of pollutants under sharp concentration conditions,and graphics processing unit acceleration technology is used to improve computational *** advection diffusion process of the model is verified numerically using two benchmark cases,and the efficiency of the model is evaluated using an engineering *** results demonstrate that the model perform well in the simulation of material transport in the presence of sharp ***,it has high computational *** acceleration ratio is 46 times the single-thread acceleration effect of the original *** efficiency of the accelerated model meet the requirements of an engineering application,and the rapid early warning and assessment of water pollution accidents is achieved.

关键词： Pollution transport and diffusion model parallel computing Compute Unified Device Architecture(CUDA) pollution event

A metal-free coordination–insertion ring-opening polymerization of tetrahydrofuran by the central metalloid bis(pentafluorophenyl)(phenoxy)borane

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Chinese Chemical Letters 2024年第3期35卷 419-422页

作者： Cheng Wu Yixuan Liu Chunsheng Xiao Chenyang Hu Xuan Pang Xuesi Chen Key Laboratory of Polymer Ecomaterials Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China School of Applied Chemistry and engineering University of Science and Technology of ChinaHefei 230026China

A new strategy for the metal-free coordination–insertion ring-opening polymerization of tetrahydrofuran by the central metalloid Boron has been first ***(pentafluorophenyl)(phenoxy)borane was used as a catalyst for the polymerization reaction *** polytetrahydrofuran with high molecular weight and narrow molecular weight distribution could be *** proposed mechanism was studied by MALDI-TOF,ESI-MS and O-18 isotope labeling analyses as a metal-free coordination insertion mechanism.

关键词： Metal-free catalyst Bis(pentafluorophenyl)(phenoxy)borane Coordination–insertion mechanism Ring-opening polymerization Polytetrahydrofuran

Benchmarking visual SLAM methods in mirror environments

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computational Visual Media 2024年第2期10卷 215-241页

作者： Peter Herbert Jing Wu Ze Ji Yu-Kun Lai School of Computer Science and Informatics Cardiff UniversityAbacws BuildingSenghennydd RdCardiff CF244AGUK School of engineering Cardiff UniversityQueen’s BuildingsThe ParadeCardiff CF243AAUK

Visual simultaneous localisation and mapping(vSLAM)finds applications for indoor and outdoor navigation that routinely subjects it to visual complexities,particularly mirror *** effect of mirror presence(time visible and its average size in the frame)was hypothesised to impact localisation and mapping performance,with systems using direct techniques expected to perform ***,a dataset,MirrEnv,of image sequences recorded in mirror environments,was collected,and used to evaluate the performance of existing representative *** ORB-SLAM3 and BundleFusion appear to show moderate degradation of absolute trajectory error with increasing mirror duration,whilst the remaining results did not show significantly degraded localisation *** mesh maps generated proved to be very inaccurate,with real and virtual reflections colliding in the reconstructions.A discussion is given of the likely sources of error and robustness in mirror environments,outlining future directions for validating and improving vSLAM performance in the presence of planar *** MirrEnv dataset is available at https://***/10.17035/d.2023.0292477898.

关键词： visual simultaneous localisation and mapping(vSLAM) mirror localisation mapping reflection datase

A call for enhanced data-driven insights into wind energy flow physics

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Theoretical & Applied Mechanics Letters 2024年第1期14卷 6-10页

作者： Coleman Moss Romit Maulik Giacomo Valerio Iungo Wind Fluids and Experiments(WindFluX)Laboratory Mechanical Engineering DepartmentThe University of Texas at DallasRichardson 75080USA College of Information Sciences and Technology The Pennsylvania State UniversityState College 16801USA

With the increased availability of experimental measurements aiming at probing wind resources and wind turbine operations,machine learning(ML)models are poised to advance our understanding of the physics underpinning the interaction between the atmospheric boundary layer and wind turbine arrays,the generated wakes and their interactions,and wind energy ***,the majority of the existing ML models for predicting wind turbine wakes merely recreate computational fluid dynamics(CFD)simulated data with analogous accuracy but reduced computational costs,thus providing surrogate models rather than enhanced data-enabled physics *** ML-based surrogate models are useful to overcome current limitations associated with the high computational costs of CFD models,using ML to unveil processes from experimental data or enhance modeling capabilities is deemed a potential research direction to *** this letter,we discuss recent achievements in the realm of ML modeling of wind turbine wakes and operations,along with new promising research strategies.

关键词： Machine learning Wake Wind turbine Wind farm Supervisory control and data acquisition

White light emission in 0D halide perovskite[(CH_(3))_(3)S]_(2)SnCl_(6)·H_(2)O crystals through variation of doping ns^(2) ions

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Frontiers of Optoelectronics 2024年第1期17卷 57-66页

作者： Yitong Lin Yu Zhong Yangpeng Lin Jiawei Lin Lei Pang Zhilong Zhang Yi Zhao Xiao‑Ying Huang Ke‑Zhao Du Fujian Provincial Key Laboratory of Advanced Materials Oriented Chemical engineering Collage of Chemistry and Material ScienceFujian Normal UniversityFuzhou 350007China State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China Qinghai Environmental Monitoring center Xining 810000China Strait Institute of Flexible Electronics(SIFE Future Technologies)Fujian Normal University and Strait Laboratory of Flexible Electronics(SLoFE)Fuzhou 350007China Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China

With the rapid development of white LEDs,the research of new and efficient white light emitting materials has attracted increasing *** dimensional(0D)organic–inorganic hybrid metal halide perovskites with superior luminescent property are promising candidates for LED application,due to their abundant and tailorable ***,[(CH_(3))_(3)S]_(2)SnCl_(6)・H_(2)O is synthesized as a host for dopant ions Bi^(3+)and Sb^(3+).The Sb^(3+)doped,or Bi^(3+)/Sb^(3+)co-doped,[(CH_(3))3S]_(2)SnCl_(6)・H_(2)O has a tunable optical emission spectrum by means of varying dopant ratio and excitation *** a result,we can achieve single-phase materials suitable for emission ranging from cold white light to warm white *** intrinsic mechanism is examined in this work,to clarify the dopant effect on the optical *** high stability of title crystalline material,against water,oxygen and heat,makes it promising for further application.

关键词： 0D Metal halide White light Perovskite Ions doping Excitation dependent