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Controllable Exciton Diffusion Length and Ultrafast Charge Generation in Ternary Organic Solar Cells

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Chinese Journal of Chemistry 2024年第11期42卷 1275-1283页

作者： Sixuan Cheng Jiawei Qiao Peng Lu Wei Qin Xiaotao Hao School of Physics State Key Laboratory of Crystal MaterialsShandong UniversityJinanShandong250100 China School of Physics National Demonstration Center for Experimental Physics EducationShandong UniversityJinanShandong250100 China arc Centre of excellence in Exciton science School of ChemistryThe University of MelbourneParkvilleVictoria3010 Australia

Charge generation,a critical process in the operation of organic solar cell(OSC),requires thorough investigation in an ultrafast *** work demonstrates that the utilization of alloy model for the non-fullerene acceptor(NFA)component can regulate the crystallization properties of active layer films,which in turn affects exciton diffusion and hole transfer(HT),ultimately influencing the charge generation *** incorporating BTP-eC7 as a third component,without expanding absorption range or changing molecular energy levels but regulating the ultrafast exciton diffusion and HT processes,the power conversion efficiency(PCE)of the optimized PM6:BTP-eC9:BTP-eC7 based ternary OSC is improved from 17.30%to 17.83%,primarily due to the enhancement of short-circuit current density(JSC).Additionally,the introduction of BTP-eC7 also reduces the trap state density in the photoactive layer which helps to reduce the loss of *** study introduces a novel approach for employing ternary alloy models by incorporating dual acceptors with similar structures,and elucidates the underlying mechanism of charge generation and JSC in ternary OSCs.

关键词： Organic photovoltaics Ternary strategy Exciton diffusion Hole transfer Trap state Kinetics Alloys Photophysics

Photoionisation detection of a single Er3+ ion with sub-100-ns time resolution

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National science Review 2024年第4期11卷 38-45页

作者： Yangbo Zhang Wenda Fan Jiliang Yang Hao Guan Qi Zhang Xi Qin Changkui Duan Gabriele G.de Boo Brett C.Johnson Jeffrey C.Mc Callum Matthew J.Sellars Sven Rogge Chunming Yin Jiangfeng Du CAS Key Laboratory of Microscale Magnetic Resonance and School of Physical sciences University of Science and Technology of China CAS center for excellence in Quantum Information and Quantum Physics University of Science and Technology of China Hefei National Laboratory University of Science and Technology of China Centre of excellence for Quantum Computation and Communication Technology School of Physics University of New South Wales Centre of excellence for Quantum Computation and Communication Technology School of Engineering RMIT University Centre of excellence for Quantum Computation and Communication Technology School of Physics University of Melbourne Centre of excellence for Quantum Computation and Communication Technology Research School of Physics and Engineering Australian National University

Efficient detection of single optical centres in solids is essential for quantum information processing, sensing and single-photon generation *** this work,we use radio-frequency（RF） reflectometry to electrically detect the photoionisation induced by a single Er3+ion in *** high bandwidth and sensitivity of the RF reflectometry provide sub-100-ns time resolution for the photoionisation *** this technique,the optically excited state lifetime of a single Er3+ion in a Si nano-transistor is measured for the first time to be 0.49±0.04μ*** results demonstrate an efficient approach for detecting a charge state change induced by Er excitation and *** approach could be used for fast readout of other single optical centres in solids and is attractive for large-scale integrated optical quantum systems thanks to the multi-channel RF reflectometry demonstrated with frequency multiplexing techniques.

关键词： single optical centres erbium ions RF reflectometry photoionisation detection

Rapid and Sensitive Biosensing of Salmonella Using Mechanical Step Rotation and Gold@platinum Nanozymatic Amplification

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Journal of Analysis and Testing 2024年第3期8卷 262-269页

作者： Meixuan Li Lei Wang Ai Xu Ying Ding Fengzhen Yang Yanbin Li Jianhan Lin Key Laboratory of Agricultural Information Acquisition Technology Ministry of Agriculture and Rural AffairsChina Agricultural University center of excellence for Poultry science University of Arkansas

Inspired by ballpoint pen, an optical biosensor is developed for detection of Salmonellausing a mechanical step rotator with a dropper to greatly simplify operation, a high gradient magnetic field with immune magnetic nanobeads to specifically separate bacteria, and immune gold@platinum nanozymes with a smartphone to sensitively detect bacteria. First, the preloaded bacterial sample is drawn by the dropper to react with the immune magnetic nanobeads through repeated squeezing and releasing of the dropper, and the rotator is successively rotated and the dropper is repeatedly squeezed and released to achieve mixing of the bacteria, magnetic nanobeads and gold@platinum nanozymes, followed by magnetic separation to remove the background. Then, the conjugates are eff ectively washed with skim milk and ultrapure water, and the substrate are rapidly catalyzed into the product. Finally, the blue product is photographed and analyzed using a smartphone to obtain the Salmonella concentration. This biosensor could detect Salmonellaas low as 56 CFU/mL in～25 min.

关键词： gold@platinum nanozyme magnetic grid separation mechanical step rotator optical biosensor Salmonella detection

Alkali Metal Ion Substituted Carboxymethyl Cellulose as Anode Polymeric Binders for Rapidly Chargeable Lithium-Ion Batteries

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Energy & Environmental Materials 2024年第1期7卷 77-82页

作者： Seoungwoo Byun Zhu Liu Dong Ok Shin Kyuman Kim Jaecheol Choi Youngjoon Roh Dahee Jin Seungwon Jung Kyung-Geun Kim Young-Gi Lee Stefan Ringe Yong Min Lee Department of Energy science and Engineering Daegu Gyeongbuk Institute of Science and Technology(DGIST)Daegu 42988Korea ZJU-Hangzhou Global Scientific and Technological Innovation center Zhejiang UniversityHangzhou 311215China Intelligent Sensors Research Section Electronics and Telecommunications Research Institute(ETRI)Daejeon 34129Korea Department of Advanced Device Technology University of Science and Technology(UST)Daejeon 34113Korea Intelligent Polymer Research Institute and arc Centre of excellence for Electromaterials science University of WollongongWollongong NSW 2522Australia Department of Chemistry Korea UniversitySeoul 02841Korea Energy science and Engineering Research center Daegu Gyeongbuk Institute of Science and Technology(DGIST)Daegu 42988Korea

The increasing demand for short charging time on electric vehicles has motivated realization of fast chargeable lithium-ion batteries(LIBs).However,shortening the charging time of LIBs is limited by Li^(+)intercalation process consisting of liquid-phase diffusion,de-solvation,SEI crossing,and solid-phase ***,we propose a new strategy to accelerate the de-solvation step through a control of interaction between polymeric binder and solvent-Li^(+)*** this purpose,three alkali metal ions(Li^(+),Na^(+),and K^(+))substituted carboxymethyl cellulose(Li-,Na-,and K-CMC)are prepared to examine the effects of metal ions on their *** lowest activation energy of de-solvation and the highest chemical diffusion coefficient were observed for ***,Li-CMC cell with a capacity of 3 mAh cm^(-2)could be charged to>95%in 10 min,while a value above>85%was observed after 150 ***,the presented approach holds great promise for the realization of fast charging.

关键词： de-solvation digital twins fast charging graphite anodes polymeric binders

Enhanced adaptive nonlinear extended state observer for pure feedback systems with matched and mismatched disturbances

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Control Theory and Technology 2024年第2期22卷 254-268页

作者： Mahtab Delpasand Mohammad Farrokhi School of Electrical Engineering Iran University of Science and TechnologyTehran16846-13114Iran center of excellence for Modelling and Control of Complex Systems Iran University of Science and TechnologyTehran16846-13114Iran

In this paper, an enhanced adaptive nonlinear extended state observer (EANESO) for single-input single-output pure feedback systems in the presence of external time-varying disturbances is proposed. In this paper, a nonlinear system with matched and mismatched disturbances is considered. The conventional extended state observer (ESO) can only be applied to systems that are in the form of integral chains. Moreover, this method has limitations in the face of mismatched disturbances. In the presence of time-varying disturbances, the traditional ESOs cannot estimate the disturbances accurately. To overcome this limitation, an EANESO is proposed in this paper. The main idea is to design the nonlinear ESO (NESO) to estimate the states of the system and multiple disturbances simultaneously. The observer gains are considered time-varying and adjusted with adaptation laws to improve the estimation accuracy and overcome the peaking phenomenon. Next, the proposed controller is designed based on output feedback to eliminate the effects of multiple disturbances and stabilize the closed-loop system. Subsequently, the stability analysis of the closed-loop system and convergence of the observer error are discussed. Finally, the proposed method is applied to the inverted pendulum system. The simulated results show good performance of the proposed method as compared with a recently published scheme in the related literature.

关键词： Nonlinear extended state observer Enhanced adaptive extended state observer Adaptation law Multiple-channel disturbances Inverted pendulum system Time-varying gain

Correction of microwave pulse reflection by digital filters in superconducting quantum circuits

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Chinese Physics B 2024年第9期33卷 117-123页

作者： Liang-Liang Guo Peng Duan Lei Du Hai-Feng Zhang Hao-Ran Tao Yong Chen Xiao-Yan Yang Chi Zhang Zhi-Long Jia Wei-Cheng Kong Zhao-Yun Chen Guo-Ping Guo CAS Key Laboratory of Quantum Information University of Science and Technology of ChinaHefei 230026China CAS center for excellence and Synergetic Innovation center in Quantum Information and Quantum Physics University of Science and Technology of ChinaHefei 230026China Origin Quantum Computing Company Limited Hefei 230088China Institute of Artificial Intelligence Hefei Comprehensive National Science CenterHefei 230088China

Reducing the control error is vital for high-fidelity digital and analog quantum *** superconducting circuits,one disagreeable error arises from the reflection of microwave signals due to impedance mismatch in the control ***,we demonstrate a reflection cancelation method when considering that there are two reflection nodes on the control *** propose to generate the pre-distortion pulse by passing the envelopes of the microwave signal through digital filters,which enables real-time reflection correction when integrated into the field-programmable gate array(FPGA).We achieve a reduction of single-qubit gate infidelity from 0.67%to 0.11%after eliminating microwave ***-time correction of microwave reflection paves the way for precise control and manipulation of the qubit state and would ultimately enhance the performance of algorithms and simulations executed on quantum processors.

关键词： reflection cancelation digital filter single-qubit gate superconducting circuit

Field induced Chern insulating states in twisted monolayer–bilayer graphene

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Chinese Physics B 2024年第6期33卷 69-73页

作者：王政文韩英卓 Kenji Watanabe Takashi Taniguchi 姜宇航毛金海 School of Physical science and CAS center for excellence in Topological Quantum Computation University of Chinese Academy of SciencesBeijing 100049China College of Materials science and Optoelectronic Technology Center of Materials Science and Optoelectronics EngineeringUniversity of Chinese Academy of SciencesBeijing 100049China Advanced Materials Laboratory National Institute for Materials ScienceTsukuba 305-0044Japan

Unraveling the mechanism underlying topological phases, notably the Chern insulators(Ch Is) in strong correlated systems at the microscopy scale, has captivated significant research interest. Nonetheless, Ch Is harboring topological information have not always manifested themselves, owing to the constraints imposed by displacement fields in certain experimental configurations. In this study, we employ density-tuned scanning tunneling microscopy(DT-STM) to investigate the Ch Is in twisted monolayer–bilayer graphene(t MBG). At zero magnetic field, we observe correlated metallic *** under a magnetic field, a metal–insulator transition happens and an integer Ch I is formed emanating from the filling index s = 3 with a Chern number C = 1. Our results underscore the pivotal role of magnetic fields as a powerful probe for elucidating topological phases in twisted Van der Waals heterostructures.

关键词： Chern insulators strong correlation effects two-dimensional van der Waals heterostructure density-tuned scanning tunneling microscopy(DT-STM)

Context Processing in Contextual and Cued Fear Extinction

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Neuroscience Bulletin 2024年第6期40卷 835-839页

作者： Yimu Zhang Chun Xu Yu Gu State Key Laboratory of Medical Neurobiology and MOE Frontiers center for Brain science Institutes of Brain ScienceFudan UniversityShanghai200032China Institute of Neuroscience State Key Laboratory of NeuroscienceCenter for Excellence in Brain Science and Intelligence TechnologyChinese Academy of SciencesShanghai200031China

Anxiety disorders such as post-traumatic stress disorder(PTSD)are prevalent mental disorders that disturb millions *** disorders often manifest as excessive fear,anxiety,and distress,significantly impacting daily *** fear extinction paradigms in animals were established decades ago and have been widely used in research,providing a scientific basis for exposure therapies for anxiety disorders in humans.

关键词： distress disorders traumatic

Seasonal Characteristics of Forecasting Uncertainties in Surface PM_(2.5)Concentration Associated with Forecast Lead Time over the Beijing-Tianjin-Hebei Region

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Advances in Atmospheric sciences 2024年第5期41卷 801-816页

作者： Qiuyan DU Chun ZHAO Jiawang FENG Zining YANG Jiamin XU Jun GU Mingshuai ZHANG Mingyue XU Shengfu LIN Deep Space Exploration Laboratory/School of Earth and Space sciences University of Science and Technology of ChinaHefei 230026China CAS center for excellence in Comparative Planetology University of Science and Technology of ChinaHefei 230026China

Forecasting uncertainties among meteorological fields have long been recognized as the main limitation on the accuracy and predictability of air quality ***,the particular impact of meteorological forecasting uncertainties on air quality forecasts specific to different seasons is still not well *** this study,a series of forecasts with different forecast lead times for January,April,July,and October of 2018 are conducted over the Beijing-Tianjin-Hebei(BTH)region and the impacts of meteorological forecasting uncertainties on surface PM_(2.5)concentration forecasts with each lead time are *** increased lead time,the forecasted PM_(2.5)concentrations significantly change and demonstrate obvious seasonal *** general,the forecasting uncertainties in monthly mean surface PM_(2.5)concentrations in the BTH region due to lead time are the largest(80%)in spring,followed by autumn(~50%),summer(~40%),and winter(20%).In winter,the forecasting uncertainties in total surface PM_(2.5)mass due to lead time are mainly due to the uncertainties in PBL heights and hence the PBL mixing of anthropogenic primary *** spring,the forecasting uncertainties are mainly from the impacts of lead time on lower-tropospheric northwesterly winds,thereby further enhancing the condensation production of anthropogenic secondary particles by the long-range transport of natural *** summer,the forecasting uncertainties result mainly from the decrease in dry and wet deposition rates,which are associated with the reduction of near-surface wind speed and precipitation *** autumn,the forecasting uncertainties arise mainly from the change in the transport of remote natural dust and anthropogenic particles,which is associated with changes in the large-scale circulation.

关键词： PM_(2.5) forecasting uncertainties forecast lead time meteorological fields Beijing-Tianjin-Hebei region