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A flexible,thin-film microchannel electrode array device for selective subdiaphragmatic vagus nerve recording

Microsystems & Nanoengineering 2024年第1期10卷 115-128页

作者： Jongcheon Lim Peter A.Zoss Terry L.Powley Hyowon Lee Matthew P.Ward Weldon School of Biomedical Engineering Purdue UniversityWest LafayetteINUSA birck Nanotechnology center Purdue UniversityWest LafayetteINUSA center for Implantable Devices Purdue UniversityWest LafayetteINUSA Department of Psychological Sciences Purdue UniversityWest LafayetteINUSA Purdue Institute of Integrative Neuroscience Purdue UniversityWest LafayetteINUSA Indiana University School of Medicine IndianapolisINUSA

The vagus nerve(VN)plays an important role in regulating physiological conditions in the gastrointestinal(GI)tract by communicating via the parasympathetic pathway to the enteric nervous system(ENS).However,the lack of knowledge in the neurophysiology of the VN and GI tract limits the development of advanced treatments for autonomic dysfunctions related to the *** better understand the complicated underlying mechanisms of the VN-GI tract neurophysiology,it is necessary to use an advanced device enabled by microfabrication *** several candidates including intraneural probe array and extraneural cuff electrodes,microchannel electrode array devices can be used to interface with smaller numbers of nerve fibers by securing them in the separate channel *** microchannel electrode array devices to interface teased nerve structures are relatively bulky with thickness around 200µ*** thick design can potentially harm the delicate tissue structures,including the nerve *** this paper,we present a flexible thin film based microchannel electrode array device(thickness:11.5µm)that can interface with one of the subdiaphragmatic nerve branches of the VN in a *** demonstrated recording evoked compound action potentials(ECAP)from a transected nerve ending that has multiple nerve ***,our analysis confirmed that the signals are from C-fibers that are critical in regulating autonomic neurophysiology in the GI tract.

关键词： electrode recording film

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Organic semiconductor-incorporated two-dimensional halide perovskites

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National Science Review 2022年第5期9卷 17-19页

作者： Yao Gao Letian Dou Davidson School of Chemical Engineering Purdue University birck Nanotechnology center Purdue University

Recently,the search for novel two-dimensional (2D) organic-inorganic halide perovskite materials has come to a *** is significant interest not only in terms of their intriguing optoelectronic properties,but also their structural diversity and improved *** 2D perovskite structure can be visualized as atomically thin slabs cut from 3D parent structures along different crystal directions that are sandwiched between two layers of large organic *** bulky organic cations/ligands play a governing role in2D structure formation via suppression of the out-of-plane growth and promotion of in-plane ***,

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Unexpected thermal conductivity enhancement in aperiodic superlattices discovered using active machine learning

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npj Computational Materials 2022年第1期8卷 99-105页

作者： Prabudhya Roy Chowdhury Xiulin Ruan School of Mechanical Engineering and the birck Nanotechnology center Purdue UniversityWest LafayetteIN47907-2088USA

While machine learning(ML)has shown increasing effectiveness in optimizing materials properties under known physics,its application in discovering new physics remains challenging due to its interpolative *** this work,we demonstrate a general-purpose adaptive ML-accelerated search process that can discover unexpected lattice thermal conductivity(κ_(l))enhancement in aperiodic superlattices(SLs)as compared to periodic superlattices,with implications for thermal management of multilayer-based electronic *** use molecular dynamics simulations for high-fidelity calculations ofκ_(l),along with a convolutional neural network(CNN)which can rapidly predictκ_(l)for a large number of *** ensure accurate prediction for the target unknown SLs,we iteratively identify aperiodic SLs with structural features leading to locally enhanced thermal transport and include them as additional training data for the *** identified structures exhibit increased coherent phonon transport owing to the presence of closely spaced interfaces.

关键词： thermal conductivity transport

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Electronic properties of 2D materials and their junctions

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Nano Materials Science 2024年第1期6卷 1-23页

作者： Taposhree Dutta Neha Yadav Yongling Wu Gary J.Cheng Xiu Liang Seeram Ramakrishna Aoussaj Sbai Rajeev Gupta Aniruddha Mondal Zheng Hongyu Ashish Yadav Department of Chemistry Indian Institute of Engineering Science and TechnologyShibpurWest Bengal711103India center for Advanced Laser Manufacturing(CALM) Shandong University of TechnologyZibo255000PR China School of Industrial Engineering Purdue University315 N.Grant St.West LafayetteIN47907United States birck Nanotechnology center Purdue University1205 W State St.West LafayetteIN47907United States Advanced Materials Institute Qilu University of TechnologyShandong Academy of SciencesJinan250014PR China Nanoscience and Nanotechnology Initiative National University of Singapore10 Kent Ridge Crescent119260Singapore Faculty of Applied Phsyics and Mathematics Gdansk University of Technology Narutowicza 11/1280233GdanskPoland Department of Physics School of EngineeringUniversity of Petroleum&Energy StudiesDehradun248007UttarakhandIndia Department of Physics National Institute of Technology DurgapurDurgapur713209West BengalIndia

With an extensive range of distinctive features at nano meter-scale thicknesses,two-dimensional(2D)materials drawn the attention of the scientific *** tremendous advancements in exploratory research on 2D materials,knowledge of 2D electrical transport and carrier dynamics still in its ***,here we highlighted the electrical characteristics of 2D materials with electronic band structure,electronic transport,dielectric constant,carriers *** atomic thinness of 2D materials makes substantially scaled field-effect transistors(FETs)with reduced short-channel effects conceivable,even though strong carrier mobility required for high performance,low-voltage device *** also discussed here about factors affecting 2D materials which easily enhanced the activity of those materials for various ***,Those 2D materials used in state-of-the-art electrical and optoelectronic devices because of the extensive nature of their electronic band structure.2D materials offer unprecedented freedom for the design of novel p-n junction device topologies in contrast to conventional bulk *** also,describe the numerous 2D p-n junctions,such as homo junction and hetero junction including mixed dimensional ***,we talked about the problems and potential for the future.

关键词： 2D materials Electrical properties p-n junctions Mixed hereto junctions Homo junctions Electrical transport

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Modeling the gene delivery process of the needle array-based tissue nanotransfection

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Nano Research 2022年第4期15卷 3409-3421页

作者： Zhigang Li Yi Xuan Subhadip Ghatak Poornachander RGuda Sashwati Roy Chandan K.Sen Indiana center for Regenerative Medicine and Engineering Indiana University Health Comprehensive Wound CenterDepartment of SurgeryIndiana University School of MedicineIndianapolisIN 46202USA birck Nanotechnology center and Weldon School of Biomedical Engineering Purdue UniversityWest LafayetteIN 47907USA

Hollow needle array-based tissue nanotransfection(TNT)presents an in vivo transfection approach that directly translocate exogeneous genes to target tissues by using electric *** this work,the gene delivery process of TNT was simulated and experimentally *** adopted the asymptotic method and cell-array-based model to investigate the electroporation behaviors of cells within the skin *** distribution of nonuniform electric field across the skin results in various electroporation behavior for each *** underneath the hollow microchannels of the needle exhibited the highest total pore numbers compared to others due to the stronger localized electric *** percentage of electroporated cells within the skin structure,with pore radius over 10 nm,increases from 25%to 82%as the applied voltage increases from 100 to 150 V/***,the gene delivery behavior across the skin tissue was investigated through the multilayer-stack-based *** delivery distance increased nonlinearly as the applied voltage and pulse number increased,which mainly depends on the diffusion characteristics and electric conductivity of each *** was also found that the skin is required to be exfoliated prior to the TNT procedure to enhance the delivery *** work provides the foundation for transition from the study of murine skin to translation use in large animals and human settings.

关键词： tissue nanotransfection silicon needle array hollow needle array electroporation electrophoresis gene delivery

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Fast and accurate machine learning prediction of phonon scattering rates and lattice thermal conductivity

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npj Computational Materials 2023年第1期9卷 1367-1376页

作者： Ziqi Guo Prabudhya Roy Chowdhury Zherui Han Yixuan Sun Dudong Feng Guang Lin Xiulin Ruan Department of Mechanical Engineering Purdue UniversityWest Lafayette 47907-2088 INUSA The birck Nanotechnology center Purdue UniversityWest Lafayette 47907-2088 INUSA Department of Mathematics Purdue UniversityWest Lafayette 47907-2088 INUSA

Lattice thermal conductivity is important for many applications,but experimental measurements or first principles calculations including three-phonon and four-phonon scattering are expensive or even *** learning approaches that can achieve similar accuracy have been a long-standing open *** recent progress,machine learning models using structural information as descriptors fall short of experimental or first principles *** study presents a machine learning approach that predicts phonon scattering rates and thermal conductivity with experimental and first principles *** success of our approach is enabled by mitigating computational challenges associated with the high skewness of phonon scattering rates and their complex contributions to the total thermal *** learning between different orders of phonon scattering can further improve the model *** surrogates offer up to two orders of magnitude acceleration compared to first principles calculations and would enable large-scale thermal transport informatics.

关键词： spite learning principles

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A generalized synthesis method for freestanding multiferroic twodimensional layered supercell oxide films via a sacrificial buffer layer

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Nano Research 2023年第7期16卷 10559-10566页

作者： Jianan Shen Benson Kunhung Tsai Ke Xu Anyu Shang James PBarnard Yizhi Zhang Rahul Tripathi Zhihong Chen Xinghang Zhang Haiyan Wang School of Materials Engineering Purdue UniversityWest LafayetteIndiana 47907USA Elmore Family School of Electrical and Computer Engineering Purdue UniversityWest LafayetteIndiana 47907USA birck Nanotechnology center Purdue UniversityWest LafayetteIndiana 47907USA

Multiferroics are an intriguing family of materials due to the simultaneous presence of two ferroic orderings,namely,ferroelectricity and *** are scientifically and technologically important and have numerous potential applications,such as four-state logic memories and multiferroic tunneling ***,the growth of epitaxial singlephase multiferroic thin films typically requires single crystalline oxide substrates,which hinders their future integration with Sibased *** this study,we report a generalized synthesis method that uses the polydimethylsiloxane(PDMS)-assisted wetetching method with an Sr_(3)Al_(2)O_(6)(SAO)sacrificial layer to transfer freestanding single-phase multiferroic Bi_(2)NiMnO_(6)(BNMO)films from conventional SrTiO_(3)(STO)substrates onto a Si *** structures and properties of the films have been characterized before and after the *** transferred films possess good multiferroic properties on Si wafers,indicating full compatibility with modern Si *** method can be generally applicable to other Bi-based multiferroic materials as ***,the original STO substrates after the transfer process have been recycled for preparing new batches of freestanding BNMO films,indicating a low-cost and sustainable method for manufacturing large-volume freestanding complex oxide thin films.

关键词： multiferroics freestanding films wet-transfer SAO sacrificial layer recyclable substrates sustainable

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Biopolymers-based skin-interfaced triboelectric sensors

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Nano Research 2023年第9期16卷 11753-11782页

作者： Shujia Xu Pedro Henrique de Souza Barbosa Wenzhuo Wu School of Industrial Engineering Purdue UniversityWest LafayetteIN 47907USA Flex Laboratory Purdue UniversityWest LafayetteIN 47907USA Regenstrief center for Healthcare Engineering Purdue UniversityWest LafayetteIN 47907USA birck Nanotechnology center Purdue UniversityWest LafayetteIN 47907USA The center for Education and Research in Information Assurance and Security(CERIAS) Purdue UniversityWest LafayetteIN 47907USA

Rapid advances in artificial intelligence,robotics,and remote healthcare have increased the demand for sustainable and highperformance wearable *** devices are gaining traction due to their self-powered operation capability and potential as wearable energy ***-interfaced triboelectric sensors(SITSs)can detect various mechanical signals and monitor physiological signals in ***-based SITSs are ideal for skin-interfaced applications since they are biocompatible and *** review focuses on the recent advancements of SITS made from biocompatible polymer materials,such as plant-based,animal-based,and synthetic polymers,and highlights their potential for various applications,including human–machine interface(HMI)and physiological *** addition,the fundamentals,challenges,and prospects of SITS based on biocompatible polymers are discussed.

关键词： skin interfaced triboelectric sensors wearable devices biopolymers

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Perspective: Predicting and optimizing thermal transport properties with machine learning methods

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能源与人工智能(英文) 2022年第2期8卷 148-161页

作者： Han Wei Hua Bao Xiulin Ruan University of Michigan-Shanghai Jiao Tong University Joint Institute Shanghai Jiao Tong UniversityShanghai 200240China School of Mechanical Engineering and birck Nanotechnology center Purdue UniversityWest LafayetteIN 47907United States

In recent years, (big) data science has emerged as the “fourth paradigm” in physical science research. Data-driven techniques, e.g. machine learning, are advantageous in dealing with problems of high-dimensional features and complex mappings between quantities, which are otherwise of great difficulty or huge cost with other scientific paradigms. In the past five years or so, there has been a rapid growth of machine learning-assisted research on thermal transport. In this perspective, we review the recent progress in the intersection between machine learning and thermal transport, where machine learning methods generally serve as surrogate models for predicting the thermal transport properties, or as tools for designing structures for the desired thermal properties and exploring thermal transport mechanisms. We provide perspectives about the advantages of machine learning methods in comparison to the physics-based methods for studying thermal transport properties. We also discuss how to improve the accuracy of predictive analytics and efficiency of structural optimization, to provide guidance for better utilizing machine learning-based methods to advance thermal transport research. Finally, we identify several outstanding challenges in this active area as well as opportunities for future developments,including developing machine learning methods suitable for small datasets, discovering effective physics-based descriptors, generating dataset from experiments and validating machine learning results with experiments, and making breakthroughs via discovering new physics.

关键词： Thermal transport properties Machine learning Prediction Optimization

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Symmetry breaking in thermal photonics

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Light(Science & Applications) 2022年第12期11卷 2835-2836页

作者： Xueji Wang Zubin Jacob birck Nanotechnology center Elmore Family School of Electrical and Computer EngineeringPurdue UniversityWest LafayetteIN 47907USA

Engineering symmetries in nanostructures and metasurfaces provides a new paradigm to control incoherent heat radiation for applications in energy conversion,thermal sources,infrared imaging,and radiative cooling.

关键词： thermal breaking radiative

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