检索结果-南通市图书馆

Sulfhydryl-functionalized COF-based electrolyte strengthens chemical affinity toward polysulfides in quasi-solid-state Li-S batteries

在线全文

学校读者我要写书评

暂无评论

Carbon Energy 2024年第9期6卷 221-234页

作者： Linnan Bi Jie Xiao Yaochen Song Tianrui Sun Mingkai Luo Yi Wang Peng Dong Yingjie Zhang Yao Yao Jiaxuan Liao Sizhe Wang Shulei Chou yangtze delta region {3.(Quzhou) University of Electronic Science and Technology of ChinaQuzhouChina National and Local Joint Engineering Research Center of Lithium-ion Batteries and Materials Preparation Technology Key Laboratory of Advanced Battery Materials of Yunnan ProvinceFaculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunmingChina institute for Carbon Neutralization College of Chemistry and Materials EngineeringWenzhou UniversityWenzhouChina School of Materials and Energy University of Electronic Science and Technology of ChinaChengduChina School of Materials Science and Engineering Shaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic MaterialsShaanxi University of Science&TechnologyXi'anChina

For lithium-sulfur batteries(Li-S batteries),a high-content electrolyte typically can exacerbate the shuttle effect,while a lean electrolyte may lead to decreased Li-ion conductivity and reduced catalytic conversion efficiency,so achieving an appropriate electrolyte-to-sulfur ratio(E/S ratio)is essential for improving the battery cycling efficiency.A quasi-solid electrolyte(COF-SH@PVDF-HFP)with strong adsorption and high catalytic conversion was constructed for in situ covalent organic framework(COF)growth on highly polarized polyvinylidene fluoride-hexafluoropropylene(PVDF-HFP)***-SH@PVDF-HFP enables efficient Li-ion conductivity with low-content liquid electrolyte and effectively suppresses the shuttle *** results based on in situ Fourier-transform infrared,in situ Raman,UV–Vis,X-ray photoelectron,and density functional theory calculations confirmed the high catalytic conversion of COF-SH layer containing sulfhydryl and imine groups for the lithium *** plating/stripping tests based on Li/COF-SH@PVDF-HFP/Li show excellent lithium compatibility(5 mAh cm^(-2) for 1400 h).The assembled Li-S battery exhibits excellent rate(2 C 688.7 mAh g^(-1))and cycle performance(at 2 C of 568.8 mAh g^(-1) with a capacity retention of 77.3.after 800 cycles).This is the first report to improve the cycling stability of quasi-solid-state Li-S batteries by reducing both the E/S ratio and the designing strategy of sulfhydryl-functionalized COF for quasi-solid *** process opens up the possibility of the high performance of solid-state Li-S batteries.

关键词： lithium-sulfur batteries low electrolyte-to-sulfur ratio polysulfide shuttle PVDF-HFP/COF

Liquid-like polymer lubricating surfaces:Mechanism and applications

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Nano Research 2024年第2期17卷 476-491页

作者： Dagui Wang Jinglong Yang Junchang Guo Zhijuan Duan Deihui Wang Fan Xia Fei Deng Xu Deng yangtze delta region {3.(Huzhou) University of Electronic Science and Technology of ChinaHuzhou 313001China institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of ChinaChengdu 610054China State Key Laboratory of Biogeology and Environmental Geology Engineering Research Center of Nano-Geomaterials of Ministry of EducationFaculty of Materials Science and ChemistryChina University of GeosciencesWuhan 430070China Department of Nephrology Sichuan Provincial People’s HospitalUniversity of Electronic Science and Technology of ChinaChengdu 610054China Department of Nephrology Sichuan Provincial People’s Hospital Jinniu HospitalChengdu Jinniu District People’s HospitalChengdu 610054China Shenzhen institute for Advanced Study University of Electronic Science and Technology of ChinaShenzhen 518110China

Liquid-like polymer lubricating surfaces(LPLSs)are solid substrates with highly flexible polymer chains grafted via covalent *** unique modification enables ultralow contact-angle hysteresis,repellency of various liquids and bulk ice,and *** distinctive wettability and universality of LPLSs have potential applications in liquid motion,biological detection,and environmental *** this review,we summarize the mechanisms,preparation,and applications of *** discuss the wettability and lubrication mechanisms of liquid droplets on *** then categorize LPLS fabrication into“grafted onto”and“grafted from”groups,depending on the type of *** highlight representative applications with recent developments in anti-complex liquid,anti-icing,anti-biological adhesions,biosensing,and photocatalytic ***,we discuss future challenges and outlooks for LPLSs.

关键词： liquid-like polymer surface lubricating wettability

Magnetoresistance hysteresis in the superconducting state of kagome CsV_(3.Sb_(5)

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chinese Physics B 2024年第10期33卷 30-34页

作者： Tian Le Jinjin Liu Zhiwei Wang Xiao Lin institute of Natural Sciences Westlake Institute for Advanced StudyHangzhou 310024China Key Laboratory for Quantum Materials of Zhejiang Province Department of PhysicsSchool of Science and Research Center for Industries of the FutureWestlake UniversityHangzhou 310030China Centre for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement(MOE)School of PhysicsBeijing Institute of TechnologyBeijing 100081China Beijing Key Laboratory of Nanophotonics and Ultrafine Optoelectronic Systems Beijing Institute of TechnologyBeijing 100081China Material Science Center Yangtze Delta Region Academy of Beijing Institute of TechnologyJiaxing 314011China

The hysteresis of magnetoresistance observed in superconductors is of great interest due to its potential connectionwith unconventional *** this study,we perform electrical transport measurements on kagome superconductorCsV_(3.Sb_(5)nanoflakes and uncover unusual hysteretic behavior of magnetoresistance in the superconducting *** hysteresis can be induced by applying either a large DC or AC current at temperatures(T)well below the superconductingtransition temperature(T_(c)).As T approaches T_(c),similar weak hysteresis is also detected by applying a *** scenarios are discussed,with particular focus on the effects of vortex pinning and the presence of timereversal-symmtery-breaking superconducting *** findings support the latter,hinting at chiral superconductivityin kagome superconductors.

关键词： hysteresis magnetoresistance kagome superconductor chiral superconductor

Anti-swarm UAV radar system based on detection data fusion

在线全文

学校读者我要写书评

暂无评论

Journal of Systems Engineering and Electronics 2024年第5期35卷 1167-1176页

作者： WANG Pengfei HU Jinfeng HU Wen WANG Weiguang DONG Hao School of Information and Communication Engineering University of Electronic Science and Technology of ChinaChengdu 611731China China Airborne Missile Academy Luoyang 471009China yangtze delta region {3.(Quzhou) University of Electronic Science and Technology of ChinaQuzhou 324003China College of Electronic and Information Engineering Nanjing University of Aeronautics and AstronauticsNanjing 211106China

There is a growing body of research on the swarm unmanned aerial vehicle(UAV)in recent years,which has the characteristics of small,low speed,and low height as radar *** confront the swarm UAV,the design of anti-UAV radar system based on multiple input multiple output(MIMO)is put forward,which can elevate the performance of resolution,angle accuracy,high data rate,and tracking flexibility for swarm UAV *** resolution and detection are the core problem in detecting the swarm *** distinct advantage of MIMO system in angular accuracy measurement is demonstrated by comparing MIMO radar with phased array *** MIMO radar has better performance in resolution,swarm UAV detection still has difficulty in target *** paper proposes a multi-mode data fusion algorithm based on deep neural networks to improve the detection ***,signal processing and data processing based on the detection fusion algorithm above are designed,forming a high resolution detection *** simulations are designed to illustrate the feasibility of the designed system and the proposed algorithm.

关键词： swarm radar high resolution deep neural network fusion algorithm

超薄锡掺杂氧化镓结合高k栅介质:硅基兼容的4英寸功率场效应晶体管阵列

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Science Bulletin 2024年第12期69卷 1848-1851页

作者：刘子淳李佳诚杨惠霞杨涵黄元张逸韵黎沛涛马远骁王业亮 School of Integrated Circuits and Electronics and yangtze delta region Academy Beijing Institute of TechnologyBeijing 100081China Department of Electrical and Electronic Engineering The University of Hong KongHong Kong 999077China R&D Center for Solid-state Lighting Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China

Gallium oxide(Ga_(2)O_(3.),a novel ultrawide-bandgap(UWBG)semiconductor,has attracted considerable attention owing to its large bandgap of up to 4.9 eV,a high breakdown electric field of 8 MV/cm,and a high Baliga's figure of merit exceeding 3.00[1,2].These remarkable properties strongly support its potential applications in power electronics,extreme environmentresistance devices,and solar-blind detectors[1–3..

关键词：功率场效应晶体管高k栅介质氧化镓

Physicochemical characterization of Dendrobium officinale polysaccharides and regulation of immunometabolic homeostasis in Sub-health mice based on the CD4-Th17/Treg immunity axis

在线全文

学校读者我要写书评

暂无评论

Food Science and Human Wellness 2024年

作者： Bo Li Ze-Hua Zhang Hao-Ru Guan Xing-Li-Shang He Ning Wang Ying-Jie Dong Mei Rong Jiu-Jie Jia Ting-Ting Chen Zhi-Yuan Li Gui-Yuan Lv Lin-Nan Zhang Su-Hong Chen Collaborative Innovation Center of yangtze River delta region Green Pharmaceuticals， Zhejiang {3. of Technology Zhejiang Provincial Key Laboratory of TCM for Innovative R & D and Digital Intelligent Manufacturing of TCM Great Health Products.Huzhou College of Pharmaceutical Science， Zhejiang Chinese Medical university

The aim of this study was to investigate the role of DOPS and DOPS100 in attenuating immune dysfunction in subfertile mice. The results of the study revealed several noteworthy findings. First， DOPS and DOPS100 treatments led to significant improvement in weight gain and reversal of fatigue-related behaviors compared to the normal group. Second， both DOPS and DOPS100 showed effectiveness in reducing immune organ swelling， modulating immunoglobulin （IgA and IgM） levels， and restoring complement （C3. and C4） levels. In addition， they demonstrated a significant ability to enhance the integrity of the intestinal mechanical barrier by differentially upregulating the tight junction proteins Occludin and ZO-1. In addition， it was found that DOPS100 specifically enhanced the CD4+-Th17/Treg immune axis in the gut， as evidenced by increased expression of Foxp3.as well as decreased expression of RORγt， and further modulation of IL-10， IL-22， and IL-17A expression levels of inflammatory factors. These findings collectively suggest that DOPS100 holds significant potential in improving sub-healthy status by repairing the intestinal barrier， restoring local immune homeostasis， and activating the intestinal immune regulatory network. The study's outcomes provide valuable insights into the therapeutic implications of DOPS and DOPS100 in addressing immune dysfunction in sub-healthy conditions.

关键词：

Sequence-controlled dynamic covalent units enable decoupling of mechanical and self-healing performance of polymers

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Science China Chemistry 2024年

作者： Luzhi Zhang Hongfei Huang Lijie Sun Xiaopeng Ma Hui Tan Zhengwei You Respiratory Department Shenzhen Children's Hospital Affiliated to Shantou University Medical College State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringInstitute of Functional MaterialsShanghai Key Laboratory of Lightweight CompositeShanghai Engineering Research Center of Nano-Biomaterials and Regenerative MedicineDonghua University yangtze delta region {3. (Huzhou) University of Electronic Science and Technology of China

Sequence regulation provides an effective approach to controlling the properties of polymer ***,this approach remains an open question in the field of dynamic polymers,which emerge as more and more important new generation ***,we systematically investigate the effect of sequence control of dynamic covalent units in tuning the properties of *** sequence-controlled poly(oxime-urethanes) are *** dynamic oxime-urethane groups are relatively dispersed (SCP-1) or concentrated (SCP-2) distributed in their molecular *** sequence control strategy provides an efficient way to decouple the mechanical and self-healing performance of polymers,which is one of the most pressing challenges in the *** relatively dispersed oxime-urethane groups in SCP-1 not only facilitate the reorganization of the dynamic covalent bonds but also increase the probability of the reformation of hydrogen *** reversible dissociation/reassociation of dynamic bonds is conducive to dissipating energy to enhance mechanical performance and promote self-healing *** a result,SCP-1 exhibits much faster self-healing than SCP-2,and its tensile strength is nearly twice that of *** addition,energy dissipation capacity and degradation behavior also show significant sequence ***,this work reveals a new molecular structure-property relationship and provides a powerful strategy to construct high-performance polymers.

关键词：

Design and fabrication of an embedded wire-grid nanograting

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Journal of Semiconductors 2009年第1期30卷 34-38页

作者：周立兵朱伟 Zhejiang yangtze delta region {3. of tsinghua university

An embedded wire-grid nanograting was designed and fabricated for using as a broadband polarizing beam splitter to reflect s-polarized light and transmit p-polarized light. A protected cladding layer of the same material as the grating＇s was deposited on the ridge, whereas the wire-grid is deposited in the grating trenches, which makes it more firm during application. High polarization extinction ratios of above 40 and 20 dB for transmission and reflection, respectively, with a broad wavelength range for the whole optical communication bandwidth （850 -1700 nm） and a wide angular tolerance （〉 ±20 °） are obtained by optimization of the designed structures, and the grating period is 200 nm.

关键词： polarizing beam splitter wire-grid nanograting extinction ratio

Reinforced Lewis covalent bond by twinborn nitride heterostructure for lithium-sulfur batteries

在线全文

学校读者我要写书评

暂无评论

Journal of Energy Chemistry 2024年第1期88卷 363-372,I0009页

作者： Yaochen Song Pengkai Tang Yanjie Wang Yi Wang Linnan Bi Qi Liang Liang He Qingyu Xie Yiyong Zhang Peng Dong Yingjie Zhang Yao Yao Jiaxuan Liao Sizhe Wang yangtze delta region {3.(QuZhou) University of Electronic Science and Technology of ChinaQinzhou 324000ZhejiangChina School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731SichuanChina National and Local Joint Engineering Laboratory for Lithium-ion Batteries and Materials Preparation Technology Key Laboratory of Advanced Battery Materials of Yunnan ProvinceFaculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunming 650093YunnanChina School of Materials Science and Engineering Shaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic MaterialsShaanxi University of Science&TechnologyXi’an 710021ShaanxiChina School of Environmental Science and Engineering North China Electric Power UniversityBaoding 071003HebeiChina

The practical application of lithium-sulfur(Li-S)batteries,as promising next-generation batteries,is hindered by their shuttle effect and the slow redox ***,a tungsten and molybdenum nitride heterostructure functionalized with hollow metal-organic framework-derived carbon(W_(2)N/Mo_(2)N)was proposed as the sulfur *** hollow spherical structure provides storage space for sulfur,enhances electrical conductivity,and inhibits volume *** metal atoms in the nitrides bonded with lithium polysulfides(Li PSs)through Lewis covalent bonds,enhancing the high catalytic activity of the nitrides and effectively reducing the energy barrier of Li PSs redox ***,the high intrinsic conductivity of nitrides and the ability of the heterostructure interface to accelerate electron/ion transport improved the Li+*** leveraging the combined properties of strong adsorption and high catalytic activity,the sulfur host effectively inhibited the shuttle effect and accelerated the redox kinetics of Li ***-efficiency Li+transmission,strong adsorption,and the efficient catalytic conversion activities of Li PSs in the heterostructure were experimentally and theoretically *** results indicate that the W_(2)N/Mo_(2)N cathode provides stable,and long-term cycling(over 2000 cycles)at 3.C with a low attenuation rate of 0.0196%per *** design strategy of a twinborn nitride heterostructure thus provides a functionalized solution for advanced Li-S batteries.

关键词： Heterostructure Adsorption Redox kinetics