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Recent advances in core-shell organic framework-based photocatalysts for energy conversion and environmental remediation

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Journal of Energy Chemistry 2024年第8期95卷 168-199,I0004页

作者： Qibing Dong Ximing Li Yanyan Duan Qingyun Tian Xinxin Liang Yiyin Zhu Lin Tian Junjun Wang Atif Sial Yongqian Cui Ke Zhao Chuanyi Wang School of Environmental Science and Engineering Shaanxi University of Science and TechnologyXi’an 710021ShaanxiChina Guangdong Engineering Technology Research center for Environmental Purification and Functional Materials Guangzhou Institute of Industrial IntelligenceGuangzhou 511400GuangdongChina Jiangxi Key Lab of Flexible Electronics Flexible Electronics Innovation InstituteJiangxi Science and Technology Normal UniversityNanchang 330013JiangxiChina Helmholtz-Zentrum Berlin für Materialien und Energie Kekuléstraße 512489 BerlinGermany

Direct conversion of solar energy into chemical energy in an environmentally friendly manner is one of the most promising strategies to deal with the environmental pollution and energy *** a variety of materials developed as photocatalysts,the core-shell metal/covalent-organic framework(MOF or COF)photocatalysts have garnered significant attention due to their highly porous structure and the adjustability in both structure and *** existing reviews on core-shell organic framework photocatalytic materials have mainly focused on core-shell MOF ***,there is still a lack of indepth reviews specifically addressing the photocatalytic performance of core-shell COFs and MOFs@***,there is an urgent need for a comprehensive review encompassing these three types of core-shell *** on this,this review aims to provide a comprehensive understanding and useful guidelines for the exploration of suitable core-shell organic framework photocatalysts towards appropriate photocatalytic energy conversion and environmental ***,the classification,synthesis,formation mechanisms,and reasonable regulation of core-shell organic framework were ***,the photocatalytic applications of these three kinds of core-shell structures in different areas,such as H_(2)evolution,CO_(2)reduction,and pollutants degradation are ***,the main challenges and development prospects of core-shell organic framework photocatalysts were *** review aims to provide insights into the development of a novel generation of efficient and stable core-shell organic framework materials for energy conversion and environmental remediation.

关键词： Organic framework Core-shell structure Photocatalysis Energy conversion Environmental remediation

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Exploring reservoir computing:Implementation via double stochastic nanowire networks

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Chinese Physics B 2024年第3期33卷 572-582页

作者：唐健峰夏磊李广隶付军段书凯王丽丹 College of Artificial intelligence Southwest UniversityChongqing 400715China Brain-inspired Computing & Intelligent Control of Chongqing Key Laboratory Chongqing 400715China National & Local Joint Engineering Laboratory of Intelligent Transmission and Control Technology Chongqing 400715China Chongqing Brain Science Collaborative Innovation center Chongqing 400715China Key Laboratory of Luminescence Analysis and Molecular Sensing Ministry of EducationSouthwest UniversityChongqing 400715China State Key Laboratory of Intelligent Vehicle Safety Technology Chongqing 400715China

Neuromorphic computing,inspired by the human brain,uses memristor devices for complex *** studies show that self-organizing random nanowires can implement neuromorphic information processing,enabling data *** paper presents a model based on these nanowire networks,with an improved conductance variation *** suggest using these networks for temporal information processing via a reservoir computing scheme and propose an efficient data encoding method using voltage *** nanowire network layer generates dynamic behaviors for pulse voltages,allowing time series prediction *** experiment uses a double stochastic nanowire network architecture for processing multiple input signals,outperforming traditional reservoir computing in terms of fewer nodes,enriched dynamics and improved prediction *** results confirm the high accuracy of this architecture on multiple real-time series datasets,making neuromorphic nanowire networks promising for physical implementation of reservoir computing.

关键词： double-layer stochastic(DS)nanowire network architecture neuromorphic computation nanowire network reservoir computing time series prediction

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Portfolio optimization based on network centralities:Which centrality is better for asset selection during global crises?

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Journal of Management Science and Engineering 2024年第3期9卷 348-375页

作者： Gang-Jin Wang Huahui Huai You Zhu Chi Xie Gazi Salah Uddin Business School and center for Finance and Investment Management Hunan UniversityChangsha410082China Hunan Province Key Laboratory of Philosophy and Social Science of Industrial Digital intelligence Finance Changsha410082China Department of Management and Engineering Linköping University58183LinköpingSweden Cambridge Centre for Economic and Public Policy(CCEPP) University of CambridgeCambridgeUnited Kingdom

We construct correlation-based networks linking 86 assets(stock indices,bond indices,foreign exchange rates,commodity futures,and cryptocurrencies)and analyze the impact of asset selection on portfolio optimization using different centrality measures(including degree,eigenvector,eccentricity,betweenness,PageRank,and hybrid centralities).In times of a global crisis,peripheral assets located in cross-market networks are more suitable for *** comparing portfolio performance based on different centrality measures,we find that(i)hybrid,eigenvector,and PageRank centralities can best improve portfolio performance;(ii)degree centrality is suitable for larger portfolios;and(iii)eccentricity and betweenness centralities are unsuitable for network optimization *** response,we explain them based on the construction principle of centrality ***,our optimal portfolios suggest that investors pay more attention to the role of emerging countries,which are less exposed to external shocks and whose financial markets are more likely to remain stable.

关键词： Financial network Centrality measures Portfolio optimization Asset selection Global crisis

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Rationale and design of a randomised double-blind 2×2 factorial trial comparing the effect of a 3-month intensive statin and antiplatelet therapy for patients with acute mild ischaemic stroke or high-risk TIA with intracranial or extracranial atherosclerosis(INSPIRES)

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Stroke & Vascular Neurology 2023年第3期8卷 249-258,I0096-I0110页

作者： Ying Gao Yuesong Pan Shangrong Han Weiqi Chen Jing Jing Chunjuan Wang Yingying Yang Tingting Wang Xia Meng Xingquan Zhao Liping Liu Hao Li S Claiborne Johnston Pierre Amarenco Philip M Bath Yongjun Wang Yilong Wang Department of Neurology Beijing Tiantan HospitalCapital Medical UniversityBeijingChina China National Clinical Research center for Neurological Diseases Beijing Tiantan HospitalCapital Medical UniversityBeijingChina Dean's Office Dell Medical SchoolUniversity of Texas at AustinAustinTexasUSA Department of Neurology and Stroke center Assistance Publique-Hôpitaux de Paris(APHP)Bichat HospitalINSERM LVTS-U1148University of ParisParisFrance Population Health Research Institute McMaster UniversityHamiltonOntarioCanada Stroke Trials Unit Mental Health&Clinical NeuroscienceUniversity of NottinghamNottinghamUK Advanced Innovation center for Human Brain Protection Capital Medical UniversityBeijingChina National center for Neurological Diseases BeijingChina Research Unit of Artificial intelligence in Cerebrovascular Disease Chinese Academy of Medical SciencesBeijingChina Chinese Institute for Brain Research BeijingChina

Background It remains unclear if intensive antiplatelet and statin treatments begun within 24-72 hours of cerebral ischaemic events from intracranial or extracranial atherosclerosis is effective or *** The Intensive Statin and Antiplatelet Therapy for High-risk Intracranial or Extracranial Atherosclerosis(INSPIRES)trial is a randomised,double-blind,placebo-controlled,multicentre and 2×2 factorial trial.6100 individuals between the ages of 35 and 80 who have experienced a mild ischaemic stroke or high-risk transient ischaemic attack(TIA)within the previous 72 hours that is attributed to≥50%atherosclerotic stenosis of a major intracranial or extracranial artery or multiple infarctions of atherosclerotic origin will be enrolled in the *** subjects will be randomised 1:1:1:1 to one of four groups:(1)intensive antiplatelet therapy(combined clopidogrel and aspirin for days 1-21,then aspirin placebo and clopidogrel for days 22-90)plus immediate intensive statin therapy(atorvastatin at a dose of 80 mg daily for the first 21 days,then 40 mg daily for days 22-90);(2)intensive antiplatelet therapy plus delayed intensive statin therapy(atorvastatin placebo for days 1-3,followed by 40 mg per day of atorvastatin for days 4-90);(3)standard antiplatelet therapy(combination of clopidogrel placebo with aspirin for 90 days)plus immediate intensive statin therapy and(4)standard antiplatelet therapy plus delayed intensive statin *** primary efficacy endpoint is any new stroke(ischaemic or haemorrhagic)within 90 days after *** primary safety endpoint is moderate to severe bleeding at 90 *** The INSPIRES trial will assess the efficacy and safety of intensive antiplatelet therapy and immediate intensive statin therapy begun within 72 hours of onset in decreasing the recurrent stroke at 90 days in patients with acute mild ischaemic stroke or high-risk TIA of intracranial or extracranial atherosclerosis origin.

关键词： intracranial atherosclerosis random

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The standardized design and application guidelines: A primary-oriented artificial intelligence screening system of the lesion sign in the macular region based on fundus color photography

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Intelligent Medicine 2023年第3期3卷 213-227页

作者： Ocular Fundus Diseases Group of Chinese Ophthalmological Society Expert Group for Artificial intelligence Research,Development,and Application Xiaoxin Li Ming Zhang Yanwu Xu 不详 Fujian Provincial Key Laboratory of Ocular Surface and Corneal Diseases Eye Institute and Affiliated Xiamen Eye Center of Xiamen UniversitySchool of MedicineXiamen UniversityXiamenFujian 361001China Department of Ophthalmology West China HospitalSichuan UniversityChengduSichuan 610044China Beijing baidu Netcom Science Technology Co.Ltd.Beijing 100085 China

With the popularity and development of artificial intelligence(AI),disease screening systems based on AI algorithms are gradually emerging in the medical *** systems can be used for primary screening of diseases to relieve the pressure on primary health *** recent years,AI algorithms have demonstrated good performance in the analysis and identification of lesion signs in the macular region of fundus color photography,and a screening system for fundus lesion signs applicable to primary screening is bound to emerge in the ***,to standardize the design and clinical application of macular region lesion sign screening systems based on AI algorithms,the Ocular Fundus Diseases Group of Chinese Ophthalmological Society,in collaboration with relevant experts,developed this guideline after investigating issues,discussing production evidence,and holding guideline *** aimed to establish uniform standards for the definition of the macular region and lesion signs,AI adoption scenarios,algorithm model construction,dataset establishment and labeling,architecture and function design,and image data acquisition for the screening system to guide the implementation of the screening work.

关键词： Artificial intelligence Screening of the lesion sign in the macular region Primary screening Fundus color photography Lesion sign analysis

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Embracing the era of neuromorphic computing

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Journal of Semiconductors 2021年第1期42卷 5-7页

作者： Yanghao Wang Yuchao Yang Yue Hao Ru Huang Department of Micro/nanoelectronics Peking UniversityBeijing 100871China center for Brain Inspired Chips Institute for Artificial IntelligencePeking UniversityBeijing 100871China School of Microelectronics Xidian UniversityXi'an 710071China

In recent years,deep learning has made tremendous achievements in computer vision,natural language processing,man-machine games and so on,where artificial intelligence can reach or go beyond the level of human ***,behind so many glories,some serious challenges exist in the bottom hardware,hindering the further development of Artificial intelligence.

关键词： hardware hinder artificial

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Characterization of glutamatergic VTA neural population responses to aversive and rewarding conditioning in freely-moving mice

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Science Bulletin 2019年第16期64卷 1167-1178页

作者： Quentin Montardy Zheng Zhou Zhuogui Lei Xuemei Liu Pengyu Zeng Chen Chen Yuanming Liu Paula Sanz-Leon Kang Huang Liping Wang Shenzhen Key Lab of Neuropsychiatric Modulation and Collaborative Innovation center for Brain Science Guangdong Provincial Key Laboratory of Brain Connectome and BehaviorCAS Center for Excellence in Brain Science and Intelligence TechnologyThe Brain Cognition and Brain Disease Institute(BCBDI)Shenzhen Institutes of Advanced TechnologyChinese Academy of SciencesShenzhen-Hong Kong Institute of Brain Science-Shenzhen Fundamental Research InstitutionsShenzhen 518055China University of Chinese Academy of Sciences Beijing 100049China School of Physics the University of SydneySydney 2006Australia Centre for Integrative Brain Function the University of SydneySydney 2006Australia Department of Biomedical Sciences City University of Hong KongTat Chee AvenueKowloonHong KongSAR 999077China

The Ventral Tegmental Area(VTA) is a midbrain structure known to integrate aversive and rewarding stimuli, but little is known about the role of VTA glutamatergic(VGluT2) neurons in these *** activation of VGluT2 soma evokes rewarding behaviors, while activation of their downstream projections evokes aversive behaviors. To facilitate our understanding of these conflicting properties, we recorded calcium signals from VTAVGluT2+ neurons using fiber photometry in VGluT2-cre mice to investigate how this population was recruited by aversive and rewarding stimulation, both during unconditioned and conditioned protocols. Our results revealed that, as a population, VTAVGluT2+neurons responded similarly to unconditioned-aversive and unconditioned-rewarding stimulation. During aversive and rewarding conditioning, the CS-evoked responses gradually increased across trials whilst the US-evoked response remained stable. Retrieval 24 h after conditioning, during which mice received only CS presentation, resulted in VTAVGluT2+ neurons strongly responding to CS presentation and to the expected-US but only for aversive conditioning. To help understand these differences based on VTAVGluT2+ neuronal networks, the inputs and outputs of VTAVGluT2+ neurons were investigated using Cholera Toxin B(CTB) and rabies virus. Based on our results, we propose that the divergent VTAVGluT2+ neuronal responses to aversion and reward conditioning may be partly due to the existence of VTAVGluT2+ subpopulations that are characterized by their connectivity.

关键词： Ventral Tegmental Area Aversion Reward Conditioning Behavior

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X-MOL: large-scale pre-training for molecular understanding and diverse molecular analysis

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Science Bulletin 2022年第9期67卷 899-902,M0003页

作者： Dongyu Xue Han Zhang Xiaohan Chena Dongling Xiao Yu kang Gonga Guohui Chuai Yu Sun Hao Tian Hua Wu Yukun Li Qi Liu These authors contributed equally to this work.a Translational Medical center for Stem Cell Therapy and Institute for Regenerative Medicine Shanghai East HospitalBioinformatics DepartmentSchool of Life Sciences and TechnologyTongji UniversityShanghai 200092China Shanghai Research Institute for Intelligent Autonomous Systems Shanghai 201210China Department of Natural Language Processing Baidu Inc.Beijing 100085China

In silico modeling and analysis of small molecules substantially accelerates the process of drug development. Representing and understanding molecules is the fundamental step for various in silico molecular analysis t... 详细信息

关键词： accelerate analysis development

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Towards characterizing bug fixes through dependency-level changes in Apache Java open source projects

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Science China(Information Sciences) 2022年第7期65卷 102-120页

作者： Di CUI Lingling FAN Sen CHEN Yuanfang CAI Qinghua ZHENG Yang LIU Ting LIU School of Computer Science and Technology Xi'an Jiaotong University College of Cyber Science Nankai University College of intelligence and Computing Tianjin University Department of Computer Science Drexel University School of Computer Science and Engineering Nanyang Technological University School of Cyber Science and Engineering Xi'an Jiaotong University

The complexity and diversity of bug fixes require developers to understand bug fixes from multiple perspectives in addition to fine-grained code changes. The dependencies among files in a software system are an important dimension to inform software quality. Recent studies have revealed that most bug-prone files are always architecturally connected with dependencies, and as one of the best practices in the industry,changes in dependencies should be avoided or carefully made during bug fixing. Hence, in this paper, we take the first attempt to understand bug fixes from the dependencies perspective, which can complement existing code change perspectives. Based on this new perspective, we conducted a systematic and comprehensive study on bug fixes collected from 157 Apache open source projects, involving 140456 bug reports and182621 bug fixes in total. Our study results show that a relatively high proportion of bug fixes(30%) introduce dependency-level changes when fixing the corresponding 33% bugs. The bugs, whose fixes introduce dependency-level changes, have a strong correlation with high priority, large fixing churn, long fixing time,frequent bug reopening, and bug inducing. More importantly, patched files with dependency-level changes in their fixes, consume much more maintenance costs compared with those without these changes. We further summarized three representative patch patterns to explain the reasons for the increasing costs. Our study unveils useful findings based on qualitative and quantitative analysis and also provides new insights that might benefit existing bug prediction techniques. We release a large set of benchmarks and also implement a prototype tool to automatically detect dependency-level changes from bug fixes, which can warn developers and remind them to design a better fix.

关键词： empirical software engineering software maintenance software evolution software architecture software design

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Stay in touch with the endoplasmic reticulum

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Science China(Life Sciences) 2024年第2期67卷 230-257页

作者： Sha Sun Gan Zhao Mingkang Jia Qing Jiang Shulin Li Haibin Wang Wenjing Li Yunyun Wang Xin Bian Yan G.Zhao Xun Huang Ge Yang Huaqing Cai Jose C.Pastor-Pareja Liang Ge Chuanmao Zhang Junjie Hu National Laboratory of Biomacromolecules Institute of BiophysicsUniversity of Chinese Academy of SciencesChinese Academy of SciencesBeijing 100101China The Ministry of Education Key Laboratory of Cell Proliferation and Differentiation College of Life SciencesPeking UniversityBeijing 100871China State Key Laboratory of Membrane Biology Tsinghua-Peking Center for Life SciencesSchool of Life SciencesTsinghua UniversityBeijing 100084China Laboratory of Computational Biology&Machine intelligence School of Artificial IntelligenceUniversity of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of Medicinal Chemical Biology College of Life SciencesNankai UniversityTianjin 300071China Brain Research center Department of BiologySchool of Life SciencesSouthern University of Science and TechnologyShenzhen 518055China State Key Laboratory of Molecular Developmental Biology Institute of Genetics and Developmental BiologyInnovation Academy for Seed DesignChinese Academy of SciencesBeijing 100101China Institute of Neurosciences Consejo Superior de Investigaciones Científicas-Universidad Miguel HernándezSan Juan de Alicante 03550Spain

The endoplasmic reticulum(ER),which is composed of a continuous network of tubules and sheets,forms the most widely distributed membrane system in eukaryotic *** a result,it engages a variety of organelles by establishing membrane contact sites(MCSs).These contacts regulate organelle positioning and remodeling,including fusion and fission,facilitate precise lipid exchange,and couple vital signaling ***,we systematically review recent advances and converging themes on ER-involved organellar *** molecular basis,cellular influence,and potential physiological functions for ER/nuclear envelope contacts with mitochondria,Golgi,endosomes,lysosomes,lipid droplets,autophagosomes,and plasma membrane are summarized.

关键词： endoplasmic reticulum nuclear envelope mitochondria Golgi apparatus endosome lysosome lipid droplets autophagosome plasma membrane membrane contact site

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